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Large‑scale Fabrication of Snake‑skin‑inspired Protective Composite Textiles

advanced Fiber materials 2024年第4期6卷 978-992页

作者： Qing Liu Fengxiang Chen Tingting Dong Woong‑Ryeol Yu Chaoyu Chen Gaoming Jiang Zhijia Dong Pibo Ma Engineering Research Center of Knitting Technology Ministry of EducationCollege of Textile Science and EngineeringJiangnan UniversityWuxi 214122P.R.China State Key Laboratory of New Textile Materials and Advanced Processing Technologies/National Local Joint Laboratory for Advanced Textile Processing and Clean Production/Hubei Key Laboratory of Digital Textile Equipment Wuhan Textile UniversityWuhan 430200P.R.China Department of Materials Science and Engineering and Research Institute of Advanced Materials Seoul National UniversitySeoul 08826Republic of Korea

Inspired by the overlapping structure of snake scales,a reinforced scale-like knitted fabric(R-SLKF)was created in this *** achieve this,short carbon fibers in an epoxy resin(ER)matrix were incorporated into the scales of an *** resulting textile is a highly stable protective composite that is flexible,warm,and thermally *** addition,supe-rior stab-resistance is ensured through rigid protective blocks in the R-SLKF,making up a hard overlapping scale region,besides satisfactory flexibility via soft twisted ultra-high-molecular-weight polyethylene yarn-based *** R-SLKF achieves high stab resistance(peak load of approximately 600 N for a single scale thickness of 2 mm),good flexibility(~290 mN cm),and breathability(100 MPa,423 mm/s),coupled with good warmth retention and thermal insulation prop-erties(0.28℃/s),which are superior to previously reported protective composite *** the results,the combination of desirable individual protection,excellent wearability and comfort enables human beings to survive in extremely danger-ous *** element simulations provided valuable insights into the factors influencing the stab resistance of R-SLKF and elucidated the underlying anti-puncture mechanism in accordance with the experimental *** study presents a novel strategy for the facile industrial fabrication of flexible and lightweight protective composite textiles,which is expected to enhance the structure and material design for future innovations and provide advantages for personal protec-tive equipment in various industrial fields.

关键词： Scale-like knitted fabric Stab-resistance Flexibility Air permeability Warmth retention and thermal insulation properties

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Enhancing energy density of poly(vinylidene fluoride) composite film via addition of N-doped carbon modified boron nitride and sandwich-structural engineering

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Applied Surface Science 2023年第1期640卷

作者： Huang, Huabo Mei, Wentao Wang, Yucong Huang, Juan Li, Liang Ji, Jiayou Xiong, Chuanxi Hubei Key Laboratory of Plasma Chemistry and Advanced Materials Key Laboratory for Green Chemical Process of Ministry of Education School of Materials Science and Engineering Wuhan Institute of Technology Wuhan430205 China Key Laboratory of Green Processing and Functional New Textile Materials of Ministry of Education School of Textile Science and Engineering Wuhan Textile University Wuhan430200 China State Key Laboratory of Advanced Technology for Materials Synthesis and Processing School of Materials Science and Engineering Wuhan University of Technology Wuhan430070 China

It is a challenge to simultaneously enhance dielectric constant and breakdown strength of dielectrics and achieve a greatly elevated energy density. Herein, polyaniline was first coated onto the surface of boron nitride nanosheets (BN), and then nitrogen-doped carbon (NC) was formed through a carburization process, resulting in BN@NC composite, which was subsequently added to poly(vinylidene fluoride) (PVDF) to prepare a composite film with high dielectric performance. The characterization showed that BN@NC effectively preserved the nanosheet structure of BN and formed strong hydrogen bonding interactions with the PVDF matrix, promoting the β-PVDF formation. This not only improved the compatibility but also enhanced the interfacial polarization between conductive NC and the polymer, leading to a high dielectric constant. Moreover, the electrically insulating BN prevented the formation of leakage current, resulting in a high breakdown strength. Finally, a sandwich-structured film was constructed, and exhibited a dielectric constant of 10.2 (at 1 kHz), a breakdown strength of 380 MV m−1, and an energy density of 6.1 J cm−3, which were 20%, 36%, and 74% higher, respectively, than those of pure PVDF film (8.5, 280 MV m−1, and 3.5 J cm−3). This work highlights significant potential for applications in low-cost and high-energy density dielectric composites. © 2023 Elsevier B.V.

关键词： Boron nitride

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Review of functionally graded materials processed by additive manufacturing

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China Welding 2023年第3期32卷 41-50页

作者：宋学平黄健康樊丁 State Key Laboratory of Advanced Processing and Recycling of Non-ferrous Metals Lanzhou University of TechnologyLanzhou 730050China School of Materials Science and Engineering Lanzhou University of TechnologyLanzhou 730050China School of Mechanical Engineering Lanzhou Petrochemical University of Vocational TechnologyLanzhou 730060China

Additive manufacturing(AM)technology makes parts through layer-by-layer deposition,which can regulate the microstructure and properties of different parts of a single part *** provides a new idea for the preparation of functionally gradient materials(FGM),and has become a research hotspot at *** referring to and analyzing the recent research achievements in the additive manufacturing tech-nology of FGM,the latest research progress at domestic and abroad from four aspects were summaried:selective laser melting additive man-ufacturing,electron beam additive manufacturing,arc additive manufacturing,path planning,and material ***,the existing problems in the research are pointed out,and the future research direction and focus are prospected.

关键词： functionally graded materials additive manufacture research progress

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Biomimetic brain-like nanostructures for solid polymer electrolytes with fast ion transport

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Science China materials 2022年第6期65卷 1476-1484页

作者： Ahmed Eissa Abdelmaoula Lulu Du Lin Xu Yu Cheng Amir AMahdy Muhammad Tahir Ziang Liu Liqiang Mai State Key Laboratory of Advanced Technology for Materials Synthesis and Processing School of Materials Science and EngineeringWuhan University of TechnologyWuhan 430070China Foshan Xianhu Laboratory of the Advanced Energy Science and Technology Guangdong Laboratory Xianhu Hydrogen ValleyFoshan 528200China Mining and Metallurgical Department Faculty of EngineeringAl-Azhar UniversityCairo 11884Egypt

The intrinsic drawbacks of electrolytes and the growth of lithium dendrites limit the development of commercial lithium *** address the aforementioned challenges,a novel biomimetic brain-like nanostructure(BBLN)solid polymer electrolyte was created by manipulating the shape of the incorporated *** designed BBLN solid polymer electrolyte was created by incorporating spherical core-shell(UIO-66@67)fillers into polymer electrolyte,which is significantly different from traditional polymer-based composite ***-66@67 spherical nanoparticles are highly favorable to eliminating polymer electrolyte stress and deformation during solidification,indicating a great potential for fabricating highly uniform BBLN solid polymer electrolytes with a substantial number of continuous ***,spherical nanoparticles can significantly reduce the crystalline structure of polymer electrolytes,improving polymer chain segmental movement and providing continuous pathways for rapid ion *** a result,BBLN solid polymer electrolyte shows excellent ionic conductivity(9.2×10^(−4)S cm^(−1)),a high lithium transference number(0.74),and outstanding cycle stability against lithium electrodes over 6500 h at room *** concept of biomimetic brain-like nanostructures in this work demonstrates a novel strategy to enhance ion transport in polymerbased electrolytes for solid-state batteries.

关键词： brain structure spherical nanoparticles continuous interphase nanophase separation MOF-in-MOF

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Optimal design approach of interpenetrating pre-stressed metal-ceramic composites based on deep learning neural network

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Composite Structures 2025年 368卷

作者： Liu, Kun Lai, Xin Liu, Lisheng Zhang, Jinyong Liu, Yifei Hubei Longzhong Laboratory Wuhan University of Technology Demonstration Zone XiangYang537134 China Hubei Key Laboratory of Theory and Application of Advanced Materials Mechanics Wuhan University of Technology Wuhan430070 China State Key Laboratory of Advanced Technology for Materials Synthesis and Processing Wuhan University of Technology Wuhan430070 China University of Rochester RochesterNY14527 United States

In this work, we proposed a new pre-stressed metal-ceramic interpenetrating structure to improve the apparent tensile strength of ceramic. In addition, an optimization design framework was constructed by integrating machine learning and gradient descent optimization algorithm for the optimization design of ceramic interpenetrating composites. The optimized metal-ceramic interpenetrating structure can achieve a balance of the stress state of the ceramic phase between intensity and distribution by ingeniously control the confinement and topology of the metal phase. More specifically, the surrogate model we constructed through deep neural network (DNN) can efficiently predict the relationship between the structure and its stress state. The final result obtained can achieve excellent pre-stress effect while making the structure lightweight. © 2025 Elsevier Ltd

关键词： Deep neural networks

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High‑Energy and High‑Power Pseudocapacitor–Battery Hybrid Sodium‑Ion Capacitor with Na^(+) Intercalation Pseudocapacitance Anode

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Nano-Micro Letters 2021年第3期13卷 209-221页

作者： Qiulong Wei Qidong Li Yalong Jiang Yunlong Zhao Shuangshuang Tan Jun Dong Liqiang Mai Dong‑Liang Peng Department of Materials Science and Engineering Fujian Key Laboratory of Materials GenomeCollege of MaterialsXiamen UniversityXiamen 361005People’s Republic of China State Key Laboratory of Advanced Technology for Materials Synthesis and Processing Wuhan University of TechnologyWuhan 430070People’s Republic of China Shenzhen Geim Graphene Center Tsinghua Shenzhen International Graduate SchoolTsinghua UniversityShenzhen 518055People’s Republic of China Advanced Technology Institute University of SurreyGuildford Surrey GU27XHUK

High-performance and low-cost sodium-ion capacitors(SICs)show tremendous potential applications in public transport and grid energy ***,conventional SICs are limited by the low specific capacity,poor rate capability,and low initial coulombic efficiency(ICE)of anode ***,we report layered iron vanadate(Fe5V15O39(OH)9·9H2O)ultrathin nanosheets with a thickness of~2.2 nm(FeVO UNSs)as a novel anode for rapid and reversible sodium-ion *** to in situ synchrotron X-ray diffractions and electrochemical analysis,the storage mechanism of FeVO UNSs anode is Na+intercalation pseudocapacitance under a safe potential *** FeVO UNSs anode delivers high ICE(93.86%),high reversible capacity(292 mAh g^−1),excellent cycling stability,and remarkable rate ***,a pseudocapacitor–battery hybrid SIC(PBH-SIC)consisting of pseudocapacitor-type FeVO UNSs anode and battery-type Na3(VO)2(PO4)2F cathode is assembled with the elimination of presodiation *** PBH-SIC involves faradaic reaction on both cathode and anode materials,delivering a high energy density of 126 Wh kg^−1 at 91 W kg^−1,a high power density of 7.6 kW kg^−1 with an energy density of 43 Wh kg−1,and 9000 stable *** tunable vanadate materials with high-performance Na+intercalation pseudocapacitance provide a direction for developing next-generation highenergy capacitors.

关键词： Sodium-ion capacitors Pseudocapacitance Hybrid capacitors Two-dimensional materials Iron vanadate

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Atomically dispersed Zn-Co-N-C catalyst boosting efficient and robust oxygen reduction catalysis in acid via stabilizing Co-N bonds

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Fundamental Research 2023年第6期3卷 909-917页

作者： Feng Ma Xuan Liu Xiaoming Wang Jiashun Liang Jianyu Huang Cameron Priest Jinjia Liu Shuhong Jiao Tanyuan Wang Gang Wu Yunhui Huang Qing Li State Key Laboratory of Material Processing and Die&Mould Technology School of Materials Science and EngineeringHuazhong University of Science and TechnologyWuhanHubei 430074China State Key Laboratory of Refractories and Metallurgy Institute of Advanced Materials and NanotechnologyKey Laboratory of Hubei Province for Coal Conversion and New Carbon MaterialsSchool of Chemistry and Chemical EngineeringWuhan University of Science and TechnologyWuhan 430081China Clean Nano Energy Center State Key Laboratory of Metastable Materials Science and TechnologyYanshan UniversityQinhuangdao 066004China Department of Chemical and Biological Engineering University at BuffaloThe State University of New YorkBuffaloNY 14260United States State Key Laboratory of Coal Conversion Institute of Coal ChemistryChinese Academy of SciencesTaiyuan 030001China National Energy Center for Coal to Clean Fuels Synfuels China Co.LtdHuairou DistrictBeijing 101400China Department of Materials Science and Engineering Key Laboratory of Materials for Energy Conversion Chinese Academy of Science(CAS)University of Science and Technology of ChinaHefei 230026China Department of Chemistry and Key Laboratory for Preparation and Application of Ordered Structural Materials of Guangdong Province Shantou UniversityShantou 515063China

Transition metal supported N-doped carbon(M-N-C)catalysts for oxygen reduction reaction(ORR)are viewed as the promising candidate to replace Pt-group metal(PGM)for proton exchange membrane fuel cells(PEMFCs).However,the stability of M-N-C is extremely challenging due to the demetalation,H_(2)O_(2)attack,*** the strongly oxidative conditions of *** this study,we demonstrate the universal effect of Zn on promoting the stability of atomically dispersed M-Nx/C(M=Co,Fe,Mn)catalysts and the enhancement mechanism is unveiled for the first *** best-performing dual-metal-site Zn-Co-N-C catalyst exhibits a high half-wave potential(E1/2)value of 0.81 V *** hydrogen electrode(RHE)in acid and outstanding durability with no activity decay after 15,000 accelerated degradation test(ADT)cycles at 60℃,surpassing most reported Co-based PGM-free catalysts in acid *** comparison,the Co-N-C in the absence of Zn suffers from a rapid degradation after ADT due to the demetalation and higher H_(2)O_(2)yield.X-ray adsorption spectroscopy(XAS)and density functional theory(DFT)calculations suggest the more negative formation energy(by 1.2 eV)and increased charge transfer of Zn-Co dual-site structure compared to Co-N-C could strength the Co-N bonds against the demetalation and the optimized d-band center accounts for the improved ORR kinetics.

关键词： Electrocatalysis Oxygen reduction reaction Non-noble metal catalysts Metal-nitrogen carbon catalysts Demetalation Structural stability

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Recently deepened insights regarding Mg corrosion and advanced engineering applications of Mg alloys

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Journal of Magnesium and Alloys 2023年第11期11卷 3948-3991页

作者： Guang-Ling Song Andrej Atrens Department of Ocean Science and Engineering Southern University of Science and Technology1088 Xueyuan BoulevardShenzhen 518055China The University of Queensland School of Mechanical and Mining EngineeringCentre for Advanced Materials Processing and Manufacturing(AMPAM)St LuciaQld 4072 Australia State Key Laboratory of Physical Chemistry of Solid Surfaces Xiamen University422 S.Siming RdXiamen 361005China

This review summarizes recent insights into the Mg corrosion mechanism, clarifies many critical controversial points regarding the Mg corrosion behaviour, and updates some efforts made to extend the industrial application of Mg alloys. Based on the new understandings gained so far, future research directions are also suggested in the review. This review has the following logic. The first section "1. Scope"is a consolidation of the new understandings or developments regarding the Mg corrosion mechanism and the new applications for Mg alloys. It also highlights some key points for the review. The second section "2. Widely accepted knowledge" briefly summarizes the general understanding of Mg corrosion gained so far, which acts as the foundation for the following sections. The third section "3. Recently deepened insights" mainly briefs on some new insights into Mg corrosion phenomena based on recent findings. Different interpretations on the corrosion behaviours are comprehensively discussed in the fourth section "4. Controversial points" and the conclusions are drawn in the subsection"4.5 Clarified points". Apart from the fundamental understandings, various efforts in the application of Mg alloys are presented in the fifth section "5. New applications". Following the research tendency as indicated in the review, prioritized research areas are suggested in "*** directions". The review is concluded with "7. Concluding remarks" at last.

关键词： Mg Corrosion Hydrogen Anode Intelligentization

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Interwoven Poly(Anthraquinonyl Sulfide)Nanosheets-Decorated Carbon Nanotubes as Core-Sheath Heteroarchitectured Cathodes for Polymer-Based Asymmetrical Full Batteries

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Energy & Environmental materials 2023年第5期6卷 468-476页

作者： Yonglin Wang Kai Chen Yunhai Zhu Jiazhi Wang Nan Jiang Yingkui Yang Key Laboratory of Catalysis and Energy Materials Chemistry of Ministry of Education&Hubei Key Laboratory of Catalysis and Materials Science South-Central Minzu UniversityWuhan 430074China State Key Laboratory of New Textile Materials and Advanced Processing Technologies Wuhan Textile UniversityWuhan 430200China School of Chemistry and Materials Science University of Science and Technology of ChinaHefei 230026China

Organic redox-active polymers provide promising alternatives to metal-containing inorganic compounds in Li-ion batteries(LIBs),whereas suffer from low actual capacities,poor rate/power capabilities,and inferior cycling ***,poly(anthraquinonyl sulfide)-coated carbon nanotubes(CNT@PAQS)are readily performed by in situ polymerization to form core-sheath ***,flower-like PAQS nanosheets are interwoven around CNTs to synergistically create robust 3D hierarchical networks with abundant cavities,internal channels,and sufficiently-exposed surfaces/edges,thereby promoting electron transport and making more active sites accessible for electrolytes and guest ***,the as-fabricated CNT@PAQS cathode delivers the large reversible capacity(200.5 mAh g^(-1)at 0.05 A g^(-1)),high-rate capability(161.5 mAh g^(-1)at 5.0 A g^(-1)),and impressive cycling stability(retaining 88.0%over 1000 cycles).In addition,an asymmetric full-battery using CNT@PAQS as a cathode and cyclized polyacrylonitrile-encapsulated CNTs as an anode is assembled that delivers a high energy density of 86.3 Wh kg^(-1),and retains 81.3%of initial capacity after 1000 *** work opens up an efficient strategy to combine highly conductive and redox-active phases into core-sheath heterostructures to unlock the barrier of high-rate charge *** further integration of two polymer-based electrodes into asymmetric full cells would also consolidate the development of low-cost,sustainable,and powerful batteries.

关键词： all-organic batteries core-sheath heterostructures lithium-ion batteries polymer electrode materials

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Bioinspired mechanically interlocking holey graphene@SiO_(2)anode

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Interdisciplinary materials 2022年第4期1卷 517-525页

作者： Fei Wang Xiaobin Liao Haoyu Wang Yan Zhao Jian Mao Donald G.Truhlar College of Materials Science and Engineering Sichuan UniversityChengduChina State Key Laboratory of Advanced Technology for Materials Synthesis and Processing Wuhan University of TechnologyWuhanChina School of Materials Science and Engineering University of New South WalesSydneyNew South WalesAustralia The Institute of Technological Sciences Wuhan UniversityWuhanChina Department of Chemistry Chemical Theory CenterMinnesota Supercomputing InstituteUniversity of MinnesotaMinneapolisMinnesotaUSA

Mechanically interlocking structures that can enhance adhesion at the interface and regulate the stress distribution have been widely observed in biological *** by the biological structures in the wings of beetles,we synthesized a holey graphene@SiO_(2)anode with strong mechanical interlocking,characterized it electrochemically,and explained its performance by finite element analysis and density functional calcula*** mechanically interlocking structure enhances lithium-ion(Li^(+))storage by transmitting the strain from SiO_(2)to the holey graphene and by a mechano-electrochemical coupling *** interlocking fit hinders the abscission of SiO_(2)and the distinctive structure reduces the stress and strain of SiO_(2)during(de)*** positive mechano-electrochemical coupling effect preserves the amount of electrochemically active phase(LixSi)during cycles and facilitates Li+***,the capacity shows only a slight attenuation after 8000 cycles(cycling stability),and the specific capacity is~1200 mA h g^(−1)at 5 A/g(rate-performance).This study furnishes a novel way to design high-performance Li^(+)/Na+/K^(+)/Al3^(+)anodes with large volume expansion.

关键词： holey graphene mechanically interlocking mechano-electrochemical coupling effect simulation SiO_(2) anode

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