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Compatible matching and synergy operation optimization of hydrogen-electric hybrid energy storage system in DC microgrid

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Energy Conversion and Management: X 2025年 26卷

作者： Du, Banghua Peng, Yanyu Li, Yang Xie, Changjun Zhu, Shihao Zhu, Wenchao Yang, Yang You, Li Zhang, Leiqi Zhao, Bo Hubei Key Laboratory of Advanced Technology for Automotive Components Wuhan University of Technology Wuhan430070 China School of Automation Wuhan University of Technology Wuhan430070 China Department of Electrical Engineering Chalmers University of Technology Gothenburg41258 Sweden State Key Laboratory of Advanced Technology for Materials Synthesis and Processing Wuhan430070 China State Grid Hubei Electric Power Research Institute Wuhan430077 China State Grid Zhejiang Electric Power Research Institute Hangzhou310014 China

Hydrogen energy storage (HES) systems could balanced source-load mismatches in DC microgrids. By combining HES with electrical energy storage (EES), the start-up delay and rapid degradation of HES under fluctuating inputs can be mitigated, enhancing system adaptability. However, without proper power allocation and operational optimization, system efficiency and the lifespan of HES and EES decrease. Accordingly, this paper proposes a compatible matching and synergy operation optimization for hydrogen-electric hybrid energy storage systems (H-E HESS). Firstly, Complete Ensemble Empirical Mode Decomposition with Adaptive Noise (CEEMDAN) is developed to decompose power fluctuation signals into frequency components, and the Hilbert transform calculates the energy value to determine high- and low-frequency dividing points. Next, a system power allocation strategy is formulated through the fast response of the EES to compensate for the delay in the start-up of the HES. A multi-objective optimization model is then developed to balance efficiency and lifespan, which is solved by the NSGA-III algorithm. Finally, case studies show that the proposed strategy improves efficiency by 17.95 % and 8.34 %, reduces degradation rates by 1 % and 0.71 %, and shortens system response time in 1 s, compared to Schemes I and II. The strategy's effectiveness is also validated through an experimental platform in a hydrogen-electric coupled DC microgrid demonstration project. © 2025 The Author(s)

关键词： Hydrogen storage

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Sym- and Asym-Expanded Heterohelicene Isomers Featuring Extended Multi-Resonance Skeleton for Narrowband Deep-Blue Fluorescence

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Angewandte Chemie - International Edition 2025年第13期64卷

作者： Zeng, Xuan Luo, Xiaofeng Meng, Guoyun Wang, Xuewen Zhang, Dongdong Duan, Lian School of Chemistry Chemical Engineering and Life Science State Key Laboratory of Advanced Technology for Materials Synthesis and Processing Wuhan University of Technology Wuhan430070 China Key Lab of Organic Optoelectronics and Molecular Engineering of Ministry of Education Department of Chemistry Tsinghua University Beijing100084 China Foshan Xianhu Laboratory of the Advanced Energy Science and Technology Guangdong Laboratory Xianhu hydrogen Valley Foshan528200 China Center for Flexible Electronics Technology Tsinghua University Beijing100084 China

Expanded heterohelicenes composed of alternating linearly and angularly fused multi-resonance (MR) skeletons have gained wide interest owing to their promising narrowband emissions. Herein, a pair of sym- and asym-expanded heterohelicene isomers was obtained by merging boron/oxygen (B/O)-embedded MR triangulene and indolo[3,2,1-jk]carbazole units via one-pot synthesis. Owing to their fully resonating extended helical skeleton, the target heterohelicenes exhibit a significantly narrowed spectra bandwidth while emission red-shifting, thus affording deep-blue narrowband emission with a peak at approximately 460 nm, full-width-at-half-maximum (FWHM) of only 18 nm, and near-unity photoluminescence quantum yields. In comparison to the symmetrical structure, the asym-expanded heterohelicene displays suppressed aggregation within doped films, thereby showing superior narrowband electroluminescence in devices with CIE coordinates of (0.12, 0.18) and a high external quantum efficiency of up to 25 %, which retains 18.1 % even at a high luminance of 10,000 cd m−1. Overall, this work provides a novel paradigm for the development of narrowband expanded heterohelicenes. © 2025 Wiley-VCH GmbH.

关键词： Electroluminescence

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Boosting oxygen evolution of LiCoO2 electrocatalysts via lithium defect

Materials Today Catalysis

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materials Today Catalysis 2025年 8卷

作者： Li, Huamei Li, Mengyuan Liao, Lingling Yang, Han Xiang, Kun Luo, Guoqiang Xie, Mingjiang School of Chemistry and Environmental Engineering Engineering Research Center of Phosphorus Resources Development and Utilization of Ministry of Education Wuhan Institute of Technology Wuhan430205 China State Key Laboratory of Advanced Technology for Materials Synthesis and Processing Wuhan University of Technology Wuhan430070 China Hubei Key Lab for Processing and Application of Catalytic Materials College of Chemical Engineering Huanggang Normal University Huanggang438000 China

The challenge of the complex oxygen evolution reaction (OER) currently impedes the efficient production of hydrogen via electrolytic water splitting. To address this issue, the development and improvement of effective electrocatalysts are required. LiCoO2, a key material in lithium-ion batteries, has shown promising potential as an electrocatalyst for electrochemical energy conversion. However, OER catalysts derived from LiCoO2 have faced obstacles such as high overpotential and a complicated preparation process. In this study, the preparation method is adjusted to optimize the synthesis of Li1-xCoO2 with a defective structure, resulting in an impressive overpotential of only 290 mV at a current density of 100 mA cm−2 and a remarkable Tafel slope of 15.2 mV dec−1. The exceptional catalytic activity of Li1-xCoO2 can be attributed to the absence of Li, which triggers oxidative alterations in the electronic structure of Co. Density functional theory (DFT) calculations reveal that Li defects can influence the d-band center of active Co sites, enhancing the adsorption capabilities of Co sites towards *OOH intermediates and increasing the conductivity of the electrocatalyst during the OER process. These alterations improve the velocity of the crucial step in the reaction, ultimately boosting the catalyst's overall performance and efficiency. © 2024 The Authors

关键词： Lithium-ion batteries

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A numerical method for predicting bursting strength of composite rocket motor case considering filament winding process-induced stress

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Chinese Journal of Aeronautics 2025年第02期 509-522页

作者： Jiqiu LIANG Fei ZHAO Dan WU Anxin DING Hubei Key Laboratory of Advanced Aerospace Propulsion Technology System Design Institute of Hubei Aerospace Technology Academy School of Materials Science and Engineering Wuhan University of Technology State Key Laboratory of Advanced Technology for Materials Synthesis and Processing Wuhan University of Technology

A numerical method to predict the bursting strength of filament wound composite rocket motor case is proposed here. This method can evaluate the longitudinal stress evolution of each composite layer as impregnated filaments with fiber tension are wound layer by layer, and consider the effects of accumulated stress and deformation during filament winding on the bursting strength of composite case. Taking ?520 mm composite cases as a case study, the filament-winding-processinduced stress and deformation as well as progressive damage behavior are numerically predicted,followed by a comparison with experimental results. The numerical results show that the predicted bursting pressures for composite cases manufactured on the mandrels with and without a flexible component are 14.20 MPa and 21.40 MPa, respectively. These values exhibit slight deviation from the measured pressures of 13.50 MPa and 21.57 MPa. Moreover, the predicted damage locations,situated respectively in the dome and cylinder, agree well with the experimental observation. These observations indicate that use of flexible component reduces the load-bearing capacity of the ***, it validates the reliability and accuracy of the proposed numerical method in predicting the bursting strength of composite cases.

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Ionic liquid-grafted MXene composite polymer electrolytes for high-performance solid-state batteries

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Chemical Engineering Journal 2025年 514卷

作者： Qian, Zhi Qiu, Zhao-Dong Wang, Rui-Qing Wei, Mei-Tong Fei, An-Min Hu, Zhi-Yi Mohamed, Hemdan S.H. Chen, Li-Hua Li, Yu Su, Bao-Lian State Key Laboratory of Advanced Technology for Materials Synthesis and Processing Wuhan University of Technology Wuhan430070 China Wuhan University of Technology Wuhan430070 China Physics Department Faculty of Science Fayoum University El Gomhoria Street Fayoum63514 Egypt University of Namur NamurB-5000 Belgium

All-solid-state batteries (ASSBs) have obtained much attention due to the high energy density and security. At present, PEO-based solid-state batteries are considered to be one of the most promising candidates for high-performance ASSBs due to the excellent processability and good interfacial stability. However, low ionic conductivity and Li+ transference number seriously hinder their progress in practical applications. Here, a novel filler is developed by embedding ionic liquid (IL) grafted onto the surface of MXene to improve the electrochemical performance of PEO-based solid composite polymer electrolyte (MXene-IL-SPE) for ASSBs. The 2D MXene can significantly reduce the crystallinity of PEO, and the presence of IL not only enhances the dispersion of MXene in the polymer matrix, but also promotes the dissociation of lithium salts and anchors anions. As a result, the MXene-IL-SPE possesses high ionic conductivity (7.19 × 10−4 S cm−1) and Li+ transference number (0.51), together with wide electrochemical window (5.2 V) at 60 °C. The assembled LiFePO4|MXene-IL-SPE|Li full cell exhibits remarkable rate capability and exceptional capacity of 154.8 mAh g−1 over 120 cycles with an impressive 95.3 % capacity retention at 0.5 C. This design opens up a new way to prepare high performance CPEs for ASSBs. © 2025 Elsevier B.V.

关键词： Solid-state Batteries

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Lattice Boltzmann simulation of droplet dynamics in proton exchange membrane fuel cell channel with mechanical vibration

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Chemical Engineering Research and Design 2025年 218卷 302-311页

作者： Zhou, Zijian Zhai, Shuai Liu, Xunchen Fang, Yuan Chen, Mingzhang Zhang, Ju Guan, Shanyue Hubei Longzhong Laboratory Wuhan University of Technology Hubei Xiangyang441000 China School of Automotive Engineering Wuhan University of Technology Wuhan430070 China State Key Laboratory of Advanced Technology for Materials Synthesis and Processing Wuhan430070 China Key Laboratory of Catalysis and Energy Materials Chemistry of Ministry of Education College of Chemistry and Materials Science South-central University for Nationalities Wuhan430074 China School of Vehicle Engineering Hubei University of Automotive Technology Shiyan442002 China

Handling water is a critical challenge for proton exchange membrane (PEM) fuel cells, significantly impacting their lifespan and reliability. While most PEM cells operate in vibrational environments, no studies have examined how mechanical vibrations affect water handling. This research investigates water droplet behavior in a vibrating airflow channel and proposes a new design featuring a hydrophilic band to enhance water management. key findings include: (1) an optimal hydrophilic band width of 0.6 that facilitates droplet movement;(2) a decrease in droplet velocity from 0.107 to 0.024 m s−1 as amplitude increases from 5 mm to 20 mm;and (3) an increase in velocity from 0.0669 to 0.15 m s−1 with higher frequency, highlighting the significant effects of vibration on droplet dynamics and overall water management in PEM fuel cells. © 2025 Institution of Chemical Engineers

关键词： Machine vibrations

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Correction to: Durable Fe3O4/PPy Particle Flow Spun Textile for Electromagnetic Interference Shielding and Joule Heating (advanced Fiber materials, (2025), 7, 2, (513-527), 10.1007/s42765-024-00498-2)

引用

advanced Fiber materials 2025年 1-1页

作者： Liu, Jiaxin Qi, Shuo Wang, Hongshan Fu, Chiyu Xu, Weilin Su, Bin Tang, Wenyang Xia, Zhigang State Key Laboratory of New Textile Materials and Advanced Processing Technologies School of Textile Science and Engineering Industry Research and Development Center of Functional Materials and Textile New Technology Textile Industry Key Laboratory of Yarn and Its Functionalization Wuhan Textile University Hubei Wuhan430200 China State Key Laboratory of Material Processing and Die and Mould Technology School of Materials Science and Engineering Huazhong University of Science and Technology Hubei Wuhan430074 China National Local Joint Engineering Laboratory of Resin-Based Structure and Functional Material Technology Hubei Xiaogan432100 China

In this article the first affiliation details for Jiaxin Liu were incorrectly given as 'state key laboratory of New Textile materials and advanced processing Technologies, School of Textile Science and Engineering, Wuhan Textile University, Wuhan, 430200, Hubei, People’s Republic of China' but should have been 'state key laboratory of New Textile materials and advanced processing Technologies, School of Textile Science and Engineering, Industry Research and Development Center of Functional materials and Textile New technology, Textile Industry key laboratory of Yarn and Its Functionalization, Wuhan Textile University, Wuhan, 430200, Hubei, People’s Republic of China'. The original article has been corrected. © Donghua University, Shanghai, China 2025.

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Industrial applicable, Be-Ni-free Y-doped Zr-based bulk metallic glasses with high glass-forming ability and superior mechanical properties

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Journal of Alloys and Compounds 2025年 1027卷

作者： Fu, X.Q. Li, C.Y. Gao, K. Zhu, X.G. Li, X.S. Pei, C.Q. Zhou, J. Kou, S.Z. Sun, B.A. State Key Laboratory of Advanced Processing and Recycling of Non-ferrous Metals School of Materials Science and Engineering Lanzhou University of Technology Gansu Lanzhou730050 China Songshan Lake Materials Laboratory Guangdong Dongguan523808 China Dongguan Yihao Metal Material Technology Co LTD Guangdong Dongguan523686 China

Zr-based bulk metallic glasses (BMGs) exhibit significant potential for a wide range of applications, owing to their exceptional glass-forming ability (GFA) and mechanical properties. However, while the addition of beryllium (Be) or rare-earth elements can improve the GFA of Zr-based BMGs, it often raises safety concerns or compromises their mechanical performance, limiting their industrial applicability. Therefore, the development of Be-Ni-free Zr-based BMGs with both superior GFA and mechanical properties remains a considerable challenge. In this study, we successfully prepared an industrially applicable Be-Ni-free (Zr61Ti2Cu25Al12)100-xYx BMG via Y-doping, demonstrating high GFA and excellent mechanical properties. We found that trace Y-doping significantly enhances both GFA and plasticity, with Y0.1 achieving a critical diameter of 13 mm and Y0.3 exhibiting a remarkable compressive strain of 18.91 %. Additionally, using the (Zr61Ti2Cu25Al12)100-xYx BMGs, we successfully fabricated industrial BMGs plates with thicknesses of 2 mm via high-vacuum, high-pressure die casting (HV-HPDC). The industrial BMGs plates of Y0.3 also exhibited the unexceptionable flexural strength of the 2.46 GPa. This work provides a novel approach for the exploration of BMGs for industrial applications and represents a significant step toward their commercialization and structural use. © 2025 Elsevier B.V.

关键词： Machinability

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Effects of PSMA and experimental conditions on the morphologies of BaCO_3 whiskers

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Rare Metals 2006年第4期25卷 382-388页

作者： CHENG Bei YU Xiaoxiao YU Jiaguo ZHAO Xiujian State Key Laboratory of Advanced Technology for Material Synthesis and Processing Wuhan University of Technology Wuhan 430070 China

BaCO3 whiskers exhibiting different morphologies were fabricated by a simple precipitation reaction of barium ch/oride with sodium carbonate in the absence and presence of poly-（styrene-alt-maleic acid）（PSMA） as a crystal growth modifier at room temperature. The as-prepared products were characterized by scanning electron microscopy （SEM）, transmission electron microscopy （TEM）, and X-ray diffraction （XRD）. The influences of experimental parameters on the size and morphology of BaCO3 whiskers were investigated and discussed. It was found that the as-prepared BaCO3 whiskers are single crystals with diameter ranging from 100 to 300 run, and grow along the crystallographic a-axis or [100] direction. BaCO3 whiskers with different morphologies, such as branching and dendritic structure, can be obtained depending on the experimental conditions. With increasing PSMA concentration, the diameter of BaCO3 whiskers decreases.

关键词： BaCO3 whiskers morphological control poly-(styrene-alt-maleic acid) single crystal

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Local structural origin of relaxor antiferroelectric behavior in NaNbO3-based ceramics

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Chemical Engineering Journal 2025年 514卷

作者： Meng, Xiangyu Yuan, Liran Li, Dongxu Wang, Pengbin Guo, Qinghu Gan, Xiaoyan Yao, Zhonghua Liu, Hanxing Wu, Jinsong Zhang, Shujun Hao, Hua State Key Laboratory of Advanced Technology for Materials Synthesis and Processing Wuhan University of Technology Wuhan430070 China National Energy Key Laboratory for New Hydrogen-Ammonia Energy Technologies Foshan Xianhu Laboratory Foshan528200 China Nanostructure Research Center Wuhan University of Technology Wuhan430070 China Institute for Superconducting and Electronic Materials Faculty of Engineering and Information Sciences University of Wollongong WollongongNSW2500 Australia

Relaxor-antiferroelectrics (relaxor-AFEs), known for their double polarization–electric field (P-E) hysteresis loops and relaxor characteristics, exhibit outstanding energy storage performance compared to other dielectric materials. However, the origins of their antiferroelectric-like behavior and relaxor features remain unclear due to their complex local structure. In this study, we designed relaxor-AFEs with a high degree of relaxor component and stable antiferroelectric behavior. The recoverable energy density (Wrec) of up to 4.6J/cm3 and energy efficiency of ∼ 79 % were achieved in a 0.76NaNbO3-0.16Na0.5Bi0.5TiO3-0.08CaTiO3 ceramic, demonstrating excellent thermal and frequency stability. The multiphase local polarization configuration was confirmed by atomic-resolution annular dark-field scanning transmission electron microscopy (ADF STEM). Additionally, integrated differential phase contrast (iDPC) images revealed an enhanced antiferrodistortion (AFD) induced by incorporating component with low tolerance factor, contributing to stable antiferroelectric behavior. The relationship between chemical heterogeneity, polarization configuration and energy storage performance was systematically established. This work provides insights into the structure origin and underlying mechanisms for relaxor-AFE performance, with potential implications to guide the development of advanced energy-storage dielectric materials. © 2025 Elsevier B.V.

关键词： Antiferroelectric materials

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