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Development in the application of laser-induced breakdown spectroscopy in recent years:A review

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Frontiers of physics 2021年第2期16卷 45-69页

作者： Lian-Bo Guo Deng Zhang Lan-Xiang Sun Shun-Chun Yao Lei Zhang Zhen-Zhen Wang Qian-Qian Wang Hong-Bin Ding Yuan Lu Zong-Yu Hou Zhe Wang Wuhan National Laboratory for Optoelectronics(WNLO) Huazhong University of Science and TechnologyWuhan 430074China State Key Laboratory of Robotics Shenyang Institute of AutomationChinese Academy of SciencesSheyang 110016China School of Electric Power South China University of TechnologyGuangzhou 510640China State Key Laboratory of Quantum Optics and Quantum Optics Devices Institute of Laser SpectroscopyShanxi UniversityTaiyuan 030006China State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong UniversityXi'an 710049China Key Laboratory of Photonic Information Technology School of Optics and PhotonicsBeijing Institute of TechnologyBeijing 100081China School of Physics Dalian University of TechnologyNo.2 Linggong RoadGanjingzi DistrictDalian 116024China Optics and Optoelectronics Laboratory Ocean University of ChinaQingdao 266100China State Key Lab of Power Systems Department of Energy and Power EngineeringTsinghua UniversityBeijing 100084China

Laser-induced breakdown spectroscopy(LIBS)has been widely studied due to its unique advantages such as remote sensing,real-time multi-elemental detection and none-to-little *** the efforts of researchers around the world,LIBS has been developed by leaps and ***,in recent years,more and more Chinese LIBS researchers have put tremendous energy in promoting LIBS *** is worth mentioning that the application of LIBS in a specific field has its special application background and technical difficulties,therefore it may develop in different stages.A review summarizing the current development status of LIBS in various fields would be helpful for the development of LIBS technology as well as its applications especially for Chinese LIBS community since most of the researchers in this field work in *** the present work,we summarized the research status and latest progress of main research groups in coal,metallurgy,and water,*** on the current research status,the challenges and opportunities of LIBS were evaluated,and suggestions were made to further promote LIBS applications.

关键词： laser-induced breakdown spectroscopy application

Numerical Study on the Impact Characteristics of a Single Molten Lead Bismuth Droplet on Water

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SSRN 2024年

作者： Lin, Yue Zhang, Dalin Chen, Yutong Zhang, Xisi Deng, Jian Du, Peng Tian, Wenxi Qiu, Suizheng Su, Guanghui Department of Nuclear Science and Technology State Key Lab. of Multiphase Flow in Power Engineering Shaanxi Key Lab. of Advanced Nuclear Energy and Technology Xi’an Jiaotong University No.28 Xianningxilu Beilinqu Shaanxi Xi’an710049 China Institute of Reactor Engineering Technology China Institute of Atomic Energy Beijing102413 China Science and Technology on Reactor System Design Technology Laboratory Nuclear Power Institute of China Sichuan Chengdu610213 China

As an important link in the possible occurrence of steam explosions, the interaction between molten materials and coolant is of great significance for safety analysis in severe accidents of nuclear reactors. This study is based on the two-dimensional multiphase and multi-component fluid dynamics code ACENA to model the process of single molten lead bismuth droplet impacting a water tank and obtain the velocity changes of the molten droplet as it moves through the water tank. Furthermore, a sensitivity analysis of relevant factors such as the heat transfer area fraction and drag coefficient of the droplet is carried out. To verify models in ACENA, the computation results are compared to experimental data. It is demonstrated that the overall trend of the velocity curve acquired by the ACENA code during the interaction between a molten lead bismuth droplet and water is consistent with the experimental results. The droplet falling velocity increases with the increase in droplet temperature when the temperature of water is the same, and the droplet falling velocity increases with the increase of water temperature at the same droplet temperature. The simulation results by ACENA code for MFCI are in good agreement with experiments which verifies the accuracy of relevant models in ACENA. It can provide an effective means for safety analysis of nuclear reactors in China. © 2024, The Authors. All rights reserved.

关键词： Drops

Numerical Study on Thermal-Hydraulic Characteristics of Lead-Bismuth Loop System Under Moving Conditions

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SSRN 2022年

作者： Yuan, Lanfei Wang, Chenglong Liu, Zhipeng Tian, Wenxi Qiu, Suizheng Su, G.H. Department of Nuclear Science and Technology State Key Lab. of Multiphase Flow in Power Engineering Shaanxi Key Lab. of Advanced Nuclear Energy and Technology Xi’an Jiaotong University Shaanxi Xi'An710049 China

The investigation of flow and heat transfer of lead-bismuth eutectic (LBE) under moving conditions is vital to the design optimization of LBE loop system in offshore engineering. In this paper, the calculation model of lead-bismuth loop system and the calculation method of moving conditions are developed by using commercial CFD software, and experiments were carried out to verify the numerical results. The calculation results demonstrate that the moving conditions will cause periodic fluctuations in the natural circulation flow rate of the loop system. The period of the flow rate fluctuation is consistent with the motion period, and the amplitude of the fluctuation will increase with the increase of the maximum range of motion and the decrease of the motion period. When the maximum heaving amplitude is 0.3m and the period is 8s, the instantaneous fluctuation of the flow rate reaches a maximum of 0.8%, and the reverse flow phenomenon occurs under rolling motion. Rolling and heaving motion also make heat transfer characteristic parameters of the system have periodic instantaneous fluctuation. The maximum instantaneous fluctuation of Nu number reaches 4.63%, and the maximum time average Nu can reach -2.15% under heaving motion of 0.3m-8s. In addition, the influence of rolling on system parameters is more severe than that of heaving. These results obtained in this study have important engineering application value for the design of LBE loop system under moving conditions. © 2022, The Authors. All rights reserved.

关键词： Computational fluid dynamics

Experimental Study on Thermoelectric Characteristics of Heat Pipe Reactor (Nuster-100) Single Assembly

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SSRN 2022年

作者： Yang, Haiwang Wang, Chenglong Tian, Wenxi Qiu, Suizheng Su, Guanghui H. Department of Nuclear Science and Technology State Key Lab. of Multiphase Flow in Power Engineering Shaanxi Key Lab. of Advanced Nuclear Energy and Technology Xi’an Jiaotong University Shaanxi Xi’an710049 China

The heat pipe cooled reactor has the advantages of miniaturization,modularization and high inherent safety,having broad application prospects in the fields of national defense and military,space exploration and energy supply in remote *** this paper, a heat pipe-thermoelectric generator integrated experimental device similar to the heat pipe cooled reactor (NUSTER-100) Single Assembly is *** heat transfer performance of sodium heat pipe and thermoelectric performance of Half-Heusler thermoelectric generator are *** results show that after the sodium heat pipe is started,the axial temperature difference of the heat pipe is 85°C,the equivalent heat transfer coefficient is 40886W/K·m,which can provide stable heat to the thermoelectric *** performance parameters of thermoelectric generator such as open voltage,output power increase with the hot side temperature *** maximum thermoelectric conversion efficiency of single thermoelectric generator reaches 7.2%,but the efficiency of integrated experimental device is only 3.5%. © 2022, The Authors. All rights reserved.

关键词： Heat pipes

Degradation of Polystyrene to Aromatic Oils with Nio@C Catalyst in Supercritical Co2

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SSRN 2024年

作者： Liu, Yanbing Mao, Liuhao Kang, Xing Li, Yi Zhao, Qiuyang Jin, Hui Meng, Wei Shi, Jinwen Guo, Liejin International Research Center for Renewable Energy State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong University 28 West Xianning Road Shaanxi Xi’an710049 China Hunan Provincial Key Lab of Dark Tea and Jin-Hua Departmet of Material & Chemical Engineering Hunan City University 518 East Yingbin Road Hunan Yiyang413000 China

One of the most promising ways to dispose of plastic pollution in the future is chemical recycling of plastic, and in particular supercritical fluids with excellent fluidity and transferability have shown great attraction in the disposal of plastic. Herein, catalytic degradation of polystyrene (PS) plastic in supercritical carbon dioxide (Sc-CO2) was realized with high yield of aromatic oils. NiO with simple preparation process, and high catalytic activity and stability in Sc-CO2 was doped with carbon material to prepare NiO@C catalyst with improved catalytic performance. Compared with NiO, NiO@C catalyst had rich porous structure and strong acidic sites, resulting in higher catalytic activity. The NiO@C catalyzed degradation of PS in Sc-CO2 yielded aromatic oils as high as 89.3 ± 0.6 wt% at 300oC with a reaction time of 2 h and a catalyst loading amount of 10 wt%. Moreover, the NiO@C catalyst degraded PS in Sc-CO2 for three cycles without obvious change in the catalytic performance. Sc-CO2 not only played a favorable role in swelling PS, but also inhibited the formation of coke, beneficial for the degradation of PS. Furthermore, CO2 was be consumed as an oxidant to generate new products and reduce greenhouse gas emission. The highly efficient catalytic conversion of PS to aromatic oils in Sc-CO2 via NiO@C catalyst provides a potential route for simultaneously recycling plastic and sequestering carbon. © 2024, The Authors. All rights reserved.

关键词： Carbon dioxide

Sacos-Plate: A New Thermal-Hydraulic Subchannel Analysis Code for Plate Type Fuel Assemblies

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SSRN 2023年

作者： Sun, Ruiyu Wang, Jianjun Wang, Jinshun Chen, Ronghua Jiang, Xing Tian, Wenxi Qiu, Suizheng Su, Guanghui Gui, Minyang Harbin Engineering University China School of Nuclear Science and Technology Xi’an Jiaotong University Shaanxi Xi’an710049 China Shaanxi Key Lab. of Advanced Nuclear Energy and Technology Xi’an Jiaotong University China State Key Lab. of Multiphase Flow in Power Engineering Xi’an Jiaotong University China Shanghai Nuclear Engineering Research Design Institute Shanghai China

Over the past few decades, plate-type fuel elements have been widely used in advanced research reactors, small modular pressurized water reactors, production reactors, etc., with the advantages of compact structure arrangement, good heat transfer characteristics and high fuel consumption. Currently, a thermal-hydraulic subchannel analysis code, namely SACOS-PLATE code, was newly designed to satisfy the calculation of different types of plate fuel elements under various steady-state operating conditions. Based on the original SACOS code, this updated version modifies the flow distribution model, the plate heat conduction model, the heat distribution model as well as the flow heat transfer model, and then realizes the simulation of the special thermal-hydraulic phenomena of the fuel and the rectangular flow channel. In this present study, the RA-6 experimental data was used to validate the code, and the simulation calculation was performed on the JRR-3 research reactor, which proved the good computing capability of SACOS-PLATE code. © 2023, The Authors. All rights reserved.

关键词： Plates (structural components)

Constructing electron transport channel of SnO2/BaSO4 on g-C3N4 for enhanced visible-light-driven photocatalytic H2 production

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Materials Today Catalysis

Materials Today Catalysis 2025年 9卷

作者： Dong, Gongyue Guo, Xiaojuan Cheng, Cheng Chen, Feng Zhang, Jinfeng Du, Yanping Meng, Wei Liu, Maochang Shi, Jinwen International Research Center for Renewable Energy State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong University Xi'an710049 China Guangdong Provincial Key Laboratory of Multi-energy Complementary Distributed Energy Systems Dongguan University of Technology Dongguan523808 China School of Engineering Lancaster University LancasterLA1 4YW United Kingdom Gansu Company PipeChina Lanzhou730060 China Hunan Provincial Key Lab of Dark Tea and Jin-Hua Department of Material & Chemical Engineering Hunan City University Yiyang413000 China

Graphitic carbon nitride (g-C3N4) is confronted with the issue of poor utilization of photogenerated charge carriers, thereby leading to limited performance of photocatalytic hydrogen (H2) production, which restricts its potential application. Herein, the electron transport material SnO2/BaSO4 was synthesized to integrate with g-C3N4 for addressing the above problem. Various characterizations were conducted to investigate the g-C3N4-SnO2/BaSO4 photocatalyst, and it demonstrated that photogenerated electrons from g-C3N4 expeditiously migrate to SnO2/BaSO4 nanoparticles, which markedly hindered photogenerated carriers’ recombination. Subsequently, the g-C3N4-SnO2/BaSO4 photocatalyst demonstrated promoted photocatalytic H2 production at a rate of 14.2 μmol h−1 under visible-light illumination, which was 2.5 times higher than that of pristine g-C3N4. © 2025 The Authors

关键词： Barium sulfate

flow Fluctuations and flow Friction Characteristics of Lead-Bismuth Eutectic in a Vertical Tube Under Rolling Conditions

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SSRN 2022年

作者： Liu, Zhipeng Zhao, Yafeng Tian, Wenxi Wang, Chenglong Qiu, Suizheng Su, Guanghui H. School of Nuclear Science and Technology Shaanxi Key Lab. of Advanced Nuclear Energy and Technology Xi’an Jiaotong University Shaanxi Xi’an710049 China State Key Laboratory of Multiphase Flow in Power Engineering China

The effects of rolling motion on the flow characteristics of lead-bismuth eutectic in a vertical circular tube are investigated experimentally. The results show that the pressure drop and flow rate of the forced LBE circulation fluctuate under rolling conditions. The effect of rolling motion on the flow characteristics decreases with the increase of the corresponding static Reynolds number. The rolling motion may increase the time-averaged frictional resistance coefficient of the LBE when flow rate is low. The critical value of the impact Reynolds number is about 125,000. As a result, the time-averaged flow rate decreases. The analysis shows that it is mainly the transverse additional force caused by the rolling motion increases the frictional resistance of the LBE. An empirical correlation is established to predict the frictional resistance coefficient under rolling conditions. This study may be useful in the thermal-hydraulic analysis of LBE as a working fluid under moving conditions. © 2022, The Authors. All rights reserved.

关键词： Reynolds number

Steady-state Multi-Physics Coupling Analysis of Heat Pipe Cooled Reactor Core

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SSRN 2022年

作者： Zhang, Zhipeng Wang, Chenglong Guo, Kailun Tian, Wenxi Qiu, Suizheng Su, Guanghui Department of Nuclear Science and Technology Shaanxi Key Lab. of Advanced Nuclear Energy and Technology Xi’an Jiaotong University Shaanxi Xi’an710049 China State Key Laboratory of Multiphase Flow in Power Engineering China

Due to the advantages of mobility, safety and universality, the heat pipe reactors have great competitiveness in many applications such as strategic defense locations, remote communities, and emergency locations. In addition, most of the heat pipe reactors are designed as solid-state reactors, which avoid the two-phase flow problem caused by the coolant transformation and make it possible to analyze the reactor with multiple physical field coupling. In this work, a typical heat pipe reactor has been carried out a 3-D neutronic-thermal-mechanical analysis, and steady state analysis is performed by OpenMC coupled with COMSOL. Coupling calculation results show that under normal operation, the maximum temperature and thermal expansion of core is 1338.94 K and 2.53 mm. In the steady-state coupling process, the influence of temperature parameters on physical calculation is mainly reflected in k eff and its power level, the maximum temperature drops from 1347.26 K to 1338.94 K, but it has little influence on power distribution. By coupling calculations, the maximum stress of the reactor is reduced by 5.78 MPa. The research results will support the subsequent development of multi-physics coupled transient analysis code for heat pipe reactors. © 2022, The Authors. All rights reserved.

关键词： Heat pipes