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SSRN 2023年

作者： Ke, Shaoqiu Nie, Xiaolei Ai, Xiaoling Li, Xiangyu Xu, Wenjie Fu, Kai Chen, Tiantian Liu, Chengshan Zhu, Wanting Wei, Ping Zhao, Wenyu Zhang, Qingjie State Key Laboratory of Advanced Technology for Materials Synthesis and Processing Wuhan University of Technology Wuhan430070 China Nanostructure Research Center Wuhan University of Technology Wuhan430070 China

The poor electrical transport performance of flexible thermoelectric (TE) films is a major bottleneck for the development of in-plane heat dissipation technology based on Peltier effect. Herein, ordered Fe nanoparticles (Fe-NPs) and in-situ Fe3O4 nanoparticles (Fe3O4-NPs) as magnetic functional elements (MFEs) were embedded into Bi0.5Sb1.5Te3 (BST)/epoxy flexible films in order to enhance the TE performance. The remarkable increases in electrical conductivity of BST/MFEs/BST/epoxy flexible films have been confirmed to originate from the carrier mobility increases. The retention of large Seebeck coefficient is attributed to the negative magnetoresistance (MR-) induced by spin-dependent scattering and weak localization effect from MFEs. As a result, the maximum power factor of BST/MFEs/BST/epoxy flexible films increased by 45%, and the maximum cooling temperature difference enhanced by 1.6 times. This work reveals that the ordered MFEs can significantly boost the electro-thermal conversion performance of flexible TE films and the magnetoresistance theory can reveal the scattering mechanism of charge carriers in thermo-electromagnetic flexible films. © 2023, The Authors. All rights reserved.

关键词： Magnetoresistance

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Ammonium Ion and Structural Water Co-Assisted Zn^(2+) Intercalation/De-Intercalation in NH_(4)V_(4)O_(10)∙0.28H_(2)O

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Chinese Journal of Chemistry 2021年第7期39卷 1885-1890页

作者： Ting Zhu Bo Mai Ping Hu Ziang Liu Congcong Cai Xuanpeng Wang Liang Zhou State Key Laboratory of Advanced Technology for Materials Synthesis and Processing Wuhan University of TechnologyWuhanHubei430070 China Department of Physical Science&Technology School of ScienceWuhan University of TechnologyWuhanHubei430070 China Foshan Xianhu Laboratory of the Advanced Energy Science and Technology Guangdong Laboratory Xianhu Hydrogen ValleyFoshanGuangdong528200 China

Main observation and conclusion The cathode material plays a crucial role in the performances of aqueous zinc-ion batteries(ZIBs).Herein,we report an ammonium vanadate(NH_(4)V_(4)O_(10)∙0.28H_(2)O,NHVO)aqueous ZIB cat... 详细信息

关键词： Aqueous zinc-ion battery Cathode material Vanadates Zincates Electrochemistry

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Articular cartilage and osteochondral tissue engineering techniques:Recent advances and challenges

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Bioactive materials 2021年第12期6卷 4830-4855页

作者： Wenying Wei Honglian Dai State Key Laboratory of Advanced Technology for Materials Synthesis and Processing Biomedical Materials and Engineering Research Center of Hubei ProvinceWuhan University of TechnologyWuhan430070China International School of Materials Science and Engineering Wuhan University of TechnologyWuhan430070China Foshan Xianhu Laboratory of the Advanced Energy Science and Technology Guangdong Laboratory Xianhu Hydrogen ValleyFoshan528200China

In spite of the considerable achievements in the field of regenerative medicine in the past several decades,osteochondral defect regeneration remains a challenging issue among diseases in the musculoskeletal system because of the spatial complexity of osteochondral units in composition,structure and *** order to repair the hierarchical tissue involving different layers of articular cartilage,cartilage-bone interface and subchondral bone,traditional clinical treatments including palliative and reparative methods have showed certain improvement in pain relief and defect *** is the development of tissue engineering that has provided more promising results in regenerating neo-tissues with comparable compositional,structural and functional characteristics to the native osteochondral *** in this review,some basic knowledge of the osteochondral units including the anatomical structure and composition,the defect classification and clinical treatments will be first *** we will highlight the recent progress in osteochondral tissue engineering from perspectives of scaffold design,cell encapsulation and signaling factor incorporation including bioreactor *** products for osteochondral defect repair will be analyzed and summarized ***,we will discuss the current obstacles and future directions to regenerate the damaged osteochondral tissues.

关键词： Osteochondral tissue engineering Cartilage tissue engineering Gradient scaffold Bioreactors

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High‑Energy and High‑Power Pseudocapacitor–Battery Hybrid Sodium‑Ion Capacitor with Na^(+) Intercalation Pseudocapacitance Anode

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Nano-Micro Letters 2021年第3期13卷 209-221页

作者： Qiulong Wei Qidong Li Yalong Jiang Yunlong Zhao Shuangshuang Tan Jun Dong Liqiang Mai Dong‑Liang Peng Department of Materials Science and Engineering Fujian Key Laboratory of Materials GenomeCollege of MaterialsXiamen UniversityXiamen 361005People’s Republic of China State Key Laboratory of Advanced Technology for Materials Synthesis and Processing Wuhan University of TechnologyWuhan 430070People’s Republic of China Shenzhen Geim Graphene Center Tsinghua Shenzhen International Graduate SchoolTsinghua UniversityShenzhen 518055People’s Republic of China Advanced Technology Institute University of SurreyGuildford Surrey GU27XHUK

High-performance and low-cost sodium-ion capacitors(SICs)show tremendous potential applications in public transport and grid energy ***,conventional SICs are limited by the low specific capacity,poor rate capability,and low initial coulombic efficiency(ICE)of anode ***,we report layered iron vanadate(Fe5V15O39(OH)9·9H2O)ultrathin nanosheets with a thickness of~2.2 nm(FeVO UNSs)as a novel anode for rapid and reversible sodium-ion *** to in situ synchrotron X-ray diffractions and electrochemical analysis,the storage mechanism of FeVO UNSs anode is Na+intercalation pseudocapacitance under a safe potential *** FeVO UNSs anode delivers high ICE(93.86%),high reversible capacity(292 mAh g^−1),excellent cycling stability,and remarkable rate ***,a pseudocapacitor–battery hybrid SIC(PBH-SIC)consisting of pseudocapacitor-type FeVO UNSs anode and battery-type Na3(VO)2(PO4)2F cathode is assembled with the elimination of presodiation *** PBH-SIC involves faradaic reaction on both cathode and anode materials,delivering a high energy density of 126 Wh kg^−1 at 91 W kg^−1,a high power density of 7.6 kW kg^−1 with an energy density of 43 Wh kg−1,and 9000 stable *** tunable vanadate materials with high-performance Na+intercalation pseudocapacitance provide a direction for developing next-generation highenergy capacitors.

关键词： Sodium-ion capacitors Pseudocapacitance Hybrid capacitors Two-dimensional materials Iron vanadate

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The effect of hierarchical single-crystal ZSM-5 zeolites with different Si/Al ratios on its pore structure and catalytic performance

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Frontiers of Chemical Science and Engineering 2021年第2期15卷 269-278页

作者： Yuexin Hou Xiaoyun Li Minghui Sun Chaofan Li Syed ul Hasnain Bakhtiar Kunhao Lei Shen Yu Zhao Wang Zhiyi Hu Lihua Chen Bao-Lian Su Laboratory of Living Materials at the State Key Laboratory of Advanced Technology for Materials Synthesis and Processing Wuhan University of TechnologyWuhan 430070China State Key Laboratory of Silicate Material for Architectures Wuhan University of TechnologyWuhan 430070China Laboratory of Inorganic Materials Chemistry(CMI) University of NamurB-5000 NamurBelgium Nanostructure Research Centre(NRC) Wuhan University of TechnologyWuhan 430070China Clare Hall University of CambridgeCambridgeCB39ALUK

Hierarchical single-crystal ZSM-5 zeolites with different Si/Al ratios(Hier-ZSM-5-x,where x=50,100,150 and 200)were synthesized using an ordered mesoporous carbon-silica composite as hard ***-ZSM-5-x exhibits improved mass transport properties,excellent mechanical and hydrothermal stability,and higher catalytic activity than commercial bulk zeolites in the benzyl alcohol self-etherification *** show that a decrease in the Si/Al ratio in hierarchical single-crystal ZSM-5 zeolites leads to a significant increase in the acidity and the density of micropores,which increases the final catalytic *** effect of porous hierarchy on the diffusion of active sites and the final catalytic activity was also studied by comparing the catalytic conversion after selectively designed poisoned acid *** poisoned Hier-ZSM-5-x shows much higher catalytic conversion than the poisoned commercial ZSM-5 zeolite,which indicates that the numerous intracrystalline mesopores significantly reduce the diffusion path of the reactant,leading to the faster diffusion inside the zeolite to contact with the acid sites in the micropores predominating in ZSM-5 *** study can be extended to develop a series of hierarchical single-crystal zeolites with expected catalytic performance.

关键词： hierarchical zeolites single crystalline interconnected pores improved diffusion performance benzyl alcohol self-etherification reaction

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Thermoelectric Energy Extraction in Motion Scenarios: Self-Powered Temperature and Pressure Detector in an Automobile Tire

SSRN

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SSRN 2023年

作者： Yang, Dongwang Wang, Jiang Xing, Yubing Hu, Kai Lyu, Jianan Li, Junhao Liu, Yutian Xiao, Yani Yan, Yonggao Tang, Xinfeng State Key Laboratory of Advanced Technology for Materials Synthesis and Processing Wuhan University of Technology Wuhan430070 China Nanostructure Research Center Wuhan University of Technology Wuhan430070 China

This study employs finite element simulation methods to meticulously analyze the temperature distribution within swiftly moving car tires to assess energy recovery possibilities. Results show that at 20 °C ambient temperature and a speed of 120 km/h, the maximum tire surface temperature due to friction and rubber deformation hysteresis reaches 91.2 °C. Additionally, a micro thermoelectric generator (micro-TEG) installed on the aluminum alloy wheel hub, functioning as a heat sink, demonstrates an effective temperature difference of 3.9 °C. When subjected to a temperature difference of 20 °C, the micro-TEG module exhibits open circuit voltage and maximum power of 1.47 V/1.41V and 12.06 mW/11.58 mW in the flat and curved states, respectively. To ensure module reliability, rigorous testing is conducted, including 10,000 cycles of bending, barometric shocking, and 20 cycles of temperature variations ranging from 0-100 °C. Remarkably, the module exhibits minimal alterations in internal resistance and open circuit voltage throughout the testing process. Additionally, the module is seamlessly integrated with energy management and Bluetooth signal transmission circuits (total weight: 8.96 g). During simulated car driving, the temperature and pressure signals received by the mobile phone software demonstrate high accuracy, with over 94% consistency compared to the measured results. © 2023, The Authors. All rights reserved.

关键词： Open circuit voltage

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Thermoelectric Energy Extraction in Motion Scenarios: Self-Powered Temperature and Pressure Detector in an Automobile Tire

SSRN

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SSRN 2023年

关键词： Open circuit voltage

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In Situ Tin Doping to Enhance the Cycling Performance of 4.9 V LNMO Cathode materials

In Situ Tin Doping to Enhance the Cycling Performance of 4.9...

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IEEE International Conference on Power and Energy Applications (ICPEA)

作者： Yan Li Jinqiao Du Zhaojie Liang Jie Tian Pei Wang Wen Luo Electric Power Scientific Research Institute Shenzhen Power Supply Bureau Co. Ltd Shenzhen China State Key Laboratory of Advanced Technology for Materials Synthesis and Processing Wuhan University of Technology Wuhan China

ISBN: (数字)9798350356113

ISBN: (纸本)9798350356120

LiNi 0.5 Mn 1.5 O 4 (LNMO) cathode material has the advantages of high energy density (650 Wh/kg), high discharge voltage (4.7 V vs Li+/Li), low raw material cost, low pollution, and high lithium ion transmission efficiency. It is a potential high power, low cost cobalt-free lithium-ion battery cathode material. However, the capacity decline of LNMO during high voltage charge and discharge processes leads to short cycle life, which limits its wide application and commercialization. To address this issue, this article uses in-situ Sn doping to enhance the cycle stability of LNMO. By uniformly mixing acetate salts in stoichiometric ratio and using one-step spray drying method to prepare undoped and Sn-doped LNMO cathode materials, this study systematically investigates the structural changes, morphological characteristics, and electrochemical performance before and after doping. The capacity retention rates of Sn-doped LNMO materials after 350 cycles at 0.7C are 93.5% and 94.5%, respectively, significantly higher than the undoped 80.8%, indicating that in-situ Sn doping can significantly enhance cycle performance. This study demonstrates that the LiNi 0.5 Mn 1.46 O 0.04 electrode prepared by spray drying method, with its simple and straightforward synthesis process and excellent electrochemical performance, has the potential to become a high-performance lithium-ion batteries cathode material.

关键词： Lithium-ion batteries Salt Electric potential Doping High-voltage techniques Voltage Lithium Ions Discharges (electric) Cathodes

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The staggered-layer induced elasticity strengthening mechanism in flexible Bi2Te3

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Matter 2025年

作者： Huang, Xiege Wu, Luoqi Hu, Mingyuan Feng, Xiaobin Zhai, Pengcheng Li, Wenjuan Duan, Bo He, Jiaqing Li, Guodong Zhang, Qingjie Goddard, William A. Hubei Key Laboratory of Theory and Application of Advanced Materials Mechanics School of Physics and Mechanics Wuhan University of Technology Wuhan430070 China Guangdong Provincial Key Laboratory of Advanced Thermoelectric Materials and Device Physics Shenzhen Key Laboratory of Thermoelectric Materials and Department of Physics Southern University of Science and Technology Shenzhen518055 China State Key Laboratory of Advanced Technology for Materials Synthesis and Processing Wuhan University of Technology Wuhan430070 China Materials and Process Simulation Center California Institute of Technology PasadenaCA91125 United States

Wearable flexible devices require the development of thermoelectric (TE) materials with high strength, excellent elastic bendability, and superior ductility. Here we report a staggered-layer strategy that overcomes the strength-flexibility dilemma. Our findings indicate that the newly formed strong Bi–Bi covalent bond between the staggered layer leads to an average 40% increase in the bond energy of the van der Waals Te–Te bond. A large Poisson's ratio leads to a high maximum linear elastic strain (ΕEmax), enhancing shear strength by 83.3%, which is consistent with a 92.2% increase in micro-pillar compressive strength. The narrow stiffness gap and bond energy gap facilitate the coordinated deformation that maintains sustained linear elasticity during compression. Moreover, the low BFCs of the Te–Te and Te–Bi bonds (0.72 eV/Å2 and 3.85 eV/Å2) contribute to the experimentally observed bending flexibility. This staggered-layer-induced elasticity strengthening mechanism offers a promising strategy for the rational design of highly reliable wearable TE devices. © 2025 Elsevier Inc.

关键词： Compressive strength

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Dynamic response of B4C, TiB2 and TiB2-B4C under shock wave compression

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Ceramics International 2025年

作者： Shu, Zaiqin Jing, Qiang Wan, Mingming Zhang, Jinyong School of Physics and Mechanics Wuhan University of Technology Wuhan430070 China School of Material Science and Engineering Wuhan University of Technology Wuhan430070 China State Key laboratory of Advanced Technology for Materials Synthesis and Processing Wuhan University of Technology Wuhan430070 China Inner Mongolian Metal Materials Research Institute Yantai264003 China

TiB2-B4C (TBC) has been widely utilized in lightweight armor due to its exceptional mechanical properties. The Hugoniot elastic limit (HEL) has been considered as an important dynamic property of ceramics. This paper presents the shock responses of pure B4C, pure TiB2, and TiB2-B4C composite. By microstructure analysis, the amorphization in B4C and dislocations in TiB2 at shock pressures around 37 GPa in the recycled debris were observed. The dislocations in TiB2 are believed to be the reason for ‘two HELs’ in TiB2. The addition of TiB2 has little effect on the shock properties of B4C, while the shock pressure exceeds HEL. Additionally, a failure wave was detected in the ceramics at shock pressures lower than HEL. A damage parameter was defined to quantify the extent of damage in the failure zone. The incorporation of TiB2 into B4C can significantly slow down failure propagation in TBC at pressure lower than HEL. Furthermore, the analysis of the damage parameter suggests that TBC exhibits superior impact resistance compared to pure B4C and TiB2. © 2025 Elsevier Ltd and Techna Group S.r.l.

关键词： Amorphization

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