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An artificial interphase enables stable PVDF-based solid-state Li metal batteries

Nano Research 2024年第3期17卷 1482-1490页

作者： Mengjun Wu Jiangping Song Jiaheng Lei Haolin Tang State Key Laboratory of Advanced Technology for Materials Synthesis and Processing Wuhan University of TechnologyWuhan 430070China Department of Chemistry School of ChemistryChemical Engineering and Life SciencesWuhan University of TechnologyWuhan 430070China Foshan Xianhu Laboratory of the Advanced Energy Science and Technology Guangdong Laboratory Foshan 528200China

Composite polymer electrolytes(CPEs)have attracted much attention for high energy density solid-state lithium-metal batteries owing to their flexibility,low cost,and easy ***,the unstable Li/CPE interface is always challengeable for the practical utilization of ***,a polymer interlayer containing K+prepared by ultraviolet(UV)-curing precursor solution is coated on Li surface to stabilize the interface between poly(vinylidene difluoride)(PVDF)composite electrolytes and Li *** from the physical barrier of the interlayer,the continuous decomposition of PVDF is restrained and the intimate contact between electrode and electrolyte is also achieved to reduce the interface ***,the added K+is utilized to further regulate smooth Li *** a consequence,the symmetric Li|Li cell with coated Li demonstrates steady cycling at 0.4 mAh·cm^(-2) and a high critical current density of 1 mA·cm^(-2).The assembled Li|LiFePO_(4) cell presents outstanding cycling stability(capacity retention of 90%after 400 cycles at 1 C)and good rate *** associated pouch cell performs impressive flexibility and *** work provides a convenient strategy to achieve stable Li/PVDF interface for high-performance PVDF-based solid state Li metal batteries.

关键词： interfacial modification solid-state batteries composite polymer electrolytes interfacial compatibility lithium dendrite

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Deformation mechanism of Cu-Al-Ni shape memory alloys fabricated via laser powder b e d fusion:Tension-compression asymmetry

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Journal of Materials Science & technology 2023年第36期167卷 14-26页

作者： Yankun Zhang Lianyong Xu Lei Zhao Danyang Lin Minqian Liu Wei Chen Yongdian Han School of Materials Science and Engineering Tianjin UniversityTianjin 300350China Tianjin Key Laboratory of Advanced Joining Technology Tianjin 300350China State Key Laboratory of Engines Tianjin UniversityTianjin 300350China State Key Laboratory of Advanced Welding and Joining Harbin Institute of TechnologyHarbin 150001China

Introducing the unique advantage of additive manufacturing technology into copper-based shape memory alloys(SMAs)to fabricate high-performance alloys has garnered great attention in recent years,but the intrinsic relationships between microstructure and mechanical properties need to be further *** this paper,the microstructural evolution of ternary CuAlNi SMAs fabricated by laser powder bed fusion(LPBF)under the tensile-compressive loading was investigated to determine the underlying mechanism of tension-compression asymmetry,that is,excellent compressive but poor tensile *** characterization of the different deformation stages revealed the numerous activated deformation mech-anism on the 18R martensite matrix.A twin-related transformation dominated the main plastic defor-mation process due to lower stacking faults energy and high-density pre-existing planer defects in the CuAlNi *** twinning nucleated at prior austenite boundaries and developed into parallel and network structures inside the parent grain of different *** addition,the preferred orientation in different stages,the stress-inducedγphase transformation,and the interaction between dislocations and stacking faults are *** results not only provide significant insights to understand the detwinning and deformation twinning process of SMAs but also establish the essential framework of mi-crostructure and mechanical properties of Cu-based SMAs fabricated by LPBF.

关键词： Shape memory alloys Cu-based Laser powder bed fusion Microstructural evolution Deformation mechanism

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Mixed Alkali-zinc Effects on Thermo-mechanical Properties in Borosilicate Glasses

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Journal of Wuhan University of technology(Materials Science) 2024年第5期39卷 1093-1099页

作者： XIAO Guanzhou TAO Yunhang ZHOU Hemin ZHENG Qingshuang QIAO Ang TAO Haizheng State Key Laboratory of Silicate Materials for Architectures Wuhan University of TechnologyWuhan 430070China Wuhan University of Technology Advanced Engineering Technology Research Institute of Zhongshan City Zhongshan 528437China

A series of mixed alkali-zinc borosilicate glasses with various r values(r=molar ratio of[ZnO]/([R^(2)O]+[ZnO]))from 0.00 to 1.00 were fabricated to probe the mixed alkali-zinc effects on thermo-mechanical *** nonlinear evolution of glass transition temperature(T_(g))with the addition of ZnO is ascribed to the competition of two converse factors,i e,the T_(g)depression as one of the colligative properties for a solution,on the one hand,and the enhancement of T_(g)due to the higher field strength of zinc cations compared to that of alkali ***,the nonlinear evolution of elastic moduli and coefficients of thermal expansion with r is attributed to the variance of intermediate-range clusters,which is confirmed by infrared and Raman scattering *** findings are very helpful in tailoring the performance of borosilicate glasses.

关键词： glass transition temperature elastic moduli coefficient of thermal expansion borosilicate glass

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An improved efficient adaptive method for large-scale multiexplosives explosion simulations

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Defence technology(防务技术) 2025年第3期45卷 28-47页

作者： Tao Li Cheng Wang Baojun Shi School of Mechanical Engineering Key Laboratory of Advanced Intelligent Protective Equipment TechnologyMinistry of EducationHebei University of TechnologyTianjin300401China State Key Lab of Explosion Science and Safety Protection Beijing Institute of TechnologyBeijing 100081China

Shock wave caused by a sudden release of high-energy,such as explosion and blast,usually affects a significant range of *** utilization of a uniform fine mesh to capture sharp shock wave and to obtain precise results is inefficient in terms of computational *** is particularly evident when large-scale fluid field simulations are conducted with significant differences in computational domain *** this work,a variable-domain-size adaptive mesh enlargement(vAME)method is developed based on the proposed adaptive mesh enlargement(AME)method for modeling multi-explosives explosion *** vAME method reduces the division of numerous empty areas or unnecessary computational domains by adaptively suspending enlargement operation in one or two directions,rather than in all directions as in AME method.A series of numerical tests via AME and vAME with varying nonintegral enlargement ratios and different mesh numbers are simulated to verify the efficiency and order of *** estimate of speedup ratio is analyzed for further efficiency *** large-scale near-ground explosion experiments with single/multiple explosives are performed to analyze the shock wave superposition formed by the incident wave,reflected wave,and Mach ***,the vAME method is employed to validate the accuracy,as well as to investigate the performance of the fluid field and shock wave propagation,considering explosive quantities ranging from 1 to 5 while maintaining a constant total *** results show a satisfactory correlation between the overpressure versus time curves for experiments and numerical *** vAME method yields a competitive efficiency,increasing the computational speed to 3.0 and approximately 120,000 times in comparison to AME and the fully fine mesh method,*** indicates that the vAME method reduces the computational cost with minimal impact on the results for such large-scale high-energy release problems with signi

关键词： Large-scale explosion Shock wave Adaptive method Fluid field simulations Efficient method

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A homogeneous atmospheric pressure air plasma in a 10 mm gap based on a three-electrode configuration

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Plasma Science and technology 2023年第10期25卷 75-80页

作者：李志宇刘大伟卢新培聂兰兰 State Key Laboratory of Advanced Electromagnetic Engineering and Technology School of Electrical and Electronic EngineeringHuazhong University of Science and TechnologyWuhan 430074People's Republic of China

Generation of atmospheric pressure homogeneous air plasma in a large gap(>4 mm)is a *** this study,an atmospheric pressure homogeneous air plasma generated in a gap up to 10 mm is reported,which is based on a three-electrode configuration,where a high-voltage(HV)electrode and a middle electrode form a surface dielectric barrier discharge(S-DBD),and together with the ground electrode form the main volume ***-speed photographs confirm that the discharge in the main gap is *** gas temperature of the plasma estimated from the N_(2)(C^(3)∏_(u)-B^(3)∏_(g))(Δv=-2)emission is about 320 K,which is close to room temperature.A detailed analysis shows that the discharge ignited between the HV electrode and the middle electrode is serving as an electron source,and the electrons deposited on the dielectric plate are due to the S-DBD along with the applied voltage generating a driving force,which results in a high concentration of seed electrons in the main gap and induces the homogeneous *** analysis shows that the electric field in the main gap is only about18.45 k V·cm^(-1),which is much lower than the typical breakdown electric field of 30 k V·cm^(-1)for atmospheric pressure air discharge.

关键词： atmospheric pressure plasma homogeneous discharge glow discharge air plasma

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engineering Thermoelectric Performance of α-GeTe by Ferroelectric Distortion

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Energy & Environmental Materials 2024年第2期7卷 171-179页

作者： Yuting Fan Chenghao Xie Jun Li Xiangyu Meng Jinchang Sun Jinsong Wu Xinfeng Tang Gangjian Tan State Key Laboratory of Advanced Technology for Materials Synthesis and Processing Wuhan University of TechnologyWuhan 430070China International School of Materials Science and Engineering Wuhan University of TechnologyWuhan 430070China

The rhombohedralα-GeTe can be approximated as a slightly distorted rock-salt structure along its[111]direction and possesses superb thermoelectric ***,the role of such a ferroelectric-like structural distortion on its transport properties remains ***,we performed a systematic study on the crystal structure and electronic band structure evolutions of Ge_(1-x)Sn_(x)Te alloys where the degree of ferroelectric distortion is continuously *** is revealed that the band gap is maximized while multiple valence bands are converged at x=0.6,where the ferroelectric distortion is the least but still *** undistorted,the band gap is considerably reduced,and the valence bands are largely separated ***,near the ferro-to-paraelectric phase transition Curie temperature,the lattice thermal conductivity reaches its minima because of significant lattice softening enabled by ferroelectric *** predict a peak ZT value of 2.6 at 673 K inα-GeTe by use of proper dopants which are powerful in suppressing the excess hole concentrations but meanwhile exert little influence on the ferroelectric distortion.

关键词： electronic band structures ferroelectric distortion lattice softening thermoelectric α-GeTe

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Peak-like three-dimensional CoFe_(2)O_(4)/carbon nanotube decorated bamboo fabrics for simultaneous solar-thermal evaporation of water and photocatalytic degradation of bisphenol A

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Journal of Materials Science & technology 2024年第12期179卷 40-49页

作者： Rui-Jie Pan Jing Wu Jin Qu Tingting Zhang Fan-Zhen Jiao Mang Zhao Meng-Yan Han Xiaofeng Li Zhong-Zhen Yu State Key Laboratory of Organic-Inorganic Composites College of Materials Science and EngineeringBeijing University of Chemical TechnologyBeijing 100029China Beijing Key Laboratory of Advanced Functional Polymer Composites Beijing University of Chemical TechnologyBeijing 100029China

Catalytic CoFe_(2)O_(4) and solar-thermal carbon nanotube decorated bamboo fabrics(CCBF)are fabricated for integrating efficient solar steam generation from wastewater with catalytic degradation of its organic *** to the numerous porous channels and polar groups of bamboo fabric and the efficient solar-thermal energy conversion of black carbon nanotubes,the porous and hydrophilic CCBF exhibits fast upward transport of water,efficient solar light absorption,and high solar-thermal energy conversion *** decorated CoFe_(2)O_(4) not only enhances the solar-thermal energy conversion efficiency of CCBF but also activates potassium peroxymonosulfate to generate abundant highly active species for catalytic degradation of bisphenol A(BPA).Furthermore,folding the CCBF into a peak-like 3D evaporator can en-hance solar energy utilization,and gain environmental energy for promoting solar-thermal water evapo-ration and catalytic degradation *** 3D CCBF evaporator achieves a water evaporation rate of 2.72 kg m^(-2) h^(-1) under 1-sun ***,100%of the BPA in the seawater can be degraded within 10 *** exceptional high purification efficiency of 27.72 kg m^(-2) h^(-1) is achieved with the 3D evaporator during a long-term treatment of BPA-containing seawater under 1-sun *** work demonstrates efficient purification of seawater/wastewater with both metal ions and organic pollutants by simultaneous solar-thermal evaporation of water and catalytic degradation of organic pollutants.

关键词： Solar-thermal water evaporation Seawater desalination Catalytic degradation Carbon nanotubes CoFe_(2)O_(4)

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Local chemical ordering and its impact on radiation damage behavior of multi-principal element alloys

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Journal of Materials Science & technology 2023年第4期135卷 13-25页

作者： Leqing Liu Xiongjun Liu Qing Du Hui Wang Yuan Wu Suihe Jiang Zhaoping Lu Beijing Advanced Innovation Center for Materials Genome Engineering State Key Laboratory for Advanced Metals and MaterialsUniversity of Science and Technology BeijingBeijing 100083China

Multi-principal element alloys(MPEAs)have attracted much attention as future nuclear materials due to their extraordinary radiation *** this work,we have elucidated the development of local chemical orderings(LCOs)and their influences on radiation damage behavior in the typical CrFeNi MPEA by hybrid-molecular dynamics and Monte Carlo *** was found that considerable LCOs consist-ing of the Cr-Cr and Ni-Fe short-range orders existed in the ordered configuration with optimized system *** modeling the accumulation cascades up to 1000 recoils,we revealed that the size of de-fect clusters and dislocation loops is smaller in the ordered configuration than those in the random one,although the former formed more Frenkel pairs(i.e.,self-interstitials and vacancies).In addition,the dis-tribution of dislocation loops is relatively more dispersed in the ordered configuration,and the stair-rod dislocations related to irradiation swelling are also smaller,implying that the existence of LCOs is con-ducive to enhancing radiation damage *** understand the underlying mechanism,the effects of LCOs on the formation and evolution of defects and radiation resistance were discussed from the aspects of atomic bonding,migration path,and energy of defect diffusion,which provides theoretical guidance for the design of MPEAs with enhanced radiation resistance.

关键词： Multi-principal element alloys Local chemical ordering Radiation damage Dislocation evolution Molecular dynamics simulation

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Precipitation Behavior of MnS Inclusion in Unidirectionally-solidified Fe–18Mn–1Al–0.3C Steels

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Tetsu-To-Hagane/Journal of the Iron and Steel Institute of Japan 2025年第3期111卷 122-130页

作者： Fan, Yuewen Kameda, Kouki Hu, Xiaojun Matsuura, Hiroyuki State Key Laboratory of Advanced Metallurgy University of Science and Technology Beijing China Department of Materials Engineering Graduate School of Engineering The University of Tokyo Japan

In order to reasonably control the precipitation of inclusions during solidification in TWIP steels, the precipitation behavior of typical MnS inclusions in high manganese steel was investigated by unidirectional solidification experiments. Through the combined analyses using ASEM-EDS, optical microscope, and thermodynamic calculation, it was found that Mn concentration in the liquid metal region were higher than those in the solid metal region. Furthermore, closer to the inclusion the liquid phase was, higher its Mn content was. In Fe–18mass%Mn–1Al–0.3C, MnS inclusions can precipitate at the positions located in the junction of dendrites at the end of the solidification (solid fraction fS = 0.96), Mn content reaching 34.88 mass%. Already existing Al2O3 particles could become the core of MnS to form composite inclusions to promote the MnS precipitation during the solidification process. When fS achieved 0.7 leading the Mn segregation in the liquid phase to 25 mass%, MnS starts to precipitate to attach the Al2O3 surface to form composite inclusion. © 2025 The Iron and Steel Institute of Japan.

关键词： Manganese steel

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Development of a toroidal soft x-ray imaging system and application for investigating three-dimensional plasma on J-TEXT

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Plasma Science and technology 2024年第3期26卷 94-99页

作者：赵传旭李建超张晓卿王能超丁永华杨州军江中和严伟李杨波毛飞越任正康 the J-TEXT Team International Joint Research Laboratory of Magnetic Confinement Fusion and Plasma Physics State Key Laboratory of Advanced Electromagnetic Engineering and TechnologySchool of Electrical and Electronic Engineering and School of PhysicsHuazhong University of Science and TechnologyWuhan 430074People's Republic of China Hubei Key Laboratory of Optical Information and Pattern Recognition Wuhan Institute of TechnologyWuhan 430205People's Republic of China International Joint Research Laboratory of Magnetic Confinement Fusion and Plasma Physics State Key Laboratory of Advanced Electromagnetic Engineering and TechnologySchool of Electrical and Electronic EngineeringHuazhong University of Science and TechnologyWuhan 430074People's Republic of China

A toroidal soft x-ray imaging(T-SXRI)system has been developed to investigate threedimensional(3D)plasma physics on *** T-SXRI system consists of three sets of SXR *** sets are newly developed and located on the vacuum chamber wall at toroidal positionsφof 126.4°and 272.6°,respectively,while one set was established previously atφ=*** set of SXR arrays consists of three arrays viewing the plasma poloidally,and hence can be used separately to obtain SXR images via the tomographic *** sawtooth precursor oscillations are measured by T-SXRI,and the corresponding images of perturbative SXR signals are successfully reconstructed at these three toroidal positions,hence providing measurement of the 3D structure of precursor *** observed 3D structure is consistent with the helical structure of the m/n=1/1 *** experimental observation confirms that the T-SXRI system is able to observe 3D structures in the J-TEXT plasma.

关键词： SXR imaging J-TEXT tokamak three-dimensional measurement MHD

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