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Proton/Mg2+Co-Insertion Chemistry in Aqueous Mg-Ion Batteries: From the Interface to the Inner

Angewandte Chemie 2023年第37期135卷

作者： Meng Huang Xuanpeng Wang Junjun Wang Jiashen Meng Xiong Liu Qiu He Lishan Geng Qinyou An Jinlong Yang Liqiang Mai Guangdong Research Center for Interfacial Engineering of Functional Materials College of Materials Science and Engineering Shenzhen University Shenzhen 518060 China College of Physics and Optoelectronic Engineering Shenzhen University Shenzhen 518060 China Hainan Institute Wuhan University of Technology Sanya 572000 P. R. China Department of Physical Science & Technology School of Science Wuhan University of Technology Hubei Wuhan 430072 P. R. China State Key Laboratory of Advanced Technology for Materials Synthesis and Processing Wuhan University of Technology Wuhan 430070 China School of Materials Science and Engineering Zhengzhou University Zhengzhou 450001 China College of Materials Science and Engineering Sichuan University Chengdu 610065 China Hubei Longzhong Laboratory Wuhan University of Technology (Xiangyang Demonstration Zone) Xiangyang 441000 P. R. China

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Reinforcement of epoxy-based composites by magnetically aligned multi walled carbon nanotube

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IOP Conference Series: materials Science and Engineering 2015年第1期87卷

作者： Xianjuan Xu Song Lin Moyu Li Wusheng Li Xiaolong Jia Qing Cai Xiaoping Yang State Key Laboratory of Organic-Inorganic Composites College of Materials Science and Engineering Beijing University of Chemical Technology Beijing 100029 P. R. China Aerospace Research Institute of Materials and Processing Technology Beijing 100076 China China Petroleum Engineering Co. Ltd. Beijing Company Beijing 100085 China Changzhou Institute of Advanced Materials Beijing University of Chemical Technology Jiangsu 213164 P. R. China

Multi walled carbon nanotubes decorated with ferriferrous oxide nanoparticle (MWCNTs-Fe3O4) complex was used as an effective reinforcement in the polymer composites. The MWCNTs-Fe3O4 with various grafting contents of Fe3O4 nanoparticles were successfully prepared by combining in situ atom transfer radical polymerization (ATRP) and coprecipitation process, which was characterized with Fourier transform infrared spectroscopy (FT-IR) and transmission electron microscope (TEM). The MWCNTs-Fe3O4 complex showed the strong magnetic response behavior, which could be easily aligned in an external magnetic field. The alignment state of MWCNTs-Fe3O4 complex could be modulated by adjusting the intensity of external magnetic field, grafting content of Fe3O4 nanoparticles and viscosity of the solvent. Moreover, with the addition of MWCNTs-Fe3O4, tensile strength and modulus of epoxy composites were enhanced by 12.3 and 10.9%, respectively, which was due to the reinforcing effect of the aligned MWCNTs-Fe3O4 within magnetic field.

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Positron annihilation study of Fe-ion irradiated reactor pressure vessel model alloys

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Journal of Physics: Conference Series 2016年第1期674卷

作者： L Chen Z C Li H Schut N Sekimura State Key Laboratory of New Ceramics and Fine Processing School of Materials Science and Engineering Tsinghua University Beijing 100084 China Department of Nuclear Engineering and Management The University of Tokyo 7-3-1 Hongo Bunkyo-ku Tokyo 113-8656 Japan Key Laboratory of Advanced Materials (MOE) School of Materials Science and Engineering Tsinghua University Beijing 100084 China To whom any correspondence should be addressed. Department of Radiation Science and Technology Delft University of Technology Mekelweg 15 2629 JB Delft the Netherlands

The degradation of reactor pressure vessel steels under irradiation, which results from the hardening and embrittlement caused by a high number density of nanometer scale damage, is of increasingly crucial concern for safe nuclear power plant operation and possible reactor lifetime prolongation. In this paper, the radiation damage in model alloys with increasing chemical complexity (Fe, Fe-Cu, Fe-Cu-Si, Fe-Cu-Ni and Fe-Cu-Ni-Mn) has been studied by Positron Annihilation Doppler Broadening spectroscopy after 1.5 MeV Fe-ion implantation at room temperature or high temperature (290 oC). It is found that the room temperature irradiation generally leads to the formation of vacancy-type defects in the Fe matrix. The high temperature irradiation exhibits an additional annealing effect for the radiation damage. Besides the Cu-rich clusters observed by the positron probe, the results show formation of vacancy-Mn complexes for implantation at low temperatures.

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In Vivo Imaging: Multiplexed NIR‐II Probes for Lymph Node‐Invaded Cancer Detection and Imaging‐Guided Surgery (Adv. Mater. 11/2020)

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advanced materials 2020年第11期32卷

作者： Rui Tian Huilong Ma Shoujun Zhu Joseph Lau Rui Ma Yijing Liu Lisen Lin Swati Chandra Sheng Wang Xingfu Zhu Hongzhang Deng Gang Niu Mingxi Zhang Alexander L. Antaris Kenneth S. Hettie Bai Yang Yongye Liang Xiaoyuan Chen Key Laboratory of Organ Regeneration and Transplantation of the Ministry of Education The First Hospital of Jilin University Changchun 130061 P. R. China Laboratory of Molecular Imaging and Nanomedicine National Institute of Biomedical Imaging and Bioengineering (NIBIB) National Institutes of Health (NIH) Bethesda MD 20892 USA Department of Materials Science and Engineering Shenzhen Key Laboratory of Printed Organic Electronics Southern University of Science and Technology Shenzhen 518055 P. R. China State Key Laboratory of Supramolecular Structure and Materials College of Chemistry Jilin University Changchun 130012 P. R. China State Key Laboratory of Advanced Technology for Materials Synthesis and Processing Wuhan University of Technology Wuhan 430070 P. R. China Intuitive Surgical Kifer Rd Sunnyvale CA 94086 USA Molecular Imaging Program at Stanford (MIPS) Department of Radiology Stanford University School of Medicine Stanford CA 94305 USA

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Catalysis: Enhanced Catalytic Efficiency of Pt Nanoparticles Supported on 3D Ordered Macro-/Mesoporous Ce0.6Zr0.3Y0.1O2for Methane Combustion (Small 20/2015)

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Small 2015年第20期11卷

作者： Hamidreza Arandiyan Hongxing Dai Kemeng Ji Hongyu Sun Yanyan Zhao Junhua Li State Key Joint Laboratory of Environment Simulation and Pollution Control School of Environment Tsinghua University Beijing 100084 China Particles and Catalysis Research Group School of Chemical Engineering The University of New South Wales Sydney NSW 2052 Australia Key Laboratory of Beijing on Regional Air Pollution Control Beijing Key Laboratory for Green Catalysis and Separation and Laboratory of Catalysis Chemistry and Nanoscience Department of Chemistry and Chemical Engineering College of Environmental and Energy Engineering Beijing University of Technology Beijing 100124 China National Center for Electron Microscopy in Beijing School of Materials Science and Engineering The State Key Laboratory of New Ceramics and Fine Processing Key Laboratory of Advanced Materials (MOE) Tsinghua University Beijing 100084 China

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On the Origin of Capacity Increase in Rechargeable Magnesium Batteries with Manganese Oxide Cathodes and Copper Metal Current Collectors

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Angewandte Chemie 2024年第5期137卷

作者： Zhao Li Yi Li Yang Zhan Xiaodong Lin Yingying Yao Tianshuo Zhao Fengzhan Sun Hao Xu Zhewen Ma Wei Zhang Yanling Xue Xiaolong Li Alexandru Vlad Jianxin Zou National Engineering Research Center of Light Alloy Net Forming State Key Laboratory of Metal Matrix Composite Center of Hydrogen Science School of Materials Science and Engineering Shanghai Jiao Tong University 200240 Shanghai China Institute of Condensed Matter and Nanosciences Université Catholique de Louvain B-1348 Louvain-la-Neuve Belgium Institute for Clean Energy & Advanced Materials School of Materials and Energy Southwest University 400715 Chongqing China State Key Laboratory of Advanced Processing and Recycling of Nonferrous Metals School of Materials Science and Engineering Lanzhou University of Technology 730050 Lanzhou China Shanghai Synchrotron Radiation Facility Shanghai Advanced Research Institute Chinese Academy of Sciences 201204 Shanghai China

Rechargeable magnesium batteries (RMBs), with Cu as positive electrode current collector (CC), typically display a gradual capacity increase with cycling. Whereas the origin of this was suggested in gradual active material electro-activation, the fact that this is prevalent in many positive electrode material systems remains unexplained. Herein, we elucidate the underlying mechanism through a series of multiscale joint operando X-ray characterizations, including operando synchrotron X-ray diffraction and imaging technology. We select a series of manganese oxides as benchmark positive electrodes and find that no magnesium ions are stored within the lattices of these materials, despite an apparent cell capacity increase with cycling. The origin of capacity increase is rooted in the gradual electrochemical corrosion of metallic Cu, release of Cu(I, II) species in electrolyte, and their subsequent redox activity, resulting in apparent electrode capacity gains. Furthermore, the shuttle and redox speciation of Cu ions trigger the irreversible depletion of both the Cu CC (or any other source) and the magnesium metal, ultimately leading to cell failure. Our work suggests the need to reconsider the appropriateness of using Cu as a positive electrode CC for RMBs.

关键词： Magnesium metal batteries synchrotron X-ray characterizations X-ray imaging operando X-ray characterizations copper current collector

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Correction: Additive-mediated intercalation and surface modification of MXenes

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Chemical Society reviews 2022年第8期51卷 3314页

作者： Jing Zou Jing Wu Yizhou Wang Fengxia Deng Jizhou Jiang Yizhou Zhang Song Liu Neng Li Han Zhang Jiaguo Yu Tianyou Zhai Husam N Alshareef School of Environmental Ecology and Biological Engineering School of Chemistry and Environmental Engineering Key Laboratory of Green Chemical Engineering Process of Ministry of Education Engineering Research Center of Phosphorus Resources Development and Utilization of Ministry of Education Wuhan Institute of Technology Wuhan Hubei 430205 P. R. China. 027wit@***. Key Laboratory of Rare Mineral Ministry of Natural Resources Geological Experimental Testing Center of Hubei Province Wuhan Hubei 430034 P. R. China. Physical Science and Engineering Division Materials Science & Engineering King Abdullah University of Science and Technology (KAUST) Thuwal 23955-6900 Kingdom of Saudi Arabia. husam.alshareef@kaust.edu.sa. State Key Laboratory of Urban Water Resources and Environment School of Environment Harbin Institute of Technology Harbin 150090 P. R. China. Institute of Advanced Materials and Flexible Electronics (IAMFE) School of Chemistry and Materials Science Nanjing University of Information Science & Technology Nanjing 210044 P. R. China. yizhou.zhang@***. Key Laboratory for Organic Electronics & Information Displays and Institute of Advanced Materials Nanjing University of Posts and Telecommunications Nanjing 210023 P. R. China. Institute of Chemical Biology and Nanomedicine (ICBN) State Key Laboratory of Chemo/Biosensing and Chemometrics College of Chemistry and Chemical Engineering Hunan University Changsha 410082 P. R. China. State Key Laboratory of Advanced Technology for Materials Synthesis and Processing State Key Laboratory of Silicate Materials for Architectures Wuhan University of Technology Wuhan Hubei 430070 P. R. China. Shenzhen Engineering Laboratory of Phosphorene and Optoelectronics and Key Laboratory of Optoelectronic Devices and Systems of Ministry of Education and Guangdong Province Shenzhen University Shenzhen 518060 P. R. China. State Key Laboratory of Material Processing and Die & Mould Technology School of Materials Science and Engineering H

Correction for 'Additive-mediated intercalation and surface modification of MXenes' by Jing Zou , , 2022, DOI: 10.1039/d0cs01487g.

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Microstructure and Mechanical Properties of AISI 304L Austenitic Stainless Steel Processed by Various Schedules of Rolling

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Journal of Physics: Conference Series 2020年第1期1688卷

作者： A G Raab G I Raab A A Tokar O V Rybalchenko A N Belyakov S V Dobatkin P La Institute of Physics of Advanced Materials Ufa State Aviation Technical University K. Marx st. 12 450008 Ufa Russia A A Baikov Institute of Metallurgy and Materials Science of RAS Leninsky pr. 49 119334 Moscow Russia National University of Science and Technology 'MISIS' Leninskiy pr. 4 119049 Moscow Russia Belgorod State University Pobeda st. 85 308015 Belgorod Russia State Key Laboratory of Advanced Processing and Recycling of Nonferrous Metals Lanzhou University of Technology Lanzhou China

The paper studies various rolling schedules implemented at 500°C (incl. direct, reverse, and cross rolling) and their effect on the structure formation and mechanical properties in AISI 304L stainless steel samples. Both TEM and SEM research techniques were applied. An ultrafine grain-subgrain microstructure was found to be formed inside elongated original grains. Rolling-processed microstructural elements were close in their size with the minimum value observed after a reverse rolling (240 nm). Mechanical properties were studied using microhardness measurements and tensile testing revealing a considerable increase in strength accompanied by a density reduction upon deformation. The strength values in the material subjected to all three rolling schedules are relatively close to the highest yield strength and ultimate tensile stress observed after reverse rolling with a strain degree of 70%.

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Corrigendum to “Fabrication of PbBi 4 Ti 4 O 15 microplatelets with different TiO 2 reactants) composites with high permittivity and low loss” [Mater. Lett. 274 (2020) 128018]

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materials Letters 2022年 310卷

作者： Leilei Li Junting Liu Shuyao Cao Jie Xu Emilia Pawlikowska Mikołaj Szafran Feng Gao State Key Laboratory of Solidification Processing MIIT Key Laboratory of Radiation Detection Materials and Devices NPU-QMUL Joint Research Institute of Advanced Materials and Structures (JRI-AMAS) School of Materials Science and Engineering Northwestern Polytechnical University Xi’an Shaanxi 710072 PR China Institute of High Pressure Physics of the Polish Academy of Sciences ul. Sokolowska 29/37 01-142 Warsaw Poland Faculty of Chemistry Warsaw University of Technology Noakowskiego 3 00-664 Warsaw Poland

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Electron-Phonon Coupling Suppression by Enhanced Lattice Rigidity in 2D Perovskite Single Crystals for High-Performance X-Ray Detection

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advanced materials (Deerfield Beach, Fla.) 2023年第7期35卷 e2208875页

作者： Bobo Zhang Tao Zheng Jiaxue You Chuang Ma Yucheng Liu Lu Zhang Jun Xi Guohua Dong Ming Liu Shengzhong Frank Liu Key Laboratory of Applied Surface and Colloid Chemistry Ministry of Education Shaanxi Key Laboratory for Advanced Energy Devices Shaanxi Engineering Lab for Advanced Energy Technology International Joint Research Center of Shaanxi Province for Photoelectric Materials Science Institute for Advanced Energy Materials School of Materials Science and Engineering Shaanxi Normal University Xi'an 710119 China. State Key Laboratory of Solidification Processing Northwestern Polytechnical University Xi'an 710072 China. Key Laboratory for Physical Electronics and Devices of the Ministry of Education & Shaanxi Key Lab of Information Photonic Technique School of Electronic Science and Engineering Xi'an Jiaotong University No. 28 Xianning West Road Xi'an 710049 China. The Electronic Materials Research Laboratory Key Laboratory of the Ministry of Education & International Center for Dielectric Research School of Electronic Science and Engineering State Key Laboratory for Mechanical Behavior of Materials Xi'an Jiaotong University Xi'an 710049 China. Dalian National Laboratory for Clean Energy iChEM Dalian Institute of Chemical Physics Chinese Academy of Sciences Dalian 116023 China. University of the Chinese Academy of Sciences Beijing 100039 China.

2D Dion-Jacobson (DJ) perovskite single crystals (PSCs) usually demonstrate better X-ray detection performance than Ruddlesden-Popper (RP) PSCs. However, the mechanism of the improved performance is still elusive. Here, by the aid of strong interactions between dimethylbiguanide (DGA) and PbI , a novel DJ-perovskitoid (DGA)PbI is designed. From the comparison of (DGA)PbI to other 2D PSCs, it is discovered that the tiniest lattice distortion and increased hydrogen bonds in the atom-scaled analysis strengthen lattice rigidity and weaken electron-phonon coupling to suppress disordered scattering of carriers, resulting in significantly improved carrier transport and stability. Therefore, high carrier mobility (78.1 cm V s ) and a pronounced sensitivity of 4869.0 µC Gy cm are achieved using (DGA)PbI , which are the best in 2D Pb-based PSC devices to date. Finally, the (DGA)PbI devices exhibit good spatial resolution in X-ray imaging and excellent long-term stability to work as a promising candidate for medical diagnostics and nondestructive determination.

关键词： 2D perovskite X-ray detection electron-phonon coupling high sensitivity lattice rigidity

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