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Air pollutant emissions induced by rural-to-urban migration during China's urbanization(2005-2015)

environmental Science and Ecotechnology 2022年第2期10卷 45-53页

作者： Guang Shi Xi Lu Hongxia Zhang Haotian Zheng Zhonghua Zhang Shi Chen Jia Xing Shuxiao Wang State Key Joint Laboratory of Environment Simulation and Pollution Control and School of Environment Tsinghua UniversityBeijing100084PR China Institute for Carbon Neutrality Tsinghua UniversityBeijing100084PR China Beijing Laboratory of Environmental Frontier Technologies Tsinghua UniversityBeijing100084PR China State Environmental Protection Key Laboratory of Sources and Control of Air Pollution Complex Beijing100084PR China School of Applied Economics Renmin University of ChinaBeijing100872PR China

As the world's most populous country,China has witnessed rapid urbanization in recent decades,with population migration from rural to urban(RU)regions as the major driving *** to the large gap between rural and urban consumption and investment level,large-scale RU migration impacts air pollutant emissions and creates extra uncertainties for air quality ***,we integrated population migration assessment,an environmentally extended inputeoutput model and structural decomposition analysis to evaluate the NOx,SO2 and primary PM2.5 emissions induced by RU migration during China's urbanization from 2005 to *** results show that RU migration increased air pollutant emissions,while the increases in NOx and SO2 emissions peaked in approximately 2010 at 2.4 Mt and 2.2 Mt,accounting for 9.2%and 8.7%of the national emissions,*** primary PM2.5 emissions induced by RU migration also peaked in approximately 2012 at 0.3 Mt,accounting for 2.8%of the national *** indirect emissions embodied in consumption and investment increased,while household direct emissions *** widening gap between urban and rural investment and consumption exerted a major increasing effect on migration-induced emissions;in contrast,the falling emission intensity contributed the most to the decreasing effect benefitting from end-of-pipe control technology applications as well as improving energy *** peak of air pollutant emissions induced by RU migration indicates that although urbanization currently creates extra environmental pressure in China,it is possible to reconcile urbanization and air quality improvement in the future with updating urbanization and air pollution control policies.

关键词： Urbanization Population migration Air pollutant emission reduction Inputeoutput model Structural decomposition analysis

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Identifying priority areas of Four Major Chinese carps’ species in the Pearl River basin based on the MaxEnt model

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Watershed Ecology and the Environment 2023年第1期5卷 18-23页

作者： Shao, Xiaojing Liu, Xing Cai, Jie Cai, Yanzi Cui, Baoshan Research Center for Monitoring and Environmental Sciences Taihu Basin & East China Sea Ecological Environment Supervision and Administration Authority Ministry of Ecology and Environment of the People's Republic of China Shanghai 200125 China State Key Joint Laboratory of Environmental Simulation and Pollution Control School of Environment Beijing Normal University Beijing 100875 China

The Pearl River basin (PRB) is an important producing area and the gene pool of wild resources of Four Major Chinese carps (FMCC). However human activities and climate changes causes the area shrink of the river network in PRB, the pollution aggregation, the serious habitat destroy of aquatic organisms, and the threat of biological resources and their living environment. Based on the accurate location and distribution data of FMCC from the literature and the field survey report of 2015–2016, this study used the MaxEnt model to predict the hot spot distribution area of FMCC in PRB. The simulation results show that the distribution of FMCC in the PRB gradually increases from the upper reaches to the middle and lower reaches. According to the MaxEnt model, the hot spots of FMCC in the PRB are mainly distributed in the south reaches and the lower reaches of the southeast. The model simulation also demonstrates that the hottest spots for the distribution of FMCC species in the PRB are the Yujiang basin, the Qianjiang basin and the lower reaches of the Xijiang basin. This study can provide the scientific guidance for the protection and the restoration of FMCC species in the PRB. © 2022 The Authors

关键词： Biodiversity MaxEnt model Pearl River basin Prior conservation area

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Grey Prediction Based Input–Output Model for Analyzing Potential Energy-Related Emission Mitigation Pathways: A Case Study of Fujian 14th

Grey Prediction Based Input–Output Model for Analyzing Pote...

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14th International Conference on environmental Science and Technology, ICEST 2023

作者： Sun, Z.M. Liu, J. Li, Y.P. School of Environmental Science and Engineering Xiamen University of Technology Xiamen361024 China State Key Joint Laboratory of Environmental Simulation and Pollution Control School of Environment Beijing Normal University Beijing100875 China Faculty of Engineering and Applied Science University of Regina ReginaSKS4S 0A2 Canada

ISBN: (纸本)9783031546839

Economic activities release pollutants and carbon (mainly CO2) directly by consuming energy resources and indirectly by using energy-intensive goods. This research put forwards a grey model (GM) (1, 1) based input–output model (GIOM) for simulating pollutants and CO2 emissions in Fujian Province under varied socio-economic development scenarios. Major findings are: (i) in the planning period, Agriculture, forestry, animal husbandry and fishery (AGR) is the main sector for wastewater emissions in the planning period, and manufacturing and materials and energy conversion (MEC) sectors will be the main sectors for emissions of waste gases and CO2 in the planning period;(ii) through the simulation, the total energy consumption in Fujian Province increases by 13.53–51.08%, Metal and nonmetal products (MAN), MEC and Wholesale and retail transportation and warehousing (WRT) are the main energy consumers;(iii) the COD, NH3–N, SO2, and NOx emissions decrease 24.55–70.11%, 24.53–70.83%, 27.11–70.55% and 22.47–72.00% over time, and the CO2 emissions range from an increase of 36.35% to a decrease of 5.98% over time. © The Author(s), under exclusive license to Springer Nature Switzerland AG 2024.

关键词： Carbon dioxide

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Chemical characteristics and water stability evaluation of groundwater in the CKDu Zone of Sri Lanka

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Journal of environmental Sciences 2024年第12期146卷 67-80页

作者： Dazhou Hu Suresh Indika Madhubhashini Makehelwala COORAY Titus Liying Zhu Zhonghe Pang Hui Zhong Sujithra K.Weragoda K.B.S.N.Jinadasa Rohan Weerasooriya Yuansong Wei State Key Joint Laboratory of Environment Simulation and Pollution Control Research Center for Eco-Environmental SciencesChinese Academy of SciencesBeijing 100085China Laboratory of Water Pollution Control Technology Research Center for Eco-Environmental SciencesChinese Academy of SciencesBeijing 100085China University of Chinese Academy of Sciences Beijing 100049China Department of Applied Earth Sciences Uva Wellassa UniversityBadulla 90000Sri Lanka China-Sri Lanka Joint Research and demonstration Center for Water Technology Ministry of Water SupplyE.O.E.Pereira MawathaPeradeniya 24000Sri Lanka National Water Supply and Drainage Board Katugastota 20800Sri Lanka Department of Civil Engineering Faculty of EngineeringUniversity of PeradeniyaPeradeniya 20400Sri Lanka National Institute of Fundamental Studies Kandy 20000Sri Lanka

Groundwater is the main source of drinking water for the rural population in the chronic kidney disease of unknown etiology(CKDu)zone of the North Central Province(NCP)in Sri *** this study,a total of 334 groundwater samples(311 dug wells,21 tube wells and 2 springs)during the wet season from two aquifers in the NCP were collected,and inves-tigated their chemical characteristics and evaluate their water quality,including ground-water chemistry,main ion sources,the corrosion and scaling potential of *** results showed that the two hydrochemical types of groundwater in the NCP were mainly of the Ca-HCO_(3),Na·Ca-HCO_(3)types,with the main HCO_(3)−,Na^(+)and Ca^(2+)ions in both types of groundwater originating from silicate and evaporite salt dissolution and influenced by alternating cation adsorption,while the presence of NO_(3)−was mainly ***-uation ofwater stability using namely Langelier saturation index(LSI),Ryznar stability index(RSI),Puckorius scaling index(PSI)and Larson-Skold index(LS),indicated that most ground-water presents corrosion potential and has corrosion behavior tendency of metals to some *** water quality of Polonnaruwa was better than that of Anuradhapura in the NCP,and when the groundwater was worse than the“good”grade,which must be properly treated before it is used as drinking water.

关键词： CKDu zone Rock weathering Cation alternating adsorption Water stability Water quality assessment

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Evaluation of laboratory and environmental exposure systems for protein modification upon gas pollutants and environmental factors

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Journal of environmental Sciences 2024年第9期143卷 213-223页

作者： Zhiwei Pan ShiyiWu Qiaoze Zhu Fobang Liu Yongjian Liang Chenglei Pei Haoyu Jiang Yingyi Zhang Senchao Lai The Key Lab of Pollution Control and Ecosystem Restoration in Industry Clusters Ministry of EducationSchool of Environment and EnergySouth China University of TechnologyGuangzhou 510006China Department of Environmental Science and Engineering Xi’an Jiaotong UniversityXi’an 710049China Guangzhou Sub-branch of Guangdong Ecological and Environmental Monitoring Center Guangzhou 510006China State Key Laboratory of Organic Geochemistry Guangdong Key Laboratory of Environmental Protection and Resources Utilizationand Joint Laboratory of the Guangdong-Hong Kong-Macao Greater Bay Area for the EnvironmentGuangzhou Institute of GeochemistryChinese Academy of SciencesGuangzhou 510640China School of Marine Sciences Sun Yat-sen UniversityZhuhai 519082China

Chemical modifications of proteins induced by ambient ozone(O_(3))and nitrogen oxides(NOx)are of public health concerns due to their potential to trigger respiratory *** laboratory and environmental exposure systems have been widely used to investigate their relevant mechanism in the *** bovine serum albumin(BSA)as a model protein,we evaluated the two systems and aimed to reduce the uncertainties of both the reactants and products in the corresponding kinetic *** the laboratory simulation system,the generated gaseous pollutants showed negligible *** layers of BSA were coated on the flow tube with protein extraction recovery of 87.4%.For environmental exposure experiment,quartz fiber filter was selected as the upper filter with low gaseous O_(3)(8.0%)and NO_(2)(1.7%)losses,and cellulose acetate filter was appropriate for the lower filter with protein extraction efficiency of 95.2%.The protein degradation process was observed without the exposure to atmospheric oxidants and contributed to the loss of protein monomer mass fractions,while environmental factors(e.g.,molecular oxygen and ultraviolet)may cause greater protein monomer *** on the evaluation,the study exemplarily applied the two systems to protein modification and both showed that O_(3) promotes the protein oligomerization and nitration,while increased temperature can accelerate the oligomerization and increased relative humidity can inhibit the nitration in the environmental exposure *** developed laboratory and environmental systems are suitable for studying protein modifications formed under different atmospheric conditions.A combination of the two will further reveal the actual mechanism of protein modifications.

关键词： Protein modification laboratory simulation environmental exposure Oligomerization Nitration

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Ambient volatile organic compounds at a receptor site in the Pearl River Delta region:Variations,source apportionment and effects on ozone formation

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Journal of environmental Sciences 2022年第1期34卷 104-117页

作者： Yao Meng Junwei Song Lewei Zeng Yingyi Zhang Yan Zhao Xufei Liu Hai Guo Liuju Zhong Yubo Ou Yan Zhou Tao Zhang Dingli Yue Senchao Lai The Key Lab of Pollution Control and Ecosystem Restoration in Industry Clusters Ministry of Educationand Guangdong Provincial Key Laboratory of Atmospheric Environment and Pollution ControlSchool of Environment and EnergySouth China University of TechnologyGuangzhou 510006China Institute of Meteorology and Climate Research Karlsruhe Institute of TechnologyHermann-von-Helmholtz-Platz 1Eggenstein-Leopoldshafen 76344Germany Department of Civil and Environmental Engineering The Hong Kong Polytechnic UniversityHong KongChina Guangdong Environmental Monitoring Center State Environmental Protection Key Laboratory of Regional Air Quality MonitoringGuangzhou 510308China Guangdong Polytechnic of Environmental Protection Engineering Foshan 528216China

We present the continuously measurements of volatile organic compounds(VOCs)at a receptor site(Wan Qing Sha,WQS)in the Pearl River Delta(PRD)region from September to November of *** average mixing ratios of total VOCs(TVOCs)was 36.3±27.9 ppbv with the dominant contribution from alkanes(55.5%),followed by aromatics(33.3%).The diurnal variation of TVOCs showed a strong photochemical consumption during daytime,resulting in the formation of ozone(O_(3)).Five VOC sources were resolved by the positive matrix factorization(PMF)model,including solvent usage(28.6%),liquid petroleum gas(LPG)usage(24.4%),vehicle exhaust(21.0%),industrial emissions(13.2%)and gasoline evaporation(12.9%).The regional transport air masses from the upwind cities of south China can result in the elevated concentrations of *** ratios of TVOCs/NO_(x)(1.53±0.88)suggested that the O_(3) formation regime at WQS site was VOC-limited,which also confirmed by a photochemical box model with the master chemical mechanism(PBM-MCM).Furthermore,the observation on high-O_(3) episode days revealed that frequent O_(3) outbreaks at WQS were mainly caused by the regional transport of anthropogenic VOCs especially for aromatics and the subsequent photochemical *** study provides valuable information for policymakers to propose the effective control strategies on photochemical pollution in a regional perspective.

关键词： Volatile organic compounds(VOCs) Pearl River Delta(PRD)region Source apportionment Ozone(O_(3)) Regional transport

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Variation characteristics of fine particulate matter and its components in diesel vehicle emission plumes

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Journal of environmental Sciences 2021年第9期33卷 138-149页

作者： Xianbao Shen Jiateng Hao Lei Kong Yue Shi Xinyue Cao Jiacheng Shi Zhiliang Yao Xin Li Bobo Wu Yiming Xu Kebin He State Environmental Protection Key Laboratory of Food Chain Pollution Control Beijing Technology and Business UniversityBeijing 100048China Key Laboratory of Cleaner Production and Integrated Resource Utilization of China National Light Industry Beijing Technology and Business UniversityBeijing 100048China School of Ecology and Environment Beijing Technology and Business UniversityBeijing 100048China State Key Joint Laboratory of Environment Simulation and Pollution Control School of EnvironmentTsinghua UniversityBeijing 100084China State Environmental Protection Key Laboratory of Sources and Control of Air Pollution Complex Beijing 100084China

A rapid reaction occurs near the exhaust nozzle when vehicle emissions contact the *** diesel vehicles were studied using a new multipoint sampling system that is suitable for studying the exhaust plume near the exhaust *** variation characteristics of fine particle matter(PM_(2.5)) and its components in diesel vehicle exhaust plumes were *** PM_(2.5) emissions gradually increased with increasing distance from the nozzle in the *** carbon emissions remained basically unchanged, organic carbon and total carbon(TC) increased with increasing *** concentrations of SO_(4)^(2-),NO_(3)^(-) and NH_(4)^(+) (SNA) directly emitted by the vehicles were very low but increased rapidly in the exhaust *** selective catalytic reduction(SCR) reduced 42.7% TC, 40% NO_(3)^(-) emissions, but increased 104% SO_(4)^(2-) and 36% NH_(4)^(+) emissions, *** summary,the SCR reduced 29% primary PM_(2.5) emissions for the tested diesel *** NH_(4)NO_(3) particle formation maybe more important in the plume, and there maybe other forms of formation of NH_(4)^(+) (***4Cl).The generation of secondary organic carbon(SOC) plays a leading role in the generation of secondary PM_(2.5).The SCR enhanced the formation of SOC and SNA in the plume, but comprehensive analysis shows that the SCR more enhanced the SNA formation in the plume, which is mainly new particles formation *** inconsistency between secondary organic aerosol(SOA) and primary organic aerosol definitions is one of the important reasons for the difference between SOA simulation and observation.

关键词： Variation characteristics Diesel vehicle Emission plume PM2.5 Components

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CeO_(2)-supported Fe,Co and Ni toward CO_(2) hydrogenation:Tuning catalytic performance via metal-support interaction

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Journal of Rare Earths 2023年第6期41卷 926-932,I0005页

作者： Bolang Li Fei Wang Kai Li Ping Ning Min Chen Changbin Zhang Faculty of Environmental Science and Engineering Kunming University of Science and TechnologyKunming 650500China National-Regional Engineering Center for Recovery of Waste Gases from Metallurgical and Chemical Industries Kunming University of Science and TechnologyKunming 650500China State Key Joint Laboratory of Environment Simulation and Pollution Control Research Center for Eco-Environment SciencesChinese Academy of SciencesBeijing 100085China University of Chinese Academy of Sciences Beijing 100049China

The chemical transformation of CO_(2) produces carbon compounds that can be used as precursors for the production of chemicals and ***,we investigated the activity and selectivity of the transition metals(Fe,Co,and Ni)supported on CeO_(2) catalyst for CO_(2) hydrogenation at atmospheric *** found that Ni/CeO_(2) shows the highest CO_(2)conversion compared with Fe/CeO_(2) and Co/CeO_(2).Besides,Co/CeO_(2)and Ni/CeO_(2) exhibit nearly 100%CH_(4)selectivity while Fe/CeO_(2) inclines to produce *** characterization results show that the metal-support interaction order is Fe/CeO_(2)>Co/CeO_(2)>Ni/CeO_(2),the weak metal-support inte raction over Ni/CeO_(2)benefits the activation of H_(2) and then promotes the activity of CO_(2) ***,in situ DRIFTS results demonstrate that monodentate formate species rather than bidentate formate are the active *** main route of CO_(2) hydrogenation to CH_(4) is that CO_(2) is firstly transformed to m-HCOO*and then direct hydrogenation of the m-HCOO*to CH_(4).This study provides insights into the understanding of the mechanisms of CO_(2) hydrogenation on CeO_(2)based catalysts.

关键词： Ni CeO_(2) Metal-support interaction CO_(2)hydrogenation Rare earths

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Atmospheric heterogeneous reactions on soot:A review

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Fundamental Research 2023年第4期3卷 579-591页

作者： Yuan Liu Guangzhi He Biwu Chu Qingxin Ma Hong He State Key Joint Laboratory of Environment Simulation and Pollution Control Research Center for Eco-Environmental SciencesChinese Academy of SciencesBeijing 100085China Center for Excellence in Regional Atmospheric Environment and Key Laboratory of Urban Pollutant Conversion Institute of Urban EnvironmentChinese Academy of SciencesXiamen 361021China University of Chinese Academy of Sciences Beijing 100049China

Soot particles,composed of elemental carbon and organic compounds,have attracted widespread attention in recent years due to their significant impacts on climate,the environment and human *** has been found to be chemically and physically active in atmospheric aging processes,which leads to alterations in its composition,morphology,hygroscopicity and optical properties and thus changes its environmental and health *** heterogeneous reactions on soot also have a significant impact on the transformation of gaseous pollutants into secondary ***,the interactions between soot and atmospheric substances have been widely investigated to better understand the environmental behaviors of *** this review,we systematically summarize the progress and developments in the heterogeneous chemistry on soot over the past_(3)0 *** trace constituents such as NO_(2),O_(3),SO_(2),N_(2)O_(5),HNO_(3),H_(2)SO_(4),OH radical,HO_(2)radical,peroxyacetyl nitrate etc.,are presented in detail from the aspect of their heterogeneous reactions on *** possible mechanisms and the effects of environmental conditions on these heterogeneous reactions are also ***,the impacts of the heterogeneous reactions of soot on the atmospheric environment are discussed,and some aspects of soot-related research which require further investigation are proposed as well.

关键词： Soot NO_(2) SO_(2) O_(3) Heterogeneous reactions

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Accumulation, transportation, and distribution of tetracycline and cadmium in rice

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Journal of environmental Sciences 2023年第4期126卷 58-69页

作者： Chunfeng He Jini Zhou Chen Yang Zhiyi Song Junheng He Ziqing Huang Yurong Deng Jinling Wang Yu Xiong Zhi Dang College of Environment and Energy South China University of TechnologyGuangzhou 510006China The Key Lab of Pollution Control and Ecosystem Restoration in Industry Clusters Ministry of EducationGuangzhou 510006China Department of Environmental Sciences The State University of New JerseyRutgers UniversityNew BrunswickNJ 08901USA Guangdong Institute of Ecological Environment and Soil Guangzhou 510650China

Co-exposure to heavy metal and antibiotic pollution might result in complexation and synergistic interactions,affecting rice growth and further exacerbating pollutant ***,our study sought to clarify the influence of different Tetracycline (TC) and Cadmium(Cd) concentration ratios (both alone and combined) on rice growth,pollutant accumulation,and transportation during the tillering stage in hydroponic ***,our findings indicated that the interaction between TC and Cd could alleviate the toxic effects of TC/Cd on aerial rice structures and decrease pollutant burdens during root *** contrast,TC and Cd synergistically promoted the accumulation of TC/Cd in rice ***,their interaction increased the accumulation of TC in roots while decreasing the accumulation of Cd when the toxicant doses *** strong affinity of rice to Cd promoted its upward transport from the roots,whereas the toxic effects of TC reduced TC ***,the combined toxicity of the two pollutants inhibited their upward ***,a low concentration of TC promoted the accumulation of Cd in rice mainly in the root ***,a certain dose of TC promoted the upward migration of Cd from the root *** ablation-inductively coupled plasma mass spectrometry demonstrated that Cd mainly accumulated in the epidermis and stele of the root,whereas Fe mainly accumulated in the epidermis,which inhibited the absorption and accumulation of Cd by the rice roots through the generation of a Fe *** findings thus provide insights into the effects of TC and Cd co-exposure on rice growth.

关键词： Laser ablation-inductively coupled plasma mass spectrometry Tetracycline Cadmium Accumulation Distribution

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