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CdS nanosheets decorated with Ni@graphene core-shell cocatalyst for superior photocatalytic H_(2) production

Journal of materials Science & technology 2020年第21期56卷 170-178页

作者： Tingmin Di Liuyang Zhang Bei Cheng Jiaguo Yu Jiajie Fan School of Materials Science and Engineering Wuhan Institute of TechnologyWuhan 430205China State Key Laboratory of Advanced Technology for Materials Synthesis and Processing Wuhan University of TechnologyWuhan 430070China School of Materials Science and Engineering Zhengzhou UniversityZhengzhou 450002China

A novel cocatalyst,*** nickel nanoparticles encapsulated in few-layer graphene(Ni@C),is obtained by carbonization of metal–organic frameworks(MOF)and leaching treatment of hydrochloric *** is selected as the cocatalyst for CdS nanosheets,forming CdS-Ni@C *** remarkably improves the photocatalytic activities of CdS nanosheets due to the synergistic effect of Ni nanoparticles and graphene *** addition,the Ni nanoparticles encapsulated by graphene layers effectively isolate Ni from the ambient,which avoids contamination and curbs *** larger work function of Ni@C and outstanding conductivity of graphene promote the electron transfer from CdS to Ni@C,suppressing the recombination of photogenerated carriers and facilitating the separation of photogenerated electronhole *** strategy by adopting this novel cocatalyst provides a new solution to the improvement of the photocatalytic hydrogen production.

关键词： CdS nanosheets Photocatalytic hydrogen production Nickel Graphene Core-shell cocatalyst Metal-organic frameworks(MOF)

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受水车启发的、在饱和盐水中也能实现高效和稳定的太阳能淡化的旋转蒸发器

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Science Bulletin 2023年第15期68卷 1640-1650,M0004页

作者：蒋函锦刘行航王海涛王德文郭亚楠王冬高岗王笑夷胡超权 State Key Laboratory of Superhard Materials Key Laboratory of Automobile Materials of Ministry of EducationJilin Provincial International Cooperation Key Laboratory of High-Efficiency Clean Energy MaterialsSchool of Materials Science and EngineeringJilin UniversityChangchun 130012China School of Fashion and Textiles The Hong Kong Polytechnic UniversityHong KongChina State Key Laboratory of Inorganic Synthesis and Preparative Chemistry College of ChemistryJilin UniversityChangchun 130012China College of Chemical Engineering Northeast Electric Power UniversityJilin 132012China National Key Laboratory of Science and Technology on Advanced Composites in Special Environments Harbin Institute of TechnologyHarbin 150080China Key Laboratory of Optical System Advanced Manufacturing Technology Changchun Institute of OpticsFine Mechanics and PhysicsChinese Academy of SciencesChangchun 130033China State Key Laboratory of Applied Optics Changchun Institute of OpticsFine Mechanics and PhysicsChinese Academy of SciencesChangchun 130033China

太阳能海水淡化是解决全球淡水短缺的最有前景方法之一.然而,传统的蒸发体在高盐度海水中遭遇了盐累积带来的蒸发速率下降甚至失效的瓶颈.受古代水车的启发,本文开发了一种自适应旋转蒸发器,其可以在任意浓度的盐水中实现长期高效的太... 详细信息

太阳能海水淡化是解决全球淡水短缺的最有前景方法之一.然而,传统的蒸发体在高盐度海水中遭遇了盐累积带来的蒸发速率下降甚至失效的瓶颈.受古代水车的启发,本文开发了一种自适应旋转蒸发器,其可以在任意浓度的盐水中实现长期高效的太阳能海水淡化.这种蒸发器是一种双硫化物负载的滚筒式生物质炭.借助了木材天然的水传输通道和分层结构,蒸发器具有杰出的水供应和热定位能力.实验和数值模拟表明,归因于其低密度及独特的亲疏水特性,这个蒸发器能够在盐结晶产生的重心偏移下周期性转动以实现自动盐移除.这使得这个蒸发体甚至可以在饱和盐水(26.47%)中,24 h内保持2.8 kg m^(-2)h^(-1)的高蒸发速率,这是过去一直无法实现的.因此,这项概念验证工作展示了一种不受浓度和运行时间限制的、自旋转诱导脱盐的蒸发器.

关键词： Adaptively rotating evaporator Self-removal of salt Waterwheel-inspired Stable solar desalination

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Recent progress in perovskite solar cells:from device to commercialization

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Science China Chemistry 2022年第12期65卷 2369-2416页

作者： Xinhui Luo Xuesong Lin Feng Gao Yang Zhao Xiaodong Li Liqing Zhan Zexiong Qiu Jin Wang Cong Chen Lei Meng Xiaofeng Gao Yu Zhang Zijian Huang Rundong Fan Huifen Liu Yanrun Chen Xiaoxue Ren Jiahong Tang Chun-Hao Chen Dong Yang Yongguang Tu Xiao Liu Dongxue Liu Qing Zhao Jingbi You Junfeng Fang Yongzhen Wu Hongwei Han Xiaodan Zhang Dewei Zhao Fuzhi Huang Huanping Zhou Yongbo Yuan Qi Chen Zhaokui Wang Shengzhong(Frank)Liu Rui Zhu Jotaro Nakazaki Yongfang Li Liyuan Han State Key Laboratory of Metal Matrix Composites School of Material Science and EngineeringShanghai Jiao Tong UniversityShanghai 200240China State Key Lab for Mesoscopic Physics and Frontiers Science Center for Nano-optoelectronics School of PhysicsPeking UniversityBeijing 100871China Key Laboratory of Semiconductor Materials Science Institute of SemiconductorsChinese Academy of SciencesBeijing 100083China School of Physics and Electronic Science Engineering Research Center of Nanophotonics&Advanced InstrumentMinistry of EducationEast China Normal UniversityShanghai 200241China Key Laboratory for Advanced Materials and Institute of Fine Chemicals School of Chemistry and Molecular EngineeringEast China University of Science and TechnologyShanghai 200237China Wuhan National Laboratory for Optoelectronics Huazhong University of Science and TechnologyWuhan 430074China Institute of Photoelectronic Thin Film Devices and Technology Renewable Energy Conversion and Storage CenterSolar Energy Research CenterNankai UniversityTianjin 300350China College of Materials Science and Engineering&Engineering Research Center of Alternative Energy Materials&Devices Ministry of EducationSichuan UniversityChengdu 610065China Beijing National Laboratory for Molecular Sciences CAS Key Laboratory of Organic SolidsInstitute of ChemistryChinese Academy of SciencesBeijing 100190China State Key Laboratory of Advanced Technology for Materials Synthesis and Processing Wuhan University of TechnologyWuhan 430070China Beijing Key Laboratory for Theory and Technology of Advanced Battery Materials Key Laboratory of Polymer Chemistry and Physics of Ministry of EducationSchool of Materials Science and EngineeringPeking UniversityBeijing 100871China School of Physics and Electronics Hunan Key Laboratory of Nanophotonics and DevicesCentral South UniversityChangsha 410083China Experimental Center for Advanced Materials School of Materials Science and EngineeringBeijing Institute of TechnologyBeijing 100081China Jia

Perovskite solar cells(PSCs) are undergoing rapid development and the power conversion efficiency reaches 25.7% which attracts increasing attention on their commercialization *** this review,we summarized the recent progress of PSCs based on device structures,perovskite-based tandem cells,large-area modules,stability,applications and ***,the challenges and perspectives are discussed,aiming at providing a thrust for the commercialization of PSCs in the near future.

关键词： perovskite solar cells device engineering stability application

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Effect of calcination temperatures on photocatalytic H_(2)O_(2)-production activity of ZnO nanorods

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Chinese Journal of Catalysis 2022年第2期43卷 226-233页

作者： Zicong Jiang Yong Zhang Liuyang Zhang Bei Cheng Linxi Wang State Key Laboratory of Advanced Technology for Materials Synthesis and Processing Wuhan University of TechnologyWuhan 430070HubeiChina Foshan Xianhu Laboratory of the Advanced Energy Science and Technology Guangdong Laboratory Xianhu Hydrogen ValleyFoshan 528200GuangdongChina College of Chemistry and Chemical Engineering Hubei Polytechnic UniversityHuangshi435003HubeiChina Laboratory of Solar Fuel Faculty of Materials Science and ChemistryChina University of GeosciencesWuhan 430074HubeiChina

Photocatalytic hydrogen peroxide(H_(2)O_(2))production from O_(2) and H2O is an ideal process for solar‐to‐chemical energy ***,ZnO nanorods are prepared via a simple hydrothermal method for photocatalytic H_(2)O_(2) *** ZnO nanorods exhibit varied performance with different calcination *** from calcination,the separation efficiency of photo‐induced carriers is significantly improved,leading to the superior photocatalytic activity for H_(2)O_(2) *** H_(2)O_(2) produced by ZnO calcined at 300℃ is 285μmol L^(−1),which is over 5 times larger than that produced by untreated *** work provides an insight into photocatalytic H2O2 production mechanism by ZnO nanorods,and presents a promising strategy to H2O2 production.

关键词： Photocatalysis Hydrogen peroxide production ZnO nanorod Calcination temperature Oxygen reduction

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Progress on Transition Metal Ions Dissolution Suppression Strategies in Prussian Blue Analogs for Aqueous Sodium-/Potassium-Ion Batteries

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Nano-Micro Letters 2024年第7期16卷 142-168页

作者： Wenli Shu Junxian Li Guangwan Zhang Jiashen Meng Xuanpeng Wang Liqiang Mai Department of Physical Science and Technology School of ScienceWuhan University of TechnologyWuhan 430070People’s Republic of China School of Materials Science and Engineering State Key Laboratory of Advanced Technology for Materials SynthesisWuhan University of TechnologyWuhan 430070People’s Republic of China Sanya Science and Education Innovation Park Wuhan University of TechnologySanya 572000People’s Republic of China Hubei Longzhong Laboratory Wuhan University of TechnologyXiangyang Demonstration ZoneXiangyang 441000People’s Republic of China

Aqueous sodium-ion batteries(ASIBs)and aqueous potassium-ion batteries(APIBs)present significant potential for large-scale energy storage due to their cost-effectiveness,safety,and environmental ***,the intricate energy storage mechanisms in aqueous electrolytes place stringent require-ments on the host *** blue analogs(PBAs),with their open three-dimensional framework and facile synthesis,stand out as leading candidates for aqueous energy ***,PBAs possess a swift capacity fade and limited cycle longevity,for their structural integrity is compromised by the pronounced dis-solution of transition metal(TM)ions in the aqueous *** manuscript provides an exhaustive review of the recent advancements concerning PBAs in ASIBs and *** dissolution mechanisms of TM ions in PBAs,informed by their structural attributes and redox processes,are thoroughly ***,this study delves into innovative design tactics to alleviate the dissolution issue of TM *** conclusion,the paper consolidates various strategies for suppressing the dissolution of TM ions in PBAs and posits avenues for prospective exploration of high-safety aqueous sodium-/potassium-ion batteries.

关键词： Prussian blue analogs Transition metal ions dissolution Suppression strategies Aqueous sodium-ion batteries Aqueous potassium-ion batteries

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Bio-based materials for sustainable energy harvesting: Applications in TENGs, PENGs, and solar-powered seawater desalination systems

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Chemical Engineering Journal 2025年 516卷

作者： Ding, Yutong Deng, Linbing Liu, Xiao-Xiao Wang, Lili Meng, Yanrong Ouyang, Mi Chen, Feng Huang, Zhao-Xia Kuang, Tairong Lab State Key Laboratory of Advanced Separation Membrane Materials Zhejiang Key Laboratory of Advanced Polymer Materials Modification and Application Technology College of Materials Science and Engineering Zhejiang University of Technology Hangzhou310014 China National Engineering Research Center of Novel Equipment for Polymer Processing Key Laboratory of Polymer Processing Engineering Ministry of Education Guangdong Provincial Key Laboratory of Technique and Equipment for Macromolecular Advanced Manufacturing Department of Mechanical and Automotive Engineering South China University of Technology Guangzhou510641 China School of Advanced Manufacturing Technology Guangdong Mechanical & Electrical Polytechnic Guangzhou510550 China Department of General Medicine First Medical Center of Chinese PLA General Hospital Beijing100039 China

The global energy crisis has intensified the need for sustainable energy solutions, yet conventional energy production still relies on non-renewable, environmentally damaging materials. Although significant advances have been made in green energy technologies, a critical gap remains in the development of materials that are both renewable and environmentally friendly. Bio-based materials, derived from renewable resources, offer a timely and sustainable alternative that can significantly improve the efficiency, functionality, and environmental compatibility of energy conversion devices. This review highlights the role of bio-based materials in addressing these challenges, focusing on their applications in emerging green energy technologies, particularly triboelectric nanogenerators (TENGs), piezoelectric nanogenerators (PENGs), and solar-powered seawater desalination systems. It provides a comprehensive overview of the latest advances in preparation methods, material properties, and their practical applications in energy conversion systems. By discussing the unique advantages and material selection challenges, this review underscores the importance of bio-based materials in the continued development of sustainable, high-performance energy harvesting devices. Furthermore, it emphasizes their potential to contribute to global sustainability goals, offering a critical pathway to more eco-friendly and cost-effective energy solutions. © 2025 Elsevier B.V.

关键词： Solar power generation

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Effect of micro/nano-sheet array structures on the osteo-immunomodulation of macrophages

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Regenerative Biomaterials 2022年第1期9卷 888-899页

作者： Xinhui Zheng Lan Chen Ji Tan Jianhua Miao Xuanyong Liu Tieyi Yang Zhihong Ding Department of Orthopedics Gongli Hospital of Shanghai Pudong New AreaShanghai 200135China Department of Orthopedics Zhengzhou Central Hospital Affiliated Zhengzhou UniversityZhengzhou 450007China State Key Laboratory of High-Performance Ceramics and Superfine Microstructure Shanghai Institute of CeramicsChinese Academy of SciencesShanghai 200050China School of Materials Science and Engineering&Henan Key Laboratory of Advanced Magnesium Alloy&Key Laboratory of Materials Processing and Mold Technology(Ministry of Education) Zhengzhou UniversityZhengzhou 450001China

The immune response induced by surface topography crucially determines the implant ***,how the immune response is mediated by the size of surface topography remains ***,various biocompatible Mg-Al layered double hydroxides sheet-array films with different sizes(nano,micro and nano/micro mixture)were constructed on the biomedical titanium,and their osteo-immunomodulation effects on the macrophages were *** nano-sheet array structures significantly promoted the polarization of M2 macrophages by activating the PI3K-AKT-mTOR signaling pathway with high gene expressions of integrin b2 and *** the micro-sheet array structures enhanced osteogenic differentiation of mouse bone marrow mesenchymal stem cells(mBMSCs)via ROCK-YAP/TAZ-mediated ***,the nano-sheet array structures promoted the osteogenic differentiation of mBMSCs with a high proportion of M2 macrophages through a shared *** study gave further information concerning integrin-induced focal adhesions in cells of different sheet array structures and their role in macrophage polarization and osteogenic differentiation of mBMSCs,which might help to design biomaterial surfaces with optimal geometry for a desired immunemodulation.

关键词： micro-nano topography immunomodulation macrophages osteogenesis

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Evolution in wear, corrosion, and tribocorrosion behavior of Ni-based alloys induced by Mn addition

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Wear 2025年 570卷

作者： Chen, Jia Lu, Wenlan Dai, Pinqiang Wen, Xiaochun Wang, Zhenjun Fan, Hengzhong Chen, Hongxiang Zhang, Yongsheng School of Materials Science and Engineering Fujian University of Technology Fuzhou350118 China State Key Laboratory of Solid Lubrication Lanzhou Institute of Chemical Physics Chinese Academy of Sciences Lanzhou730000 China Fujian Provincial Key Laboratory of Advanced Materials Processing and Application Fuzhou350118 China

Ni-based alloys have attracted much attention due to their exceptional mechanical and corrosion properties. The combination of these excellent properties has increased researchers’ interest in studying passivation mechanism during corrosion and tribocorrosion. In the present study, the effects of Mn addition (Mn = 0, 5, 10, and 20 at.%) on wear, corrosion, and tribocorrosion behavior of Ni-based alloys were investigated under room temperature. The microstructures of as-fabricated and post-test Ni alloys were characterized by X-ray diffraction and scanning electron microscopy. The elemental distribution and chemical states in worn and unworn areas were identified by using energy dispersive X-ray spectroscopy and X-ray photoelectron spectroscopy. The addition of Mn in the alloy was found to increase wear and tribocorrosion resistance. Pitting potential of Mn-free alloys was higher than that of Mn-containing alloys, reducing from 0.56 V to −0.05 V. Higher Mn concentration in the alloy offered a wear-induced corrosion during tribocorrosion process. In addition, substituting Cr with Mn content can promote the passivation of Ni, which was confirmed by X-ray photoelectron spectroscopy. Although Ni-Mn alloys does not passivate thermodynamically, passive layers can be found by transmission electron microscopy analysis due to the formation of metastable oxide phases. © 2025 Elsevier B.V.

关键词： X ray photoelectron spectroscopy

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Emerging Applications of Optical Fiber‑Based Devices for Brain Research

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advanced Fiber materials 2022年第1期4卷 24-42页

作者： Roya Nazempour Bozhen Zhang Zhongyin Ye Lan Yin Xianli Lv Xing Sheng Department of Electronic Engineering Center for Flexible Electronics TechnologyIDG/McGovern Institute for Brain ResearchBeijing National Research Centre for Information Science and TechnologyTsinghua UniversityBeijing 100084China School of Materials Science and Engineering The Key Laboratory of Advanced MaterialsState Key Laboratory of New Ceramics and Fine ProcessingCenter for Flexible Electronics TechnologyTsinghua UniversityMinistry of EducationBeijing 10084China Neurosurgery Department School of Clinical MedicineBeijing Tsinghua Changgung HospitalTsinghua UniversityBeijing 102218China

Research in neuroscience and neuroengineering has attracted tremendous interest in the past ***,the complexity of the brain tissue,in terms of its structural,chemical,mechanical,and optical properties,makes the interrogation of biophysical and biochemical signals within the brain of living animals extremely *** a viable and versatile tool for brain studies,optical fber based technologies have provided exceptional opportunities to unravel the mysteries of the brain and open the door for clinical applications in the treatment,diagnosis,and prevention of neurological ***,optical fbers with diameters from 10 to 1000μm are capable of guiding and delivering light to deep levels of the living ***,small dimensions of such devices along with their fexibility and light weight paved the way for understanding the complex behaviours of living and freely moving *** article provides a review of the emerging applications of optical fbers in neuroscience,specifcally in the mammalian *** utilities,including optogenetics,fuorescence sensing,drug administration and phototherapy,are *** also discuss other biological applications of such implantable fbers,which may provide insights into the future study of *** is envisioned that these and other optical fber based techniques ofer a powerful platform for multi-functional neural activity sensing and modulation.

关键词： Optical fbers Neuroscience Optogenetics Biosensing

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Discovering the Role of Moisture in Spray-Coating High-Quality Perovskite Films Under Ambient Conditions

SSRN

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SSRN 2023年

作者： Yu, Xinxin Mo, Yanping Li, Jing Ku, Zhiliang Xiao, Junyan Long, Fei Han, Liyuan Peng, Yong Cheng, Yi-Bing State Key Laboratory of Advanced Technology for Materials Synthesis and Processing Wuhan University of Technology Hubei Wuhan430070 China College of Materials Science and Engineering Guilin University of Technology Guangxi Guilin541004 China State Key Laboratory of Metal Matrix Composites Shanghai Jiao Tong University Shanghai200240 China

The effect of moisture on the crystallization and morphological control of spray-prepared Cs0.19FA0.81PbI2.5Br0.5 perovskite films is elucidated. Moisture in air functions to (1) enhance droplet spreading as a result of humidity-suppressed solvent evaporation;(2) solvate organic salts in conjunction with added water in the precursor solution to facilitate the penetration of organic salts into inorganic halide films and accelerate their interaction. These conjunct contributions, on the one hand, relieve inhomogeneous solute distribution and suppress the "coffee-ring effect", on the other hand, promote phase transition and improve the crystallinity of resultant perovskite, ultimately enabling the formation of high-quality Cs0.19FA0.81PbI2.5Br0.5 perovskite films with homogeneous morphology and good crystallization. The power conversion efficiency (PCE) of the champion perovskite solar cell increases from 18.25% to 19.74%, with improved thermal stability, maintaining 80% of its initial efficiency after operating at 50 °C for >800 h. The large-area perovskite film (10 × 10 cm2) exhibits significant uniformity over the entire film, and the corresponding devices exhibit high consistency and reproducibility. The average PCE of small-area devices employing the same large-area perovskite film is 19.53±0.25%. Mini-modules with an active area of 64.8 cm2 yield an optimal PCE of 16.75%, with an average PCE of 16.08±0.32%. © 2023, The Authors. All rights reserved.

关键词： Perovskite solar cells

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