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Smart ZnS@C filler for super-anticorrosive self-healing zinc-rich epoxy coating

Nano Research 2022年第5期15卷 4756-4764页

作者： Kai Yang Yixue Duan Guicheng Liu Guoyan Ma Hao Fu Xuyong Chen Manxiang Wang Gangqiang Zhu Woochul Yang Yiding Shen Shaanxi Key Laboratory of Chemical Additives for Industry Shaanxi University of Science and TechnologyXi’an 710021China Department of Physics Dongguk UniversitySeoul 04620Republic of Korea State Key Laboratory of Advanced Technology for Materials Synthesis and Processing Wuhan University of TechnologyWuhan 430070China College of Chemistry and Chemical Engineering Xi'an Shiyou UniversityXi'an 710065China School of physics and Information Technology Shaanxi Normal UniversityXi’an 710062China

The zinc-rich epoxy cathodic protection coating is the most widely used anticorrosion material for marine ***,traditional conductive fillers lack the intelligent self-healing effect,which limits the long-term anticorrosion ***,with uniform carbon-coated ZnS(ZnS@C)nanoballs as the smart active release filler,we propose an anticorrosive and self-healing zinc-rich maleic anhydride epoxy *** to the high pore filling efficiency of the nanoballs,the water vapor transmission rate of the coating with an initial corrosion efficiency of 99.92%and a low-frequency impedance of|Z|f=10mHz=3.88×10^(10) Ω·cm^(2),was reduced by 52%.The carbon-shell of the nanoball increases electron transmission paths in the coating and improves conductivity by nearly two orders of magnitude,which effectively activates more Zn-sites and extends the cathodic protection ***,once the steel-substrate undergoes regional corrosion,the SO_(4)^(2-)hydrolyzes from the ZnS-core of the nanoball and reacts with iron ions on the corroded area accurately and intelligently to fill the gap and self-heals into a new dense barrier layer(Fe_(2)(SO_(4))_(3),etc.),which significantly improves the shielding protection ability during the long-term usage of the *** effective anticorrosion time of the proposed coating could be up to 3,400 h.

关键词： smart ZnS@C fller microemulsion-carbonization method zinc-rich epoxy coating anticorrosion self-healing

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Ballistic Behavior of Three-Dimensional Orthotropic Woven Fabric Based on Virtual Fiber Model

SSRN

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SSRN 2024年

作者： Zhang, Jian Zhou, Yi Lu, Zhenqian Yue, Jianing Han, Jing Zhou, Kanghui Liu, Shengkai Jiang, Qian Wu, Liwei Tianjin and Ministry of Education Key Laboratory for Advanced Textile Composite Materials Tiangong University Tianjin300387 China Innovation Platform of Intelligent and Energy-Saving Textiles School of Textile Science and Engineering Tiangong University Tianjin300387 China State Key Laboratory of New Textile Materials and Advanced Processing Technologies Wuhan Textile University Wuhan China College of Textiles and Clothing Yancheng Institute of Technology Jiangsu 224051 China

This study proposes a novel virtual fiber model (VFM)1 on a fiber scale to capture the ballistic behavior of fabrics. The model effectively accounts for yarn deformation during 3D orthogonal woven fabric (3DOWF) weaving, yarn pull-out, interfiber friction, and yarn interactions during the ballistic response. The optimized VFM was used to explore the ballistic behaviors of the fabrics. The results revealed that the VFM exhibited a ballistic response consistent with high-speed photography observations and successfully captured fiber slippage and pull-out behavior under impact. Compared to the yarn model (YM), the VFM enables the observation of nonsimultaneous fiber breakage and fiber interactions. Moreover, it illustrates the role of yarn pull-out in the penetration resistance of the 3DOWF, dissipating the kinetic energy of the projectile in the form of friction. Furthermore, the VFM delineated the specific functions of each system yarn. Specifically, the warp and weft yarns primarily serve as impediments to the projectile, whereas the Z yarn binds the weft, promoting the increased involvement of the weft in dissipating kinetic energy. Building on this investigation, the impact of the clamping method on the ballistic performance of the 3DOWF was explored. The findings revealed that yarn pullout emerged as the primary failure mode under the weft sides. Notably, the warp yarns predominantly experienced pullout, which enhanced the friction energy. The Z yarn binds to weft yarns that gather with warp yarns to form a strip-like protrusion, impeding the projectile motion owing to the increased number of yarns. The VFM contributes significantly to the exploration of the impact of fabric structures on ballistic performance, offering valuable insights for designing and enhancing ballistic fabric *** study proposes a novel, fiber-scale virtual fiber model (VFM) to capture the ballistic behavior of fabrics. The model accounts for yarn deformation during 3D orthogonal

关键词： Yarn

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Highly active bifunctional catalyst: Constructing FeWO_(4)-WO_(3) heterostructure for water and hydrazine oxidation at large current density

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Nano Research 2021年第11期14卷 4356-4361页

作者： Fang Shen Zhenglin Wang Yamei Wang Guangfu Qian Miaojing Pan Lin Luo Guoning Chen Hailang Wei Shibin Yin College of Chemistry and Chemical Engineering Key Laboratory of New Processing Technology for Nonferrous Metals and MaterialsState Key Laboratory of Processing for Non-Ferrous Metal and Featured MaterialsGuangxi UniversityNanning530004China Guangxi Bossco Environmental Protection Technology Co. Ltd12 Kexing RoadNanning530007China

Developing high performance anode catalysts for oxygen evolution reaction (OER) and hydrazine oxidation reaction (HzOR) at large current density is an efficient pathway to produce hydrogen. Herein, we synthesize a FeWO_(4)-WO_(3) heterostructure catalyst growing on nickel foam (FeWO_(4)-WO_(3)/NF) by a combination of hydrothermal and calcination method. It shows good catalytic activity with ultralow potentials for OER (ζ_(10) = 1.43 V, ζ_(1.000) = 1.56 V) and HzOR (ζ_(10) = −0.034 V, ζ_(1.000) = 0.164 V). Moreover, there is little performance degradation after being tested for _(10)0 h at 1,000 (OER) and _(10)0 (HzOR) mA·cm−2, indicating good stability. The superior performance could be attributed to the wolframite structure and heterostructure: The former provides a high electrical conductivity to ensure the electronic transfer capability, and the later induces interfacial electron redistribution to enhance the intrinsic activity and stability. The work offers a brand-new way to prepare good performance catalysts for OER and HzOR, especially at large current density.

关键词： catalyst heterostructure large current density oxygen evolution reaction hydrazine oxidation reaction

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Loofah-Inspired Biomass Polysaccharide-Based Aerogels for All-Weather Super-Viscous Crude Oil Adsorption and Wastewater Treatment in Harsh Environment

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SSRN 2023年

作者： Chen, Zhicheng Zheng, Long Song, Yiheng Tan, Yeqiang Xianze, Yin College of Materials Science and Engineering State Key Laboratory of New Textile Materials & Advanced Processing Technology Wuhan Textile University Wuhan430200 China State Key Laboratory of Bio-Fibers and Eco-Textiles Collaborative Innovation Center of Marine Biobased Fiber and Ecological Textile Technology Institute of Marine Biobased Materials College of Materials Science and Engineering Qingdao University Qingdao China

Solar-driven viscosity reduction of highly viscous crude oil has emerged as an environmentally friendly method to address large-scale oil spills. However, the challenge lies in the limited availability of sunlight during cloudy days and at night, which hinders the effectiveness of green advanced porous materials. This study developed all-weather-available advanced porous materials in the form of loofah-like structured aerogels composed of 1H, 1H, 2H, 2H-perfluorooctyltriethoxysilane/MXene/carbon nanotubes (CNTs)/sodium alginate (SA)/cellulose fibers (CFs). MXene and CNTs formed a continuous and stable network that enabled PMCSCAs to rapidly reduce crude oil viscosity for all-day based on photothermal and electrothermal conversions. Additionally, loofah-like porous structure and oriented pipeline biomass skeleton endowed PMCSCAs with stable and rapid adsorption capacity and speed. Considering the complexity of the external environment and oily wastewater composition, we verified the separation performance of PMCSCAs for metal ions and dyes and the ice-breaking ability under icy conditions. PMCSCAs provided a novel approach to achieving clean, high-efficiency, all-day remediation of ultra-viscous crude oil. This "Three birds with one stone" approach is expected to be obtained from nature and used on a large scale, replacing conventional porous adsorbent materials. © 2023, The Authors. All rights reserved.

关键词： Crude oil

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Electrolyte Engineering for High-Voltage Lithium Metal Batteries

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Research 2022年第4期2022卷 781-832页

作者： LiweiDong Shijie Zhong Botao Yuan Yuanpeng Ji Jipeng Liu Yuanpeng Liu Chunhui Yang Jiecai Han Weidong He MIIT Key Laboratory of Critical Materials Technology for New Energy Conversion and Storage School of Chemistry and Chemical EngineeringHarbin Institute of TechnologyHarbin 150080China National Key Laboratory of Science and Technology on Advanced Composites in Special Environments and Center for Composite Materials and Structures Harbin Institute of TechnologyHarbin 150080China State Key Laboratory of Urban Water Resource and Environment Harbin Institute of TechnologyHarbin 150080China Chongqing Research Institute Harbin Institute of TechnologyChongqing 401151China School of Mechanical Engineering Chengdu UniversityChengdu610106China

High-voltage lithium metal batteries(HVLMBs)have been arguably regarded as the most prospective solution to ultrahigh-density energy storage devices beyond the reach of current ***,the only component inside the HVLMBs in contact with both aggressive cathode and Li anode,is expected to maintain stable electrode/electrolyte interfaces(EEIs)and facilitate reversible Li+***,traditional electrolytes with narrow electrochemical windows fail to compromise the catalysis of high-voltage cathodes and infamous reactivity of the Li metal anode,which serves as a major contributor to detrimental electrochemical performance fading and thus impedes their practical *** stable electrolytes is vital for the further development of ***,optimization principles,design strategies,and future perspectives for the electrolytes of the HVLMBs have not been summarized in *** review first gives a systematical overview of recent progress in the improvement of traditional electrolytes and the design of novel electrolytes for the *** strategies of conventional electrolyte modification,including high concentration electrolytes and CEI and SEI formation with additives,are *** electrolytes including fluorinated,ionic-liquid,sulfone,nitrile,and solid-state electrolytes are also *** addition,theoretical studies and advanced characterization methods based on the electrolytes of the HVLMBs are probed to study the internal mechanism for ultrahigh stability at an extreme *** also foresees future research directions and perspectives for further development of electrolytes in the HVLMBs.

关键词： electrolyte maintain summarized

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Different surface modification methods and coating materials of zinc metal anode

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Journal of Energy Chemistry 2022年第3期31卷 397-412,I0011页

作者： Feng Tao Yong Liu Xinyuan Ren Jing Wang Yazhou Zhou Yingjie Miao Fengzhang Ren Shizhong Wei Jianmin Ma Provincial and Ministerial Co-construction of Collaborative Innovation Center for Non-ferrous Metal New Materials and Advanced Processing Technology Henan Key Laboratory of Non-Ferrous Materials Science&Processing TechnologySchool of Materials Science and EngineeringHenan University of Science and TechnologyLuoyang 471023HenanChina National Joint Engineering Research Center for Abrasion Control and Molding of Metal Materials Henan Key Laboratory of High-Temperature Structural and Functional MaterialsHenan University of Science and TechnologyLuoyang 471003HenanChina School of Art&Design Henan University of Science and TechnologyLuoyang 471023HenanChina School of Physics and Electronics Hunan UniversityChangsha 410082HunanChina School of Materials and Energy University of Electronic Science and Technology of ChinaChengdu 611731SichuanChina

Rechargeable aqueous Zn-ion batteries(AZIBs)are one of the most promising energy storage devices for large-scale energy storage owing to their high specific capacity,eco-friendliness,low cost and high ***,zinc metal anodes suffer from severe dendrite growth and side reactions,resulting in the inferior electrochemical performance of *** address these problems,surface modification of zinc metal anodes is a facile and effective method to regulate the interaction between the zinc anode and an *** this review,the current challenges and strategies for zinc metal anodes are ***,recent advances in surface modification strategies to improve their electrochemical performance are concluded and ***,challenges and prospects for future development of zinc metal anodes are *** hope this review will be useful for designing and fabricating highperformance AZIBs and boosting their practical applications.

关键词： Zn-ion batteries Zinc metal anode Surface modification Solvent casting method Wet chemistry method

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Review of functionally graded materials processed by additive manufacturing

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China Welding 2023年第3期32卷 41-50页

作者：宋学平黄健康樊丁 State Key Laboratory of Advanced Processing and Recycling of Non-ferrous Metals Lanzhou University of TechnologyLanzhou 730050China School of Materials Science and Engineering Lanzhou University of TechnologyLanzhou 730050China School of Mechanical Engineering Lanzhou Petrochemical University of Vocational TechnologyLanzhou 730060China

Additive manufacturing(AM)technology makes parts through layer-by-layer deposition,which can regulate the microstructure and properties of different parts of a single part *** provides a new idea for the preparation of functionally gradient materials(FGM),and has become a research hotspot at *** referring to and analyzing the recent research achievements in the additive manufacturing tech-nology of FGM,the latest research progress at domestic and abroad from four aspects were summaried:selective laser melting additive man-ufacturing,electron beam additive manufacturing,arc additive manufacturing,path planning,and material ***,the existing problems in the research are pointed out,and the future research direction and focus are prospected.

关键词： functionally graded materials additive manufacture research progress

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MnO Stabilized in Carbon-Veiled Multivariate Manganese Oxides as High-Performance Cathode Material for Aqueous Zn-Ion Batteries

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Energy & Environmental materials 2021年第4期4卷 603-610页

作者： Wanwei Jiang Haiting Shi Xijun Xu Jiadong Shen Zhiwei Xu Renzong Hu State Key Laboratory of Separation Membranes and Membrane Processes School of Textile Science and EngineeringTiangong UniversityTianjin 300387China School of Materials Science and Engineering Guangdong Provincial Key Laboratory of Advanced Energy Storage MaterialsSouth China University of TechnologyGuangzhou 510640China

Aqueous Zn-ion battery has emerged as one of the most prospective energy storage devices due to its low cost,high safety,and ***,Zn-ion batteries are bottlenecked by significant capacity fading during long-term cycling and poor performance at high current ***,we report an available cooperation of multivariate manganese oxides@carbon hybrids(MnO_(2)/MnO@C and MnO_(2)/Mn_(3)O_(4)@C)via a plasma-assisted design as an attractive Zn-ion *** them,the MnO_(2)/MnO@C cathode exhibits a reversible specific capacity of 165 m Ah g^(-1)over 200 cycles at a high rate of 0.5 A g^(-1),and possesses great rate performance with high capacities of 110 and 100 m Ah g^(-1)at a high rate of 0.8 and 1 A g^(-1),*** good cathode performance significantly results from the facile charge transfer and ions(Zn^(2+)and H^(+))insertion in the manganese oxides/carbon hybrids featuring phase stability behavior in the available cooperation of multivalence and carbon conductive *** work will promote the Zn-manganese dioxide system for the design of low-cost and high-performance aqueous rechargeable Zn-ion batteries.

关键词： aqueous rechargeable Zn batteries conductive substrates multivariate manganese oxides phase stability plasma

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Recently deepened insights regarding Mg corrosion and advanced engineering applications of Mg alloys

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Journal of Magnesium and Alloys 2023年第11期11卷 3948-3991页

作者： Guang-Ling Song Andrej Atrens Department of Ocean Science and Engineering Southern University of Science and Technology1088 Xueyuan BoulevardShenzhen 518055China The University of Queensland School of Mechanical and Mining EngineeringCentre for Advanced Materials Processing and Manufacturing(AMPAM)St LuciaQld 4072 Australia State Key Laboratory of Physical Chemistry of Solid Surfaces Xiamen University422 S.Siming RdXiamen 361005China

This review summarizes recent insights into the Mg corrosion mechanism, clarifies many critical controversial points regarding the Mg corrosion behaviour, and updates some efforts made to extend the industrial application of Mg alloys. Based on the new understandings gained so far, future research directions are also suggested in the review. This review has the following logic. The first section "1. Scope"is a consolidation of the new understandings or developments regarding the Mg corrosion mechanism and the new applications for Mg alloys. It also highlights some key points for the review. The second section "2. Widely accepted knowledge" briefly summarizes the general understanding of Mg corrosion gained so far, which acts as the foundation for the following sections. The third section "3. Recently deepened insights" mainly briefs on some new insights into Mg corrosion phenomena based on recent findings. Different interpretations on the corrosion behaviours are comprehensively discussed in the fourth section "4. Controversial points" and the conclusions are drawn in the subsection"4.5 Clarified points". Apart from the fundamental understandings, various efforts in the application of Mg alloys are presented in the fifth section "5. new applications". Following the research tendency as indicated in the review, prioritized research areas are suggested in "*** directions". The review is concluded with "7. Concluding remarks" at last.

关键词： Mg Corrosion Hydrogen Anode Intelligentization

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Stabilizing oxygen vacancies and promoting electrostrain in leadfree potassium niobate-based piezoelectrics over wide temperature ranges

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Journal of advanced Ceramics 2024年第12期13卷 1965-1973页

作者： Bingcheng Luo Wei Feng Suwei Dai Hongzhou Song Yunyi Wu Jie Zhang College of Science China Agricultural UniversityBeijing 100083China State Key Laboratory of New Ceramics and Fine Processing School of Materials Science and EngineeringTsinghua UniversityBeijing 100084China School of Materials Science and Technology China University of Geosciences BeijingBeijing 100083China Institute of Applied Physics and Computational Mathematics Beijing 100094China Research Center for Comprehensive Energy Technology CTG Science and Technology Research InstituteBeijing 100038China Research Center for Metamaterials Wuzhen LaboratoryJiaxing 314500China

Piezoelectric ceramics provide high strain and large driving forces in actuators.A large electrostrain can be realized by the introduction of point defects such as vacancies,interstitial defects,and substitution *** Mn doping,a significant increase in the reversible electrostrain from 0.05%to 0.17%could be achieved in potassium niobite lead-free piezoelectric *** origins of the large electrostrain were analyzed via in situ X-ray diffraction(XRD)under an electric *** electrostrain and other typical electrical properties of the samples were measured at various temperatures,which enabled the ceramics to perform under a very wide temperature range,such as−80–130℃ for the 0.5 mol%Mn-doped sample with low dielectric loss(≤0.02).More importantly,combined with characterizations of the defect behavior by thermally stimulated depolarization current(TSDC),the failure mechanisms of electrostrain in a hightemperature environment could be revealed,which was associated with synergistic damage to the defects caused by the electric field and high *** results can provide good ideas and a basis for the design of piezoelectric materials with good electrostrain stability over a wide temperature range.

关键词： piezoelectric ceramic lead-free point defect electrostrain thermally stimulated depolarization current(TSDC)

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