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The rise of intelligent fabric agent from mass-produced advanced fiber materials

Science Bulletin 2024年第23期69卷 3644-3647页

作者： Pan Li Maiping Yang Yueheng Liu Jing Zhang Sisi He Cuiwei Yang Weizhong Yang Xinyuan Cai Liping Zhu Shenglin Ye Hongyu Sun Chong Hou Ning Zhou Meifang Zhu Guangming Tao Wuhan National Laboratory for Optoelectronics Huazhong University of Science and TechnologyWuhan 430074China School of Mechanical Engineering and Electronic Information China University of Geosciences(Wuhan)Wuhan 430074China Shenzhen Key Laboratory of Flexible Printed Electronics Technology School of ScienceHarbin Institute of TechnologyShenzhen 518055China Department of Biomedical Engineering School of Information Science and TechnologyFudan UniversityShanghai 200433China Shanghai Different Advanced Material Co. Ltd.Shanghai 201502China School of Architecture and Urban Planning Huazhong University of Science and TechnologyWuhan 430074China State Key Laboratory for Modification of Chemical Fibers and Polymer Materials College of Materials Science and EngineeringDonghua UniversityShanghai 201620China Meta Reality Lab Meta PlatformsInc.SunnyvaleCA 94089USA School of Nursing Peking UniversityBeijing 100191China School of Optical and Electronic Information Huazhong University of Science and TechnologyWuhan 430074China Department of Cardiology Beijing Anzhen HospitalCapital Medical UniversityNational Clinical Research Center for Cardiovascular DiseasesBeijing 100029China Key Laboratory of Vascular Aging Ministry of EducationTongji Hospital Tongji Medical CollegeHuazhong University of Science and TechnologyWuhan 430030China State Key Laboratory of Material Processing and Die&Mould Technology School of Materials Science and EngineeringHuazhong University of Science and TechnologyWuhan 430074China School of Physical Education Huazhong University of Science and TechnologyWuhan 430074China

Artificial intelligence(AI)is crucial in driving scientific,technological,and industrial advancements,and it has given rise to an ambient intelligence that can potentially improve the physical execution of healthcare delivery[1,2].Among diverse advanced AI technologies,an intelligent agent with multi-parameter perception,decision-making,and execution capabilities demonstrates the potential for facilitating the development of next-generation optoelectronic *** intelligent agent is a physical or abstract entity that acts autonomously,perceives and interacts with its environment,and communicates with other agents[3].It could perceive dynamic environmental conditions,execute actions,and make appropriate *** emerges as an ideal carrier for human-centered intelligent agents,providing various properties such as perceptibility,adaptability,and *** fabric,known for its unique functionality,has attracted considerable attention from academia and *** 2014,Germany proposed a national strategy called FutureTEX to upgrade the entire textile industry by promoting integration between textiles and other *** years later,the United states announced the establishment of the Revolutionary Fibers and Textiles Manufacturing Innovation Institute,which intends to accelerate the revival of fabric *** with conventional fibers,revolutionary fibers focus on the design of multiple materials and structures,enabling the integration of various functionalities into a single *** in the United states,the advent of the digital revolution,advancements in Internet of Things technology,and mature fiber technology significantly boost the development of the intelligent fiber *** commercial applications of intelligent fibers are gradually *** Jacquard,a collab.rative effort by Google and Levi’s,presents an intelligent jacket that combines the washability and texture of standard fabrics with the

关键词： agent execution fiber

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二维材料最新研究进展

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物理化学学报 2021年第12期37卷 1-151页

作者：常诚陈伟陈也陈永华陈雨丁峰樊春海范红金范战西龚成宫勇吉何其远洪勋胡晟胡伟达黄维黄元季威李德慧李连忠李强林立凌崇益刘鸣华刘楠刘庄 Kian Ping Loh 马建民缪峰彭海琳邵明飞宋礼苏邵孙硕谭超良唐智勇王定胜王欢王金兰王欣王欣然 Andrew T.S.Wee 魏钟鸣吴宇恩吴忠帅熊杰熊启华徐伟高尹鹏曾海波曾志远翟天佑张晗张辉张其春张铁锐张翔赵立东赵美廷赵伟杰赵运宣周凯歌周兴周喻朱宏伟张华刘忠范 Institute of Science and Technology Austria Am Campus 13400 KlosterneuburgAustria Department of Chemistry National University of Singapore3 Science Drive 3117543Singapore Department of Chemistry The Chinese University of Hong KongShatinNew TerritoriesHong KongChina Key Laboratory of Flexible Electronics and Institute of Advanced Materials Nanjing Tech UniversityNanjing 211816China School of Life Sciences Shanghai UniversityShanghai 200444China Centre for Multidimensional Carbon Materials Institute for Basic ScienceUlsan 44919Korea School of Chemistry and Chemical Engineering Shanghai Jiao Tong UniversityShanghai 200240China School of Physical and Mathematical Sciences Nanyang Technological UniversitySingapore 637371Singapore Department of Chemistry City University of Hong KongKowloonHong KongChina Department of Electrical and Computer Engineering and Quantum Technology Center University of MarylandCollege ParkMaryland 20742USA School of Materials Science and Engineering Beihang UniversityBeijing 100191China Department of Materials Science and Engineering City University of Hong KongKowloonHong KongChina Center of Advanced Nanocatalysis(CAN) Hefei National Laboratory for Physical Sciences at the MicroscaleDepartment of Applied ChemistryUniversity of Science and Technology of ChinaHefei 230026China College of Chemistry and Chemical Engineering State Key Laboratory of Physical Chemistry of Solid SurfacesCollaborative Innovation Center of Chemistry for Energy Materials(iChEM)Xiamen UniversityXiamen361005Fujian ProvinceChina State Key Laboratory of Infrared Physics Shanghai Institute of Technical PhysicsChinese Academy of SciencesShanghai 200083China Advanced Research Institute of Multidisciplinary Science Beijing Institute of TechnologyBeijing100081China Beijing Key Laboratory of Optoelectronic Functional Materials&Micro-Nano Devices Department of PhysicsRenmin University of ChinaBeijing 100872China School of Optical and Electronic Information Wuhan National Laboratory

Research on two-dimensional(2D) materials has been explosively increasing in last seventeen years in varying subjects including condensed matter physics, electronic engineering, materials science, and chemistry since the mechanical exfoliation of graphene in 2004. Starting from graphene, 2D materials now have become a big family with numerous members and diverse categories. The unique structural features and physicochemical properties of 2D materials make them one class of the most appealing candidates for a wide range of potential applications. In particular, we have seen some major breakthroughs made in the field of 2D materials in last five years not only in developing novel synthetic methods and exploring new structures/properties but also in identifying innovative applications and pushing forward commercialisation. In this review, we provide a critical summary on the recent progress made in the field of 2D materials with a particular focus on last five years. After a brief backgroundintroduction, we first discuss the major synthetic methods for 2D materials, including the mechanical exfoliation, liquid exfoliation, vapor phase deposition, and wet-chemical synthesis as well as phase engineering of 2D materials belonging to the field of phase engineering of nanomaterials(PEN). We then introduce the superconducting/optical/magnetic properties and chirality of 2D materials along with newly emerging magic angle 2D superlattices. Following that, the promising applications of 2D materials in electronics, optoelectronics, catalysis, energy storage, solar cells, biomedicine, sensors, environments, etc. are described sequentially. Thereafter, we present the theoretic calculations and simulations of 2D materials. Finally, after concluding the current progress, we provide some personal discussions on the existing challenges and future outlooks in this rapidly developing field.

关键词： Two-dimensional materials Transition metal dichalcogenides Phase engineering of nanomaterials Electronics Optoelectronics Catalysis Energy storage and conversion

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Removal: “Ultra-Simple synthesis of Ordered Mesoporous γ-Alumina: High Thermal Stability and Catalytic Activity”

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European Journal of Inorganic Chemistry 2007年第35期2007卷 5605-5605页

作者： Le-Yue Li Quan Yuan Lei Liao Chun-Hua Yan Jun Chen State Key Lab of Advanced Technology for Materials Synthesis and Processing Department of Chemistry Wuhan University Wuhan 430070 China Fax: +86-27-68754112 Beijing National Laboratory for Molecular Sciences State Key Lab of Rare Earth Materials Chemistry and Applications & PKU-HKU Joint Lab in Rare Earth Materials and Bioinorganic Chemistry Peking University Beijing China

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A C156 Molecular Nanocarbon: Planar/Rippled Nanosheets Hybridization

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Angewandte Chemie 2024年第6期137卷

作者： Ruihua Fu Xingyu Chen Fei Qiu Xinyue Liu Prof. Jianlong Xia Prof. Lei Zhang Beijing Advanced Innovation Center for Soft Matter Science and Engineering State Key Lab of Organic-Inorganic Composites Beijing University of Chemical Technology 100029 Beijing P. R. China State Key Laboratory of Advanced Technology for Materials Synthesis and Processing Center of Smart Materials and Devices Wuhan University of Technology 430070 Wuhan P. R. China

A novel hybrid nanocarbon consisting of one rippled and two planar nanosheets has been synthesized and characterized. Two meso pairs of [5]helicenes are formed along the long molecular axis of the hybrid to connect rippled and planar subunits, leading to a stable conformation. It is shown that the hybrid possesses the individual electronic properties of the rippled and planar subunits. Compared to the rippled subunit, such hybrid has a better geometric match to C 60 and complexes with C 60 in a 1 : 1 stoichiometry, with the association constant on the order of 10 5 M −1 . The hybrid displays unusual anti -Kasha fluorescence emission. The transient absorption spectroscopy revealed that the singlet fission (SF) from higher level singlet excited states (S n ) is operative in the film of the hybrid.

关键词： nanocarbon hybridization nanosheet supramolecular complexation transient absorption

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Front Cover: 3D Nitrogen-Doped Graphene Encapsulated Metallic Nickel–Iron Alloy Nanoparticles for Efficient Bifunctional Oxygen Electrocatalysis (Chem. Eur. J. 18/2020)

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Chemistry – A European Journal 2020年第18期26卷 3894-3894页

作者： Zhaoyang Wang Xiaobin Liao Zifeng Lin Prof. Fuzhi Huang Yalong Jiang Kwadwo Asare Owusu Prof. Lin Xu Ziang Liu Dr. Jiantao Li Prof. Yan Zhao Prof. Yi-Bing Cheng Prof. Liqiang Mai State Key Laboratory of Advanced Technology for Materials Synthesis and Processing State Key Laboratory of Silicate Materials for Architectures Wuhan University of Technology Wuhan 430070 P. R. China ARC Centre of Excellence in Exciton Science Monash University Clayton Victoria 3800 Australia

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H2-free Semi-hydrogenation of Butadiene by the Atomic Sieving Effect of Pd Membrane with Tree-like Pd Dendrites Array

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Angewandte Chemie (International ed. in English) 2023年第38期62卷 e202309013页

作者： Yong-Qin Yan Zhao Wei Zhao Wang Yao Li Wei-Hao Wang Bo Jiang Bao-Lian Su Wuhan University of Technology - Mafangshan Campus: Wuhan University of Technology State Key Laboratory of Advanced technology for Materials Synthesis and Processing Luoshi Road 122 Wuhan 430070 Wuhan CHINA. Wuhan University of Technology - Mafangshan Campus: Wuhan University of Technology State Key Laboratory of Advanced technology for Materials Synthesis and Processing Luoshi Road 122 430070 Wuhan CHINA. University of Namur: Universite de Namur Chemistry 61 rue de Bruxelles 5000 Namur BELGIUM.

H2-free semi-hydrogenation at room temperature shows great advantage for replacing the thermocatalytic process in industry owing to the high energy and resource saving, however, remains great challenges. Herein, a tree-like Pd dendrites array decorated Pd membrane was constructed as the core device in an electrochemistry assisted gas-fed membrane reactor for butadiene semi-hydrogenation. It reveals that hydrogen atomic sieving effect of this Pd-based membrane under electrochemical condition was the key for semi-hydrogenation. The configuration study of Pd nanostructured membrane demonstrates that the penetration of hydrogen atoms through Pd membrane from electrochemical side to chemical side is affected by the consumption of hydrogen atom in semi-hydrogenation step. Such atomic sieving property of nanostructured Pd membrane with 5.1 times increase in catalytic active surface area brings above 14 times higher in butadiene conversion than that of bare Pd foil, with ~90% of butenes selectivity at butadiene conversion ~98% over 300h of H2-free reaction under 15 mA cm-2.

关键词： 1,3-Butadiene Pd Membrane Semi-Hydrogenation Unsaturated Hydrocarbons Water Electrolysis

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Yolk–shell vanadium pentoxide integrated electrode for high-performance stretchable lithium metal battery

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Journal of Energy Storage 2024年 98卷

作者： Nathan, Muthu Gnana Theresa Yeon, Seon-Young Lee, Jae Seob Jo, Min Su Hwang, Gil Chan Kim, Hong-Il Wu, Fanglin Kim, Guk-Tae Liu, Ying Kim, Jin-Hee Cho, Jung Sang Kim, Jae-Kwang Department of Energy Convergence Engineering Cheongju University 258 Daeseong-ro Chungbuk Cheongju28503 Korea Republic of Department of Engineering Chemistry Chungbuk National University Chungbuk 28644 Korea Republic of Department of Earth System Sciences Yonsei University Seoul03722 Korea Republic of State Key Laboratory of Advanced Technology for Materials Synthesis and Processing Wuhan University of Technology Wuhan430070 China Department of Biomedical Laboratory Science College of Health Science Cheongju University Chungbuk Cheongju28503 Korea Republic of Biomedical Research Institute Chungbuk National University Hospital Chungbuk 361-763 28644 Korea Republic of

Vanadium pentoxide (V2O5) stands out as a preferred cathode material for stretchable lithium-ion batteries due to its high specific capacity, robust structural stability, cost-effectiveness, and ease of synthesis. However, its practical application is limited by a low Li+ diffusion coefficient (10−12–10−13 cm2 s−1) and poor electrical conductivity. To address these challenges, we have developed an innovative yolk-shell V2O5 architecture using a facile synthesis method involving spray pyrolysis followed by thermal treatment. This yolk-shell V2O5 is coated with a poly(ethylene oxide) (PEO) electrolyte to enhance ion transport contact areas and flexibility. The yolk-shell V2O5@PEO is then integrated with a PEO-based polymer electrolyte in a thin film configuration, paired with zig-zag truncated lithium metal anodes for stretchable lithium metal batteries. The integrated film demonstrates superior electrochemical performance due to highly reversible Li+ insertion/extraction and enhanced Li ion diffusion. The unique design of the stretchable Li-yolk-shell V2O5@PEO battery achieves an excellent specific discharge capacity of 261 mAh g−1, compared to 158 mAh g−1 for pure V2O5 at 0.1C. Additionally, the stretchable Li-yolk-shell V2O5@PEO cell exhibits a discharge capacity of 250 mAh g−1 under zero-strain conditions and 233.7 mAh g−1 under 40 % strain at 0.1C and 40 °C. Characterization through X-ray diffraction (XRD) and scanning electron microscopy (SEM) confirms the nano-sized morphology and high crystallinity of the yolk-shell V2O5. X-ray photoelectron spectroscopy (XPS) analysis reveals the transformation of yolk-shell V2O5@PEO into α-V2O5, Ε-Li0.5V2O5, δ-LiV2O5, and γ-Li2V2O5 phases during lithium-ion (de)intercalation. This cutting-edge battery design paves the way for the development of high-performance, stretchable, and flexible batteries, ideal for next-generation portable electronic devices. © 2024 Elsevier Ltd

关键词： Scanning electron microscopy

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Activation of subnanometric Pt on Cu-modified CeO2 via redox-coupled atomic layer deposition for CO oxidation (vol 11, 4240, 2020)

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NATURE COMMUNICATIONS 2020年第1期11卷 4240-4240页

作者： Liu, Xiao Jia, Shuangfeng Yang, Ming Tang, Yuanting Wen, Yanwei Chu, Shengqi Wang, Jianbo Shan, Bin Chen, Rong State Key Laboratory of Digital Manufacturing Equipment and Technology School of Mechanical Science and Engineering Huazhong University of Science and Technology 430074 Wuhan Hubei People’s Republic of China State Key Laboratory of Materials Processing and Die and Mould Technology School of Materials Science and Engineering Huazhong University of Science and Technology 430074 Wuhan Hubei People’s Republic of China School of Physics and Technology Center for Electron Microscopy MOE Key Laboratory of Artificial Micro- and Nano-structures and Institute for Advanced Studies Wuhan University 430072 Wuhan Hubei People’s Republic of China General Motors Global Research and Development Chemical Sciences and Materials Systems Lab 3500 Mound Road Warren Michigan 48090 USA Institute of High Energy Physics Chinese Academy of Sciences 100049 Beijing People’s Republic of China Present Address: Department of Chemical and Biomolecular Engineering Clemson University Clemson South Carolina 29634 USA

A Correction to this paper has been published: 10.1038/s41467-020-19663-3.

关键词： Heterogeneous catalysis Pollution remediation materials for energy and catalysis synthesis and processing

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Testing statistical isotropy in cosmic microwave background polarization maps

arXiv

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arXiv 2017年

作者： Rath, Pranati K. Samal, Pramoda Kr. Panda, Srikanta Mishra, Debesh D. Aluri, Pavan K. Institute of High Energy Physics Chinese Academy of Sciences Beijing100049 China Theoretical Physics Center for Science Facilities Chinese Academy of Sciences Beijing100049 China Department of Physics Utkal University Bhubaneswar Odisha751004 India State Key Laboratory of Advanced Technology for Materials Synthesis and Processing Wuhan University of Technology Wuhan430070 China Korea Institute for Advanced Study Quantum Universe Center 85 Hoegi-ro Dongdaemun-gu Seoul02455 Korea Republic of Korea Astronomy and Space Science Institute 776 Daedeokdae-ro Yuseong-gu Daejeon305348 Korea Republic of

We apply our symmetry based Power tensor technique to test conformity of PLANCK Polarization maps with statistical isotropy. On a wide range of angular scales (l = 40 − 150), our preliminary analysis detects many statistically anisotropic multipoles in foreground cleaned full sky PLANCK polarization maps viz., COMMANDER and NILC. We also study the effect of residual foregrounds that may still be present in the galactic plane using both common UPB77 polarization mask, as well as the individual component separation method specific polarization masks. However some of the statistically anisotropic modes still persist, albeit significantly in NILC map. We further probed the data for any coherent alignments across multipoles in several bins from the chosen multipole range. Copyright © 2017, The Authors. All rights reserved.

关键词： Polarization

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Revealing the Interfacial Chemistry of Fluoride Alkyl Magnesium Salts in Magnesium Metal Batteries

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Angewandte Chemie 2023年第21期135卷

作者： Juncai Long Dr. Shuangshuang Tan Junjun Wang Dr. Fangyu Xiong Lianmeng Cui Prof. Qinyou An Prof. Liqiang Mai State Key Laboratory of Advanced Technology for Materials Synthesis and Processing Wuhan University of Technology Wuhan 430070 China College of Materials Science and Engineering Chongqing University Chongqing 400030 China Wuhan University of Technology (Xiangyang Demonstration Zone) Xiangyang 441000 China

Exploring promising electrolyte-system with high reversible Mg plating/stripping and excellent stability is essential for rechargeable magnesium batteries (RMBs). Fluoride alkyl magnesium salts (Mg(OR F ) 2 ) not only possess high solubility in ether solvents but also compatible with Mg metal anode, thus holding a vast application prospect. Herein, a series of diverse Mg(OR F ) 2 were synthesized, among them, perfluoro-tert-butanol magnesium (Mg(PFTB) 2 )/AlCl 3 /MgCl 2 based electrolyte demonstrates highest oxidation stability, and promotes the in situ formation of robust solid electrolyte interface. Consequently, the fabricated symmetric cell sustains a long-term cycling over 2000 h, and the asymmetric cell exhibits a stable Coulombic efficiency of 99.5 % over 3000 cycles. Furthermore, the Mg||Mo 6 S 8 full cell maintains a stable cycling over 500 cycles. This work presents guidance for understanding structure–property relationships and electrolyte applications of fluoride alkyl magnesium salts.

关键词： Electrolyte Fluoride Alkyl Magnesium Salts Rechargeable Magnesium Batteries Solid Electrolyte Interface

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