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Energy transfer enhanced photocatalytic hydrogen evolution in organic heterostructure nanoparticles via flash nanoprecipitation processing

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Green Energy & Environment 2025年第2期10卷 390-398页

作者： Miaojie Yu Weiwei Zhang Xueyan Liu Guohui Zhao Jun Du Yongzhen Wu Wei-Hong Zhu Key Laboratory for Advanced Materials and Institute of Fine Chemicals Joint International Research Laboratory of Precision Chemistry and Molecular EngineeringFeringa Nobel Prize Scientist Joint Research CenterFrontiers Science Center for Materiobiology and Dynamic ChemistrySchool of Chemistry and Molecular EngineeringEast China University of Science and TechnologyShanghai200237China State Key Laboratory of Molecular Reaction Dynamics Dalian Institute of Chemical PhysicsChinese Academy of SciencesDalianLiaoning116023China

Organic nanophotocatalysts are promising candidates for solar fuels production,but they still face the challenge of unfavorable geminate recombination due to the limited exciton diffusion ***,we introduce a binary nanophotocatalyst fabricated by blending two polymers,PS-PEG5(PS)and PBT-PEG5(PBT),with matched absorption and emission spectra,enabling a Forster resonance energy transfer(FRET)process for enhanced *** heterostructure nanophotocatalysts are processed using a facile and scalable flash nanoprecipitation(FNP)technique with precious kinetic control over binary nanoparticle *** resulting nanoparticles exhibit an exceptional photocatalytic hydrogen evolution rate up to 65 mmol g^(-1) h^(-1),2.5 times higher than that single component *** through fluorescence spectra and transient absorption spectra confirm the hetero-energy transfer within the binary nanoparticles,which prolongs the excited-state lifetime and extends the namely“effective exciton diffusion length”.Our finding opens new avenues for designing efficient organic photocatalysts by improving exciton migration.

关键词： Polymer photocatalysts Nanoparticles Hydrogen evolution Forster resonance energy transfer

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Energy routing strategy of laser power transmission network based on two-layer optimization

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Kongzhi Lilun Yu Yingyong/Control Theory and Applications 2025年第4期42卷 703-712页

作者： Yuan, Ao-Te Cai, Tao Lan, Jian-Yu State Key Laboratory of Advanced Electromagnetic Technology Huazhong University of Science and Technology Hubei Wuhan430074 China Key Laboratory of Power Electronics and Energy Management for Ministry of Education of China School of Electrical and Electronic Engineering Huazhong University of Science and Technology Hubei Wuhan430074 China Shanghai Space Power Research Institute Shanghai200245 China

The low transfer efficiency and poor robustness are important obstacles restricting the development of laser power transmission. The routing strategy of the network has been studied for efficient and reliable energy transfer. The paper analyzed the architecture of the laser power transmission network, modified the calculation formula of laser transmission efficiency in the atmosphere, and abstracted the network into a weight graph. Considering the multidimensional coupling characteristics in the laser power transmission network, a two-layer optimization strategy with spatio-temporal decoupling is proposed. The first layer optimization realizes path planning based on Dijkstra algorithm to find the most efficient energy transmission path. The second layer optimization is based on the optimal paths, takes the total loss as the objective function, builds mathematical models and solves it with inner iterative PSO algorithm. Through the simulation of a unmanned aerial vehicle (UAV) cruise system under different control strategies, the effectiveness and feasibility of the two-layer optimization strategy are verified. © 2025 South China University of technology. All rights reserved.

关键词： Particle swarm optimization (PSO)

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KCl acts as a flux to assist the growth of sub-millimeter-scale metallic 2D non-layered molybdenum dioxide

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Rare Metals 2025年第1期44卷 404-416页

作者： Li-Ying Deng Qing Zhang Wang-Yang Li Xiao-Yuan Ye Yi-Fan Zhao Shen-Zhong Chen Yu-Lan Wang Xing-Hui Wang Hui-Peng Chen Zhi-Yang Yu Qun Yan Shu-Ying Cheng Tai-Liang Guo Wen-Ping Hu Feng Ding Jie Sun National and Local United Engineering Laboratory of Flat Panel Display Technology College of Physics and Information EngineeringFuzhou UniversityFuzhou350100China Fujian Key Laboratory of Agricultural Information Sensing Technology College of Mechanical and Electrical EngineeringFujian Agriculture and Forestry UniversityFuzhou350002China Key Laboratory of Organic Integrated Circuit Department of ChemistrySchool of ScienceMinistry of Education and Tianjin Key Laboratory of Molecular Optoelectronic SciencesTianjin UniversityTianjin300072China Collaborative Innovation Center of Chemical Science and Engineering(Tianjin) Tianjin300072China College of Physics and Information Engineering Institute of Micro-Nano Devices and Solar CellsFuzhou UniversityFuzhou350108China State Key Laboratory of Photocatalysis on Energy and Environment College of ChemistryFuzhou UniversityFuzhou350116China Faculty of Materials Science and Engineering/Institute of Technology for Carbon Neutrality Shenzhen Institute of Advanced TechnologyChinese Academy of SciencesShenzhen518000China

Two-dimensional(2D)metal oxides(2DMOs),such as MoO_(2),have made impressive strides in recent years,and their applicability in a number of fields such as electronic devices,optoelectronic devices and lasers has been ***,2DMOs present challenges in their synthesis using conventional methods due to their non-van der Waals *** report that KCl acts as a flux to prepare large-area 2DMOs with sub-millimeter *** systematically investigate the effects of temperature,homogeneous time and cooling rate on the products in the flux method,demonstrating that in this reaction a saturated homogenous solution is obtained upon the melting of the salt and ***,the cooling rate was adjusted to regulate the thickness of the target crystals,leading to the precipitation of 2D non-layered material from the supersaturated solution;by applying this method,the highly crystalline non-layered 2D MoO_(2)flakes with so far the largest lateral size of up to sub-millimeter scale(~464μm)were *** studies have revealed that the 2D MoO_(2)features metallic properties,with an excellent sheet resistance as low as 99Ω·square^(-1 )at room temperature,and exhibits a property of charge density wave in the measurement of resistivity as a function of temperature.

关键词： 2D non-layered materials Metallic Metal oxide Thickness modulation Flux method

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Giant spatial Goos-Hänchen shift achieved in superconducting hyperbolic metamaterials with graphene

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Optics Express 2025年第9期33卷 19359-19370页

作者： Yang, Junfu Xie, Zhijiang Ni, Hao Chen, Xiaoling Qin, Zhongli Zhao, Dong Zhao, Miaomiao State Key Laboratory of Mechanical Transmission for Advanced Equipment Chongqing University Chongqing400044 China College of Mechanical and Vehicle Engineering Chongqing University Chongqing400044 China School of Electronic and Information Engineering Hubei University of Science and Technology Xianning437100 China Hubei Provincial Key Laboratory of Optoelectronic Information and Intelligent Control Hubei University of Science and Technology Xianning437100 China

We have theoretically analyzed the enhancement and regulation of the Goos-Hänchen (GH) shift within hyperbolic metamaterials in the near-infrared band under low-temperature conditions. Given a fixed incident wavelength, photonic crystals constructed from graphene and superconductor present hyperbolic dispersion characteristics in the dispersion space by modulating the Fermi energy of graphene. Near the critical phase transition point from elliptic dispersion to hyperbolic dispersion, the phase of the reflection coefficient undergoes an abrupt alteration. Consequently, a remarkably large GH shift occurs precisely at the resonant state. A substantial GH shift can be effectively realized by regulating the layers of graphene, the thickness of the superconductor, and the temperature. The largest positive GH shift reaches up to 4000λ at T = 200 K. This research is anticipated to provide theoretical guidance for devising high-sensitivity temperature sensors based on the GH shift effect in hyperbolic materials within a low-temperature environment. © 2025 Optica Publishing Group under the terms of the Optica Open Access Publishing Agreement.

关键词： Metamaterials

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A High-Power Wave Energy Harvester with Mag-Boost Mechanism 5th

A High-Power Wave Energy Harvester with Mag-Boost Mechanism

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5th International Conference on Vibration and Energy Harvesting Applications, VEH 2024

作者： Tang, Tianyi Li, Yunfei Sun, Lining Liu, Huicong State Key Laboratory of Robotics and System Harbin Institute of Technology Harbin China School of Mechanical and Electrical Engineering Jiangsu Provincial Key Laboratory of Advanced Robotics Soochow University Suzhou China

ISBN: (纸本)9789819611904

Ocean wave energy is a widely anticipated new type of renewable energy. However, due to the ultra-low-frequency and random motion characteristics of ocean waves, effectively harnessing it presents a significant challenge. This paper proposes a Mag-Boost mechanism based on the phenomenon that the magnetic torque undergoes a sudden change when the magnetic poles of two magnets are orthogonal. This innovative mechanism, requiring just a trigger below 1 Hz, can stimulate a power-magnet to generate high-frequency oscillation without direct contact. Utilizing this mechanism, a high-power wave energy harvester (WEH) with ultra-low-frequency response capabilities has been developed. Tested on a six-degree-of-freedom platform, the WEH demonstrated a high-output power of 1.44W and a power density of 1.2 kW/m3 at a frequency of 1 Hz and an inclination angle of 30°. The peak open-circuit voltage of the WEH reached 5 V, ensuring a completely independent and stable power supply for wireless temperature and humidity sensors. Furthermore, the Mag-Boost mechanism also shows considerable potential for harvesting other forms of low-frequency environmental energy, including wind, vibration, and human kinetic energy. © The Author(s), under exclusive license to Springer Nature Singapore Pte Ltd. 2025.

关键词： Water waves

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Understanding the iodine electrochemical behaviors in aqueous zinc batteries

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Journal of Energy Chemistry 2025年第2期101卷 402-415,I0009页

作者： Xuefang Xie Xiaoxin Xu Shuquan Liang Guozhao Fang College of Physical Science and Technology Xinjiang UniversityUrumqi 830017XinjiangChina Xinjiang Key Laboratory of Solid State Physics and Devices Xinjiang UniversityUrumqi 830046XinjiangChina School of Materials Science&Engineering Key Laboratory of Electronic Packaging and Advanced Functional Materials of Hunan ProvinceCentral South UniversityChangsha 41003 HunanChina National Energy Metal Resources and New Materials Key Laboratory Central South UniversityChangsha 410083HunanChina

Iodine is widely used in aqueous zinc batteries(ZBs)due to its abundant resources,low cost,and active redox *** addition to the active material in zinc-iodine batteries,iodine also plays an important role in other ZBs,such as regulating the electrochemical behavior of zinc ions,promoting the reaction kinetic and reversibility of other redox pairs,catalytic behaviors related to iodine reactions,coupling with other halogen ions,shuttle behaviors of polyiodides,***,there is currently a lack of comprehensive discussion on these ***,this review provides a comprehensive overview of the electrochemical behaviors of iodide in the aqueous *** effect of iodine ions on the Zn^(2+)desolvation behaviors and the interfacial behaviors of Zn anode was *** redox pairs boosting other redox pairs,such as MnO_(2)/Mn^(2+)redox pair and vanadium redox pair to obtain high reversibility and capacity was also ***,the catalytic behaviors related to iodine reactions in aqueous ZBs,synergistic reaction with other halogen ions and suppression of shuttle behaviors for high performance zinc-iodine batteries were systematically ***,future prospects for designing effective iodine electrochemical behaviors with practicability are proposed,which will provide scientific guidance for the practical application of iodine-related aqueous ZBs.

关键词： lodide ion Redox pairs Catalytic behavior Shuttle effect Zinc batteries

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Experimental Research on the Impact of Water Vapor and Solid Particles on the Air Gap DC Discharge Characteristics 11th

Experimental Research on the Impact of Water Vapor and Solid...

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11th Frontier Academic Forum of Electrical engineering, FAFEE 2024

作者： Cheng, Tingting Ji, Lanlan Su, Pengfei Li, Yuanzhen Li, Gaoyue Jiang, Xingliang Wang, Linghao State Key Laboratory of Advanced Power Transmission Technology State Grid Smart Grid Research Institute Co. Ltd. Beijing China State Key Laboratory of Power Transmission Equipment Technology School of Electrical Engineering Chongqing University Chongqing China

ISBN: (纸本)9789819788316

Long-term exposure of outdoor power transmission and distribution equipment to varying levels of water vapor and solid particles in the atmospheric environment often leads to diminished insulation strength, consequently posing safety hazards. This paper delves into a systematic exploration of the impact of water vapor and solid particles in impure air on the DC breakdown characteristics of air gaps. Through the design and implementation of a tailored discharge chamber and air filtration system, the study scrutinizes the influence of these factors on the DC breakdown characteristics of a needle-plate gap. The findings reveal that, under conditions of humidity saturation, the frequency breakdown voltage of the needle-plate gap escalates with rising water vapor concentration. With the passage of solid particles, the breakdown voltage of the needle-plate gap exhibits an upward trend correlated with increasing solid particle concentration. Conversely, larger particle sizes tend to induce a reduction in breakdown voltage. Additionally, while the relative dielectric constant of solid particulate matter generally maintains the breakdown voltage at a stable level, there is a slight inclination towards decrease. © Beijing Paike Culture Commu. Co., Ltd. 2025.

关键词： Needles

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Achieving high strength and large ductility in a Cr30Co30Ni30Al5Ti5 alloy through intergranular precipitation

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Journal of Materials Science and technology 2025年 215卷 167-179页

作者： Zou, Jiawei Chen, Siyu Cheng, Pengming Ding, Jun Zhang, Chongle Zhang, Shengze Zhang, Bozhao Fu, Xiaoqian Chen, Yujie Zhao, Yuping Qi, Xu Gu, Lin Zhang, Ze Sha, Gang Yu, Qian Center of Electron Microscopy and State Key Laboratory of Silicon and Advanced Semiconductor Materials School of Materials Science and Engineering Zhejiang University Hangzhou310027 China School of Materials Science and Engineering Herbert Gleiter Institute of Nanoscience Nanjing University of Science and Technology Nanjing210094 China State Key Laboratory for Mechanical Behavior of Materials School of Materials Science and Engineering Xi'an Jiaotong University Xi'an710049 China Center for Alloy Innovation and Design State Key Laboratory for Mechanical Xi'an Jiaotong University Xi'an710049 China Pico Electron Microscopy Center Innovation Institute for Ocean Materials Characterization Technology Center for Advanced Studies in Precision Instruments Hainan University Haikou570228 China Beijing National Center for Electron Microscopy and Laboratory of Advanced Materials School of Materials Science and Engineering Tsinghua University Beijing100084 China

Precipitation at grain boundaries is typically not regarded as an efficient method for strengthening materials since it can induce grain boundary embrittlement, which detrimentally affects ductility. In this research, we developed a multi-principal element alloy (MPEA) with the composition Cr30Co30Ni30Al5Ti5 (at.%), incorporating both intragranular and intergranular nanoprecipitates. Utilizing multiscale, three-dimensional, and in-situ electron microscopy techniques, coupled with computational simulations, we established that intergranular nanoprecipitation in this material plays a crucial role in enhancing strength and promoting dislocation plasticity. The structure of intergranular nanoprecipitation comprises multiple phases with varying composition and structure. Despite the diversity, the crystal planes conducive to the easy glide of dislocations are well-matched, allowing for the sustained continuity of dislocation slipping across different phase structures. Simultaneously, this structure generates an undulated stress field near grain boundaries, amplifying the strengthening effect and facilitating multiple slip and cross-slip during deformation. Consequently, it promotes the proliferation and storage of dislocations. As a result, our material exhibits a yield strength of approximately 1010 MPa and an ultimate tensile strength of around 1500 MPa, accompanied by a significant fracture elongation of 41 %. Our findings illuminate the potential for harnessing intergranular nanoprecipitation to optimize the strength-ductility trade-off in MPEAs, emphasizing the strategy of leveraging complex compositions for the design of sophisticated functional microstructures. © 2024

关键词： Ductility

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Corrosion behavior of MgO-C refractories with Al2O3-spinel addition by different low basicity slags

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Ceramics International 2025年第14期51卷 18439-18450页

作者： Wei, Jiawei Han, Bingqiang Ma, Lin Xiang, Xing Zhang, Yingli Dong, Binbin Wan, Zhong Yan, Junjie Zhu, Yihong Chen, Junfeng Ma, Jiuhong School of Materials Science and Engineering Luoyang Institute of Science and Technology Luoyang471023 China The State Key Laboratory of Refractories and Metallurgy Wuhan University of Science and Technology Wuhan430081 China Beijing Jinyu Tongda Refractory Technology Co. Ltd. Beijing100043 China State Key Laboratory of Advanced Refractories Sinosteel Luoyang Institute of Refractories Research Co. Ltd Luoyang471039 China

Low-carbon is the development trend in refractory industry. In order to improve the corrosion resistance of MgO-C refractories due to the reduction of carbon content, the Al2O3-spinel was used to improve their properties. The physical properties, oxidation resistance and corrosion resistance were tested to assess the influence of Al2O3-spinel on the MgO-C refractories, and thermodynamic calculation was used to investigate possible reactions during corrosion process. The introduction of Al2O3-spinel had no obvious effect on the physical properties of MgO-C refractories. However, Al2O3-spinel had adverse effects on the oxidation resistance due to the expansion caused by the in-situ formation of spinel from Al2O3-spinel and MgO-C refractories’ components. The different basicity of the slags affect its morphology and characteristics in the initial stage of corrosion and the reaction activity with refractories exhibiting different corrosion phenomena. Al2O3-spinel could improve the corrosion resistance by its inherent high temperature stability. In conclusion, MgO-C refractories with 3 wt% of Al2O3-spinel exhibited the better performance. © 2025 Elsevier Ltd and Techna Group S.r.l.

关键词： Oxidation resistance

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A review of functions and mechanisms of clay soil conditioners and catalysts in thermal remediation compared to emerging photo-thermal catalysis

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Journal of Environmental Sciences 2025年第1期147卷 22-35页

作者： Juan Zhang Shuo Wang Xin Wang Wentao Jiao Minghua Zhang Fujun Ma State Key Laboratory of Advanced Metallurgy School of Metallurgical and Ecological EngineeringUniversity of Science and Technology BeijingBeijing 100083China Research Center for Eco-Environmental Sciences Chinese Academy of SciencesBeijing 100085China College of Agricultural and Environmental Sciences University of CaliforniaDavisCA 95616USA State Key Laboratory of Environmental Criteria and Risk Assessment Chinese Research Academy of Environmental SciencesBeijing 100012China

High temperatures and providing sufficient time for the thermal desorption of persistent organic pollutants(POPs)from contaminated clay soils can lead to intensive energy ***,this article provides a critical review of the potential additives which can improve soil texture and increase the volatility of POPs,and then discusses their enhanced mechanisms for contributing to a green ***-based additives have been used to reduce plasticity of bentonite clay,absorb water and replenish system *** contrast,non-Ca-based additives have been used to decrease the plasticity of kaolin *** soil structure and soil plasticity can be changed through cation exchange and flocculation *** transitionmetal oxides and alkalimetal oxides can be applied to catalyze and oxidize polycyclic aromatic hydrocarbons,petroleum and emerging *** this system,reactive oxygen species(•O_(2)^(-)and•OH)are generated fromthermal excitation without strong chemical ***,multiple active ingredients in recycled solid wastes can be controlled to reduce soil plasticity and enhance thermal ***,the alkali,nano zero-valent iron and nano-TiN can catalyze hydrodechlorination of POPs under reductive ***,photo and photo-thermal catalysis are discussed to accelerate replacement of fossil fuels by renewable energy in thermal remediation.

关键词： Persistent organic contaminants Clay soils Thermal remediation Soil conditioning Synergistic catalysis

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