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Design and high-strength origin of novel (CoFeNi)_(80)Ti_(5)V_(15) medium entropy alloy with “fcc + L1_(2) ”structure

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Journal of Materials Science & technology 2023年第18期149卷 154-160页

作者： Lei Wang Xinyuan Wu Yuan Wu Gang Liu Zhenhua Han Yunpeng Zhang Yanning Su Shengfeng Kang Jun Shen Guojun Zhang School of Materials Science and Engineering Xi’an University of TechnologyXi’an 710048China State Key Laboratory for Advanced Metals and Materials University of Science and Technology BeijingBeijing 100083China State Key Laboratory of Solidification Processing Northwestern Polytechnical UniversityXi’an 710072China

*** The multi-component high entropy alloys(HEAs)or medium entropy alloys(MEAs)attract reseachers’extensive attention,in particular,the single-face center cubic(fcc)HEAs or MEAs due to their some advantages,such as excellent ductility[1,2],good corrosion resistance[3]and high radiation tolerance[4].However,their strength is commonly insufficient for engineering ***,many investigations are ongoing to improve their strength by traditional strengthening mechanisms,like fine-grained strengthening[5,6],solid strengthening[6-8],strain strengthening[9],polyphase strengthening[10-12],and precipitation strength-ening[13-15].Among these strengthening mechanisms,the co-herent L1_(2)-type nanoparticles precipitation strengthening has been proven to be a very effective way to improve their strength[13-15].

关键词： strengthening strength alloy

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Sandwich-Structured Solar Cells with Accelerated Conversion Efficiency by Self-Cooling and Self-Cleaning Design

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Journal of Bionic engineering 2024年第6期21卷 2955-2968页

作者： Huide Fu Ben Wang Rui He Yongpu Yang Hongyuan Li Zhiguang Guo College of Chemistry and Environmental Engineering Shenzhen UniversityShenzhen518060China State Key Laboratory for Turbulence and Complex Systems Department of Mechanics and Engineering ScienceBeijing Innovation Center for Engineering Science and Advanced TechnologyCollege of EngineeringPeking UniversityBeijing100871China Hubei Collaborative Innovation Centre for Advanced Organic Chemical Materials and Ministry of Education Key Laboratory for the Green Preparation and Application of Functional Materials Hubei UniversityWuhan430062PR China State Key Laboratory of Solid Lubrication Lanzhou Institute of Chemical PhysicsChinese Academy of ScienceLanzhou730000PR China

Photovoltaic(PV)power generation is highly regarded for its capability to transform solar energy into electrical ***,in real-world applications,PV modules are prone to issues such as increased self-heating and surface dust accumulation,which contribute to a reduction in photoelectric conversion ***,elevated temperatures can adversely affect the components’operational *** augment the efficiency and extend the lifespan of PV modules,it is crucial to implement cooling strategies and periodic surface dust *** this research,we introduce a composite PV module design that amalgamates a hygroscopic hydrogel with self-cleaning *** design incorporates a superhydrophobic polydimethylsiloxane(PDMS)film as its exposed surface layer and employs a PAM-CaCl2-SiC hygroscopic hydrogel for rear *** arrangement is intended to facilitate efficient surface self-cleaning and passive cooling of the composite PV *** studies were conducted to evaluate the performance of this innovative composite PV module design,and the results showed that the composite PV panel had an increase of about 1.39%in power generation compared to an ordinary PV panel in the spring of Shenzhen,China.

关键词： Self-cleaning Solar cell Superhydrophobic Hygroscopic hydrogel Conversion efficiency

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Enhancing rheology and mechanical properties of DLP 3D-printed Si_(3)N_(4) materials via composition optimization and gas-pressure sintering

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International Journal of Minerals,Metallurgy and Materials 2025年第5期32卷 1220-1233页

作者： Qing Qin Gang Xiong Lin Han Yujuan Zhang Zhen Shen Changchun Ge Institute of Powder Metallurgy and Advanced Ceramics School of Materials Science and EngineeringUniversity of Science and Technology BeijingBeijing 100083China State Key Laboratory of Multimodal Artificial Intelligence Systems Beijing Engineering Research Center of Intelligent Systems and TechnologyInstitute of AutomationChinese Academy of SciencesBeijing 100190China

Digital light processing(DLP)is a crucial additive manufacturing(AM)technique for producing high-precision ceramic *** study aims to optimize the formulation of Si_(3)N_(4)slurry to enhance both its performance and manufacturability in the DLP process,and investigate key factors such as particle size distribution,photopolymer resin monomer ratios,and dispersant types to im-prove the slurry’s rheological *** these optimizations,a photosensitive Si_(3)N_(4)slurry with 50vol%solid content was de-veloped,exhibiting excellent stability,and low viscosity(2.48 Pa·s at a shear rate of 12.8 s^(-1)).The effects of gas-pressure sintering on the material’s phase composition,microstructure,and mechanical properties were further explored,revealing that this technique significantly increases the flexural strength of the green sample from(109±10.24)to(618±42.15)*** sintered ceramics exhibited high hard-ness((16.59±0.05)GPa)and improved fracture toughness((4.45±0.03)MPa·m^(1/2)).Crack trajectory analysis revealed that crack deflec-tion,crack bridging,and the pull-out of rod-likeβ-Si_(3)N_(4)grains,are the main toughening mechanisms,which could effectively mitigate crack *** these mechanisms,crack deflection and bridging were particularly influential,significantly enhancing the frac-ture toughness of the Si_(3)N_(4)***,this research highlights how monomer formulation and gas-pressure sintering strengthen the performance of Si_(3)N_(4)slurry in the DLP three-dimensional printing *** work is expected to provide new insights for fabricat-ing complex Si_(3)N_(4)ceramic components with superior mechanical properties.

关键词： additive manufacturing Si_(3)N_(4)slurry low viscosity pressure sintering

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Modulated synthesis of stoichiometric and sub-stoichiometric two-dimensional covalent organic frameworks for enhanced ethylene purification

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Chinese Chemical Letters 2025年第1期36卷 272-276页

作者： Jiahao Li Guinan Chen Chunhong Chen Yuanyuan Lou Zhihao Xing Tao Zhang Chengtao Gong Yongwu Peng College of Materials Science and Engineering Zhejiang University of TechnologyHangzhou 310014China State Key Laboratory of Organic Electronics and Information Displays&Jiangsu Key Laboratory for Biosensors Institute of Advanced Materials(IAM)Jiangsu National Synergetic Innovation Center for Advanced Materials(SICAM)Nanjing University of Posts and TelecommunicationsNanjing 210023China

Controlled synthesis of two-dimensional covalent organic frameworks(2D COFs),including stoichiometric and sub-stoichiometric variations,is a topic of growing interest due to its potential in gas separation *** this study,we successfully synthesized three distinct 2D COFs by carefully adjusting solvent compositions and monomer ratios during the synthesis of[4+4]type *** included a stoichiometric[4+4]type COF and two sub-stoichiometric[4+2]type COFs,featuring unreacted amino or formyl *** resulting COFs exhibit different gas adsorption and separation ***,sub-stoichiometric COF-DA with residual amino groups shows comparable adsorption capacity for C_(2)H_(2),C_(2)H_(4),and CO_(2)to stoichiometric *** contrast,sub-stoichiometric COF-Py with residual formyl groups displays enhanced adsorption selectivity for C_(2)H_(2)/C_(2)H_(4)and C_(2)H_(2)/CO_(2)separation,with the C_(2)H_(2)/C_(2)H_(4)selectivity being the highest among reported COFs,attributed to increased pore polarity resulting from the presence of formyl *** study not only offers an additional example of substoichiometric COF synthesis but also advocates for further exploration of sub-stoichiometric COF materials,particularly in the field of gas adsorption and separation.

关键词： Two-dimensional covalent organic frameworks Stoichiometric and sub-stoichiometric Residual functional groups Ethylene purification

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Visible-light-induced controllable transformations of cumulative aryldienes through an energy transfer process

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Science China Chemistry 2025年第3期68卷 987-1001页

作者： Ling Qian Ziqi Yu Jiaxin Liu Yin Wei Min Shi Key Laboratory for Advanced Materials and Institute of Fine Chemicals Key Laboratory for Advanced Materials and Feringa Nobel Prize Scientist Joint Research CenterSchool of Chemistry&Molecular EngineeringEast China University of Science and TechnologyShanghai 200237China State Key Laboratory of Organometallic Chemistry Center for Excellence in Molecular SynthesisUniversity of Chinese Academy of SciencesShanghai Institute of Organic ChemistryChinese Academy of SciencesShanghai 200032China Key Laboratory of Fluorine and Nitrogen Chemistry and Advanced Materials Shanghai Institute of Organic ChemistryUniversity of Chinese Academy of SciencesChinese Academy of SciencesShanghai 200032China

In this work,we report a visible light-induced energy transfer process related photochemical protocol of cumulative diene containing compounds for the construction of benzocyclohexene skeletons or the corresponding aromatized structures through an energy transfer process,1,5-hydrogen atom transfer and a 6πelectrocyclization or demethoxylation in the presence of different photocatalysts such as[Ir(dF(Me)ppy)_(2)(dtbbpy)]PF_(6) or *** newly developed photochemical strategy is characterized by mild conditions,broad substrate applicability,good functional group tolerance and good *** mechanistic paradigm was clarified by deuterium labeling,kinetic,photophysical and electrochemical analyses,control experiments and density functional theory(DFT)*** transformation of the obtained product to the drug-like molecules such as Sertraline and the luminescent conjugated aromatic compounds has also been disclosed.

关键词： visible-light photocatalysis EnT process 1,5-HAT remote C(sp^(3))-H bond activation

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Dislocation behavior in Cu single crystal joints under the ultrasonically excited high-strain-rate deformation

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Journal of Materials Science & technology 2023年第10期141卷 66-77页

作者： Qiuchen Ma Jingyuan Ma Jianli Zhou Xiaoxiong Zheng Hongjun Ji The State Key Laboratory of Advanced Welding and Joining School of Materials Science and EngineeringHarbin Institute of Technology at ShenzhenShenzhen 518055China Sauvage Laboratory for Smart Materials Shenzhen Key Laboratory of Flexible Printed Electronics TechnologySchool of Materials Science and EngineeringHarbin Institute of Technology(Shenzhen)Shenzhen 518055China School of Science Harbin Institute of Technology at ShenzhenShenzhen 518055China

The coupling effects of ultrasonic excitation and high-strain-rate deformation are the core factors for weld formation during ultrasonic ***,interfacial deformation behavior still shrouds in uncer-tainty because of the contradictory features between mutual dislocation retardation caused by severely frictional deformation and ultrasonic-accelerated dislocation motion.[101]and[111]-oriented Cu single crystals which tended to form geometrically necessary boundaries(GNBs)were selected as the welding substrates to trace the uniquely acoustoplastic effects in the interfacial region under the ultrasonically excited high-strain-rate *** was indicated that for a low energy input,micro-welds localized at the specific interface region,and equiaxed dislocation cells substituting for GNBs dominated in the ini-tial single crystal rotation *** the welding energy increased,continuous shear deformation drove the dynamic recrystallization region covered by equiaxed grains to spread *** discrete dislocations inside the recrystallized grains and nascent dislocation cells at the grain boundaries were ob-served in[101]and[111]joints simultaneously,suggesting that the ultrasonic excitation promoted motion of intragranular dislocation and pile-up along the sub-grain *** interfacial morphology be-fore and after expansion of recrystallization region all exhibited the weakening of orientation constraint on dislocation motion,which was also confirmed by the similar micro-hardness in joint *** first-principle calculation and applied strain-rate analysis further revealed that ultrasonic excitation en-hanced dislocation slipping,and enabled dislocation motion to accommodate severe plastic deformation at a high-strain-rate.

关键词： Acoustoplasticity Ultrasonic welding Cu single crystal Dynamic recrystallization Dislocation cell High-strain-rate deformation

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Enhanced Electrochemical Performances of Ni Doped Cr_(8)O_(21)Cathode Materials for Lithium-ion Batteries

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Journal of Wuhan University of technology(Materials Science) 2023年第6期38卷 1242-1247页

作者： TANG Guoli LIU Hanxing YU Zhiyong YANG Bo KONG Linghua School of Materials Science and Engineering Wuhan University of TechnologyWuhan 430070China International School of Materials Science and Engineering Wuhan University of TechnologyWuhan 430070China State Key Laboratory of Advanced Technology for Materials Synthesis and Processing Wuhan 430070China

Cathode materials,nickel doped Cr_(8)O_(21),were synthesized by a solid-state *** effects of Ni doping on the electrochemical performances of Cr_(8)O_(21) were *** experimental results show that the discharge capacities of the samples depend on the nickel contents,which increases firstly and then decreases with increasing Ni *** Ni_(0.5)Cr_(7.5)O_(21)delivers a first capacity up to 392.6 m Ah·g^(-1)at *** addition,Ni doped sample also demonstrates enhanced cycling stability and rate capability compared with that of the bare Cr_(8)O_(21).At 1 C,an initial discharge capacity of 348.7 m Ah·g^(-1)was achieved for Ni_(0.5)Cr_(7.5)O_(21),much higher than 271.4 m Ah·g^(-1)of the un-doped sample,with an increase of more than 28%.Electrochemical impedance spectroscopy results confirm that Ni doping reduces the growth of interface resistance and charge transfer resistance,which is conducive to the electrochemical kinetic behaviors during charge-discharge.

关键词： Cr_(8)O_(21) cathode material doping electrochemical performances lithium-ion batteries

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Ultra-sensitive,highly linear,and hysteresis-free strain sensors enabled by gradient stiffness sliding strategy

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npj Flexible Electronics 2024年第1期8卷 817-824页

作者： Fuhua Xue Qingyu Peng Renjie Ding Pengyang Li Xu Zhao Haowen Zheng Liangliang Xu Zhigong Tang Xinxing Zhang Xiaodong He National Key Laboratory of Science and Technology on Advanced Composites in Special Environments Center for Composite Materials and StructuresHarbin Institute of Technology150080 HarbinChina State Key Laboratory of Polymer Materials Engineering Polymer Research InstituteSichuan University610065 ChengduChina

Developing strain sensors with both high sensitivity and high linearity has always been the goal of *** to resistive strain sensors,capacitive strain sensors have incomparable linearity advantages,but have always been limited by low ***,we report a gradient stiffness sliding design strategy that addresses this problem,significantly improving sensitivity while maintaining high *** controlling the distribution of the locally enhanced electric field and the heterogeneous deformation of the substrate,a strain sensor with excellent performance is successfully prepared,exhibiting a giant gauge factor(9.1×10^(6))and linearity(R^(2)=0.9997)over the entire sensing range,together with almost no hysteresis and fast response time(17 ms).The gradient stiffness sliding design is a general strategy expected to be applied to other types of sensors to achieve ultra-high sensitivity and ultra-high linearity at the same time.

关键词： stiffness strain gradient

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Theoretically predicted innovative palladium stripe dopingcobalt(111) surface with excellent catalytic performance for carbonmonoxide oxidative coupling to dimethyl oxalate

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Chinese Journal of Chemical engineering 2024年第9期73卷 235-243页

作者： Bingying Han Neng Shi Mengjie Dong Ye Liu Runping Ye Lixia Ling Riguang Zhang Baojun Wang State Key Laboratory of Clean and Efficient Coal Utilization Taiyuan University of TechnologyTaiyuan 030024China College of Chemical Engineering and Technology Taiyuan University of TechnologyTaiyuan 030024China College of Chemistry and Chemical Engineering Nanchang UniversityNanchang 330031China Shanxi-Zheda Institute of Advanced Materials and Chemical Engineering Taiyuan 030013China

Pd-based catalysts are extensively employed to catalyze CO oxidative coupling to generate DMO,while the expensive price and high usage of Pd hinder its massive application in industrial *** Pd-based catalysts with high efficiency and low Pd usage as well as expounding the catalytic mechanisms are significant for the *** this study,we theoretically predict that Pd stripe doping Co(111)surface exhibits excellent performance than pure Pd(111),Pd monolayer supporting on Co(111)and Pd single atom doping Co(111)surface,and clearly expound the catalytic mechanisms through the density functional theory(DFT)calculation and micro-reaction kinetic model *** is obtained that the favorable reaction pathway is COOCH_(3)-COOCH_(3)coupling pathway over these four catalysts,while the rate-controlling step is COOCH_(3)+CO+OCH_(3)→2COOCH_(3)on Pd stripe doping Co(111)surface,which is different from the case(2COOCH_(3)→DMO)on pure Pd(111),Pd monolayer supporting on Co(111)and Pd single atom doping Co(111)*** study can contribute a certain reference value for developing Pd-based catalysts with high efficiency and low Pd usage for CO oxidative coupling to DMO.

关键词： CO oxidative coupling to DMO Pd stripe doping Co(111)surface Catalytic mechanism DFT calculation Micro-reaction kinetic model analysis Catalytic performance

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A multi-component nanocrystalline FeCrV alloy with improved mechanical properties and excellent irradiation resistance

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Progress in Natural Science:Materials International 2022年第4期32卷 433-442页

作者： Tingting Li Sizhe Diao Pingping Liu Yong Zhang Qian Zhan School of Materials Science and Engineering University of Science and Technology Beijing Beijing Advanced Innovation Center for Materials Genome Engineering State Key Laboratory for Advanced Metals and Materials University of Science and Technology Beijing

An equiatomic low-activated Fe Cr V ternary alloy was prepared by mechanical alloying and spark plasma sintering. The BCC solid solution alloy exhibited an excellent strength-ductility synergy properties, which was 1.85GPa compressive yield strength, 3.04 GPa fracture strength and more than 28% plasticity at room *** at an elevated temperature of 600°C, its yield strength was still more than 1 GPa, revealing a pronounced high temperature resistance. The Fe Cr V alloy had a homogeneous microstructure with high-density dislocations.A nanocrystalline characteristic was demonstrated and the average grain size was about 322 nm, leading to the improved mechanical properties. The strengthening mechanism was discussed in detail and the contributions of strengthening factors were calculated. The Fe Cr V alloy was irradiated up to 160 dpa with 2 Me V Au2+ions at 573K. The nanoindentation test was carried out to simply evaluate the hardening degree under such a high dose irradiation with heavy ions. The semi-quantitative analysis results show that Fe Cr V alloy has an excellent irradiation tolerance compared with pure Fe.

关键词： Mechanical properties Nanocrystalline Strengthening mechanism Au2+ irradiation Multi-component alloy Mechanical alloying

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