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Monitoring of lubrication and wear in-situ by triboelectrification under grease lubrication

Friction 2025年第2期13卷 89-98页

作者： Yiming Lei Yange Feng Zixiang Wu Qiang Gao Zhuopei Zhang Wenpeng Wang Liucheng Wang Youqiang Wang Daoai Wang State Key Laboratory of Solid Lubrication Lanzhou Institute of Chemical PhysicsChinese Academy of SciencesLanzhou 730000China Shandong Laboratory of Advanced Materials and Green Manufacturing at Yantai Yantai 265503China School of Mechanical and Automotive Engineering Qingdao University of TechnologyQingdao 266520China Center of Materials Science and Optoelectronics Engineering University of Chinese Academy of SciencesBeijing 100049China Qingdao Center of Resource Chemistry and New Materials Qingdao 266104China

The stable operation of friction pairs is one of the most critical factors to maintain the stable operation of mechanical *** real-time monitoring of lubrication state of the friction pair is very important to ensure the normal operation of machinery and realize early warning of wear failure,but it is also a big *** this article,a new lubrication insitu monitoring system is designed,which can monitor the lubrication and wear state of friction pairs through *** current acquisition module and friction coefficient acquisition module are integrated into a high vacuum hydrodynamic oil film thickness measuring instrument to explore the intrinsic relationship between triboelectricity and friction coefficient *** severe wear occurs,the oil film at the interface of the friction pair is no longer complete,and the accumulated triboelectric charge at the interface of the friction pair breaks down the air and causes discharge,the friction current suddenly increases from nanoampere level to microampere *** time node when discharge occurs at the steel ball interface is well consistent with the time node when the friction pair suffers serious *** to the corresponding relationship between the triboelectric current and the friction and wear status of the friction pair,an early wear warning monitoring system is designed to monitor the operating status of the friction pair in real time through triboelectric *** the mechanical friction pair is worn,the early warning system will send out sound and light alarm signals and send real-time warnings to the mobile terminal through the Internet of Things,providing a new and reliable method for real-time monitoring of friction and wear of grease-lubricated machinery.

关键词： friction sensing wear warning triboelectric sensor in-situ monitoring real-time

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High Transparent and Robust Ionically Conductive Cellulose Hydrogels for Flexible and Antifreezing Strain Sensors

SSRN

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SSRN 2023年

作者： Li, Xiaoyan Tu, Hu Wang, Peng Liu, Yuncui Shao, Xiaoyu Tan, Sirui Cai, Guangming Zhang, Ruquan State Key Laboratory of New Textile Materials and Advanced Processing Technologies Hubei Key Laboratory of Advanced Textile Materials & Application Key Laboratory of Textile Fiber & Product Ministry of Education Wuhan Textile University Wuhan430200 China

The development of flexible sensors with multifunction such as high transparency, good mechanical properties and durability, biodegradability, excellent antifreezing ability and sensitivity still remains a great challenge. Herein, cellulose hydrogels were constructed from "green" LiOH/urea solvents via chemically–physically double crosslinked strategy. 1,4-butanediol diglycidyl ether as a long-chain chemical crosslinker was used to enlarge the activity domains of cellulose chains of the crosslinked networks in hydrogels, further improving their elasticity, flexibility and durability. During the physically crosslinked process Li ions were retained within the hydrogel and glycerol was introduced, which could effectively improve the hydrogels mechanical properties and significantly enhance its conductivity. At the same time, Li ions and glycerol could form hydrogen bonds with water molecules, greatly enhancing the hydrogel's freeze resistance and water retention. The ionically conductive cellulose hydrogels with high transparence could sensitively monitor the human motions including large motions and subtle actions, as well as the detection of heartbeat rate, pulse beat and body temperature changes and the usage as an electronic skin, which showed great potential for visually monitoring human physiological functions in extreme environments. © 2023, The Authors. All rights reserved.

关键词： Cellulose

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Local symmetry distortion induced anomalous thermal conduction in thermoelectric layered oxyselenides

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npj Computational materials 2023年第1期9卷 658-665页

作者： Bin Wei Jiale Li Yueyang Yang Wang Li Zhifang Zhou Yunpeng Zheng Wenyu Zhang Yifan Chai Zheng Chang Ce-Wen Nan Yuan-Hua Lin Henan Key Laboratory of Materials on Deep-Earth Engineering School of Materials Science and EngineeringHenan Polytechnic UniversityJiaozuo 454000PR China State Key Laboratory of New Ceramics and Fine Processing School of Materials Science and Engineering Tsinghua UniversityBeijing 100084PR China School of Materials and Metallurgy Inner Mongolia University of Science and TechnologyBaotou 014010PR China School of Naval Architecture and Maritime Zhejiang Ocean UniversityZhoushan 316022PR China

Polyhedral distortion,associated closely with the atomic arrangement and interatomic interactions,drives many unique behaviors in solids,such as phase transition and negative thermal *** thermoelectric heteroanionic oxides,the anionic polyhedra are widely present,but their effect on thermal transport is rarely ***,we report an anomalous thermal conduction induced by local symmetry distortion in layered oxyselenides via solving the Boltzmann transport equation based on first-principles *** found interestingly that lighter BiCuSeO exhibits lower thermal conductivity than heavier *** to the different distorted degrees of CuSe4 and AgSe4 tetrahedrons,Cu prefers the in-plane vibration,while Ag has more tendency of out-of-plane ***,the heat-carrying phonons dominated by the rattling-like vibration of Cu are significantly suppressed,resulting in lower thermal conductivity of *** study highlights the importance of polyhedral distortion in regulating thermal conduction in layered heteroanionic materials.

关键词： distortion thermal conduction

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具有气-液-固三相界面的二维/二维石墨相氮化碳@碘氧铋S型异质结高效光催化二氧化碳还原

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Science China materials 2024年第6期67卷 1830-1838页

作者：杨超张庆贺王往程蓓余家国曹少文 State Key Laboratory of Advanced Technology for Materials Synthesis and Processing Wuhan University of TechnologyWuhan 430070China Hubei Technology Innovation Center for Advanced Composites Wuhan University of TechnologyWuhan 430070China Laboratory of Solar Fuel Faculty of Materials Science and ChemistryChina University of GeosciencesWuhan 430074China

在过去几十年中,将二氧化碳光还原转化为有用的化学燃料(甲烷、一氧化碳和甲醇等)受到了极大的关注.然而,由于光生电荷的复合速度快,二氧化碳和水分子的共吸附不足,目前的二氧化碳光还原系统的效率还远远不能令人满意.本文报道了在疏水... 详细信息

在过去几十年中,将二氧化碳光还原转化为有用的化学燃料(甲烷、一氧化碳和甲醇等)受到了极大的关注.然而,由于光生电荷的复合速度快,二氧化碳和水分子的共吸附不足,目前的二氧化碳光还原系统的效率还远远不能令人满意.本文报道了在疏水碳纤维纸上构建一个紧密的二维/二维石墨相氮化碳@碘氧铋梯型(S型)异质结,用于高效的二氧化碳光还原.所制备的异质结具有良好的一氧化碳选择性(77.8%)和活性(458.0μmol h^(-1)m^(-2)).良好的光催化性能归因于良好设计的S型异质结结构,提高了电荷分离效率,以及形成了气-液-固三相界面,充分保证了二氧化碳和水的同时供给.这项工作为高效光催化二氧化碳还原系统的设计提供了新思路.

关键词： CO_(2)photoreduction S-scheme heterojunction tri-phase interface separation of charge carriers co-adsorption of CO_(2)and H2O

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Highly dispersed Ag clusters for active and stable hydrogen peroxide production

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Nano Research 2022年第7期15卷 5842-5847页

作者： Mengmeng Jin Wei Liu Jiaqiang Sun Xinzhong Wang Shusheng Zhang Jun Luo Xijun Liu Information Technology Research Institute Shenzhen Institute of Information TechnologyShenzhen 518172China Institute for New Energy Materials and Low-Carbon Technologies Tianjin Key Lab for Photoelectric Materials&DevicesSchool of Materials Science and EngineeringTianjin University of TechnologyTianjin 300384China State Key Laboratory of Coal Conversion Institute of Coal ChemistryChinese Academy of SciencesTaiyuan 030001China College of Chemistry Zhengzhou UniversityZhengzhou 450000China MOE Key Laboratory of New Processing Technology for Non-Ferrous Metals and Materials and Guangxi Key Laboratory of Processing for NonFerrous Metals and Featured MaterialsSchool of ResourceEnvironments and MaterialsGuangxi UniversityNanning 530004China

The electrosynthesis of hydrogen peroxide(H2O2)from oxygen reduction reaction(ORR)via a two-electron pathway provides an appealing alternative to the energy-intensive anthraquinone route;however,the development of ORR with high selectivity and durability for H2O2 production is still ***,we demonstrate an active and stable catalyst,composing of highly dispersed Ag nanoclusters on N-doped hollow carbon spheres(NC-Ag/NHCS),which can effectively reduce O2 molecules into H2O2 with a selectivity of 89%–91%in a potential range from 0.2 to 0.7 V(*** hydrogen electrode(RHE))in acidic ***,NC-Ag/NHCS achieve a mass activity of 27.1 A·g^(−1) and a yield rate of 408 mmol·gcat.^(−1)·h^(−1) at 0.7 V,both of which are comparable with the best-reported ***,NC-Ag/NHCS enable catalyzing H2O2 production with a stable current density over 48-h electrolysis and only about 9.8%loss in selectivity after 10,000 *** analyses indicate that Ag nanoclusters can contribute more electrons to favor the protonation of adsorbed O2,thus leading to a high H2O2 *** work confirms the great potential of metal nanocluster-based materials for H2O2 electrosynthesis under ambient conditions.

关键词： hydrogen peroxide synthesis electrochemical route Ag nanoclusters oxygen reduction reaction energy-efficient

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Ultralow-voltage hydrogen production and simultaneous Rhodamine B beneficiation in neutral wastewater

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Journal of Energy Chemistry 2023年第6期81卷 574-582,I0013页

作者： Xiang Peng Song Xie Shijian Xiong Rong Li Peng Wang Xuming Zhang Zhitian Liu Liangsheng Hu Biao Gao Peter Kelly Paul K.Chu Hubei Key Laboratory of Plasma Chemistry and Advanced Materials Hubei Engineering Technology Research Center of Optoelectronic and New Energy MaterialsSchool of Materials Science and EngineeringWuhan Institute of TechnologyWuhan 430205HubeiChina Department of Physics Department of Materials Science and EngineeringDepartment of Biomedical EngineeringCity University of Hong KongTat Chee AvenueKowloon 999077Hong KongChina State Key Laboratory of Refractories and Metallurgy and Institute of Advanced Materials and Nanotechnology Wuhan University of Science and TechnologyWuhan 430081HubeiChina Department of Chemistry and Key Laboratory for Preparation and Application of Ordered Structural Materials of Guangdong Province Shantou UniversityShantou 515063GuangdongChina Surface Engineering Group Manchester Metropolitan UniversityManchester M15GDUK

Electrocatalytic water splitting for hydrogen production is hampered by the sluggish oxygen evolution reaction(OER)and large power consumption and replacing the OER with thermodynamically favourable reactions can improve the energy conversion *** iron corrodes easily and even self-corrodes to form magnetic iron oxide species and generate corrosion currents,a novel strategy to integrate the hydrogen evolution reaction(HER)with waste Fe upgrading reaction(FUR)is proposed and demonstrated for energy-efficient hydrogen production in neutral *** heterostructured MoSe_(2)/MoO_(2) grown on carbon cloth(MSM/CC)shows superior HER performance to that of commercial Pt/C at high current *** replacing conventional OER with FUR,the potential required to afford the anodic current density of 10 m A cm^(-2)decreases by 95%.The HER/FUR overall reaction shows an ultralow voltage of 0.68 V for 10 m A cm^(-2)with a power equivalent of 2.69 k Wh per m^(3)H_(2).Additionally,the Fe species formed at the anode extract the Rhodamine B(Rh B)pollutant by flocculation and also produce nanosized magnetic powder and beneficiated Rh B for value-adding *** work demonstrates both energy-saving hydrogen production and pollutant recycling without carbon emission by a single system and reveals a new direction to integrate hydrogen production with environmental recovery to achieve carbon neutrality.

关键词： Energy-saving hydrogen production Hydrogen evolution reaction Neutral water splitting MoSe_(2)/MoO_(2)heterostructure Environmental recovery

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MXene Sediment-Based Poly(vinyl alcohol)/Sodium Alginate Aerogel Evaporator with Vertically Aligned Channels for Highly Efficient Solar Steam Generation

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Nano-Micro Letters 2024年第10期16卷 638-654页

作者： Tian Wang Meng Li Hongxing Xu Xiao Wang Mingshu Jia Xianguang Hou Shuai Gao Qingman Liu Qihang Yang Mingwei Tian Lijun Qu Zhenhua Song Xiaohu Wu Lili Wang Xiansheng Zhang Shandong Key Laboratory of Medical and Health Textile Materials College of Textiles and ClothingState Key Laboratory of Bio-Fibers and Eco-TextilesResearch Center for Intelligent and Wearable TechnologyQingdao UniversityQingdao 266071People's Republic of China Department of Pharmacology Qingdao University School of PharmacyQingdao UniversityQingdao 266071People's Republic of China Shandong Institute of Advanced Technology Jinan 250100People's Republic of China College of Electromechanical Engineering Qingdao University of Science and TechnologyQingdao 266061People's Republic of China

Solar-driven interfacial evaporation from seawater is considered an effective way to alleviate the emerging freshwater crisis because of its green and environmentally friendly ***,developing an evaporator with high efficiency,stability,and salt resistance remains a key ***,with an internal photothermal conversion efficiency of 100%,has received tremendous research interest as a photothermal ***,the process to prepare the MXene with monolayer is inefficient and generates a large amount of“waste”MXene sediments(MS).Here,MXene sediments is selected as the photothermal material,and a three-dimensional MXene sediments/poly(vinyl alcohol)/sodium alginate aerogel evaporator with vertically aligned pores by directional freezing method is innovatively *** vertical porous structure enables the evaporator to improve water transport,light capture,and high evaporation *** swabs and polypropylene are used as the water channel and support,respectively,thus fabricating a self-floating *** evaporator exhibits an evaporation rate of 3.6 kg m^(-2)h^(-1)under one-sun illumination,and 18.37 kg m^(-2)of freshwater is collected in the condensation collection device after 7 h of outdoor sun *** evaporator also displays excellent oil and salt *** research fully utilizes“waste”MS,enabling a self-floating evaporation device for freshwater collection.

关键词： MXene sediments Porous structure Desalination Self-floating

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Tailored lithium metal/polymer electrolyte interface with LiTa_(2)PO_(8) fillers in PEO-based composite electrolyte

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Rare Metals 2022年第8期41卷 2826-2833页

作者： Bing Huang Zhi-Hong Li Yu-Mei Zhu Yong Che Chang-An Wang Key Laboratory for Advanced Ceramics and Machining Technology of Ministry of Education School of Materials Science and EngineeringTianjin UniversityTianjin300072China State Key Laboratory of New Ceramics and Fine Processing School of Materials Science and EngineeringTsinghua UniversityBeijing100084China Enpower Energy Corp. Beijing102600China

The unstable Li/PEO-based electrolyte interface in allsolid-state lithium metal batteries usually leads to high interfacial resistance,low Coulombie efficiency and fast lithium dendrites growth even under a low current *** interface composition directly determines the interfacial integrity,dynamic Li^(+)/e^(-)transport processes and the subsequent Li+plating/stripping behavior;thus,it is of significance to regulate the interphase to have better safety and higher energy density for all-solid-state lithium metal ***,by incorporation of Li^+conducting LiTa_(2) PO_(8) fillers in PEO-based polymer electrolyte.

关键词： electrolyte lithium interface

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High-Performance Ag_(2)Se/Methyl Cellulose Thermoelectric Composites for Flexible Power Generators

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Energy Material Advances 2024年第1期5卷 275-282页

作者： Zuo Xiao Qiufeng Meng Yong Du Ping Wei Jie Qin Jingyu Chen Zhongchang Wang Per Eklund School of Materials Science and Engineering Shanghai Institute of Technology100 Haiquan RoadShanghai 201418China State Key Laboratory of Advanced Technology for Materials Synthesis and Processing Wuhan University of TechnologyWuhan 430070China The Center of Functional Materials for Working Fluids of Oil and Gas Field School of New Energy and MaterialsSouthwest Petroleum UniversityChengdu 610500China Sichuan Engineering Technology Research Center of Basalt Fiber Composites Development and Application State Key Laboratory of Oil and Gas Reservoir Geology and ExploitationSouthwest Petroleum UniversityChengdu 610500SichuanChina International Iberian Nanotechnology Laboratory Av.Mestre Jose Veiga s/n4715-330 BragaPortugal Thin Film Physics Division Department of PhysicsChemistry and Biology(IFM)Linköping UniversitySE-58183 LinköpingSweden

Flexible thermoelectric generators(FTEGs)offer a promising solution for powering wearable electronics,while their practical applications are mainly obstructed by the moderate properties of flexible thermoelectric(TE)***,flexible Ag_(2)Se nanowire(NW)/methyl cellulose(MC)composite films were developed via facile screen-printing technology combined with cold pressing and annealing treatment,and a highest power factor of 1,641.58μW m^(-1)K^(-2)at 360 K was *** reasons for the high TE performance of the Ag_(2)Se NW/MC composite films were because,after the annealing treatment,the Ag_(2)Se NWs were sintered to form conductive network structures,the crystallinity of Ag_(2)Se was markedly enhanced,and the content of insulating phase MC in the composite film was *** Ag_(2)Se NW/MC composite film held appreciable flexibility,as its room-temperature power factor(1,312.08μW m^(-1)K^(-2))can retain~93%after bending for 1,000 cycles at a radius of 4 ***,the assembled FTEG consisting of 4 strips can generate a maximal power density of 3.51 W m^(-2)at a temperature difference of 14.1 *** results open an effective and large-scale strategy for fabricating high-performance flexible TE materials and energy-harvesting devices.

关键词： annealing treatment cold pressing Ag Se nanowires methyl cellulose flexible thermoelectric generators ftegs offer thermoelectric composites flexible thermoelectric generators power factor

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Microfluidic synthesis of hollow CsPbBr_(3) perovskite nanocrystals through the nanoscale Kirkendall effect

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Nano Research 2024年第9期17卷 8487-8494页

作者： Yue Chen Xiaoyu Zhang Jinzhou Jiang Gaoyu Chen Kunhong Zhou Xinwen Zhang Fajing Li Caojin Yuan Jianchun Bao Xiangxing Xu Jiangsu Collaborative Innovation Center of Biomedical Functional Materials Jiangsu Key Laboratory of New Power BatteriesSchool of Chemistry and Materials ScienceNanjing Normal UniversityNanjing 210023China Key Laboratory for Organic Electronics and Information Displays Institute of Advanced Materials(IAM)Nanjing University of Posts and TelecommunicationsNanjing 210023China Frontiers Science Center for Flexible Electronics Institute of Flexible Electronics(IFE)Northwestern Polytechnical UniversityXi’an 710072China Jiangsu Key Laboratory for Opto-Electronic Technology School of Physics and TechnologyNanjing Normal UniversityNanjing 210023China State Key Laboratory of Coordination Chemistry School of Chemistry and Chemical EngineeringNanjing UniversityNanjing 210093China

All inorganic metal halide perovskite nanocrystals(NCs)have attracted much attention for their outstanding optoelectronic properties,which can be tuned by the composition,surface,size and morphology in ***,we report the microfluidic synthesis of hollow CsPbBr_(3)perovskite NCs through the nanoscale Kirkendall *** formation mechanism of the hollow structure(Kirkendall void)controlled by the temperature,flow rate,ratios of precursors and ligands was *** with the solid CsPbBr_(3)NCs of the same size,the hollow CsPbBr_(3)NCs exhibit blue shifts in ultraviolet-visible(UV-vis)absorption and photoluminescence(PL)spectra,and remarkably longer PL average lifetime(~98.2 ns).Quantum confinement effect,inner surface induced additional trap states and lattice strain of the hollow CsPbBr_(3)NCs were discussed in understanding their unique optoelectronic *** hollow CsPbBr_(3)NC based photodetector exhibits an outstanding negative photoconductivity(NPC)detectivity of 8.9×10^(12)*** also show potentials in perovskite NC based photovoltaic and light emitting diodes(LEDs).

关键词： perovskite nanocrystals hollow nanocrystals nanoscale Kirkendall effect microfluidic synthesis

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