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Recent progress and perspective on lithium metal battery with nickel-rich layered oxide cathode

eScience 2024年第6期4卷 75-87页

作者： Han Zhang Ziqi Zeng Shijie Cheng Jia Xie State Key Laboratory of Advanced Electromagnetic Technology School of Electrical and Electronic EngineeringHuazhong University of Science and TechnologyWuhan 430074China State Key Laboratory of Materials Processing and Die&Mould Technology School of Materials Science and EngineeringHuazhong University of Science and TechnologyWuhan 430074China

The pairing of lithium metal anode(LMA)with Ni-rich layered oxide cathodes for constructing lithium metal batteries(LMBs)to achieve energy density over 500 Wh kg^(-1) receives significant attention from both industry and the scientific ***,notorious problems are exposed in practical conditions,including lean electrolyte/capacity(E/C)ratio(<3 g(Ah)^(-1)),high cathode mass loading(>3 mAh cm^(-2)),and low negative/positive(N/P)ratio(<3),which creates a significant disparity between the current performance of LMBs and the desired requirements for commercial *** the review,we present a summary of the recent achievements made in understanding the mechanistic degradation of LMA,followed by practical strategies that are utilized to address these *** also consider the detrimental issues of Ni-rich layered oxide ***,we highlight current progresses in the field of practical LMBs in coin/pouch cells to stimulate further *** the end,we propose the issues and prospects for development from the perspective of practical LMBs.

关键词： Lithium metal anode Ni-rich layered oxide cathodes Lithium metal batteries Practical conditions Cyclic performance High energy density

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A Preliminary Look at the Unity of Frequency Support for Grid-Following and Grid-Forming Wind Turbines

A Preliminary Look at the Unity of Frequency Support for Gri...

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2024 IEEE China International Youth Conference on Electrical engineering, CIYCEE 2024

作者： Zhou, Hongyu Yao, Wei Zong, Qihang Wen, Jinyu Huazhong University of Science and Technology State Key Laboratory of Advanced Electromagnetic Engineering and Technology Wuhan430074 China

ISBN: (纸本)9798331530174

Grid-connected wind turbines for frequency support of the grid is conducive to improving the grid frequency security level. Grid-following (GFL) converters and gridforming (GFM) converters are two important types of equipment to support renewable energy integration into the grid. Both GFM and GFL have a variety of different control strategies when performing frequency support. Clarifying the relationship be-tween different strategies of GFM and GFL when performing frequency support will provide guidance for renewable energy frequency support. In this paper, four levels of frequency support uniformity are first established at the generation unit level. (1) The governor and damping branch of the virtual synchronous generator (VSG) control based GFM converter are unified. (2) The VSG based GFM and the droop based GFM are unified. (3) Integrated inertial control based GFL and droop based GFL are unified. Finally, the theoretical analysis is synthetically verified by MATLAB/Simulink simulation platform. © 2024 IEEE.

关键词： MATLAB

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Facile synthesis of the Mn_(3)O_(4)polyhedron grown on N-doped honeycomb carbon as high-performance negative material for lithium-ion batteries

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International Journal of Minerals,Metallurgy and Materials 2023年第6期30卷 1152-1161页

作者： Dan Zhang Chunyan Zhang Xuan Zheng Yizhuo Zhao Xinyu Shi Baomin Luo Yuzhu Li Guangyin Liu Xiaodi Liu Chuang Yu College of Chemistry and Pharmaceutical Engineering Nanyang Normal UniversityNanyang 473061China State Key Laboratory of Advanced Electromagnetic Engineering and Technology School of Electrical and Electronic EngineeringHuazhong University of Science and TechnologyWuhan 430074China

Because of their large volume variation and inferior electrical conductivity,Mn_(3)O_(4)-based oxide anode materials have short cyclic lives and poor rate capability,which obstructs their *** this study,we successfully prepared a Mn_(3)O_(4)/N-doped honeycomb carbon composite using a smart and facile synthetic *** Mn_(3)O_(4)nanopolyhedra are grown on N-doped honeycomb carbon,which evidently mitigates the volume change in the charging and discharging processes but also improves the electrochemical reaction *** importantly,the Mn-O-C bond in the Mn_(3)O_(4)/N-doped honeycomb carbon composite benefits electrochemical *** features of the Mn_(3)O_(4)/N-doped honeycomb carbon(NHC)composite are responsible for its superior electrochemical *** used for Li-ion batteries,the Mn_(3)O_(4)/N-doped honeycomb carbon anode exhibits a high reversible capacity of 598 mAh·g^(−1)after 350 cycles at 1 A·g^(−1).Even at 2 A·g^(−1),the Mn_(3)O_(4)/NHC anode still delivers a high capacity of 472 mAh·g^(−1).This work provides a new prospect for synthesizing and developing manganese-based oxide materials for energy storage.

关键词： Mn_(3)O_(4) polyhedron nitrogen-doped honeycomb carbon anode lithium-ion battery

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Experimental demonstration of 220-GHz terahertz signals wireless transmission over 4.6 km

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Science China(Information Sciences) 2025年第1期68卷 386-388页

作者： Yi WEI Jianjun YU Mingxu WANG Xiongwei YANG Qiutong ZHANG Jingwen TAN Bing ZHANG Ying WU Yang HAN Peng TIAN Wen ZHOU Kaihui WANG Feng ZHAO State Key Laboratory of ASIC and System Key Laboratory for Information Science of Electromagnetic Waves (MoE)School of Information Science and Technology Fudan University School of Electronic Engineering Xi'an University of Posts and Telecommunications

The advancement of terahertz (THz) communication technology drives the evolution of wireless communication systems,offering novel pathways and technical means for the development of future 6G communication *** wireless communication systems are often constrained by bandwidth limitations of electronic devices in high frequency ***,THz communication technology leverages the characteristics of electromagnetic waves to transcend these limitations,enabling communication athigher frequencies and wider bandwidths.

关键词： wireless terahertz over demonstration experimental signals transmission

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Design and experimental study of a field-reversed configuration plasma thruster prototype

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Plasma Science and technology 2025年第3期27卷 118-126页

作者： Yuxuan HUANG Ming ZHANG Yong YANG Fangwei LYU Xiaopeng YI Chaofan LYU Yisong ZHANG Bo RAO State Key Laboratory of Advanced Electromagnetic Technology International Joint Research Laboratory of Magnetic Confinement Fusion and Plasma PhysicsSchool of Electrical and Electronic EngineeringHuazhong University of Science and TechnologyWuhan 430074People’s Republic of China National Key Laboratory of Science and Technology on Vacuum Technology and Physics Lanzhou Institute of PhysicsLanzhou 730000People’s Republic of China

The field-reversed configuration(FRC)plasma thruster driven by rotating magnetic field(RMF),abbreviated as the RMF-FRC thruster,is a new type of electric propulsion technology that is expected to accelerate the deep space *** experimental prototype,including diagnostic devices,was designed and constructed based on the principles of the RMF-FRC thruster,with an RMF frequency of 210 kHz and a maximum peak current of 2 *** the rated operating conditions,the initial plasma density was measured to be 5×10^(17)m^(-3),and increased to 2.2×10^(19)m^(-3)after the action of *** coupling efficiency of RMF was about 53%,and the plasma current reached 1.9 *** axial magnetic field changed in reverse by 155 Gauss,successfully reversing the bias magnetic field of 60 Gauss,which verifies the formation of FRC *** optimization research,it was found that when the bias magnetic field is 100 Gauss,the axial magnetic field reverse variation caused by FRC is the highest at 164 *** experimental results are discussed and strategies are proposed to improve the performance of the prototype.

关键词： rotating magnetic field(RMF) field-reversed configuration(FRC) plasma thrusters plasma current

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Dual-Functional Organotelluride Additive for Highly Efficient Sulfur Redox Kinetics and Lithium Regulation in Lithium–Sulfur Batteries

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Energy & Environmental Materials 2023年第3期6卷 126-133页

作者： Wei Zhang Fenfen Ma Qiang Wu Ziqi Zeng Wei Zhong Shijie Cheng Xin Chen Jia Xie State Key Laboratory of Advanced Electromagnetic Engineering and Technology School of Electrical and Electronic EngineeringHuazhong University of Science and TechnologyWuhan 430074China GuSu Laboratory of Materials SuzhouJiangsu 215123China State Key Laboratory of Materials Processing and Die&Mould Technology School of Materials Science and EngineeringHuazhong University of Science and TechnologyWuhan 430074China

High energy density and low cost made lithium–sulfur(Li–S)batteries appealing for the next-generation energy storage ***,their commercial viability is seriously challenged by serious polysulfide shuttle effect,sluggish sulfur kinetics,and uncontrollable dendritic Li ***,a dual-functional electrolyte additive,diphenyl ditelluride(DPDTe)is reported for Li–S *** sulfur cathodes,DPDTe works as a redox mediator to accelerate redox kinetics of sulfur,in which Te radical-mediated catalytic cycle at the solid–liquid interface contributes significantly to the whole *** lithium anodes,DPDTe can react with lithium metal to form a smooth and stable organic–inorganic hybrid solid-electrolyte interphase(SEI),enabling homogeneous lithium deposition for suppressing dendrite ***,the Li–S battery with DPDTe exhibits remarkable cycling stability and superb rate capability,with a high capacity up to 1227.3 mAh g^(-1)and stable cycling over 300 ***,a Li–S pouch cell with DPDTe is evaluated as the proof of *** work demonstrates that organotelluride compounds can be used as functional electrolyte additives and offers new insights and opportunities for practical Li–S batteries.

关键词： electrolyte additive Li anode Li2 S deposition Li–S battery sulfur kinetics

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An Environment‑Tolerant Ion‑Conducting Double‑Network Composite Hydrogel for High‑Performance Flexible Electronic Devices

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Nano-Micro Letters 2024年第5期16卷 352-369页

作者： Wenchao Zhao Haifeng Zhou Wenkang Li Manlin Chen Min Zhou Long Zhao State Key Laboratory of Advanced Electromagnetic Technology School of Electrical and Electronic EngineeringHuazhong University of Science and TechnologyWuhan 430074People’s Republic of China School of Chemistry and Chemical Engineering Huazhong University of Science and TechnologyWuhan 430074People’s Republic of China

High-performance ion-conducting hydrogels(ICHs)are vital for developing flexible electronic ***,the robustness and ion-conducting behavior of ICHs deteriorate at extreme tempera-tures,hampering their use in soft *** resolve these issues,a method involving freeze–thawing and ionizing radiation technology is reported herein for synthesizing a novel double-network(DN)ICH based on a poly(ionic liquid)/MXene/poly(vinyl alcohol)(PMP DN ICH)*** well-designed ICH exhibits outstanding ionic conductivity(63.89 mS cm^(-1) at 25℃),excellent temperature resistance(-60–80℃),prolonged stability(30 d at ambient temperature),high oxidation resist-ance,remarkable antibacterial activity,decent mechanical performance,and ***,the ICH performs effectively in a flexible wireless strain sensor,thermal sensor,all-solid-state supercapacitor,and single-electrode triboelectric nanogenerator,thereby highlighting its viability in constructing soft electronic *** highly integrated gel structure endows these flexible electronic devices with stable,reliable signal output *** particular,the all-solid-state supercapacitor containing the PMP DN ICH electrolyte exhibits a high areal specific capacitance of 253.38 mF cm^(-2)(current density,1 mA cm^(-2))and excellent environmental *** study paves the way for the design and fabrication of high-performance mul-tifunctional/flexible ICHs for wearable sensing,energy-storage,and energy-harvesting applications.

关键词： Ionic liquids Double-network hydrogels Temperature tolerance Multifunctionality Flexible electronic devices

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Investigation of stimulated growth effect using pulsed cold atmospheric plasma treatment on Ganoderma lucidum

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Plasma Science and technology 2022年第11期24卷 106-113页

作者： Mengqi LI Xiaoyi HUANG Zilan XIONG State Key Laboratory of Advanced Electromagnetic Engineering and Technology Huazhong University of Science and TechnologyWuhan 430074People’s Republic of China

Cold atmospheric plasma(CAP)driven by pulsed high-voltage power has specific advantages in various fields,such as the growth promotion of edible fungi in plasma *** with other strains,Ganoderma lucidum has the significant advantage of high medicinal value,but the shortcomings of low yield,long growth cycle,and an uneven market *** this study,Ganoderma lucidum was treated with a CAP powered by a homemade pulsed highvoltage power *** groups of Ganoderma lucidum were treated under different *** stalk lengths and pileus areas of Ganoderma lucidum were recorded to evaluate growth *** showed that treatment frequency affected growth status *** lucidum was treated with 40 s plasma once a week and showed an improved growth status with a 33.63%increase in average stalk length and a 28%increase in the number of individuals whose pileus areas was greater than the ***,the growth speed was ***,treatment at an excessive frequency would damage and slow down the growth of Ganoderma lucidum.

关键词： low temperature plasma plasma agriculture edible fungi Ganoderma lucidum stimulated growth

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Mechanism Analysis of Instability in Grid-Connected PV Systems With Volt-Var Control 10

Mechanism Analysis of Instability in Grid-Connected PV Syste...

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10th IEEE International Power Electronics and Motion Control Conference, IPEMC 2024 ECCE Asia

作者： Yan, Shuxuan Shi, Xiaojie Liu, Xuhua Chen, Qiong Lin, Lei Huazhong University of Science and Technology State Key Laboratory of Advanced Electromagnetic Engineering and Technology Wuhan430074 China

ISBN: (纸本)9798350351330

Utilizing the flexible reactive power regulation capability of PV inverters for voltage support is proved to be an effective solution to voltage fluctuation and violation, which however can induce control of instability. To address this issue, this paper focuses on the dq-frame admittance modeling of three-phase grid-tied inverters with volt-var control, which behaves as a multi-input-multi-output (MIMO) system. It is found that the volt-var control can reshape the q-d channel output admittance in the low-frequency range and increase the risk of oscillation instability. To explore its mechanism, the MIMO model is transformed into a single-input-single (SISO) model from Iqd to Ud. Applying the impedance-based stability criterion, this paper analyzes in detail the effect of volt-var control, grid-following (GFL) control and the grid impedance on the system stability. Finally, simulations and semi-physical experiments results validate the above analysis. © 2024 IEEE.

关键词： Stability criteria

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Nanopore-rich NiFe LDH targets the formation of the high-valent nickel for enhanced oxygen evolution reaction

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Nano Research 2023年第2期16卷 2286-2293页

作者： Qunlei Wen Shuzhe Wang Ruiwen Wang Danji Huang Jiakun Fang Youwen Liu Tianyou Zhai State Key Laboratory of Materials Processing and Die&Mould Technology School of Materials Science and EngineeringHuazhong University of Science and TechnologyWuhan 430074China State Key Lab of Advanced Electromagnetic Engineering and Technology School of Electrical and Electronic EngineeringHuazhong University of Science and TechnologyWuhan 430074China

Nickel-iron layered double hydroxides(NiFe LDHs)represent a promising candidate for oxygen evolution reaction(OER),however,are still confronted with insufficient activity,due to the slow kinetics of electrooxidation of Ni^(2+)cations for the high-valent active ***,nanopore-rich NiFe LDH(PR-NiFe LDH)nanosheets were proposed for enhancing the OER activity together with *** the designed catalyst,the confined nanopores create abundant unsaturated Ni sites at edges,and decrease the migration distance of protons down to the scale of their mean free path,thus promoting the formation of high-valent Ni^(3+)/^(4+)active *** unique configuration further improves the OER stability by releasing the lattice stress and accelerating the neutralization of the local acidity during the phase ***,the optimized PR-NiFe LDH catalysts exhibit an ultralow overpotential of 278 mV at 10 mA∙cm^(−2)and a small Tafel slope of 75 mV∙dec^(−1),which are competitive among the advanced LDHs based ***,the RP-NiFe LDH catalyst was implemented in anion exchange membrane(AEM)water electrolyzer devices and operated steadily at a high catalytic current of 2 A over 80 *** results demonstrated that PR-NiFe LDH could be a viable candidate for the practical *** concept also provides valuable insights into the design of other catalysts for OER and beyond.

关键词： nickel-iron layered double hydroxides(NiFe LDHs) water oxidation nanopores high-valent sites

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