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Chlorine-Substituent Regulation in Dopant-Free Small-Molecule Hole-Transport Materials Improves the Effi ciency and Stability of Inverted Perovskite Solar Cells

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Transactions of Tianjin University 2024年第4期30卷 314-323页

作者： Xinyi Liu Xiaoye Zhang Zhanfeng Li Jinbo Chen Yanting Tian Baoyou Liu Changfeng Si Gang Yue Hua Dong Zhaoxin Wu Key Laboratory of Advanced Transducers and Intelligent Control System Ministry of Education and Shanxi ProvinceTaiyuan University of TechnologyTaiyuan 030024China School of Electrical Engineering University of South ChinaHengyang 421001China College of Physics and Optoelectronics Taiyuan University of TechnologyTaiyuan 030024China Ningxia Hui Autonomous Region Screen Display Organic Materials Engineering Technology Research Center Ningxia Sinostar Display Material Co.Ltd.Yinchuan 750003China Organic Semiconductor Centre EaStCHEM School of ChemistryUniversity of St AndrewsFife KY169STUK Key Laboratory of Photonics Technology for Information School of Electronic and Information Engineering Xi’an Jiaotong UniversityXi’an 710049China

Although doped hole-transport materials(HTMs)off er an effi ciency benefi t for perovskite solar cells(PSCs),they inevi-tably diminish the ***,we describe the use of various chlorinated small molecules,specifi cally fl uorenone-triphenylamine(FO-TPA)-x-Cl[x=para,meta,and ortho(p,m,and o)],with diff erent chlorine-substituent positions,as dopant-free HTMs for *** chlorinated molecules feature a symmetrical donor-acceptor-donor structure and ideal intramolecular charge transfer properties,allowing for self-doping and the establishment of built-in potentials for improving charge *** effi cient hole-transfer interfaces are constructed between perovskites and these HTMs by strategi-cally modifying the chlorine ***,the chlorinated HTM-derived inverted PSCs exhibited superior effi ciencies and air ***,the dopant-free HTM FO-TPA-o-Cl not only attains a power conversion effi ciency of 20.82% but also demonstrates exceptional stability,retaining 93.8%of its initial effi ciency even after a 30-day aging test conducted under ambient air conditions in PSCs without *** fi ndings underscore the critical role of chlorine-substituent regulation in HTMs in ensuring the formation and maintenance of effi cient and stable PSCs.

关键词： Hole-transport materials Inverted perovskite solar cells Chlorinated small molecules Donor–acceptor–donor structure

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Ultrasensitive Ammonia Gas Sensor Based on Ti3c2tx/Ti3alc2 Planar Composite at Room Temperature

SSRN

引用

SSRN 2022年

作者： Liu, Zhihua Han, Dan Liu, Lulu Li, Donghui Han, Xiaomei Chen, Yi Liu, Xiaoru Zhuo, Kai Cheng, Yongqiang Sang, Shengbo Shanxi Key Laboratory of Micro Nano Sensors & Artificial Intelligence Perception College of Information and Computer Taiyuan University of Technology Taiyuan030024 China Key Lab of Advanced Transducers and Intelligent Control System the Ministry of Education Taiyuan University of Technology Taiyuan030024 China

Two-dimensional (2D) transition metal carbides (MXene) have attracted great attention for device applications due to their unique structures and excellent properties, such as high electrical conductivity and abundant functional groups on the surface. However, gas sensors based on Ti3C2Tx MXene have the problems of high detection limit and poor long-term stability. Herein, we report a simple method to prepare Ti3C2Tx/Ti3AlC2 planar composite gas sensing materials using high molar ratio of HCl and LiF with Ti3AlC2 as a framework. The Ti3C2Tx/Ti3AlC2 planar composite gas sensor has a high sensitivity, good selectivity and low detection limit for NH3, which can detect 50 ppb (1.2%) at room temperature ((25 ± 2) °C). Furthermore, the gas sensor has good repeatability and long-term stability. After 120 days, the response of the gas sensor to 500 ppb of NH3 fluctuated little due to the Ti3AlC2 as a framework. The superior performances can be attributed to the special heterojunction between Ti3C2Tx and Ti3AlC2 and the high proportion of -O and -OH functional groups on the surface of Ti3C2Tx/Ti3AlC2 composite. This study provides an important reference for the realization of high performance NH3 sensing by Ti3C2Tx. © 2022, The Authors. All rights reserved.

关键词： Gases

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Design of a Novel Autonomous Docking system With a Supporting Robotic Fish

Design of a Novel Autonomous Docking System With a Supportin...

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IEEE International Conference on Real-time Computing and Robotics (RCAR)

作者： Huijie Dong Chunyang Zhao Tiezhu Qiao Jian Wang Di Chen Yan Meng Junzhi Yu Ministry of Education Key Laboratory of Advanced Transducers and Intelligent Control System Taiyuan University of Technology Taiyuan China Institute of Automation Laboratory of Cognitive and Decision Intelligence for Complex System Chinese Academy of Sciences Beijing China Department of Advanced Manufacturing and Robotics College of Engineering State Key Laboratory for Turbulence and Complex Systems Peking University Beijing China College of Electronics and Information Engineering Guangdong Ocean University Zhanjiang China

Underwater supporting robots serving as a relay of energy supplements and communication for other underwater equipment are promising for ocean exploration, development, and protection. This paper proposes a novel autonomous docking system centered on a designed supporting robotic fish named ‘CourierFish’. Specifically, CourierFish is capable of docking with a surface dock station for supplying itself and docking with a seafloor platform for supporting equipment in the platform. A visual navigation scheme integrating LED and ArUco markers is presented for accurate localization. The control approach for docking motion is also illustrated. Simulations and aquatic experiments are performed to verify the feasibility of the proposed docking system. The obtained results lay a solid foundation for the construction of various underwater equipment and robot networks.

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Bearing Fault Diagnosis Based on Dual-Data Input Convolutional Neural Network

SSRN

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SSRN 2022年

作者： He, Chaoqian Hao, Runfang Yang, Kun Yuan, Zhongyun Shang, Shengbo Wang, Xiaorui Shanxi Key Laboratory of Micro Nano Sensors & Artificial Intelligence Perception College of Information and Computer Taiyuan University of Technology Taiyuan030024 China Key Lab of Advanced Transducers and Intelligent Control System Ministry of Education Taiyuan University of Technology Taiyuan030024 China

Previous bearing fault diagnosis models show low accuracy and unstable performance in strong noise environment, which are not suitable for the actual complex industrial scenarios. In this paper, the dual-channel convolution model (DDCNN) based on dual-data inputs is established. The model used the reconstructed two-dimensional data as inputs. In one channel, convolution with small kernel is used to extract details of FE data, and large kernel obtain global information of DE data in the other. The output is classified through the full connection layer after the data features of both channels are fused. Besides, data are mixed from different loads to avoid cross-load effects as much as possible. The results demonstrate that the proposed model has good accuracy and anti-noise performance. The accuracy is as high as 92.65% when the SNR is -10. © 2022, The Authors. All rights reserved.

关键词： Failure analysis

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Achieving high-security and massive-capacity optical communications based on orbital angular momentum configured chaotic laser

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advanced Photonics Nexus 2024年第4期3卷 92-100页

作者： Yanwei Cui Jianguo Zhang Zhongquan Nie Anbang Wang Yuncai Wang Taiyuan University of Technology Ministry of EducationCollege of Electronic Information and Optical EngineeringKey Laboratory of Advanced Transducers and Intelligent Control SystemTaiyuanChina National University of Defense Technology College of Advanced Interdisciplinary StudiesChangshaChina Guangdong University of Technology School of Information EngineeringGuangzhouChina Guangdong Provincial Key Laboratory of Photonics Information Technology GuangzhouChina

Secure and high-speed optical communications are of primary focus in information *** it is widely accepted that chaotic secure communication can provide superior physical layer security,it is challenging to meet the demand for high-speed increasing communication *** theoretically propose and experimentally demonstrate a conceptual paradigm for orbital angular momentum(OAM)configured chaotic laser(OAM-CCL)that allows access to high-security and massivecapacity optical *** 11 OAM modes and an all-optical feedback chaotic laser,we are able to theoretically empower a well-defined optical communication system with a total transmission capacity of 100 Gb∕s and a bit error rate below the forward error correction threshold 3.8×10^(-3).Furthermore,the OAM-CCL-based communication system is robust to 3D misalignment by resorting to appropriate mode spacing and beam ***,the conceptual paradigm of the OAM-CCL-based communication system is *** contrast to existing systems(traditional free-space optical communication or chaotic optical communication),the OAM-CCL-based communication system has threein-one characteristics of high security,massive capacity,and *** findings demonstrate that this will promote the applicable settings of chaotic laser and provide an alternative promising route to guide high-security and massive-capacity optical communications.

关键词： chaotic secure communication orbital angular momentum configured chaotic laser high security massive capacity misalignment

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Ultrasensitive Ammonia Gas Sensor Based on Ti3c2tx/Ti3alc2 Planar Composite at Room Temperature

SSRN

引用

SSRN 2022年

作者： Liu, Zhihua Han, Dan Liu, Lulu Li, Donghui Han, Xiaomei Chen, Yi Liu, Xiaoru Zhuo, Kai Cheng, Yongqiang Sang, Shengbo Shanxi Key Laboratory of Micro Nano Sensors & Artificial Intelligence Perception College of Information and Computer Taiyuan University of Technology Taiyuan030024 China Key Lab of Advanced Transducers and Intelligent Control System of the Ministry of Education Taiyuan University of Technology Taiyuan030024 China

Two-dimensional (2D) transition metal carbides (MXene) have attracted great attention for device applications due to their unique structures and excellent properties, such as high electrical conductivity and abundant functional groups on the surface. However, gas sensors based on Ti3C2Tx MXene have the problems of high detection limit and poor long-term stability. Herein, we report a simple method to prepare Ti3C2Tx/Ti3AlC2 planar composite gas sensing materials using high molar ratio of HCl and LiF with Ti3AlC2 as a framework. The Ti3C2Tx/Ti3AlC2 planar composite gas sensor has a high sensitivity, good selectivity and low detection limit for NH3, which can detect 50 ppb (1.2%) at room temperature (25°C). Furthermore, the gas sensor has good repeatability and long-term stability. After 120 days, the response of the gas sensor to 500 ppb of NH3 fluctuated little due to the Ti3AlC2 as a framework. The superior performances can be attributed to the special heterojunction between Ti3C2Tx and Ti3AlC2 and the high proportion of -O and -OH functional groups on the surface of Ti3C2Tx/Ti3AlC2 composite. This study provides an important reference for the realization of high performance NH3 sensing by Ti3C2Tx. © 2022, The Authors. All rights reserved.

关键词： Chemical detection

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Gradient piezoelectric composites for ultrasonic transducer design and imaging applications

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Journal of Materiomics 2025年

作者： Chenxue Hou Zhaoxi Li Chunlong Fei Qibo Lin Xiaofei Luo Xiongwei Wei Yiheng Yang Qi Lu Yi Quan Guangzhi Dong Zeyu Chen Xiaozhou Lü Weimin Bao Yintang Yang Shaanxi Provincial Key Laboratory of Integrated Circuit and System Integration Faculty of Integrated Circuit Xidian University Xi’an 710071 China School of Aerospace Science and Technology Xidian University Xi’an 710071 China State Key Laboratory of Precision Manufacturing for Extreme Service Performance College of Mechanical and Electrical Engineering Central South University Changsha 410083 China College of Automotive and Mechanical Engineering Changsha University of Science and Technology Changsha 410114 China Hunan Province University Key Laboratory of Intelligent Testing and Control Technology for Engineering Equipment Changsha 410114 China School of Advanced Materials and Nanotechnology Xidian University Xi'an 710126 China Furong Laboratory (Precision Medicine) Changsha 410008 China National Engineering Research Center of Personalized Diagnostic and Therapeutic Technology Xiangya Hospital Central South University Changsha 410008 China Hunan Engineering Research Center of Skin Health and Disease Xiangya Hospital Central South University Changsha 410008 China

Ultrasonic imaging technology has advanced rapidly, the escalating demand for imaging quality has driven the continuous development of ultrasonic transducers featuring high-performance. Among them, the crucial factors constraining the further enhancement of imaging quality are the frequency of the device and the intensity of the echo signal. Piezoelectric composites have become a hotspot for ultrasonic transducers and imaging applications due to their excellent properties. However, due to the limitations of the accuracy of the cutting process, the development of piezoelectric/polymer composites is often undermined by undesirable pseudo-vibrations, especially in high-frequency applications, which will significantly reduce energy conversion efficiency. In this study, a novel design method of 1-3 piezoelectric composites with gradient nanoparticle doped polymer is proposed to eliminate the undesired lateral vibrations. Based on the optimized composites, a high-performance composite ultrasonic transducer with a center frequency of 8.51 MHz is prepared. Compared with the traditional composite transducer, the optimized transducer improves the echo voltage amplitude significantly, reaching nearly 3 times. The above advantages are further verified in high-quality ultrasound and photoacoustic imaging. The optimization method has valuable guidance for the design of high-frequency composite transducers, which have great potential in ultrasonic and photoacoustic imaging applications.

关键词： Piezoelectric composites Ultrasonic transducer Imaging applications Lateral vibration Finite element analysis

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A NSGA-Ⅱ based Peak Load Shifting Optimization Method for Customers with Distributed Generators Considering Time-of-use Price

A NSGA-Ⅱ based Peak Load Shifting Optimization Method for C...

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第37届中国控制会议

作者： Hao Zhou Min Ding Bo Hu Qingyi Wang Zhili Tan Danyun li School of Automation China University of Geosciences Hubei Key Laboratory of Advanced Control and Intelligent Automation for Complex System State Grid Energy Research Institute Co. LTD.

With the extensive use of distributed generation, the traditional demand response analysis cannot meet the current *** paper proposes a NSGA-II based peak load shifting optimization method for customers with distributed generators considering time-of-use price. Firstly, a fuzzy classification method divides the daily power into three time segments,peak hours, flat hours and valley hours. Secondly, on the basis of the time-of-use price, a peak load shifting optimization model is built with constraints and the objectives of minimizing the peak load, maximizing the valley load, and minimizing the peakvalley difference. Then, a NSGA-II based optimization method solves the optimal model and obtains the optimal electricity prices of different time segments to shift the peak load and the valley load. Finally, the simulation results shows the effectiveness of the proposed method.

关键词： Distributed Generation Demand Respond Time-of-use Price Multi-objective Genetic Algorithm

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Numerical study of nanochannel on a silicon-silver dimer gap for significantly enhanced fluorescence

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Results in Physics 2024年 62卷

作者： Wang, Qiang Chen, Zhihui Gu, Zhiyuan Li, Lingqiao Guo, Deyi Shi, Baopeng Wang, Yang Key Lab of Advanced Transducers and Intelligent Control System Ministry of Education and Shanxi Province College of Electronic Information and Optical Engineering Taiyuan University of Technology Taiyuan 030024 China Key Lab of Advanced Transducers and Intelligent Control System Ministry of Education and Shanxi Province College of Physics Taiyuan University of Technology Taiyuan 030024 China Key Laboratory of Chemical Biology and Molecular Engineering of Ministry of Education Institute of Biotechnology Shanxi University Taiyuan 030006 China

The metal-dielectric dimer is an ideal structure for enhancing single-molecule fluorescence. When a single-molecule interacts with the metal-dielectric dimer, the metal-dielectric plasmonic system creates strong resonance, which amplifies the electric field by several orders of magnitude. One-dimensional photonic crystals (1D PCs) provide a photonic bandgap (PBG) and nearly perfect reflection for specific wavelengths. These phenomena contribute significantly to fluorescence enhancement. Herein, we propose the structure of 1D PCs with a silicon-silver dimer to achieve remarkable fluorescence enhancement under numerical study. Specifically, our design involves a 20 nm gapped silicon-silver dimer with a 50 nm nanochannel positioned above it. Through the optimization of structural parameters, our results demonstrate that quantum dots with a high intrinsic quantum yield, such as 100 %, are capable of achieving a fluorescence directional emission enhancement of up to three orders of magnitude compared to the bare structure, with an average enhancement factor reaching 407-fold. These findings stand for the unique sensitivity of the device, making it a promising choice for applications in biological nanoparticle detection, environmental monitoring, and other fields in the future. © 2024

关键词： Localized surface plasmon resonance (LSPR) Resonant cavity Silicon-silver dimer Ultra-high fluorescence enhancement

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Time delay signature elimination of chaos in a semiconductor laser by dispersive feedback from a chirped FBG

arXiv

引用

arXiv 2017年

作者： Wang, Daming Wang, Longsheng Zhao, Tong Gao, Hua Wang, Yuncai Chen, Xianfeng Wang, Anbang Key Laboratory of Advanced Transducers and Intelligent Control System Ministry of Education and Shanxi Province College of Physics and Optoelectronics Taiyuan University of Technology Taiyuan030024 China School of Electronic Engineering Bangor University BangorLL571UT United Kingdom

—Time delay signature (TDS) of a semiconductor laser subject to dispersive optical feedback from a chirped fiber Bragg grating (CFBG) is investigated experimentally and numerically. Different from mirror, CFBG provides additional frequency-dependent delay caused by dispersion, and thus induces external-cavity modes with irregular mode separation rather than a fixed separation induced by mirror feedback. Compared with mirror feedback, the CFBG feedback can greatly depress and even eliminate the TDS, although it leads to a similar quasi-period route to chaos with increases of feedback. In experiments, by using a CFBG with dispersion of 2000ps/nm, the TDS is decreased by 90% to about 0.04 compared with mirror feedback. Furthermore, both numerical and experimental results show that the TDS evolution is quite different: the TDS decreases more quickly down to a lower plateau (even background noise level of autocorrelation function) and never rises again. This evolution tendency is also different from that of FBG feedback, of which the TDS first decreases to a minimal value and then increases again as feedback strength increases. In addition, the CFBG feedback has no filtering effects and does not require amplification for feedback *** Codes 37D45 (Primary), 37N20, 78A60 (Secondary) Copyright © 2017, The Authors. All rights reserved.

关键词： Time delay

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