检索结果-内蒙古大学图书馆

In-situ physical/chemical cross-linked hydrogel electrolyte achieving ultra-stable zinc anode-electrolyte interface towards dendrite-free zinc ion battery

引用

Journal of Energy Chemistry 2024年第10期97卷 342-351,I0007页

作者： Chen-Yang Li Jiang-Lin Wang Dong-Ting Zhang Min-Peng Li Hao Chen Wei-Hai Yi Xin-Ying Ren Bao Liu Xue-Feng Lu Mao-Cheng Liu State Key Laboratory of Advanced Processing and Recycling of Non-ferrous Metals Lanzhou University of TechnologyLanzhou 730050GansuChina School of Materials Science and Engineering Lanzhou University of TechnologyLanzhou 730050GansuChina Chaowei Power Group Co. LTDChangxing 313100ZhejiangChina School of Vehicle Engineering Jiangsu UniversityNanjing 210031jiangsuChina

Hydrogen evolution reaction(HER),zinc corrosion,and dendrites growth on zinc metal anode are the major issues limiting the practical applications of zinc-ion ***,an in-situ physical/chemical cross-linked hydrogel electrolyte(carrageenan/polyacrylamide/ZnSO_(4),denoted as CPZ)has been developed to stabilize the zinc anode-electrolyte interface,which can eliminate side reactions and prevent dendrites *** in-situ CPZ hydrogel electrolyte improves the reversibility of zinc anode due to eliminating side reactions caused by active water ***,the electrostatic interaction between the SO_(4)^(-)groups in CPZ and Zn^(2+)can encourage the preferential deposition of zinc atoms on(002)crystal plane,which achieve dendrite-free and homogeneous zinc *** in-situ hydrogel electrolyte offers a streamlined approach to battery manufacturing by allowing for direct integration into the ***,the Zn//Zn half battery with CPZ hydrogel electrolyte can enable an ultra-long cycle over 5500 h at a current density of 0.5 mA cm^(-2),and the Zn//Cu half battery reach an average coulombic efficiency of 99.37%.The Zn//V_(2)O_5-GO full battery with CPZ hydrogel electrolyte demonstrates94.5%of capacity retention after 2100 *** study is expected to open new thought for the development of commercial hydrogel electrolytes for low-cost and long-life zinc-ion batteries.

关键词： In-suit CPZ hydrogel electrolyte Hydrogen evolution reaction and zinc corrosion Dendrites growth Zinc anode-electrolyte interface Zn ion batteries

来源：评论

学校读者我要写书评

暂无评论

Flexible coatings with microphase separation structure attained by copolymers and ultra-fine nanoparticles for endurable antifouling

引用

Journal of materials Science & technology 2021年第23期82卷 179-186页

作者： Zhuo Chen Shun Chen Yufei Xiong Yuping Yang Yang Zhang Lijie Dong State Key Laboratory of Advanced Technology for Materials Synthesis and Processing Center for Smart Materials and DevicesWuhan University of TechnologyWuhan430070China School of Civil Engineering Architecture and EnvironmentHubei University of TechnologyWuhan430068China

Incorporating antibacterial agent into biomimetic coating inspired by natural organisms with micronano structure surface has generated more interest for antifouling *** this work,poly(dimethylsiloxane)(PDMS)-based triblock copolymers and sub-20 nm nanoparticles Ag and heterogeneous Fe_(3)O_(4)-coated Ag(Fe_(3)O_(4)@Ag)were used to construct microphase separation topography with oriented copolymer blocks *** artificial surface was verified by atomic force microscopy and scanning electron microscopy ***,the surface exhibited relative stable hydrophobic property,which was demonstrated by the water contact angle and dynamic air-bubble contact angle ***,after immersed in BSA solution 24 h and 720 h,the actual BSA absorption amount of the surface with Fe_(3)O_(4)@Ag nanoparticles was as low as 10%and 27%that of the initial BSA amount,***,the surface also showed remarkable antibacterial performance,which effectively suppressed the growth rate of Escherichia *** strategy of constructing the flexible micro p hase separation structure by introducing heterogeneous inorganic antibacterial nanoparticles into a block copolymer substrate opens up a new way to create an antifouling surface coating.

关键词： Microphase separation topography Ultra-fine nanoparticles Antifouling surfaces Antibacterial performance

来源：评论

学校读者我要写书评

暂无评论

Unraveling the reaction mechanisms of electrode materials for sodiumion and potassium‐ion batteries by in situ transmission electron microscopy

引用

Interdisciplinary materials 2022年第2期1卷 196-212页

作者： Hong Wang Fang Liu Ruohan Yu Jinsong Wu Nanostructure Research Center(NRC) Wuhan University of TechnologyWuhanHubeiChina State Key Laboratory of Advanced Technology for Materials Synthesis and Processing School of Materials Science and EngineeringWuhan University of TechnologyWuhanHubeiChina School of Mathematics and Physics Jingchu University of TechnologyJingmenHubeiChina

Sodium ion batteries(SIBs)and potassium ion batteries(PIBs)have caught numerous attention due to the low cost and abundant availability of sodium and ***,their power density,cycling stability and safety need further improvement for practical *** on the reaction mechanisms and structural degradation when cycling are of great *** situ transmission electron microscopy(TEM)is one of the most significant techniques to understand and monitor electrochemical processes at an atomic scale with real-time *** this review,the current progress in unraveling reaction mechanisms of electrode materials for SIBs and PIBs via in situ TEM is ***,the importance of in situ TEM is ***,based on the three types of electrochemical reaction,i.e.,intercalation reac-tion,conversion reaction and alloying reaction,the structural evolution and reaction kinetics at atomic resolution,and their relation to the electrochemical performance of electrode materials are reviewed and described in ***-nally,future directions of in situ TEM for SIBs and PIBs are ***,the in‐depth understanding revealed by in situ TEM will give an instructive guide in rational design of electrode materials for high performance electrode materials of SIBs and PIBs.

关键词： in situ transmission electron microscopy potassium ion batteries sodiumion batteries

来源：评论

学校读者我要写书评

暂无评论

Carrier recombination suppression and transport enhancement enable high-performance self-powered broadband Sb_(2)Se_(3) photodetectors

引用

InfoMat 2023年第4期5卷 60-76页

作者： Shuo Chen Yi Fu Muhammad Ishaq Chuanhao Li Donglou Ren Zhenghua Su Xvsheng Qiao Ping Fan Guangxing Liang Jiang Tang Shenzhen Key Laboratory of Advanced Thin Films and Applications Key Laboratory of Optoelectronic Devices and Systems of Ministry of Education and Guangdong ProvinceCollege of Physics and Optoelectronic EngineeringShenzhen UniversityShenzhenGuangdongthe People's Republic of China MOE Key Laboratory of New Processing Technology for Non-ferrous Metals and Materials Guangxi Key Laboratory of Processing for Non-ferrous Metals and Featured MaterialsGuangxi UniversityNanningGuangxithe People's Republic of China State Key Laboratory of Silicon Materials&School of Materials Science and Engineering Zhejiang UniversityHangzhouZhejiangthe People's Republic of China Wuhan National Laboratory for Optoelectronics(WNLO) School of Optical and Electronic InformationHuazhong University of Science and TechnologyWuhanHubeithe People's Republic of China

Antimony selenide(Sb_(2)Se_(3))is a promising candidate for photodetector applications boasting unique material benefits and remarkable optoelectronic *** high-performance self-powered Sb_(2)Se_(3)photodetector through a synergistic regulation of absorber layer and heterojunction interface demonstrates great potential and needs essential *** this study,an effective two-step thermodynamic/kinetic deposition technique containing sputtered and selenized Sb precursor is implemented to induce self-assembled growth of Sb_(2)Se_(3)light absorbing thin film with large crystal grains and desirable[hk1]orientation,presenting considerable thin-film photodetector ***,aluminum(Al^(3+))cation dopant is introduced to modify the optoelectronic properties of CdS buffer layer,and further optimize the Sb_(2)Se_(3)/CdS(Al)heterojunction interface *** to the suppressed carrier recombination and enhanced carrier transport kinetics,the champion Mo/Sb_(2)Se_(3)/CdS(Al)/ITO/Ag photodetector exhibits self-powered and broadband characteristics,accompanied by simultaneously high responsivity of 0.9 A W^(-1)(at 11 nW cm^(-2)),linear dynamic range of 120 dB,impressive ON/OFF switching ratio over 10^(6)and signal-to-noise ratio of 10^(9),record total noise determined realistic detectivity of 4.78×10^(12)Jones,and ultra-fast response speed with rise/decay time of 24/75 ns,representing the top level for Sb_(2)Se_(3)-based *** intriguing work opens up an avenue for its selfpowered broadband photodetector applications.

关键词： photoresponse recombination suppression Sb_(2)Se_(3) self-powered photodetector transport enhancement

来源：评论

学校读者我要写书评

暂无评论

Polyzwitterionic cross-linked double network hydrogel electrolyte enabling high-stable Zn anode

引用

Nano Research 2024年第6期17卷 5278-5287页

作者： Mengyu Shi Junlong Zhang Guochuan Tang Ben Wang Sen Wang Xiaoxian Ren Guojie Li Weihua Chen Chuntai Liu Changyu Shen State Key Laboratory of Structural Analysis Optimization and CAE Software for Industrial EquipmentNational Engineering Research Center for Advanced Polymer Processing TechnologyZhengzhou UniversityZhengzhou 450002China College of Chemistry and Green Catalysis Center Zhengzhou UniversityZhengzhou 450001China Research Institute of Interdisciplinary Science and School of Materials Science and Engineering Dongguan University of TechnologyDongguan 523808China

Zn metal anode suffers from dendrite issues and passive byproducts,which severely plagues the practical application of aqueous Zn metal ***,a polyzwitterionic cross-linked double network hydrogel electrolyte composed of physical crosslinking(hyaluronic acid)and chemical crosslinking(synthetic zwitterionic monomer copolymerized with acrylamide)is introduced to overcome these *** the one hand,highly hydrophilic physical network provides an energy dissipation channel to buffer stress and builds a H_(2)O-poor interface to avoid side *** the other hand,the charged groups(sulfonic and imidazolyl)in chemical crosslinking structure build anion/cation transport channels to boost ions’kinetics migration and regulate the typical solvent structure[Zn(H_(2)O)_(6)]^(2+)to R-SO_(3)^(−)[Zn(H_(2)O)_(4)]^(2+),with uniform electric field distribution and significant resistance to dendrites and parasitic *** on the above functions,the symmetric zinc cell exhibits superior cycle stability for more than 420 h at a high current density of 5 mA·cm^(−2),and Zn||MnO_(2)full cell has a reversible specific capacity of 150 mAh·g^(−1)after 1000 cycles at 2 C with this hydrogel ***,the pouch cell delivers impressive flexibility and cyclability for energy-storage applications.

关键词： Zn anode dendrites parasitic reactions polyzwitterion double network hydrogel electrolyte

来源：评论

学校读者我要写书评

暂无评论

Anomalous enhancing effects of electric pulse treatment on strength and ductility of TC17 linear friction welding joints

引用

Journal of materials Science & technology 2024年第36期203卷 155-166页

作者： Xin Zhang Junjie Zhang Yunkui Yao Qingsong Qiao Lixing Zhao Leichang Liu Feng Jin Mei Zhan Hongwei Li Key Laboratory of High-Performance Manufacturing for Aero Engine Ministry of Industry and Information TechnologyNorthwestern Polytechnical UniversityXi’an 710072China Engineering Research Center of Advanced Manufacturing Technology for Aero Engine Ministry of EducationNorthwestern Polytechnical UniversityXi’an 710072China Shaanxi Key Laboratory of High-Performance Precision Forming Technology and Equipment Northwestern Polytechnical UniversityXi’an 710072China School of Materials Science and Engineering Jiangsu UniversityZhenjiang 212013China State Key Laboratory of Solidification Processing School of Materials Science and EngineeringNorthwestern Polytechnical UniversityXi’an 710072China

Mechanical properties of TC17 titanium alloy undergo a significant reduction after linear friction welding(LFW),of which the strength and ductility are hard to be improved simultaneously by traditional aging heat treatment(AHT),seriously limiting the application of LFW in the manufacturing of TC17 titanium alloy *** this end,the present work proposes to use electric pulse treatment(EPT)to enhance the strength and ductility of TC17 LFW joints simultaneously by improving its *** results show that,in comparison to the uneven distribution ofαphases in the welding zone(WZ),heat-affected zone(HAZ),and base metal(BM)zone after AHT,EPT can selectively homogenize theαphase distribution of WZ and HAZ without impacting the *** selective effect of EPT is reflected as the synergistic influence of the local Joule heating effect and the electron wind effect,which promotes the diffusion ofβphase stabilizing element Mo and leads to a competitive precipitation ofβphase andαphase in theαphase transition temperature *** ratio ofαphase toβphase in the WZ and HAZ finally approaches an equilibrium point which is similar to that of BM,leading to a uniform distribution ofαphase and realizing the synergy of strength-ductility of LFW joint:the maximum strength increase observed is 12.9%,accompanied by a corresponding elongation increase of 122%(by AHT&EPT),and the maximum plasticity improvement is 185%,accompanied by a corresponding strength increase of 4.3%(by EPT for 1 h).This study provides essential insights for improving the strength and ductility of LFW TC17 titanium alloy blisks and enhancing the applications of LFW in aeroengine components.

关键词： Linear friction welding TC17 titanium alloy Electric pulse treatment Phase transformation Local joule heating effect

来源：评论

学校读者我要写书评

暂无评论

Recent Advances on Graphene Quantum Dots for Electrochemical Energy Storage Devices

引用

Energy & Environmental materials 2022年第1期5卷 201-214页

作者： Noura Zahir Pierre Magri Wen Luo Jean Jacques Gaumet Philippe Pierrat CNRS L2CM UMR 7053 Universit e de Lorraine LCP-A2MC EA4632 Institut Jean Barriol Universit e de Lorraine State Key Laboratory of Advanced Technology for Materials Synthesis and Processing Wuhan University of Technologywuhan 430070china

Graphene quantum dots(GQDs)which are nanofragments of graphene with an average size between 2 and 50 nm have attracted much attention due to their outstanding properties such as high conductivity,high surface area,and good solubility in various *** combine the quantum confinement and edges effects and the properties of ***,GQDs offers a broad range of applications in various fields(medicine,energy conversion,and energy storage devices).This review will present the recent research based on the introduction of GQDs in batteries,supercapacitors,and microsupercapacitors as electrodes materials or mixed with an active material as an auxiliary ***,discussed on selected examples,summarize the electrochemical performances and finally,challenges and perspectives are recalled for the subsequent optimization strategy of electrode *** review is expected to appeal a broad interest on functional GQDs materials and promote the further development of high-performance energy storage device.

关键词： energy storage graphene quantum dots lithium ion batteries sodium ion batteries supercapacitor

来源：评论

学校读者我要写书评

暂无评论

Rechargeable metal(Li, Na, Mg, Al)-sulfur batteries: materials and advances

引用

Journal of Energy Chemistry 2021年第10期30卷 104-134,I0004页

作者： Xue Liu Yan Li Xu Xu Liang Zhou Liqiang Mai State Key Laboratory of Advanced Technology for Materials Synthesis and Processing International School of Materials Science and EngineeringWuhan University of TechnologyWuhan 430070HubeiChina Foshan Xianhu Laboratory of the Advanced Energy Science and Technology Guangdong Laboratory Xianhu Hydrogen ValleyFoshan 528200GuangdongChina

Energy and environmental issues are becoming more and more severe and renewable energy storage technologies are vital to solve the *** metal(Li,Na,Mg,Al)-sulfur batteries with low-cost and earth-abundant elemental sulfur as the cathode are attracting more and more interest for electrical energy storage in recent ***-sulfur(Li-S),room-temperature sodium-sulfur(RT Na-S),magnesium-sulfur(Mg-S)and aluminum-sulfur(Al-S)batteries are the most prominent candidates among *** obvious obstacles are hampering the developments of metal-sulfur ***-S and Na-S batteries are encumbered mainly by anode dendrite issues,polysulfides shuttle and low conductivity of ***-S and Al-S batteries are short of suitable *** this review,relationships between various employed nanostructured materials and electrochemical performances of metal-sulfur batteries have been ***,the selections of suitable electrolytes,anode protection,separator modifications and prototype innovations are all crucial to the developments of metal-sulfur batteries and are discussed at the same ***,we give a review on the advances of Li-S,RT Na-S,Mg-S and Al-S batteries from the point of view of materials,and then focus on perspectives of their future developments.

关键词： Lithium sulfur batteries Sodium sulfur batteries Magnesium sulfur batteries Aluminum sulfur batteries Energy materials

来源：评论

学校读者我要写书评

暂无评论

Formation mechanism of partial stacking faults by incompletemixed-mode phase transformation: A case study of Fe-Ga alloys

引用

Journal of materials Science & technology 2022年第22期117卷 59-64页

作者： Tianzi Yang Tianyu Ma Feng Liu Xiaobing Ren Frontier Institute of Science and Technology State Key Laboratory for Mechanical Behavior of Materialsand MOE Key Laboratory for Nonequilibrium Synthesis and Modulation of Condensed MatterXi’an Jiaotong UniversityXi’an 710049China State Key Laboratory of Solidification Processing and Analytical and Testing Center Northwestern Polytechnical UniversityXi’an 710072China Center for Functional Materials National Institute for Materials ScienceTsukuba 305-0047IbarakiJapan

Partial stacking faults(PSFs) formed by incomplete mixed-mode phase transformation have been found to exhibit unfixed slip distance of closely-packed planes unlike those of the deformation-induced stacking faults(SFs) with fixed distance. Though engineering PSFs can yield appealing properties, such as the enhanced damping capacity, understanding of the interaction between lattice distortion and atomic diffusion and their influences on forming PSFs is still far from being clear. Herein we performed a case study on aged Fe-Ga alloy that undergoes a mixed-mode phase transformation from body-centered cubic(BCC)to ordered face-centered cubic(FCC). The TEM investigations showed that the faulted {111}-FCC distance of the PSFs is shorter than a/6<112> of the typical {111}-<112> SFs in deformed FCC materials and the PSFs have disordered Fe and Ga arrangements. Further studies revealed that such PSFs will not be completely dissociated at FCC twin boundaries(TBs) even after long term isothermal aging. Consequently,the formation of PSFs can be ascribed to the transformation-dependent atomic ordering and lattice shear strain of the parent BCC lattice, where the diffusion-controlled glides of the PSFs-associated dislocations will accelerate atomic diffusions due to the dislocation-pipe effect along <112>-FCC direction, but may hinder the atomic diffusions across the {111}-FCC TBs due to the retarding effect. This study may add important insight into the defects process during mixed-mode phase transformation and broaden the knowledge of the interaction between concurrently-happened lattice distortion and atomic diffusion.

关键词： Stacking faults Mixed-mode phase transformation Diffusion Lattice distortion Fe-Ga alloy

来源：评论

学校读者我要写书评

暂无评论

High Conduction Band Inorganic Layers for Distinct Enhancement of Electrical Energy Storage in Polymer Nanocomposites

引用

Nano-Micro Letters 2022年第9期14卷 221-236页

作者： Yingke Zhu Zhonghui Shen Yong Li Bin Chai Jie Chen Pingkai Jiang Xingyi Huang Shanghai Key Laboratory of Electrical Insulation and Thermal Ageing State Key Laboratory of Metal Matrix CompositesDepartment of Polymer Science and EngineeringShanghai Jiao Tong UniversityShanghai 200240People’s Republic of China State Key Laboratory of Advanced Technology for Materials Synthesis and Processing Center of Smart Materials and DevicesWuhan University of TechnologyWuhan 430070People’s Republic of China Institute of Applied and Physical Chemistry and Center for Environmental Research and Sustainable Technology University of Bremen28359 BremenGermany

Dielectric polymer nanocomposites are considered as one of the most promising candidates for high-power-density electrical energy storage *** nanofillers with high insulation property are frequently introduced into fluoropolymer to improve its breakdown strength and energy storage ***,inorganic nanofillers are thought to introducing traps into polymer matrix to suppress leakage ***,how these nanofillers effect the leakage current is still ***,high dopant(>5 vol%)is prerequisite for distinctly improved energy storage performance,which severely deteriorates the processing and mechanical property of polymer nanocomposites,hence brings high technical complication and ***,boron nitride nanosheet(BNNS)layers are utilized for substantially improving the electrical energy storage capability of polyvinylidene fluoride(PVDF)*** reveal that the high conduction band minimum of BNNS produces energy barrier at the interface of adjacent layers,preventing the electron in PVDF from passing through inorganic layers,leading to suppressed leakage current and superior breakdown *** by improved Young’s modulus(from 1.2 GPa of PVDF to 1.6 GPa of nanocomposite),significantly boosted discharged energy density(14.3 J cm^(-3)) and charge-discharge efficiency(75%)are realized in multilayered nanocomposites,which are 340 and 300% of PVDF(4.2 J cm^(-3),25%).More importantly,thus remarkably boosted energy storage performance is accomplished by marginal *** work offers a new paradigm for developing dielectric nanocomposites with advanced energy storage performance.

关键词： Boron nitride nanosheet Conduction band Efficiency Energy density Barrier

来源：评论

学校读者我要写书评

暂无评论

建议与咨询留下您的常用邮箱和电话号码，以便我们向您反馈解决方案和替代方法

时间限定

文献类型

馆藏选择

核心期刊

语言

文献类型

帮助

文字说明：

检索规则说明：

检索范例：

分类表

所选分类

限定检索结果

文献类型

馆藏范围

日期分布

学科分类号

主题

机构

作者

语言

请选择保存的检索档案：

请选择收藏分类：

通借通还

建议与咨询 留下您的常用邮箱和电话号码，以便我们向您反馈解决方案和替代方法

时间限定

文献类型

馆藏选择

核心期刊

语言

文献类型

帮助

文字说明：

检索规则说明：

检索范例：

分类表

所选分类

限定检索结果

文献类型

馆藏范围

日期分布

学科分类号

主题

机构

作者

语言

请选择保存的检索档案： 新增检索档案 确定 取消

请选择收藏分类： 新增自定义分类 确定 取消

通借通还

建议与咨询留下您的常用邮箱和电话号码，以便我们向您反馈解决方案和替代方法

请选择保存的检索档案：

请选择收藏分类：