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Achieving Nearly 100% Targeted Conversion of NO to NO₂ through Cooperative Activation of Lattice Oxygen and Molecular Oxygen on Dual-Defect LaMnO₃

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Environmental Science and Technology 2025年 2025 May 20页

作者： Qian, Zhen Yuan, Bo Sheng, Shiwei Lai, Fei Chen, Jianjun Mi, Jinxing Ma, Zhao Hao, Runlong Li, Junhua Wang, Lidong Hebei Key Lab of Power Plant Flue Gas Multi-Pollutants Control Department of Environmental Science and Engineering North China Electric Power University Baoding 071003 China State Key Joint Laboratory of Environment Simulation and Pollution Control School of Environment Tsinghua University Beijing 100084 China MOE Key Laboratory of Resources and Environmental Systems Optimization College of Environmental Science and Engineering North China Electric Power University Beijing 102206 China

Inhibiting the deposition of N species on the catalyst surface for the targeted oxidation of NO to NO2 is still a great challenge. Herein, a La and O dual-defective LaMnO3 (2U-L0.8MO) perovskite was fabricated using a... 详细信息

Inhibiting the deposition of N species on the catalyst surface for the targeted oxidation of NO to NO₂ is still a great challenge. Herein, a La and O dual-defective LaMnO₃ (2U-L_0.8MO) perovskite was fabricated using a urea-nonstoichiometric comodulation strategy, which achieved 97.6% NO oxidation efficiency at 210 °C and 300,000 h^-1, and was also capable of nearly 100% targeted oxidation of NO to NO₂, as well as exhibited excellent stability and recyclability. Characterizations and theoretical calculations unveiled that the urea-nonstoichiometric modulation method optimized the specific surface area and geometrical structure of perovskite, promoted the formation of La defects and oxygen vacancies (OVs), enhanced lattice oxygen activation and migration, and also facilitated the coadsorption of NO and O₂ and increased the d-band center of the perovskite. The synergistic activation of lattice oxygen and molecular oxygen along with the low-temperature oxidation mechanisms of NO was finally revealed: the comodulation strategy caused stretching and distortion of the 2U-L_0.8MO lattice, making its lattice oxygen susceptible to activation, thereby oxidizing adsorbed NO to NO₂ and simultaneously generating OVs. Afterward, O₂ would be captured by the abundant OVs on the 2U-L_0.8MO surface and converted to superoxide O₂^-, which could not only directly oxidize NO but also transform into single ¹O₂ on the adjacent Mn⁴⁺ site for the targeted oxidation of NO. This work realizes the coactivation of O₂ and lattice oxygen and also extends the understanding of the low-temperature-targeted oxidation of NO. © 2025 American Chemical Society.

关键词： cooperative activation LaMnO3 perovskite lattice oxygen activation low-temperature oxidation molecular oxygen activation targeted conversion of NO to NO2

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An Improved OPA Model in power System Considering Planning 33

An Improved OPA Model in Power System Considering Planning

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第三十三届中国控制会议

作者： GONG Yuan MEI Shengwei PENG Dong LONG Wangcheng GUO Mingxing Power Systems and Power Generation Equipment Control and Simulation National Key Laboratory Department of Electrical Engineering Tsinghua University State Power Economic Research Institute

ISBN: (纸本)9781479947249

The power system now is a typical complex system, which has inherent characteristics of SOC. Studying on cascading failures are necessary and meaningful to insure the grid's safety, national security and economic development. This paper firstly establishes the indices of power system development diagnosis, which are closely relevant to the trigger of power system evolution. Then a cascading failure model is proposed, considering planning and evolution of the power system. This model is based on OPA model, including both fast dynamics and slow dynamics. The slow dynamic process simulates the evolution of power system, which represents the functions of the planning department, while the fast dynamic process simulates power flow and cascading failures, which takes the effects of dispatch, relay protection and automation into consideration. Moreover, simulations are tested on the case of Kaifeng-Shangqiu power system in Henan Province of China, and evolution results are presented.

关键词： power system evolution,cascading failure,power system diagnosis,power grid complexity,OPA model

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Blackout Risk Analysis and control of power System Integrated with Wind Farm 28

Blackout Risk Analysis and Control of Power System Integrate...

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第28届中国控制与决策会议

作者： Zhong Yuxin Zhang Xuemin Mei Shengwei Xia Deming Wang Shuai Shi Rui Dept.of Electrical Engineering State Key Lab of Control and Simulation of Power Systems and Generation EquipmentsTsinghua University Northeast Branch of State Grid Corporation of China State Power Economic Research Institute

ISBN: (纸本)9781467397155

With the increase of wind power penetration,the characteristics of the wind farm have brought a significant impact on the security of power *** is urgent to study how to reduce the risk of cascading failures while improving the environmental *** this paper,a cascading failure model containing wind farm is proposed,which considers wind power characteristics,such as the structure of wind farm,the randomness of power of wind farm,the virtual inertia control of wind turbine,and the disconnection response of wind turbine after short-circuit *** order to identify the key factors of blackout,decision tree is used to analyze results generated from this blackout *** control is adopted to decrease the probability or effect of critical attributes that can be found in decision *** blackout risk of IEEE 30 test system integrated with wind farm is *** key factors,such as disconnection of wind turbines from the grid and certain transmission lines,are identified by decision ***,the effectiveness of the virtual inertial control of wind turbine,reactive power compensation and line construction is verified by simulation.

关键词： Wind Farm Disconnection of Wind Turbines Virtual Inertial control Blackout Risk Decision Tree

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A usage-based transmission cost allocation scheme considering impacts of DERs

A usage-based transmission cost allocation scheme considerin...

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2016 Tsinghua University-IET Electrical Engineering Academic Forum

作者： Wang, J.X. Zhong, H.W. Xia, Q. State Key Lab. of Control and Simulation of Power Systems and Generation Equipments Department of Electrical Engineering Tsinghua University Beijing China

ISBN: (纸本)9781785614170

With the rapid development of distributed energy resources (DERs), it is of vital importance to develop a well-designed transmission cost allocation scheme to reflect the contributions of DERs to the power system. In this paper, a usage-based transmission cost allocation scheme is proposed considering the capability of DERs. Based on the different intentions of transmission capacity, the transmission costs can be classified into four fractions: operating, contingency, planning and invalid transmission costs. On operating conditions, the transmission costs are identified and allocated according to the actual usage of consumers at each node. On contingency conditions, the transmission cost allocation will be influenced by the behaviors of DERs since DERs can provide emergent power support to help alleviate transmission congestion. On planning conditions, the transmission costs are useful in the future. The residual costs, i.e., the invalid transmission costs, should not allocated by consumers because this fraction is caused by the over investment of transmission owners. The case studies based on the IEEE 30-bus system validates the effectiveness of the proposed scheme and model. © 2016, Institution of Engineering and Technology. All rights reserved.

关键词： Investments

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Applications and Prospects of Online Insulation Monitoring Technique Based on Broadband Frequency Response for Transformers in Voltage Source Converter System 2nd

Applications and Prospects of Online Insulation Monitoring T...

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Conference Proceedings of 2022 2nd International Joint Conference on Energy, Electrical and power Engineering

作者： Lu, Geye Zheng, Dayong Zhang, Pinjia State Key Lab of Security Control and Simulation of Power Systems and Large Scale Generation Equipment Tsinghua University Beijing100084 China

ISBN: (纸本)9789819943333

power electronic converters are widely applied in new power system. Converter transformers have a critical risk in safe and reliable operation due to the insulation ageing. At present, conventional transformer insulation monitoring methods are limited to low sensitivity, invasive sensors and sophisticated evaluation. The goal of this paper is to improve the performance of online insulation monitoring for converter transformers based on broadband frequency response. The significance of application promotion, the disadvantages of existing methods and the challenges from offline to online implementation are clarified. A novel technique based on inherent harmonics in voltage source converter system is investigated, which provides the prospect in improving the online monitoring performance with high reliability and non-invasiveness nature. © 2023, The Author(s), under exclusive license to Springer Nature Singapore Pte Ltd.

关键词： Insulation

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Research and simulation on voltage stability control strategy for AC port of power electronic transformer 16

Research and simulation on voltage stability control strateg...

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16th IET International Conference on AC and DC power Transmission, ACDC 2020

作者： Shen, Yu Nie, Haozhe Cai, Weiqian Yuan, Liqiang Zhang, Chunpeng Zhao, Zhengming State Key Lab of Control and Simulation of Power Systems and Generation Equipment Department of Electrical Engineering Tsinghua University Beijing100084 China

ISBN: (纸本)9781839533914

With wide application of power electronic equipment in power system, voltage stability and power supply reliability need to be improved. In this paper, voltage sag caused by AC port load increase and the influencing factors are studies with a typical power electronic transformer topology as example. A calculation method which can estimate the port voltage sag performance according to the load impedance is proposed. In order to maintain the port voltage stability in the process of load increase, a voltage stability control strategy is proposed based on the double-loop control by increasing the voltage feedforward, which can improve the power supply quality and stability of power electronic transformer. Finally, the MATlab/Simulink simulation results show that the proposed scheme is accurate and effective. © 2020 Institution of Engineering and Technology. All rights reserved.

关键词： MATlab

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Evaluation of cascading failure in power system based on the operational reliability theory

Evaluation of cascading failure in power system based on the...

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2010 IEEE 11th International Conference on Probabilistic Methods Applied to power systems, PMAPS 2010

作者： Zou, Xin Cheng, Lin Sun, Yuanzhang Department of Electrical Engineering State Key Lab. of Control and Simulation of Power Systems and Generation Equipments Tsinghua University Beijing China

ISBN: (纸本)9781424457236

According to the characteristics of the cascading failures in power grid, a lot of assessment methods based on the probability theory have been proposed in recent years. However, most of them ignore the influence of the changing operating conditions on the power system planning and operation. This paper assesses the risk of the cascading failure in the power system based on the operational reliability theory which considering the variation of operating states and environment of the power system. The operational reliability of the power system is calculated based on Markov Process which describes the transient probability of states. The key conception of this theory is that the failure rate and the probability of components are changing along with the life of the equipment, the operating states and the environment conditions. A new evaluation procedure is brought up to calculate the operational reliability indices which can provide the specific information of the cascading failure. The evaluating results of the test system confirm that this approach is applicable to analyze the cascading failures in real power system. ©2010 IEEE.

关键词： Reliability theory

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Effects of temperature on creepage discharge characteristics in oil-impregnated pressboard insulation under combined AC–DC voltage

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Plasma Science and Technology 2019年第5期21卷 14-22页

作者： Fubao JIN Yuanxiang ZHOU Bin LIANG Zhongliu ZHOU Ling ZHANG Key Laboratory of Plateau Ecology and Agriculture College of Agriculture and Animal HusbandrySchool of Water Resources and Electric PowerQinghai UniversityXining 800016People's Republic of China State Key Lab of Control and Simulation of Power Systems and Generation Equipments Department of Electrical EngineeringTsinghua UniversityBeijing 100084People's Republic of China

Due to the complexity of the valve side winding voltage of the converter transformer, the insulation characteristics of the oil-impregnated pressboard(OIP) of the converter transformer are different from those of the traditional AC transformer. The study on effect of temperature on the creeping discharge characteristics of OIP under combined AC–DC voltage is seriously inadequate. Therefore, this paper investigates the characteristics of OIP creepage discharge under combined AC–DC voltage and discusses the influence of temperature on creepage discharge characteristics under different temperatures from 70 °C to 110 °C. The experimental results show that the partial discharge inception voltage and flashover voltage decrease with increasing temperature. The times of low amplitude discharge(LAD) decrease and amplitude of LAD increases. Simultaneously, the times of high amplitude discharge(HAD) gradually increase at each stage of creepage discharge with higher temperature. The analysis indicates that the charge carriers easily accumulate and quickly migrate directional movement along the electric field ahead of discharging. The residual charge carriers are more easily dissipated after *** ‘hump’ region of LAD moves to the direction of higher discharge magnitude. The interval time between two continuous discharges is shortened obviously. The concentration of HAD accelerates the development of OIP insulation creepage discharge. The temperature had an accelerating effect on the development of discharge in the OIP under applying voltage.

关键词： oil-impregnated pressboard insulation combined AC-DC voltage inception voltage creepage discharge temperature flashover voltage

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On engineering game theory with its application in power systems

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control Theory and Technology 2017年第1期15卷 1-12页

作者： Shengwei MEI Wei WEI Feng LIU Department of Electrical Engineering and Applied Electronics Technology Tsinghua Universily Beijing 100084 China State Key Laboratory of Control and Simulation of Power Systems and Generation Equipments Tsinghua University Beijing 100084 China

Due to its capability of solving decision-making problems involving multiple entities and objectives, as well as complex action sequences, game theory has been a basic mathematical tool of economists, politicians, and sociologists for decades. It helps them understand how strategic interactions impact rational decisions of individual players in competitive and uncertain environment, if each player aims to get the best payoff. This situation is ubiquitous in engineering practices. This paper streamlines the foundations of engineering game theory, which uses concepts, theories and methodologies to guide the resolution of engineering design, operation, and control problems in a more canonical and systematic way. An overview of its application in smart grid technologies and power systems related topics is presented, and intriguing research directions are also envisioned.

关键词： Decision making engineering game theory power system smart grid technology

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Steady-state security analysis of power system based on the operational reliability theory 3

Steady-state security analysis of power system based on the ...

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3rd International Conference on Reliability of Electrical Products and Electrical Contacts, ICREPEC 2009

作者： Zou, Xin Cheng, Lin Sun, Yuanzhang Department of Electrical Engineering State Key Lab of Control and Simulation of Power Systems and Generation Equipments Tsinghua University Beijing100084 China

ISBN: (纸本)9789889968489

Conventional steady-state security analysis have to compute the faults belonging to the predefined faults set in turn with out considering the small probability of the occurrence of some faults under certain circumstances. Although its results reflect the violation of the components precisely, they can not figure out how the violation affects the security of the system. The steady-state security analysis based on the operational reliability theory applies the state-depended models of the components in order to find the faults which would happen with high probability. As a result, only these faults should be calculated to decrease the computation time considerably. Further more, the reliability indices indicate the probability of the violation of the component as well as the influence of the violation on the system security, so that the security of the system can be evaluated comprehensively. IEEE RTS-79 test system is adopted in this paper to illustrate the differences between the conventional and the new steady-state security analysis methods. By contrast, it can be concluded that steady-state security analysis based on the operational reliability theory can calculate the influence of the variation of the component failure probability on the system security more specifically, which making the evaluation results more close to the practical operating system Copyright © 2009 by International Academic Publishers Ltd.

关键词： Reliability theory

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