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Manipulating Interfacial Stability via Preferential Absorption for Highly Stable and Safe 4.6 V LiCoO_(2) Cathode

Nano-Micro Letters 2025年第8期17卷 95-110页

作者： Long Chen Xin He Yiqing Chen Youmin Hou Yujie Zhang Kangli Wang Xinping Ai Yuliang Cao Zhongxue Chen Key Laboratory of Hydraulic Machinery Transients Ministry of EducationSchool of Power and Mechanical EngineeringWuhan UniversityWuhan 430072People’s Republic of China State Key Laboratory of Advanced Electromagnetic Technology School of Electrical and Electronic EngineeringHuazhong University of Science and TechnologyWuhan 430074People’s Republic of China Hubei Key Laboratory of Electrochemical Power Sources College of Chemistry and Molecular SciencesWuhan UniversityWuhan 430072People’s Republic of China

Elevating the upper cutoff voltage to 4.6 V could effec-tively increase the reversible capacity ofLiCoO_(2)(LCO)cathode,whereas the irreversible structural transition,unstable electrode/electrolyte interface and potentially induced safety hazards severely hinder its industrial *** a robust cathode/electrolyte interface film by electrolyte engineer-ing is one of the efficient approaches to boost the performance of high-voltage LCO(HV-LCO);however,the elusive interfacial chemistry poses substantial challenges to the rational design of highly compatible ***,we propose a novel electrolyte design strategy and screen proper solvents based on two factors:highest occupied molecular orbital energy level and LCO absorption ***(2,2,2-trifluoroethyl)phosphate is determined as the optimal solvent,whose low defluorination energy barrier significantly promotes the construction of LiF-rich cathode/electrolyte interface layer on the surface of LCO,thereby eventually suppresses the phase transition and enhancesLi+diffusion *** rationally designed electrolyte endows graphite||HV-LCO pouch cells with long cycle life(85.3%capacity retention after 700 cycles),wide-temperature adaptability(-60–80℃)and high safety(pass nail penetration).This work provides new insights into the electrolyte screening and rational design to constructing stable interface for high-energy lithium-ion batteries.

关键词： Electrolyte design LiF-rich interface Wide-temperature High-safe 4.6 V LCO

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A Real-Time Junction Temperature Estimating Method for SiC MOSFET Based on the Turn-on Drain-Source Current Oscillation

A Real-Time Junction Temperature Estimating Method for SiC M...

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International Conference of Electrical, Electronic and Networked Energy Systems, EENES 2024

作者： Yang, Fengming Liang, Lin Zhang, Ziyang State Key Laboratory of Advanced Electromagnetic Technology Power Electronics and Energy Management Key Laboratory Ministry of Education of China School of Electrical and Electronic Engineering Huazhong University of Science and Technology Wuhan430070 China

ISBN: (纸本)9789819618514

Online junction temperature (Tj) measurement is critical for SiC MOSFET reliability evaluation health management and life prediction. In order to make the tradeoff between availability, simplicity, as well as accuracy, this article demonstrates a real-time junction temperature estimating method by selecting the current oscillation peak of drain source (Ioscpeak) during turn-on transient as a temperature sensitive electrical parameter (TSEP). The theoretical and simulation analysis results show that the Ioscpeak is available to be a TSEP. Then, the model of Ioscpeak and Tj is derived through fitting curve based the experimental results. The voltage and load current dependency of proposed method are also discussed. The experimental results demonstrate that the bus voltage level has a negligible influence to the relationship between the Ioscpeak and the Tj, the value of Ioscpeak is increasing with the increment of current level at the specific temperature. The sensitivity of proposed method has a satisfactory performance of junction temperature estimation. The estimation circuit of proposed method has a simplicity hardware with low cost and easy to be implanted with gate drive of SiC MOSFET. © Beijing Paike Culture Commu. Co., Ltd. 2025.

关键词： MOSFET devices

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Novel Inertia Control Method with Phase-Locked Error Feedforward in PLL for DFIG-Based WTs

Novel Inertia Control Method with Phase-Locked Error Feedfor...

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International Conference of Electrical, Electronic and Networked Energy Systems, EENES 2024

作者： Yu, Jiawei Zhu, Yihua Zhou, Yini Hu, Bo Li, Zheyu Li, Xiaoyu State Key Laboratory of HVDC Electric Power Research Institute China Southern Power Grid Guangzhou510663 China State Key Laboratory of Advanced Electromagnetic Engineering and Technology School of Electrical and Electronic Engineering Huazhong University of Science and Technology Wuhan430074 China

ISBN: (纸本)9789819620418

The large-scale access of wind power causes a significant reduction in the inertia of the power system, seriously threatening the security and stability of the system frequency. Inertia control methods based on the optimized PLLs provide a solution to the low inertia problem of doubly-fed inductance generator (DFIG)-based wind turbines (WTs), but they still suffer from poor dynamic performance and obvious phase-locked error in steady state. For this reason, a novel inertia control method for DFIG-based WTs is proposed in this paper to support the system frequency with better performance in all aspects. Firstly, an equivalent inertia model is deduced considering the dynamic of control and the reason why modifying PLL can realize inertia response of WT is analyzed. Then, the existing inertia control methods based on optimized PLL is introduced and a novel inertia control method with phase-locked error feed-forward in PLL (pefPLL) is proposed. After that, the inertia characteristics, dynamic performance, and steady state performance of pefPLL and other PLLs are compared. Finally, the superiority of the novel inertia control method with pefPLL is verified by simulations. © Beijing Paike Culture Commu. Co., Ltd. 2025.

关键词： Wind turbines

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Experimental Study on Electrode Erosion Process with High Current Vacuum Arc 19th

Experimental Study on Electrode Erosion Process with High Cu...

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19th Annual Conference of China Electrotechnical Society, ACCES 2024

作者： Peng, Ruochen Li, Yilong Zhao, Yuan Chen, Lixue Ya, Penglong Lyu, Tianmao State Key Laboratory of Advanced Electromagnetic Engineering and Technology Huazhong University of Science & Technology Wuhan China School of Electrical and Electronic Engineering Huazhong University of Science & Technology Wuhan China Key Laboratory of Pulsed Power Technology Huazhong University of Science & Technology Ministry of Education China

ISBN: (纸本)9789819613861

During the breaking process, the erosion of anode contact greatly affects the result of high current vacuum breaking. Therefore, it is important to study the forming and transforming process of anode modes for improving the breaking performance and life of vacuum circuit breaker. The cup axial magnetic field (AMF) contacts is widely used in vacuum trigger switch and vacuum on-load tap changer. In order to study the vacuum arc characteristics and anode mode change of cup AMF contacts under high current density, the 40 mm diameter cup AMF contacts with six slots is observed and studied by experimental means under the gap distance of 6 mm and 10 mm. In this paper, the arc current-voltage characteristics, vacuum arc shape and surface erosion of contact are analyzed. The analysis results show that the larger the contact gap, the larger the arc voltage, the smaller the arc anode mode threshold current and the more serious the contact erosion degree. © Beijing Paike Culture Commu. Co., Ltd. 2025.

关键词： Anodes

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Analysis of Three-Phase Short-Circuit Electromotive Force on Six Vacuum-Break Parallel-Type Generator Outlet Circuit Breakers 11th

Analysis of Three-Phase Short-Circuit Electromotive Force on...

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11th Frontier Academic Forum of Electrical engineering, FAFEE 2024

作者： Sun, Likang Chen, Lixue He, Yinghui Zou, Xinyang Li, Yingzhuo State Key Laboratory of Advanced Electromagnetic Technology Huazhong University of Science and Technology Wuhan430074 China Key Laboratory of Pulsed Power Technology Ministry of Education School of Electrical and Electronic Engineering Huazhong University of Science and Technology Wuhan430074 China

ISBN: (纸本)9789819787791

Currently, vacuum type generator outlet circuit breaker dominates the large-capacity generator circuit breaker. However, due to the large short-circuit current at the generator outlet end, the generator outlet circuit breaker needs to bear a great short-circuit electromotive force, thus affecting its dynamic stability. In this paper, COMSOL is used to construct a model of a six vacuum break parallel type outlet circuit breaker for the protection of a megawatt-level generator. Based on Maxwell's electromagnetic theory, the transient calculation of three-phase short-circuit electromotive force under different phases is carried out for the generator outlet vacuum circuit breaker, and the great values of short-circuit electromotive force under different phases are obtained for each phase. The results show that the main component of the short-circuit electromotive force is the electromotive force in the y-direction. And based on the maximum transient electromotive force, the influence of the material on the short-circuit electromotive force is studied, which provides theoretical support for the analysis of the short-circuit electromotive force of the generator outlet circuit breaker and the optimized design of the shell. © Beijing Paike Culture Commu. Co., Ltd. 2025.

关键词： Electric shielding

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Al-F co-doping towards enhanced electrolyte-electrodes interface properties for halide and sulfide solid electrolytes

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Chinese Chemical Letters 2025年第1期36卷 610-617页

作者： Han Yan Jingming Yao Zhangran Ye Qiaoquan Lin Ziqi Zhang Shulin Li Dawei Song Zhenyu Wang Chuang Yu Long Zhang College of Physics and Energy Fujian Normal UniversityFuzhou 350117China Clean Nano Energy Center State Key Laboratory of Metastable Materials Science and TechnologyYanshan UniversityQinhuangdao 066004China Tianjin Key Laboratory for Photoelectric Materials and Devices School of Materials Science and EngineeringTianjin University of TechnologyTianjin 300384China Guilin Electrical Equipment Scientific Research Institute Co. Ltd.Guilin 541004China State Key Laboratory of Advanced Electromagnetic Engineering and Technology School of Electrical and Electronic EngineeringHuazhong University of Science and TechnologyWuhan 430000China

All-solid-state Li batteries(ASSLBs)using solid electrolytes(SEs)have gained significant attention in recent years considering the safety issue and their high energy *** these advantages,the commercialization of ASSLBs still faces challenges regarding the electrolyte/electrodes interfaces and growth of Li *** doping is an effective and direct method to enhance the performance of ***,we report an Al-F co-doping strategy to improve the overall properties including ion conductivity,high voltage stability,and cathode and anode ***,the Al-F co-doping enables the formation of a thin Li-Al alloy layer and fluoride interphases,thereby constructing a relatively stable interface and promoting uniform Li *** similar merits of Al-F co-doping are also revealed in the Li-argyrodite *** assembled with these optimized electrolytes gain good electrochemical performance,demonstrating the universality of Al-F co-doping towards advanced SEs.

关键词： Solid electrolytes Li halides Li_(2)ZrCl_(6) Li argyrodites Fluorine doping

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Design and Analysis of Coupled Self-charging Mechanical DC Circuit Breaker

Design and Analysis of Coupled Self-charging Mechanical DC C...

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International Conference of Electrical, Electronic and Networked Energy Systems, EENES 2024

作者： Xie, Yunlong Yuan, Zhao Chen, Lixue State Key Laboratory of Advanced Electromagnetic Technology Huazhong University of Science and Technology Wuhan430074 China Key Laboratory of Pulsed Power Technology Ministry of Education School of Electrical and Electronic Engineering Huazhong University of Science and Technology Wuhan430074 China

ISBN: (纸本)9789819620456

Mechanical DC circuit breakers have become an irreplaceable part of flexible DC power grids because of their advantages of high economy, low con-duction impedance, and reliable control. However, the large volume of the charging circuit and the high interruption pressure in low current are still the problems it faces. To address the aforementioned issues, a Coupled Self-charging Mechanical DC Circuit Breaker (CSC-DCCB) is proposed. This innovative solution mitigates the risk of switch arc reignition during the commutation process by incorporating a self-charging circuit. The energy consumption process of metal-oxide varistor will cause the capacitor to complete recharging, and this voltage will be used for the reclosing of the CSC-DCCB. Secondly, the parameter of the CSC-DCCB is optimized to achieve a lower overall capacity of the circuit breaker and the rated voltage of the converter switches, which retains the traditional low conduction loss. Finally, the feasibility of CSC-DCCB is validated through PSCAD, the technical parameters of CSC-DCCB are compared with traditional DCCB, showing that CSC-DCCB has better economic efficiency. © Beijing Paike Culture Commu. Co., Ltd. 2025.

关键词： Flexible electronics

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Numerical Study of the Current Density on the Armature and Rail Interface with Dynamic Contact

Numerical Study of the Current Density on the Armature and R...

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International Conference of Electrical, Electronic and Networked Energy Systems, EENES 2024

作者： Xu, Jinghan Xia, Shengguo Chen, Lixue Ministry of Education Hubei Wuhan430074 China State Key Laboratory of Advanced Electromagnetic Engineering and Technology Hubei Wuhan430074 China School of Electrical and Electronic Engineering Huazhong University of Science and Technology Wuhan430074 China

ISBN: (纸本)9789819620791

The electrical contact between the armature and rail is acknowledged as imperfect electrical contact (ImPEC), exhibiting characteristics distinct from bulk behavior. It is important to understand the current distribution of the ImPEC for future design and optimization. This paper proposes ImPEC boundary conditions by combining the contact layer model (CLM) and the Cooper-Mikic-Yoranovich model (CMYM), and the current distribution is numerically studied. Variations in the contact pressure and current density with time are analyzed. The results show a rapid increase in the contact pressure and area during the current ramp-up stage, being constant in the flat stage, and a gradual decline in the current ramp-down stage. The current path changes with the contact area, and the current shifts from the trailing edge to the leading edge over time. Additionally, comparative calculations are performed to analyze current variations under dynamic contact. Results suggest that the current distribution is influenced by magnetic diffusion and forced shifts of current caused by dynamic contact. © Beijing Paike Culture Commu. Co., Ltd. 2025.

关键词： Threshold current density

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Effect of electrochemical hydrogen charging on the microstructure and mechanical behavior of a duplex structured Mg-8wt.%Li alloy

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Journal of Magnesium and Alloys 2025年第2期13卷 668-680页

作者： Shuo Wang Daokui Xu Baojie Wang Dongliang Wang Zhiqiang Zhang Li Liu Jie Chen Key Lab of Electromagnetic Processing of Materials Ministry of EducationNortheastern UniversityShenyang110819China Key Laboratory of Nuclear Materials and Safety Assessment Institute of Metal ResearchChinese Academy of SciencesShenyang110016China Engineering Research Center of Advanced Materials Preparing Technology Ministry of EducationNortheastern UniversityShenyang110819China Binzhou Institute of Technology BinzhouShandong Province256606China Shandong Key Laboratory of Advanced Aluminium Materials and Technology BinzhouShandong Province256606China School of Environmental and Chemical Engineering Shenyang Ligong UniversityShenyang110159China Spallation Neutron Source Science Center Dongguan523803China

In this work,through performing microstructural characterization,tensile testing and failure analysis,the influence of electrochemical hydrogen charging on the microstructure and mechanical behavior of an as-cast Mg-8wt.%Li alloy was *** revealed that after being hydrogen charged at 50 mA/cm2 for respectively 3 h,6 h and 18 h in 0.1 M NaCl solution,obvious HID occurred and the damage degree was gradually increased with the hydrogen charging *** the sample being hydrogen charged for 3 h,micro pores with the diameter ranging from 10~30µm were formed and preferentially present inα-Mg ***,micro cracks with the length ranging from 10~50µm mainly initiated inα-Mg phase,atα-Mg/β-Li interfaces and the peripheries of *** the increase of hydrogen charging time,the numbers of pores and cracks were obviously *** results revealed that the hydrogen charging can simultaneously decrease the tensile strength and ductility of the *** with the uncharged sample,the tensile yield strength,ultimate tensile strength and the elongation ratio to failure were respectively reduced by 5.7%,7.3%,31.7%for the 3h-charged sample and 24.6%,24.8%,67.0%for the 18h-charged *** analysis indicated that hydrogen charging can induce the brittle cracking of the alloy and the size of brittle cracking region being composed of quasi-cleavage facets and interfacial cracks on the fracture surfaces was increased with the hydrogen charging time.

关键词： Magnesium-lithium alloy Microstructure Hydrogen-induced damage Hydrogen embrittlement Mechanical behavior

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Metal-organic polyhedra as dynamic cross-linker for recyclable mixed matrix membranes with promising dimension stability

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Science China Chemistry 2025年第2期68卷 705-713页

作者： Linjie Lan Mingxin Zhang Haiyan Xiao Wei Liu-Fu Yuyan Lai Jiadong Chen Jia-Fu Yin Panchao Yin State Key Laboratory of Luminescent Materials and Devices&South China Advanced Institute for Soft Matter Science and Technology Guangdong Basic Research Center of Excellence for Energy and Information Polymer MaterialsSouth China University of TechnologyGuangzhou 510641China State Key Laboratory of Marine Resource Utilization in South China Sea Hainan Provincial Key Lab of Fine ChemistrySchool of Chemical Engineering and TechnologyHainan UniversityHaikou 570228China

Mixed matrix membranes(MMMs)are designed by incorporating microporous inorganic fillers into polymer matrix for the integration of inorganics’excellent gas separation performance with polymers’promising ***,due to the complex interphase interaction,the prevention of long-term aging is still challenging and the poor processability/recyclability of MMMs hinders their extensive ***,a coordination assembly protocol is developed for the fabrication of MMMs with both excellent processability/recyclability upon thermal annealing and promising dimension stability even under high gas *** bearing isophthalic acid(IPA)as side chains are applied to coordinate with Cu^(2+)and the assembled 2.5 nm microporous metal-organic polyhedra(MOP),{Cu_(24)IPA_(24)},serves as multi-functional cross-linkers for the polymer network *** MOPs’well-defined microporosity grants MMMs the capability for O_(2)/N_(2) separation while their activated dynamics at high temperatures(>120℃)endows polymer networks with excellent *** contrast to conventional supramolecular units,the MOPs possess unique logarithmic ligand-exchange kinetics and they show nearly frozen bonding dynamics at room temperature,ensuring promising dimensional stability to overcome the long-term aging and high gas pressure *** work not only provides fundamental understanding of the unique relaxation dynamics of complex systems with intertwined dynamics of supramolecular bonds and polymer chains,but also paves new avenues for the fabrication of robust and recyclable MMMs and elastomers.

关键词： dynamic bonding metal-organic polyhedra mixed matrix membrane polymer recycling gas separation

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