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Correction: Large-scale and fast synthesis of nano-hydroxyapatite powder by a microwave-hydrothermal method

RSC advances 2019年第26期9卷 15140页

作者： Zhengwei Cai Xinyu Wang Zongrui Zhang Yingchao Han Jing Luo Mingzheng Huang BoWen Zhang Yuanjing Hou State Key Laboratory of Advanced Technology for Materials Synthesis and Processing Wuhan University of Technology Wuhan 430070 China wangxinyu@*** +86-27-87880734 +86-27-87651853. Biomedical Materials and Engineering Research Center of Hubei Province Wuhan 430070 China. College of Biochemical Engineering Anhui Polytechnic University Wuhu 241000 China.

[This corrects the article DOI: 10.1039/C9RA00091G.].

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Regulative Electronic states around Ruthenium/Ruthenium Disulphide Heterointerfaces for Efficient Water Splitting in Acidic Media

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Angewandte Chemie 2021年第22期133卷

作者： Jiawei Zhu Dr. Yao Guo Fang Liu Hanwen Xu Lei Gong Wenjie Shi Ding Chen Pengyan Wang Yue Yang Chengtian Zhang Prof. Jinsong Wu Dr. Jiahuan Luo Prof. Shichun Mu State Key Laboratory of Advanced Technology for Materials Synthesis and Processing Wuhan University of Technology Wuhan 430070 P. R. China Foshan Xianhu Laboratory of the Advanced Energy Science and Technology Guangdong Laboratory Xianhu Hydrogen Valley Foshan 528200 P. R. China Department of Chemical and Environmental Engineering Anyang Institute of Technology Anyang 455000 P. R. China NRC (Nanostructure Research Centre) Wuhan University of Technology Wuhan 430070 P. R. China

Theoretical calculations unveil the charge redistribution over abundant interfaces and the enhanced electronic states of Ru/RuS 2 heterostructure. The resulting surface electron-deficient Ru sites display optimized adsorption behavior toward diverse reaction intermediates, thereby reducing the thermodynamic energy barriers. Experimentally, for the first time the laminar Ru/RuS 2 heterostructure is rationally engineered by virtue of the synchronous reduction and sulfurization under eutectic salt system. Impressively, it exhibits extremely high catalytic activity for both OER (201 mV @ 10 mA cm −2 ) and HER (45 mV @ 10 mA cm −2 ) in acidic media due to favorable kinetics and excellent specific activity, consequently leading to a terrific performance in acidic overall water splitting devices (1.501 V @ 10 mA cm −2 ). The in-depth insight into the internal activity origin of interfacial effect could offer precise guidance for the rational establishment of hybrid interfaces.

关键词： acidic water electrolysis bifunctional electrocatalyst DFT calculation heterostructure Ru-based nanomaterial

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Tungsten Phosphide on Nitrogen and Phosphorus-Doped Carbon as a Functional Membrane Coating Enabling Robust Lithium-Sulfur Batteries

SSRN

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SSRN 2024年

作者： Li, Canhuang Yu, Jing Zhang, Chaoqi Wang, Jian Yang, Dawei Xiao, Ke Li, Hao Huang, Chen Cheng, Yapeng Ren, Yuchuan Qi, Xuede Yang, Tianxiang Li, Junshan Wang, Jiaao Henkelman, Graeme Arbiol, Jordi Nan, Junmin Cabot, Andreu Catalonia Institute for Energy Research-IREC Sant Adrià de Besòs Barcelona08930 Spain Department of Chemistry Universitat de Barcelona Barcelona08028 Spain College of Materials Science and Engineering Fuzhou University No.2 Xueyuan Road Minhou County Fujian Province Fuzhou City350108 China Department of Electronic and Biomedical Engineering Universitat de Barcelona Barcelona08028 Spain UlmD89081 Germany Henan Province Key Laboratory of Photovoltaic Materials School of Future Technology Henan University Kaifeng475004 China State Key Laboratory of Advanced Technology for Materials Synthesis and Processing Wuhan University of Technology China Chongqing University of Technology China CSIC and BIST Campus UAB Bellaterra Barcelona Catalonia08193 Spain School of Environmental Engineering and Chemistry Luoyang Institute of Science and Technology Henan Luoyang471023 China Institute for Advanced Study Chengdu University Chengdu610106 China Department of Chemistry The Oden Institute for Computational Engineering and Sciences The University of Texas at Austin AustinTX78712-0165 United States School of Chemistry South China Normal University Guangzhou510006 China ICREA Pg. Lluis Companys Barcelona Catalonia08010 Spain

Lithium-sulfur batteries (LSBs) hold great potential as future energy storage technology, but their widespread application is hampered by the slow polysulfide conversion kinetics and the sulfur loss during cycling. In this study, we detail a one-step approach to growing tungsten phosphide (WP) nanoparticles on the surface of nitrogen and phosphorus co-doped carbon nanosheets (WP@NPC). We further demonstrate that this material provides outstanding performance as a multifunctional separator in LSBs, enabling higher sulfur utilization and exceptional rate performance. These excellent properties are associated with the abundance of lithium polysulfide (LiPS) adsorption and catalytic conversion sites and rapid ion transport capabilities. Experimental data and density functional theory calculations demonstrate tungsten to have a sulfophilic character while nitrogen and phosphorus provide lithiophilic sites that prevent the loss of LiPSs. Furthermore, WP regulates the LiPS catalytic conversion, accelerating the Li-S redox kinetics. As a result, LSBs containing a polypropylene separator coated with a WP@NPC layer show capacities close to 1500 mAh g-1 at 0.1C and coulombic efficiencies above 99.5% at 3C. Batteries with high sulfur loading, 4.9 mg cm−2, are further produced to validate their superior cycling stability. This work demonstrates the use of multifunctional separators as an effective strategy to promote LSB performance. © 2024, The Authors. All rights reserved.

关键词： Polysulfides

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Hierarchical Structuring: Phases Hybriding and Hierarchical Structuring of Mesoporous TiO2Nanowire Bundles for High-Rate and High-Capacity Lithium Batteries (Adv. Sci. 7/2015)

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advanced Science 2015年第7期2卷 n/a-n/a页

作者： Jun Jin Shao-Zhuan Huang Jing Liu Yu Li Li-Hua Chen Yong Yu Hong-En Wang Clare P. Grey Bao-Lian Su Laboratory of Living Materials at the State Key Laboratory of Advanced Technology for Materials Synthesis and Processing Wuhan University of Technology 122 Luoshi Road 430070 Wuhan Hubei China Department of Chemistry University of Cambridge Lensfeild Road Cambridge CB2 1EW UK Laboratory of Inorganic Materials Chemistry (CMI) University of Namur 61 rue de Bruxelles B-5000 Namur Belgium

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Self-repairing high entropy oxides

arXiv

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arXiv 2021年

作者： Liu, Zongwen Huang, Pengru Sun, Lixian Liu, Yanping Qu, Jiangtao Cairney, Julie Zheng, Zhong Wang, Zhiming M. Khan, Naveed A. Lai, Zhiping Fu, Li Teng, Bing Zhou, Cuifeng Zhao, Hong Xu, Fen Xiong, Pan Zhu, Junwu Yuan, Peng Tsoutas, Kosta Akhavan, Behnam Bilek, Marcela M. Ringer, Simon P. Novoselov, Kostya S. School of Chemical and Biomolecular Engineering The University of Sydney NSW2006 Australia The University of Sydney Nano Institute The University of Sydney NSW2006 Australia Department of Materials Science and Engineering National University of Singapore 117575 Singapore Guangxi Key Laboratory of Information Materials Guangxi Collaborative Innovation Center of Structure and Property for New Energy and Materials School of Material Science & Engineering Guilin University of Electronic Technology Guilin541004 China School of Physics and Electronics Hunan Key Laboratory for Super-Microstructure and Ultrafast Process Central South University Hunan410083 China School of Aerospace Mechanical and Mechatronic Engineering The University of Sydney SydneyNSW2006 Australia The Australian Centre for Microscopy and Microanalysis The University of Sydney NSW2006 Australia Institute of Fundamental and Frontier Sciences University of Electronic Science and Technology of China Chengdu610054 China Advanced Membranes and Porous Materials Center Division of Physical Science and Engineering King Abdullah University of Science and Technology Thuwal23955 Saudi Arabia State Key Laboratory of Solidification Processing Northwestern Polytechnical University Xi'an710072 China College of Physics Qingdao University Qingdao266071 China Key Laboratory for Soft Chemistry and Functional Materials Ministry Education Nanjing University of Science and Technology Nanjing210094 China CAS Key Laboratory of Mineralogy and Metallogeny Guangdong Provincial Key laboratory of Mineral Physics and Materials Guangzhou Institute of Geochemistry Chinese Academy of Sciences Guangzhou510640 China School of Physics The University of Sydney NSW2006 Australia School of Biomedical Engineering The University of Sydney NSW2006 Australia

All biological organisms, from plants to living creatures, can heal minor wounds and damage. The realization of a similar self-healing capacity in inorganic materials has been a design target for many decades. This would represent a breakthrough in materials engineering, enabling many novel technological applications, since such materials would be able to resist damage caused by electromagnetic irradiation and/or mechanical impact. Here we demonstrate that a high-entropy oxide is intrinsically capable of undergoing an autonomous self-repairing process. Transmission electron microscopy revealed that the spinel structure of (AlCoCrCu0.5FeNi)3O4 can regrow and repair itself at the atomic level when damaged. Density functional theory calculations reveal that the extra enthalpy stored in the high entropy material during fabrication can be released to effectively heal macroscopic defects by regrowing into a partially ordered state. This extraordinary self-repairing phenomenon makes this new material highly desirable as a coating, enabling structures used in harsh environments to better withstand damage, such as cosmic irradiation in space, nuclear irradiation in nuclear power facilities, or tribological damage. Most importantly, our results set the general design principles for the synthesis of self-repairing materials. Copyright © 2021, The Authors. All rights reserved.

关键词： Entropy

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One-pot synthesis of hierarchical CdS/MoS 2 /rGO with enhanced (photo)electrocatalytic activities

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Chemical Physics Letters 2020年 759卷

作者： Xiu Cheng Yi Lu Yi-Xuan Liu Ge Tian Xiao-Yu Yang State Key Laboratory of Advanced Technology for Materials Synthesis and Processing & School of Materials Science and Engineering Wuhan University of Technology 122 Luoshi Road Wuhan 430070 China School of Chemical Engineering and Technology Sun Yat-sen University Zhuhai 519000 China Qingdao National Laboratory for Marine Science and Technology Qingdao 266237 China School of Engineering and Applied Sciences Harvard University Cambridge 02138 MA United States

A facile one-pot hydrothermal synthesis of 3D windmill-like CdS/MoS 2 /rGO has been reported. The MoS 2 /rGO framework prevents the aggregation of CdS and leads to a two-pathway for electron transfer, thus enhancing the electron density and more active site on the rGO surface. Compared with pure CdS, the hierarchical CdS/MoS 2 /rGO catalyst displays superior photocatalytic H 2 production activity and electrocatalytic H 2 evolution overpotential, which is 3.5 times in photoactivity and 146.7 mV decrease of overpotential. A new hierarchical structure and its characteristics and mechanism are proposed at the atomic-/nanoscale.

关键词： CdS MoS 2 /rGO framework Windmill-like Photocatalysis Electrocatalysis

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The issues on the commercialization of perovskite solar cells

材料展望（英文）

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材料展望（英文） 2024年第2期3卷 118-152页

作者： Lixiu Zhang Yousheng Wang Xiangchuan Meng Jia Zhang Pengfei Wu Min Wang Fengren Cao Chunhao Chen Zhaokui Wang Fu Yang Xiaodong Li Yu Zou Xi Jin Yan Jiang Hengyue Li Yucheng Liu Tongle Bu Buyi Yan Yaowen Li Junfeng Fang Lixin Xiao Junliang Yang Fuzhi Huang Shengzhong Liu Jizhong Yao Liangsheng Liao Liang Li Fei Zhang Yiqiang Zhan Yiwang Chen Yaohua Mai Liming Ding Center for Excellence in Nanoscience(CAS) Key Laboratory of Nanosystem and Hierarchical Fabrication(CAS)National Center for Nanoscience and TechnologyBeijing 100190People's Republic of China Institute of New Energy Technology College of Information Science and TechnologyJinan UniversityGuangzhou 510632People's Republic of China Institute of Polymers and Energy Chemistry(IPEC) Nanchang UniversityNanchang 330031People's Republic of China Institute of optoelectronics Fudan UniversityShanghai 200433People's Republic of China School of Chemical Engineering and Technology Tianjin UniversityTianjin 300072People's Republic of China School of Physical Science and Technology Soochow UniversitySuzhou 215006People's Republic of China Institute of Functional Nano & Soft Materials(FUNSOM) Soochow UniversitySuzhou 215123People's Republic of China College of Chemistry Chemical Engineering and Materials ScienceSoochow UniversitySuzhou 215123People's Republic of China School of Physics and Electronic Science East China Normal UniversityShanghai 200241People's Republic of China State Key Laboratory for Artificial Microstructure and Mesoscopic Physics Department of PhysicsPeking UniversityBeijing 100871People's Republic of China College of Biophotonics South China Normal UniversityGuangzhou 510631People's Republic of China School of Materials Science and Engineering Beijing Institute of TechnologyBeijing 100081People's Republic of China School of Physics and Electronics Central South UniversityChangsha 410083People's Republic of China School of Materials Science and Engineering Shaanxi Normal UniversityXi'an 710119People's Republic of China State Key Laboratory of Advanced Technology for Materials Synthesis and Processing Wuhan University of TechnologyWuhan 430070People's Republic of China Microquanta semiconductor Hangzhou 311121People's Republic of China School of Information Science and Technology Fudan UniversityShanghai 200433People's Republic of China

Perovskite solar cells have aroused a worldwide research upsurge in recent years due to their soaring photovoltaic performance,ease of solution processing,and low *** power conversion efficiency record is constantly being broken and has recently reached 26.1％in the lab,which is comparable to the established photovoltaic technologies such as crystalline silicon,copper indium gallium selenide and cadmium telluride(CdTe)solar ***,perovskite solar cells are standing at the entrance of industrialization,where huge opportunities and risks ***,towards commercialization,challenges of up-scaling,stability and lead toxicity still remain,the proper handling of which could potentially lead to the widespread adoption of perovskite solar cells as a low-cost and efficient source of renewable *** review gives a holistic analysis of the path towards commercialization for perovskite solar cells.A comprehensive overview of the current state-of-the-art level for perovskite solar cells and modules will be introduced first,with respect to the module efficiency,stability and current status of *** will then discuss the challenges that get in the way of commercialization and the corresponding strategies to address them,involving the upscaling,the stability and the lead toxicity *** into the future direction of commercialization of perovskite photovoltaics was also provided,including the flexible perovskite cells and modules and perovskite indoor ***,the future perspectives towards commercialization are put forward.

关键词： commercializations perovskite solar cells state-of-the-art level challenges and perspectives indoor photovoltaics

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Front Cover: Highly Dispersed Pt Nanoparticles Embedded in N-Doped Porous Carbon for Efficient Hydrogen Evolution (Chem. Asian J. 14/2021)

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Chemistry – An Asian Journal 2021年第14期16卷

作者： Yuan Dong Dr. Jie Ying Yu-Xuan Xiao Jiang-Bo Chen Prof. Xiao-Yu Yang State Key Laboratory of Advanced Technology for Materials Synthesis and Processing Wuhan University of Technology 122 Luoshi Road Wuhan 430070 P. R. China School of Chemical Engineering and Technology Sun Yat-sen University Zhuhai 519082 P. R. China School of Engineering and Applied Sciences Harvard University Cambridge Massachusetts 02138 USA

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Author Correction: Chemical fixation of carbon dioxide catalyzed via cobalt (III) ONO pincer ligated complexes

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Communications Chemistry 2019年第1期2卷 1页

作者： Habib Ullah Bibimaryam Mousavi Hussein A. Younus Zafar A. K. Khattak Somboon Chaemchuen Suleman Suleman Francis Verpoort State Key Laboratory of Advanced Technology for Materials Synthesis and Processing Wuhan University of Technology Wuhan China Chemistry Department Faculty of Science Fayoum University Fayoum Egypt National Research Tomsk Polytechnic University Tomsk Russian Federation Ghent University Global Campus Songdo Incheon South Korea College of Arts and Sciences Khalifa University of Science and Technology Abu Dhabi UAE

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Verifying the Charge-Transfer Mechanism in S-Scheme Heterojunctions Using Femtosecond Transient Absorption Spectroscopy

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Angewandte Chemie 2022年第8期135卷

作者： Chang Cheng Dr. Jianjun Zhang Dr. Bicheng Zhu Prof. Guijie Liang Prof. Liuyang Zhang Prof. Jiaguo Yu State Key Laboratory of Advanced Technology for Materials Synthesis and Processing Wuhan University of Technology 430070 Wuhan P. R. China Laboratory of Solar Fuel Faculty of Materials Science and Chemistry China University of Geosciences 68 Jincheng Street 430078 Wuhan P. R. China Hubei Key Laboratory of Low Dimensional Arts and Science Hubei University of Arts and Science 441053 Xiangyang P. R. China

The S-scheme heterojunction is flourishing in photocatalysis because it concurrently realizes separated charge carriers and sufficient redox ability. Steady-state charge transfer has been confirmed by other methods. However, an essential part, the transfer dynamics in S-scheme heterojunctions, is still missing. To compensate, a series of cadmium sulfide/pyrene- alt -difluorinated benzothiadiazole heterojunctions were constructed and the photophysical processes were investigated with femtosecond transient absorption spectroscopy. Encouragingly, an interfacial charge-transfer signal was detected in the spectra of the heterojunction, which provides solid evidence for S-scheme charge transfer to complement the results from well-established methods. Furthermore, the lifetime for interfacial charge transfer was calculated to be ca. 78.6 ps. Moreover, the S-scheme heterojunction photocatalysts exhibit higher photocatalytic conversion of 1,2-diols and H 2 production rates than bare cadmium sulfide.

关键词： 1,2-Diols Oxidation Hydrogen Production Photocatalysis S-Scheme Transient Absorption

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