检索结果-内蒙古大学图书馆

Carbon Energy 2025年第2期7卷 121-130页

作者： Tianyi Xu Dongxu Jiao Jinchang Fan Yilong Dong Zhaoyong Jin Lei Zhang Wei Zhang Jingxiang Zhao Weitao Zheng Xiaoqiang Cui State Key Laboratory of Automotive Simulation and Control Key Laboratory of Automobile MaterialsMinistry of EducationSchool of Materials Science and EngineeringJilin UniversityChangchunChina College of Chemistry Jilin UniversityChangchunChina Key Laboratory of Photonic and Electronic Bandgap Materials Ministry of EducationCollege of Chemistry and Chemical EngineeringHarbin Normal UniversityHarbinChina

Strain effects have garnered significant attention in catalytic applications due to their ability to modulate the electronic structure and surface adsorption properties of *** this study,we propose a novel approach called“similar stacking”for stress modulation,achieved through the loading of Co_(2)P on Ni_(2)P(Ni_(2)P/Co_(2)P).Theoretical simulations reveal that the compressive strain induced by Co_(2)P influences orbital overlap and electron transfer with hydrogen ***,the number of stacked layers can be adjusted by varying the precursor soaking time,which further modulates the strain range and hydrogen *** a 2-h soaking condition,the strain effect proves favorable for efficient hydrogen *** characterizations using X-ray diffraction,high-angel annular dark-field scanning transmission election microscope(HAADF-STEM),and X-ray absorption near-edge structure spectroscopy successfully demonstrate lattice contraction of Co_(2)P and bond length shortening of ***,our catalyst shows an ultrahigh current density of 1 A cm^(-2) at an overpotential of only 388 mV,surpassing that of commercial Pt/C,while maintaining long-term *** material design strategy of similar stacking opens up new avenues of strain modulation and the deeper development of electrocatalysts.

关键词： compressive strain heterogeneous phosphide hydrogen evolution reaction similar stacking

来源：评论

学校读者我要写书评

暂无评论

Research on Air Supply System control of PEMFC Based on LQR control

Research on Air Supply System Control of PEMFC Based on LQR ...

引用

China SAE Congress, 2021

作者： Zeng, Xiaohua Song, Meijie Song, Dafeng Niu, Chaofan State Key Laboratory of Automobile Simulation and Control Jilin University Changchun China

ISBN: (纸本)9789811938412

Proton exchange membrane fuel cell (PEMFC) is composed of several coupled components with complex nonlinear characteristics. Coordinating the work of each component and effectively controlling the air supply system are key measures to improve the efficiency of the system. In order to control the air supply system of PEMFC, this paper explores the influence of different input parameters on the energy consumption efficiency of the system, quantifies the relationship between the variables, and studies the change law of power consumption efficiency and peroxide ratio of the system. After that, separate feed-forward, feed-forward + feedback and LQR control algorithms are used to control the optimal peroxide ratio respectively, and the algorithms are verified by Matlab/Simulink simulation. The results show that the LQR algorithm has the best dynamic response speed, which is shortened by 17.0% and 47.1% compared with the feed-forward + feedback control and separate feed-forward control systems. At the same time, the maximum control error of LQR algorithm is the smallest, which is 52.6% and 84.6% lower than that of feed-forward + feedback control and separate feed-forward control. © 2023, The Author(s), under exclusive license to Springer Nature Singapore Pte Ltd.

关键词： MATLAB

来源：评论

学校读者我要写书评

暂无评论

Kinetically and thermodynamically expediting elementary steps via high-valence Cr-incorporated of nickel selenide for water electrolysis

引用

Nano Research 2024年第3期17卷 1199-1208页

作者： Huafeng Fan Dongxu Jiao Jinchang Fan Dewen Wang Bilal Zaman Wei Zhang Lei Zhang Weitao Zheng Xiaoqiang Cui State Key Laboratory of Automotive Simulation and Control School of Materials Science and EngineeringKey Laboratory of Automobile Materials of MOEJilin Provincial International Cooperation Key Laboratory of High-Efficiency Clean Energy MaterialsElectron Microscopy CenterJilin UniversityChangchun 130012China College of Chemistry Jilin UniversityChangchun 130012China

Designing high-performance electrocatalysts toward hydrogen evolution reaction(HER)and oxygen evolution reaction(OER)is essential to reduce the activation barrier and optimize free adsorption energy of reactive ***,we report that incorporating high-valence Cr into NiSe_(2)(Cr_(x)Ni_(1-x)Se_(2))kinetically and thermodynamically expedites elementary steps of both HER and *** as-prepared Cr_(0.05)Ni_(0.95)Se_(2) catalyst displays excellent HER and OER activities,with low overpotentials of 89 and 272 mV at the current density of 10 mA·cm^(-2)(j10),respectively,and remains stable during operation for 30 h.A low cell voltage of only 1.59 V is required to drive j10 in alkaline *** situ Raman spectroscopy reveals that Cr incorporation facilitates the formation of NiOOH active species during the OER ***,theoretical explorations demonstrate that high-valence Cr incorporation efficiently accelerates water dissociation kinetics and improves H*adsorption during HER process,lowering the activation barrier of OER and optimizing the adsorption energy of oxygen-based intermediate,thus kinetically and thermodynamically enhancing the intrinsic performance of NiSe_(2) for over water *** strategy provides a new horizon to design transition metal based electrocatalysts in the clean energy field.

关键词： nickel selenide electrocatalytic water splitting high-valence Cr density functional theory(DFT)calculation

来源：评论

学校读者我要写书评

暂无评论

Vehicle state and Bias Estimation Based on Unscented Kalman Filter with Vehicle Hybrid Kinematics and Dynamics Models

引用

Automotive Innovation 2023年第4期6卷 571-585页

作者： Shouren Zhong Yang Zhao Linhe Ge Zitong Shan Fangwu Ma State Key Laboratory of Automotive Simulation and Control Jilin UniversityChangchun 130022China

In recent years,vehicle state estimation methods incorporating different vehicle models have received extensive *** the vehicle is disturbed by external forces not considered in traditional vehicle models(for example,a certain slope,or wind resistance different from theoretical calculation),the problem of model mismatch will occur,which leads to the inaccurate estimation of the vehicle *** solve this problem,an Unscented Kalman Filter(UKF)algorithm is used to fuse inertial navigation data with the vehicle hybrid model in this *** hybrid model introduces a switching strategy that fuses the vehicle kinematics and the dynamics models while augmenting biases that need to be estimated in the vehicle *** switching strategy resolves the integration divergence problem of vehicle dynamics models at low speeds and the inaccurate estimation of vehicle kinematics models at high *** experiments demonstrate that the proposed method can accurately estimate biases induced by external forces,enhancing the accuracy and confidence of states by eliminating errors caused by these *** robustness of the method is validated in vehicle verification platform experiments,where errors in vehicle lateral speed and yaw rate are reduced by 9.7 cm/s and 0.012°/s,respectively,under large curvature maneuvers,and 9.6 cm/s and 0.004°/s under quarter-turn *** proposed method significantly improves lateral speed and vehicle position accuracies.

关键词： Vehicle state estimation Vehicle hybrid models Unscented Kalman filter Integration stability

来源：评论

学校读者我要写书评

暂无评论

Hierarchical Parking Path Planning Based on Optimal Parking Positions

引用

Automotive Innovation 2023年第2期6卷 220-230页

作者： Yaogang Zhang Guoying Chen Hongyu Hu Zhenhai Gao State Key Laboratory of Automotive Simulation and Control Jilin UniversityChangchunJilinChina

Automated valet parking(AVP)has attracted the attention of industry and academia in recent ***,there are still many challenges to be solved,including shortest path search,optimal time efficiency,and applicability of algorithm in complex *** this paper,a hierarchical AVP path planner is proposed,which divides a complete AVP path planning into the guided layer and the planning layer from the perspective of global *** guided layer is mainly used to divide a complex AVP path planning into several simple path plannings,which makes the hybrid A*algorithm more applicable in a complex parking *** planning layer mainly adopts different optimization methods for driving and parking path *** proposed method is verified by a large number of simulations which include the verification of the optimal parking position,the performance of the planner for perpendicular parking,and the scalability of the planner for parallel parking and inclined *** simulation results reveal that the efficiency of the algorithm is increased by more than 20 times,and the average path length is also shortened by more than 20%.Furthermore,the planner overcomes the problem that the hybrid A*algorithm is not applicable in complex parking scenarios.

关键词： Automated valet parking Path planning Hybrid A Visibility graph Shortest path

来源：评论

学校读者我要写书评

暂无评论

Evolution of soil DOM during thermal remediation below 100℃:concentration,spectral characteristics and complexation ability

引用

Frontiers of Environmental Science & Engineering 2024年第8期18卷 31-41页

作者： Wan Huang Ziren Wan Di Zheng Lifeng Cao Guanghe Li Fang Zhang State Key Joint Laboratory of Environment Simulation and Pollution Control State Environment Protection Key Laboratory of Microorganism Application and Risk ControlSchool of EnvironmentTsinghua UniversityBeijing 100084China National Engineering Laboratory for Site Remediation Technologies Beijing 100015China

The impact of thermal remediation on soil function has drawn increasing *** far,as the most active fraction of soil organic matter,the evolution of dissolved organic matter(DOM)during the thermal remediation lacks in-depth investigation,especially for the temperatures value below 100℃.In this study,a series of soil thermal treatment experiments was conducted at 30,60,and 90℃ during a 90-d period,where soil DOM concentration increased with heating temperature and *** molecular weight,functional groups content and aromaticity of DOM all decreased during the thermal *** excitation-emission matrices(EEM)results suggested that humic acid-like substances transformed into fulvic acid-like substances(FIII/FV increased from 0.27 to 0.44)during the heating process,and five DOM components were further identified by *** change of DOM structures and components indicated the decline of DOM stability and hydrophilicity,and can potentially change the bioavailability and *** temperature also resulted in the decline of DOM complexation ability,which may be caused by the loss of binding sites due to the decrease of polar function groups,aromatic structures and hydrophilic *** study provides valuable information about the evolution of DOM during thermal remediation,which would potentially change the fate of metal ions and the effectiveness of the post-treatment technologies in the treated region.

关键词： Thermal remediation below 100℃ Heating temperature Soil DOM concentration DOM spectral characteristics Excitation-emission matrices(EEM) Complexation ability

来源：评论

学校读者我要写书评

暂无评论

Analysis of China’s PM_(2.5)and ozone coordinated control strategy based on the observation data from 2015 to 2020

引用

Journal of Environmental Sciences 2024年第4期138卷 385-394页

作者： Liuwei Kong Mengdi Song Xin Li Ying Liu Sihua Lu Limin Zeng Yuanhang Zhang State Key Joint Laboratory of Environmental Simulation and Pollution Control College of Environmental Sciences and EngineeringPeking UniversityBeijing 100871China

The coordinated control of PM_(2.5)and ozone has become the strategic goal of national air pollution *** the gradual decline in PM_(2.5)concentration and the aggravation of ozone pollution,a better understanding of the coordinated control of PM_(2.5)and ozone is urgently ***,we collected and sorted air pollutant data for 337 cities from 2015 to 2020 to explore the characteristics of PM_(2.5)and ozone pollution based on China’s five major air pollution *** results show that it is necessary to continue to strengthen the emission reduction in PM_(2.5)and ozone precursors,and control NO_(x) and VOCs while promoting a dramatic emission reduction in PM_(2.5).The primary method of curbing ozone pollution is to strengthen the emission control of VOCs,with a long-term strategy of achieving substantial emission reductions in NO_(x),because VOCs and NO_(x) are also precursors to PM_(2.5);hence,their reductions also contribute to the reduction in PM_(2.5).Therefore,the implementation of a multipollutant emission reduction control strategy aimed at the prevention and control of PM_(2.5)and ozone pollution is the only means to realize the coordinated control of PM_(2.5)and ozone.

关键词： PM_(2.5) Ozone Coordinated control Multipollutant reduction

来源：评论

学校读者我要写书评

暂无评论

Intake of tobacco nitrosamines of smokers in various provinces of China and their cancer risk:A meta-analysis

引用

Journal of Environmental Sciences 2024年第7期141卷 249-260页

作者： Xiao Li Zhiwei Ye Jun Wang Pengfei Lin Xiaojin Zhang Shuguang Xie Chao Chen Research Institute for Environmental Innovation(Suzhou) TsinghuaSuzhouJiangsu 215163China State Key Joint Laboratory of Environmental Simulation and Pollution Control School of EnvironmentTsinghua UniversityBeijing 100084China Shenzhen Key Laboratory of Organic Pollution Prevention and Control State Key Laboratory of Urban Water Resource and EnvironmentHarbin Institute of TechnologyShenzhen 518055China State Key Joint Laboratory of Environmental Simulation and Pollution Control College of Environmental Science and EngineeringPeking UniversityBeijing 100871China

Nitrosamines are a class of carcinogens which have been detected widely in food,water,some pharmaceuticals as well as *** objectives of this paper include reviewing the basic information on tobacco consumption and nitrosamine contents,and assessing the health risks of tobacco nitrosamines exposure to Chinese *** searched the publications in English from“Web of Science”and those in Chinese from the“China National Knowledge Infrastructure”in 2022 and collected 151 literatures with valid *** content of main nitrosamines in tobacco,including 4-(methylnitrosoamino)-1-(3-pyridyl)-1-butanone(NNK),N-nitrosonornicotine(NNN),N-nitrosoanatabine(NAT),N-nitrosoanabasine(NAB),total tobacco-specific nitrosamines(TSNA),and N-nitrosodimethylamine(NDMA)were *** information of daily tobacco consumption of smokers in 30 provinces of China was also ***,the intakes of NNN,NNK,NAT,NAB,TSNAs,and NDMA via tobacco smoke were estimated as 1534ng/day,591 ng/day,685 ng/day,81 ng/day,2543 ng/day,and 484 ng/day by adult smokers in30 provinces,*** cancer risk(CR)values for NNN and NNK inhalation intake were further calculated as 1.44×10^(-5)and 1.95×10^(-4).The CR value for NDMA intake via tobacco smoke(inhalation:1.66×10^(-4))indicates that NDMA is similarly dangerous in tobacco smoke when compared with the *** China,the CR values caused by average nitrosamines intake via various exposures and their order can be estimated as the following:smoke(3.75×10^(-4))>food(1.74×10^(-4))>drinking water(1.38×10^(-5)).Smokers in China averagely suffer 200%of extra cancer risk caused by nitrosamines in tobacco when compared with non-smokers.

关键词： N-nitrosamine Tobacco Cancer risk Tobacco specific nitrosamines(TSNAs) N-nitrosodimethylamine(NDMA)

来源：评论

学校读者我要写书评

暂无评论

Efficient Metal Recovery from Industrial Wastewater:Potential Oscillation and Turbulence Mode for Electrochemical System

引用

Engineering 2024年第7期38卷 184-193页

作者： Li Chen Gong Zhang Huijuan Liu Shiyu Miao Qingbai Chen Huachun Lan Jiuhui Qu Center for Water and Ecology State Key Joint Laboratory of Environment Simulation and Pollution ControlSchool of EnvironmentTsinghua UniversityBeijing 100084China

Efficient metal recovery from industrial wastewater facilitates addressing of the environmental hazards and resource requirements of heavy *** conventional electrodeposition recovery method is hampered by the limitations of interfacial ion transport in charge-transfer reactions,creating challenges for simultaneous rapid and high-quality metal ***,we proposed integrating a transient electric field(TE)and swirling flow(SF)to synchronously enhance bulk mass transfer and promote interfacial ion *** investigated the effects of the operation mode,transient frequency,and flow rate on metal recovery,enabling determination of the optimal operating conditions for rapid and efficient sequential recovery of Cu in TE&SF *** conditions included low and high electric levels of 0 and 4 V,a 50%duty cycle,1 kHz frequency,and 400 L·h^(-1)flow *** kinetic coefficients of TE&SF electrodeposition were 3.5-4.3 and 1.37-1.97 times that of single TE and SF electrodeposition,*** the deposition process under TE and SF conditions confirmed the efficient concurrence of interfacial ion transport and charge transfer under TE and SF synergy,which achieved rapid and highquality metal ***,the combined deposition strategy is considered an effective technique for reducing metal pollution and promoting resource recycling.

关键词： Ion transport Reaction kinetics Transient electric field Swirling flow

来源：评论

学校读者我要写书评

暂无评论

Review of technologies and their applications for the speciated detection of RO2 radicals

引用

Journal of Environmental Sciences 2023年第1期123卷 487-499页

作者： Yue Gao Keding Lu Yuanhang Zhang State Key Joint Laboratory of Environmental Simulation and Pollution Control State Environmental Protection Key Laboratory of Atmospheric Ozone Pollution ControlCollege of Environmental Sciences and EngineeringPeking UniversityBeijing 100871China

Peroxy radicals(RO_(2)),which are formed during the oxidation of volatile organic compounds,play an important role in atmospheric oxidation ***,the measurement of RO_(2),especially distinct species of RO_(2)radicals,is important and greatly helps the exploration of atmospheric chemistry *** the speciated detection of RO_(2)radicals remains challenging,various methods have been developed to study them in *** methods can be divided into spectroscopy and mass spectrometry *** spectroscopy methods contain laser-induced fluorescence(LIF),UV-absorption spectroscopy,cavity ring-down spectroscopy(CRDS)and matrix isolation and electron spin resonance(MIESR).The mass spectrometry methods contain chemical ionization atmospheric pressure interface time-of-flight mass spectrometry(CI-APi-TOF),chemical ionization mass spectrometry(CIMS),CI-Orbitrap-MS and the third-generation proton transfer reaction-time-of-flight mass spectrometer(PTR3).This article reviews technologies for the speciated detection of RO_(2)radicals and the applications of these *** addition,a comparison of these techniques and the reaction mechanisms of some key species are ***,possible gaps are proposed that could be filled by future research into speciated RO_(2)radicals.

关键词： Speciated RO_(2)radicals Atmospheric chemistry Reaction mechanisms Mass spectrometry

来源：评论

学校读者我要写书评

暂无评论

建议与咨询留下您的常用邮箱和电话号码，以便我们向您反馈解决方案和替代方法

时间限定

文献类型

馆藏选择

核心期刊

语言

文献类型

帮助

文字说明：

检索规则说明：

检索范例：

分类表

所选分类

限定检索结果

文献类型

馆藏范围

日期分布

学科分类号

主题

机构

作者

语言

请选择保存的检索档案：

请选择收藏分类：

通借通还

建议与咨询 留下您的常用邮箱和电话号码，以便我们向您反馈解决方案和替代方法

时间限定

文献类型

馆藏选择

核心期刊

语言

文献类型

帮助

文字说明：

检索规则说明：

检索范例：

分类表

所选分类

限定检索结果

文献类型

馆藏范围

日期分布

学科分类号

主题

机构

作者

语言

请选择保存的检索档案： 新增检索档案 确定 取消

请选择收藏分类： 新增自定义分类 确定 取消

通借通还

建议与咨询留下您的常用邮箱和电话号码，以便我们向您反馈解决方案和替代方法

请选择保存的检索档案：

请选择收藏分类：