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Self-powered temperature-changing system driven by wind energy

Microsystems & Nanoengineering 2024年第5期10卷 171-180页

作者： Jiayu Li Boxun Liu Mingyang Li Yahui Li Wangyang Ding Guanlin Liu Jun Luo Nan Chen Lingyu Wan Wenjuan Wei Center on Nanoenergy Research Institute of Science and Technology for Carbon Peak&NeutralityGuangxi UniversityNanning 530004China State Key Laboratory of Featured Metal Materials and Life-cycle Safety for Composite Structures School of Physical Science&TechnologyGuangxi UniversityNanning 530004China Department of Chemistry and the Tsinghua Center for Frontier Polymer Research Tsinghua UniversityBeijing 100084PR China State Key Laboratory of Pollution Control and Resource Reuse School of the EnvironmentNanjing UniversityNanjing 210023China Department of Micro/Nano Electronics School of Electronic Information and Electrical EngineeringShanghai Jjao Tong UniversityShanghai 200240PR China State Key Laboratory of Featured Metal Materials and Life-cycle Safety for Composite Structures MOE Key Laboratory of New Processing Technology for Nonferrous Metals and Materialsand School of ResourcesEnvironment and MaterialsGuangxi UniversityNanning 530004China

Research on outdoor,mobile,and self-powered temperature-control devices has always been highly *** devices can reduce energy consumption for cooling and heating,and they have broad market *** this basis,a rotary disc-shaped triboelectric nanogenerator(TENG)with a maximum open-circuit voltage of 6913 V,a maximum short-circuit current of 85μA,and a maximum transferred charge of 1.3μC was *** synthesized a ferroelectric ceramic composed of 0.15PbTiO_(3)-0.85PbSc_(o.5)Ta_(o.5)O_(3)(0.15PT-0.85PST),which exhibited excellent electrothermal effects at room *** quenching,the electrothermal effect(A Tmax)and energy harvesting properties of the device were 1.574 K and 0.542 J/cm3,***,for the frst time,we proposed a self-powered temperature quantification control system with a rotary disc-shaped *** device effectively harnessed wind and water energy,in addition to other types of *** system consisted of energy collecting cups,a rotating disc-shaped FEP-rabbit fur TENG,a circuit management module,and a ferroelectric ceramic chip *** the circuit management module,the system converted external wind energy into a high-voltage electric field at the two ends of the 0.15PT-0.85PST ceramic chip to fully stimulate the electrothermal *** a speed of 200 rpm,the temperature change in the insulated cup within 276 s was 0.49 K,and the volume of the insulated cup was 300 times greater than that of the 0.15PT-0.85PST ceramic *** with the results reported in previous work,the cooling and heating times were both reduced by 31%,and the temperature changes for both cooling and heating increased by 81%.Moreover,the heating and cooling temperatures of the device optimized on this basis were increased to 1.19K and 0.93 K,*** great improvement in the temperature variation performance confrmed the great potential of the device for *** research could serve as a reference for reduci

关键词： ceramic shaped ferroelectric

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Toluene Processed All-Polymer Solar Cells with 18%Efficiency and Enhanced Stability Enabled by Solid Additive:Comparison Between Sequential-processing and Blend-Casting

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Energy & Environmental materials 2024年第4期7卷 247-254页

作者： Guoping Zhang Chaoyue Zhao Liangxiang Zhu Lihong Wang Wenzhao Xiong Huawei Hu Qing Bai Yaping Wang Chen Xie Peng You He Yan Dan Wu Tao Yang Mingxia Qiu Shunpu Li Guangye Zhang College of New Materials and New Energies Shenzhen Technology UniversityShenzhen 518118China Department of Chemistry and Hong Kong Branch of Chinese National Engineering Research Center for Tissue Restoration and Reconstruction The Hong Kong University of Science and TechnologyClear Water BayHong Kong 999077China State Key Laboratory for Modification of Chemical Fibers and Polymer Materials Center for Advanced Low-dimension MaterialsCollege of Materials Science and EngineeringDonghua UniversityShanghai 201620China Julong College Shenzhen Technology UniversityShenzhen 518118China

The emergence of polymerized small molecule acceptors(PSMAs)has significantly improved the performance of all-polymer solar cells(all-PSCs).However,the pace of device engineering lacks behind that of materials development,so that a majority of the PSMAs have not fulfilled their ***,most high-performance all-PSCs rely on the use of chloroform as the processing *** instance,the recent highperformance PSMA,named PJ1-γ,with high LUMO,and HOMO levels,could only achieve a PCE of 16.1%with a high-energy-level donor(JD40)using ***,we present a methodology combining sequential processing(SqP)with the addition of 0.5%wt PC_(71)BM as a solid additive(SA)to achieve an impressive efficiency of 18.0%for all-PSCs processed from toluene,an aromatic hydrocarbon *** to the conventional blend-casting(BC)method whose best efficiency(16.7%)could only be achieved using chloroform,the SqP method significantly boosted the device efficiency using toluene as the processing *** addition,the donor we employ is the classic PM6 that has deeper energy levels than JD40,which provides low energy loss for the *** compare the results with another PSMA(PYF-T-o)with the same ***,an improved photostability of the SqP devices with the incorporation of SA is demonstrated.

关键词： all-polymers solar cells sequential processing solid additive

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In-situ synthesis of gadolinium niobate quasi-binary composites with balanced mechanical and thermal properties for thermal barrier coatings

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Journal of advanced Ceramics 2022年第9期11卷 1445-1456页

作者： Yi HAN Peng-an ZONG Muzhang HUANG Zesheng YANG Yingjie FENG Wei PAN Peng ZHANG Chunlei WAN State Key Laboratory of New Ceramics and Fine Processing School of Materials Science and EngineeringTsinghua UniversityBeijing 100084China Institute of Welding and Surface Engineering Technology Faculty of Materials and ManufacturingBeijing University of TechnologyBeijing 100124China

Yttria-stabilized zirconia(YSZ)has been used as a thermal barrier coating(TBC)material in gas turbines for several *** continuous efforts have been made to develop novel TBC materials that can work at a higher temperature,no single material other than YSZ has all the desired attributes for the *** this paper,we report the in-situ synthesis of quasi-binary GdNbO_(4)/Gd_(3)NbO_(7)composites based on the simple Gd_(2)O_(3)-Nb_(2)O_(5)binary phase *** fracture toughness of these quasi-binary composites is remarkably enhanced compared with the value predicted by the rule of mixtures because the ferroelastic domain switching is more activated due to the residual stress in the quasi-binary composites,which triggers more crack defections due to the enlarged process ***,the Gd_(3)NbO_(7)phase provides a low thermal conductivity due to the substantial chemical inhomogeneity,which diffuses ***_(3)NbO_(7)/GdNbO_(4)exhibits a balanced thermal conductivity of 1.6 W/(m·K)at 1073 K and a toughness value of 2.76 MPa·m0.5,and these values are among the best comprehensive properties that have been obtained for new TBC *** work demonstrates a feasible approach of designing a new TBC material with balanced properties and can be easily fabricated.

关键词： thermal barrier coating(TBC) fracture toughness thermal conductivity residual stress

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Orbital-level band gap engineering of RuO₂ for enhanced acidic water oxidation

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Nature Communications 2025年第1期16卷 1-13页

作者： Wang, Xing Pi, Wei Li, Zhaobing Hu, Sheng Bao, Haifeng Xu, Weilin Yao, Na State Key Laboratory of New Textile Materials and Advanced Processing School of Materials Science and Engineering Wuhan Textile University Wuhan 430200 China

Developing efficient and stable oxygen evolution reaction electrocatalysts under acidic conditions is crucial for advancing proton-exchange membrane water electrolysers commercialization. Here, we develop a representative strategy through p-orbital atoms (N, P, S, Se) doping in RuO₂ to precisely regulate the lattice oxygen-mediated mechanism-oxygen vacancy site mechanism pathway. In situ and ex situ measurements along with theoretical calculations demonstrate that Se doping dynamically adjusts the band gap between the Ru-e_g and O-p orbitals during the oxygen evolution reaction process. This modulation accelerates electron diffusion to the external circuit, promotes the lattice oxygen-mediated process, and enhances catalytic activity. Additionally, it facilitates electron feedback and stabilizes oxygen vacancies, thereby promoting the oxygen vacancy site mechanism process and enhancing catalytic stability. The resulting Se-RuO_x catalyst achieves efficient proton-exchange membrane water electrolysers performance under industrial conditions with a minimal charge overpotential of 1.67 V to achieve a current density of 1 A cm⁻² and maintain long-term cyclability for over 1000 h. This work presents a unique method for guiding the future development of high-performance metal oxide catalysts. © The Author(s) 2025.

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Dimensionality-driven metal to Mott insulator transition in two-dimensional 1T-TaSe2

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National Science Review 2024年第3期11卷 108-118页

作者： Ning Tian Zhe Huang Bo Gyu Jang Shuaifei Guo Ya-Jun Yan Jingjing Gao Yijun Yu Jinwoong Hwang Cenyao Tang Meixiao Wang Xuan Luo Yu Ping Sun Zhongkai Liu Dong-Lai Feng Xianhui Chen Sung-Kwan Mo Minjae Kim Young-Woo Son Dawei Shen Wei Ruan Yuanbo Zhang State Key Laboratory of Surface Physics New Cornerstone Science Laboratory and Department of PhysicsFudan University Shanghai Qi Zhi Institute Shanghai Research Center for Quantum Sciences Institute for Nanoelectronic Devices and Quantum Computing Fudan University Zhangjiang Fudan International Innovation Center Fudan University State Key Laboratory of Functional Materials for Informatics Shanghai Institute of Microsystem and Information Technology(SIMIT)Chinese Academy of Sciences School of Physical Science and Technology ShanghaiTech University Korea Institute for Advanced Study School of Emerging Technology and Department of Physics University of Science and Technology of China Advanced Light Source Lawrence Berkeley National Laboratory ShanghaiTech Laboratory for Topological Physics Key Laboratory of Materials Physics Institute of Solid State Physics Hefei Institutes of Physical ScienceChinese Academy of Sciences High Magnetic Field Laboratory Hefei Institutes of Physical Science Chinese Academy of Sciences Collaborative Innovation Centre of Advanced Microstructures Nanjing University Department of Physics University of Science and Technology of China and Key Laboratory of Strongly Coupled Quantum Matter Physics Chinese Academy of Sciences National Synchrotron Radiation Laboratory University of Science and Technology of China

Two-dimensional materials represent a major frontier for research into exotic many-body quantum phenomena. In the extreme two-dimensional limit, electron-electron interaction often dominates over other electronic energy scales, leading to strongly correlated effects such as quantum spin liquid and unconventional *** dominance is conventionally attributed to the lack of electron screening in the third dimension. Here, we discover an intriguing metal to Mott insulator transition in 1T-TaSe2that defies conventional wisdom. Specifically, we find that dimensionality crossover, instead of reduced screening, drives the transition in atomically thin 1T-TaSe2. A dispersive band crossing the Fermi level is found to be responsible for the bulk metallicity in the material. Reducing the dimensionality,however, effectively quenches the kinetic energy of these initially itinerant electrons, and drives the material into a Mott insulating *** dimensionality-driven metal to Mott insulator transition resolves the long-standing dichotomy between metallic bulk and insulating surface of 1T-TaSe2. Our work further reveals a new pathway for modulating two-dimensional materials that enables exploring strongly correlated systems across uncharted parameter space.

关键词： two-dimensional materials 1T-TaSe2 dimensionality crossover metal to Mott insulator transition

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How the surface Cu layer affected the activity of Ni foil for alkaline hydrogen evolution

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Journal of materials Science & technology 2024年第2期169卷 11-18页

作者： Qingfeng Hu Yuan Liu Xuerong Zheng Jinfeng Zhang Jiajun Wang Xiaopeng Han Yida Deng Wenbin Hu School of Materials Science and Engineering Key Laboratory of Advanced Ceramics and Machining Technology of Ministry of EducationTianjin UniversityTianjin 300072China State Key Laboratory of Marine Resource Utilization in South China Sea School of Materials Science and EngineeringHainan UniversityHaikou 570228China Joint School of National University of Singapore and Tianjin University International Campus of Tianjin UniversityBinhai New CityFuzhou 350207China

Synthesizing bimetallic nanomaterials,with noble metals as the surface layers and inert metals as the substrates,has been proven to be an effective way to reduce the use of noble metals with maintained catalytic ***,an atomic diffusion from the inert substrate to the surface during the long-term operation has been reported to significantly decrease the *** this work,a series of catalysis-inert Cu-coated Ni foil were fabricated through electrodeposition and their activities for alkaline hydrogen evolution were ***,the Ni/Cu-60 sample showed a similar catalytic property with pure Ni foil and only a slight decrease in HER activity was *** X-ray photoelectron spectroscopy(XPS)results indicated a decreased electron concentration of Cu in Ni/Cu-60,and theoretical calculations further demonstrated the electron transfer between the Ni substrate and Cu *** results reveal that a specific composition or structure of an inert metal layer might not significantly decrease the electrocatalytic activity of active ***,there are more possibilities for the rational design of metal-based catalysts for electrocatalysis.

关键词： Bimetallic heterostructure Charge redistribution Water splitting Alkaline hydrogen evolution

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Manganese-based oxides cathodes for potassium-ion batteries: a review

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Journal of Energy Chemistry 2025年 108卷 1-18页

作者： Yue, Qinggang Xia, Maoting Zhou, Jiang Cheng, Juanjuan Lu, Bingan School of Physics and Electronics Hunan University Hunan Changsha410082 China State Key Laboratory of Advanced Design and Manufacturing for Vehicle Body Hunan University Hunan Changsha410082 China School of Materials Science and Engineering and Key Laboratory of Nonferrous Metal Materials Science and Engineering Ministry of Education Central South University Hunan Changsha410083 China School of Materials Science and Engineering Hunan Provincial Key Lab of Advanced Materials for New Energy Storage and Conversion Hunan University of Science and Technology Hunan Xiangtan411201 China

Potassium-ion batteries (PIBs) were recognized for their natural abundance, high theoretical output voltage, and the availability of commercialized graphite anodes. However, the development of high-performance manganese-based layered oxide cathodes—a leading candidate for PIB systems—has been fundamentally constrained by irreversible phase transitions (PT) during the cycling process, manifesting as severe structural degradation and capacity fading. This review presents a transformative paradigm integrating machine learning (ML) with multiscale characterization to analyse the complex phase transition mechanisms in Mn-based cathodes. Through systematic ML-driven interrogation of structure–property relationships, we establish quantitative descriptors for phase stability and develop predictive models for transition dynamics. Furthermore, we highlight recent breakthroughs in cross-disciplinary approaches, enabling the rational design of PT-mitigated cathode architectures. By consolidating these insights into a unified knowledge framework, this work provides strategic guidelines for developing structurally robust Mn-based cathodes and outlines future research directions for next-generation PIB systems. © 2025 Science Press and Dalian Institute of Chemical Physics, Chinese Academy of Sciences.

关键词： Setting

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Tunable Ru-Ru2P heterostructures with charge redistribution for efficient pH-universal hydrogen evolution

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InfoMat 2022年第5期4卷 164-173页

作者： Ding Chen Ruohan Yu Ruihu Lu Zonghua Pu Pengyan Wang Jiawei Zhu Pengxia Ji Dulan Wu Jinsong Wu Yan Zhao Zongkui Kou Jun Yu Shichun Mu State Key Laboratory of Advanced Technology for Materials Synthesis and Processing Wuhan University of TechnologyWuhanChina Foshan Xianhu Laboratory of the Advanced Energy Science and Technology Guangdong Laboratory Xianhu Hydrogen ValleyFoshanChina Nanostructure Research Centre(NRC) Wuhan University of TechnologyWuhanChina State Key Laboratory of Silicate Materials for Architectures International School of Materials Science and EngineeringWuhan University of TechnologyWuhanChina

Designing synergistic heterogeneous catalytic interfaces is the key to developing highly compatible pH-universal electrocatalysts for complex chemical envi*** theoretical calculation results demonstrate that the Ru-Ru2P heterointerface can not only promote the redistribution of charges,but also reduce the d-band center,and then enhances the adsorption capacity of the key ***,in situ and facile synthesis of Ru-Ru2P heterostructures is severely limited by thermodynamic ***,we propose a molten salt-assisted catalytic synthesis scheme,and successfully build a series of homologous metallic Ru-Ru2P heterostructure catalysts with different molar ratios of Ru to P under atmospheric pressure and low-temperature(400C).The resultant Ru-Ru2P with rich heterostructures show the Pt-like HER performance in different pH ***,it is prominent under alkaline conditions(18 mV@10 mA cm^(2)),which outperforms the Pt catalyst(37 mV@10 mA cm^(2)).Furthermore,Ru-Ru2P heterostructures also show certain potential in the electrolysis of seawater to produce *** work represents a significant supplement of high-efficiency pH-universal HER catalysts,and provides a new light on interface engineering in energy technology fields and beyond.

关键词： DFT calculation heterostructure molten salt-assisted synthesis pH-universal hydrogen evolution ruthenium phosphide

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Image processing based three-dimensional model reconstruction for cross-platform numerical simulation

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China Foundry 2023年第2期20卷 139-147页

作者： Yu-cheng Sun Yu-hang Huang Na Li Xiao Han Ai-long Jiang Jin-wu Kang Ji-wu Wang Hai-liang Yu State Key Laboratory of Engine Reliability Weichai Power Co.Ltd.Weifang 261061ShandongChina School of Mechanical Engineering Central South UniversityChangsha 41000China School of Mechanical Electronic and Control EngineeringBeijing Jiaotong UniversityBeijing 100044China Key Laboratory for Advanced Materials Processing Technology School of Materials Science and EngineeringTsinghua UniversityBeijing 100084China

Numerical simulation is the most powerful computational and analysis tool for a large variety of engineering and physical *** a complex problem relating to multi-field,multi-process and multi-scale,different computing tools have to be developed so as to solve particular fields at different scales and for different ***,the integration of different types of software is ***,it is difficult to perform the transfer of the meshes and simulated results among software packages because of the lack of shared data formats or encrypted data *** image processing based method for three-dimensional model reconstruction for numerical simulation was proposed,which presents a solution to the integration problem by a series of slice or projection images obtained by the post-processing modules of the numerical simulation *** means of mapping image pixels to meshes of either finite difference or finite element models,the geometry contour can be extracted to export the stereolithography *** values of results,represented by color,can be deduced and assigned to the *** the models with data can be directly or indirectly integrated into other software as a continued or new numerical *** three-dimensional reconstruction method has been validated in numerical simulation of castings and case studies were provided in this study.

关键词： cross-platform numerical simulation 3D model reconstruction image processing slice

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Enhanced breakdown strength and energy storage density of AgNbO_(3)ceramics via tape casting

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Rare Metals 2023年第2期42卷 495-502页

作者： Ming-Yuan Zhao Jing Wang Lin Chen Hao Yuan Mao-Hua Zhang Su-Wei Zhang Lei Zhao Key Laboratory of High-Precision Computation and Application of Quantum Field Theory of Hebei Province College of Physics Science and TechnologyHebei UniversityBaoding071002China State Key Laboratory of Mechanics and Control of Mechanical Structures College of Aerospace EngineeringNanjing University of Aeronautics and AstronauticsNanjing210016China Department of Materials and Earth Sciences Nonmetallic Inorganic MaterialsTechnical University of DarmstadtDarmstadt64287Germany State Key Laboratory of New Ceramics and Fine Processing School of Materials Science and EngineeringTsinghua UniversityBeijing100084China

Antiferroelectric materials are promising candidates for energy-storage applications due to their double hysteresis loops,which can deliver high power *** the antiferroelectric materials,AgNbO_(3)is proved attractive due to its environmental-friendliness and high potential for achieving excellent energy storage ***,the recoverable energy storage density of AgNbO_(3)ceramics is limited by their relatively low breakdown ***,the breakdown strength of the pure AgNbO_(3)ceramics prepared using the tape casting method is enhanced to 307 kV·cm^(-1),which is,to the best of our knowledge,among the highest values reported for pure AgNbO-3bulk *** high breakdown strength may be due to its dense microstructure and good crystallinity obtained by the tape casting method and the optimized sintering *** to its enhanced breakdown strength,AgNbO_(3)ceramics show high recoverable energy storage density of 2.8 J·cm^(-3).These results have led to the development of lead-free antiferroelectric materials and devices with high energy storage density.

关键词： AgNbO_(3) Energy storage performance Antiferroelectric Tape casting

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