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Artificial intelligence for geoscience:Progress,challenges,and perspectives

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The Innovation 2024年第5期5卷 136-160,135页

作者： Tianjie Zhao Sheng Wang Chaojun Ouyang Min Chen Chenying Liu Jin Zhang Long Yu Fei Wang Yong Xie Jun Li Fang Wang Sabine Grunwald Bryan MWong Fan Zhang Zhen Qian Yongjun Xu Chengqing Yu Wei Han Tao Sun Zezhi Shao Tangwen Qian Zhao Chen Jiangyuan Zeng Huai Zhang Husi Letu Bing Zhang Li Wang Lei Luo Chong Shi Hongjun Su Hongsheng Zhang Shuai Yin Ni Huang Wei Zhao Nan Li Chaolei Zheng Yang Zhou Changping Huang Defeng Feng Qingsong Xu Yan Wu Danfeng Hong Zhenyu Wang Yinyi Lin Tangtang Zhang Prashant Kumar Antonio Plaza Jocelyn Chanussot Jiabao Zhang Jiancheng Shi Lizhe Wang Aerospace Information Research Institute Chinese Academy of SciencesBeijing 100094China School of Computer Science China University of GeosciencesWuhan 430078China State Key Laboratory of Mountain Hazards and Engineering Resilience Institute of Mountain Hazards and EnvironmentChinese Academy of SciencesChengdu 610299China Key Laboratory of Virtual Geographic Environment(Ministry of Education of PRC) Nanjing Normal UniversityNanjing 210023China Data Science in Earth Observation Technical University of Munich80333 MunichGermany The National Key Laboratory of Water Disaster Prevention Yangtze Institute for Conservation and DevelopmentHohai UniversityNanjing 210098China Institute of Computing Technology Chinese Academy of SciencesBeijing 100190China School of Geographical Sciences Nanjing University of Information Science and TechnologyNanjing 210044China State Key Laboratory of Soil and Sustainable Agriculture Institute of Soil ScienceChinese Academy of SciencesNanjing 210008China Soil Water and Ecosystem Sciences DepartmentUniversity of FloridaPO Box 110290GainesvilleFLUSA Materials Science Engineering Program Cooperating Faculty Member in the Department of Chemistry and Department of Physics Astronomy University of CaliforniaCaliforniaRiversideCA 92521USA Institute of Remote Sensing and Geographical Information System School of Earth and Space SciencesPeking UniversityBeijing 100871China Key Laboratory of Computational Geodynamics University of Chinese Academy of SciencesBeijing 100049China International Research Center of Big Data for Sustainable Development Goals Beijing 100094China College of Geography and Remote Sensing Hohai UniversityNanjing 211100China Department of Geography The University of Hong KongHong Kong 999077SARChina Jiangsu Key Laboratory of Atmospheric Environment Monitoring and Pollution Control Nanjing 210044China School of Environmental Science and Engineering Nanjing University of Information Science&TechnologyNanjing 210044China Collaborative Inno

This paper explores the evolution of geoscientific inquiry,tracing the progression from traditional physics-based models to modern data-driven approaches facilitated by significant advancements in artificial intelligence(AI)and data collection *** models,which are grounded in physical and numerical frameworks,provide robust explanations by explicitly reconstructing underlying physical ***,their limitations in comprehensively capturing Earth’s complexities and uncertainties pose challenges in optimization and real-world *** contrast,contemporary data-driven models,particularly those utilizing machine learning(ML)and deep learning(DL),leverage extensive geoscience data to glean insights without requiring exhaustive theoretical *** techniques have shown promise in addressing Earth science-related ***,challenges such as data scarcity,computational demands,data privacy concerns,and the“black-box”nature of AI models hinder their seamless integration into *** integration of physics-based and data-driven methodologies into hybrid models presents an alternative *** models,which incorporate domain knowledge to guide AI methodologies,demonstrate enhanced efficiency and performance with reduced training data *** review provides a comprehensive overview of geoscientific research paradigms,emphasizing untapped opportunities at the intersection of advanced AI techniques and *** examines major methodologies,showcases advances in large-scale models,and discusses the challenges and prospects that will shape the future landscape of AI in *** paper outlines a dynamic field ripe with possibilities,poised to unlock new understandings of Earth’s complexities and further advance geoscience exploration.

关键词： Earth utilizing landscape

Formation of Robust Cei Film on High Voltage Lini0.6co0.2mn0.2o2 Cathode Enabled by Functional [Pivm][Tfsa] Ionic Liquid Additive

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SSRN 2022年

作者： Cai, Yingjun Xu, Tinghua Meng, Xianglei von Solms, Nicolas Zhang, Haitao Thomsen, Kaj Department of Chemical and Biochemical Engineering Technical University of Denmark Søltofts Plads Kgs. Lyngby 2800 Denmark Beijing Key Laboratory of Ionic Liquids Clean Process CAS Key Laboratory of Green Process and Engineering State Key Laboratory of Multiphase Complex Systems Institute of Process Engineering Chinese Academy of Sciences Beijing100190 China

The ionic liquid 1-(3-amino-3-oxopropyl)-3-vinylimidazolium bis(trifluoromethylsulfonyl)amide ([PIVM][TFSA]) was synthesized and applied in the electrolyte of Li/LiNi 0.6 Co 0.2 Mn 0.2 O 2 lithium ion batteries. The thermostability of this pure ionic liquid was investigated to provide a wide liquid range from -50 °C to 200 °C. The physicochemical properties of binary mixtures of this ionic liquid with DMC and EMC were measured at different temperatures and with different ionic liquid mole fractions. [PIVM][TFSA] widens the electrochemical window of the electrolyte. The ionic liquid inhibits the increasing of water and HF content in the electrolyte. A comparison of charge and discharge performances in different electrolytes with various content of ionic liquid is reported. The electrolyte with the concentration of 1.0 wt % [PIVM][TFSA] has the best electrochemical properties. It enhances the initial capacity, the capacity retention and the high current rate performance of the cells. The surface film on the electrodes was confirmed by SEM and XPS that the ionic liquid [PIVM][TFSA] participated in membrane formation and played an active role. © 2022, The Authors. All rights reserved.

关键词： Electrolytes

Strategic Design of High-Directional Scaffold Enabling Accelerated Kinetics for High-Loading Low-Temperature Lithium-Sulfur Batteries

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SSRN 2025年

作者： Shi, Junye Yu, Chenxi Ning, Yuchen Li, Bao Wang, Bao Zheng, Shumin Institute of Refrigeration and Cryogenics Shanghai Jiao Tong University Shanghai200433 China State Key Laboratory of Biochemical Engineering Institute of Process Engineering Chinese Academy of Sciences Beijing100190 China Key Laboratory of Biopharmaceutical Preparation and Delivery Chinese Academy of Sciences Beijing100190 China School of Chemistry and Chemical Engineering Henan Normal University Xinxiang453007 China College of Chemistry and Materials Jiangxi Agricultural University Nanchang330045 China

Electronic market starves for efficient batteries at low temperatures. Herein, a free-standing and highly directional scaffold filled with NiCo-decorated carbon nanotube bushes (HDS-NCCNT) is synthesized and employed as a three-dimensional thick host for low-temperature lithium-sulfur (Li-S) batteries. This unique structure can ensure the high loading of active material and improve the sluggish reaction kinetics at low temperatures. The NCCNT bushes can further suppress the shuttle effect of lithium polysulfides and prolong the lifespan. As a result, the Li2S6@HDS-NCCNT cathode with a loading mass of 5 mg cm-2 exhibits a remarkable capacity of 1026 mAh g-1 at 0.1 C under -20 ℃. Even under -40 ℃, the Li2S6@HDS-NCCNT cathode also shows favorable performance with a high sulfur loading of 10 mg cm-2. This pioneering work demonstrates the rational design of components and architectures ranging from micrometer to nanometer scale, which inspires the development of high-loading Li-S batteries under cryogenic conditions. © 2025, The Authors. All rights reserved.

关键词： Lithium sulfur batteries

Desorption of VOC from polymer adsorbent in multistage fluidized bed

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Chinese Journal of Chemical engineering 2020年第6期28卷 1709-1716页

作者： Jiale Zheng Wenli Song Lin Du Lina Wang Songgeng Li State Key Laboratory of Multiphase Complex Systems Institute of Process EngineeringChinese Academy of SciencesBeijing 100190China University of Chinese Academy of Sciences Beijing 100049China

The desorption process of volatile organic compounds(VOC)from a polymer adsorbent in counter-current multistage fluidized bed was *** a mathematical model considering the mass transfer dynamics was developed,which was validated from experiment *** gaseous ethyl acetate mass transfer was discussed,and the limiting step is the intraparticle mass transfer of the desorption *** value of intraparticle mass transfer coefficient is between 1.85×10-6 and 1.38×10-5 m·s-1 under temperature of 100–160°*** under different operating conditions were carried *** effects of operating conditions such as gas–solid flow ratio,gas inlet temperature and total stage number of multistage fluidized bed on outlet VOCs concentration and desorption efficiency were *** maximum outlet VOCs concentration and corresponding desorption efficiency of the multistage fluidized bed desorber was calculated under different gas inlet temperatures and total stage numbers.

关键词： VOC Desorption Mass transfer Fluidized bed

Targeted inhibition of osteoclastogenesis reveals the pathogenesis and therapeutics of bone loss under sympathetic neurostress

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International Journal of Oral Science 2022年第4期14卷 479-488页

作者： Bingdong Sui Jin Liu Chenxi Zheng Lei Dang Ji Chen Yuan Cao Kaichao Zhang Lu Liu Minyan Dang Liqiang Zhang Nan Chen Tao He Kun Xuan Fang Jin Ge Zhang Yan Jin Chenghu Hu State Key Laboratory of Military Stomatology and National Clinical Research Center for Oral Diseases and Shaanxi International Joint Research Center for Oral Diseases Center for Tissue EngineeringSchool of StomatologyThe Fourth Military Medical UniversityXi'anChina Law Sau Fai Institute for Advancing Translational Medicine in Bone and Joint Diseases School of Chinese MedicineHong Kong Baptist UniversityHong Kong SARChina Xi'an Key Laboratory of Stem Cell and Regenerative Medicine Institute of Medical ResearchNorthwestern Polytechnical UniversityXianChina Xi'an Institute of Tssue Engineering and Regenerative Medicine XianChina Department of Biochemistry and Molecular Biology School of Basic Medical SciencesXi'an Jiaotong UniversityXi'anChina

Sympathetic cues via the adrenergic signaling critically regulate bone homeostasis and contribute to neurostress-induced bone loss,but the mechanisms and therapeutics remain incompletely ***,we reveal an osteoclastogenesis-centered functionally important osteopenic pathogenesis under sympatho-adrenergic activation with characterized micro RNA response and efficient *** discovered that osteoclastic mi R-21 was tightly regulated by sympatho-adrenergic cues downstream theβ2-adrenergic receptor(β2AR)signaling,critically modulated osteoclastogenesis in vivo by inhibiting programmed cell death 4(Pdcd4),and mediated detrimental effects of both isoproterenol(ISO)and chronic variable stress(CVS)on ***,without affecting osteoblastic bone formation,bone protection against ISO and CVS was sufficiently achieved by a(D-Asp8)-lipid nanoparticle-mediated targeted inhibition of osteoclastic mi R-21 or by clinically relevant drugs to suppress ***,these results unravel a previously underdetermined molecular and functional paradigm that osteoclastogenesis crucially contributes to sympatho-adrenergic regulation of bone and establish multiple targeted therapeutic strategies to counteract osteopenias under stresses.

关键词： osteoclast pathogenesis homeostasis

Simultaneously Enhanced Gas Separation Performance and Long-Term Stability by Thermally Treated Zif-8-Based Nanocomposite Membranes

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SSRN 2024年

作者： Li, Kaihua Ma, Yuchao Zhao, Wei Yang, Leixin Zhang, Jinwei Zhang, Qian Xiaohua, Ma Jiao, Long Yin, Zhen Cheng, Bowen State Key Laboratory of Biobased Fiber Manufacturing Technology Tianjin University of Science & Technology Tianjin300457 China College of Chemical Engineering and Materials Science Tianjin University of Science & Technology Tianjin300457 China College of Light Industry Science and Engineering Tianjin University of Science & Technology Tianjin300457 China SINOPEC Research Institute of Petroleum Processing State Key Laboratory of Petroleum Molecular & Process Engineering Beijing100083 China School of Materials Science and Engineering State Key Laboratory of Separation Membranes and Membrane Processes Tiangong University Tianjin300387 China

The challenges of trade-off effect and long-term stability pose huge obstacles in the application of polymer-based gas separation membranes. In this study, we proposed a novel strategy to overcome these problems by in-situ thermally treating ZIF-8/polyimide mixed-matrix membranes (MMMs) at 300 oC. After thermally treatment, the T-ZIF-8 produced some unsaturated Zn site as defects that decreased BET surface area and the shrunk of micropore size as compared with *** MMMs with T-ZIF-8 significantly affects their gas separation performance and long-term stability, in which, the H2/CH4 and CO2/CH4 separation performance of T-ZIF-8/PI(3:10) and T-ZIF-8/PI(6:10) increased from far below the 2008 trade off lines for their PI matrix to approach or even above ***, both higher permeability and selectivity were observed for T-ZIF-8/PI(6:10) as compared with its precursor for H2/CH4 separation, which was contributed by its higher H2 diffusion coefficient (3834 vs 580 ×10-8 cm2 s-1) and H2/CH4 diffusion selectivity (240 vs 154). Furthermore, the T-ZIF-8/PI (1:10) and T-ZIF-8/PI(3:10) MMMs demonstrate less than 15% H2 decreasing after 150 days, which is much better than that of the pristine PI membrane (26.7%). These results probably contributed by the defected ZIF-8 loading induced extra ultra-micropore that caused size sieving effect and strong interaction with polyimide matrix that formed more rigid polymer chains. These findings propose a strategy to effectively enhance the gas separation performance and long-term stability by in-situ introducing the defect MOF in the polymer matrix. © 2024, The Authors. All rights reserved.

关键词： Economic and social effects

PRMT6 promotes tumorigenicity and cisplatin response of lung cancer through triggering 6PGD/ENO1 mediated cell metabolism

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Acta Pharmaceutica Sinica B 2023年第1期13卷 157-173页

作者： Mingming Sun Leilei Li Yujia Niu Yingzhi Wang Qi Yan Fei Xie Yaya Qiao Jiaqi Song Huanran Sun Zhen Li Sizhen Lai Hongkai Chang Han Zhang Jiyan Wang Chenxin Yang Huifang Zhao Junzhen Tan Yanping Li Shuangping Liu Bin Lu Min Liu Guangyao Kong Yujun Zhao Chunze Zhang Shu-Hai Lin Cheng Luo Shuai Zhang Changliang Shan State Key Laboratory of Medicinal Chemical Biology College of Pharmacy and Tianjin Key Laboratory of Molecular Drug ResearchNankai UniversityTianjin 300350China Biomedical Translational Research Institute Jinan UniversityGuangzhou 510632China State Key Laboratory of Cellular Stress Biology Innovation Center for Cell Signaling NetworkSchool of Life SciencesXiamen UniversityXiamen 361102China School of Integrative Medicine Tianjin University of Traditional Chinese MedicineTianjin 301617China Department of Pathology and Institute of Precision Medicine Jining Medical UniversityJining 272067China Department of Pathology Medical SchoolDalian UniversityDalian 116622China Department of Biochemistry and Molecular Biology School of Basic Medical SciencesHengyang Medical SchoolUniversity of South ChinaHengyang 421001China School of Laboratory Medicine and Life Sciences Wenzhou Medical UniversityWenzhou 325035China Institute of Biomedical Sciences Shandong Provincial Key Laboratory of Animal Resistance BiologyCollaborative Innovation Center of Cell Biology in Universities of ShandongCollege of Life SciencesShandong Normal UniversityJinan 250014China National Local Joint Engineering Research Center of Biodiagnostics and Biotherapy the Second Affiliated Hospital of Xi'an Jiaotong UniversityXi'an 710004China State Key Laboratory of Drug Research Shanghai Institute of Materia MedicaChinese Academy of SciencesShanghai 201203China Department of Colorectal Surgery Tianjin Union Medical Center Nankai UniversityTianjin 300121China

Metabolic reprogramming is a hallmark of cancer,including lung ***,the exact underlying mechanism and therapeutic potential are largely *** we report that protein arginine methyltransferase 6(PRMT6)is highly expressed in lung cancer and is required for cell metabolism,tumorigenicity,and cisplatin response of lung ***6 regulated the oxidative pentose phosphate pathway(PPP)flux and glycolysis pathway in human lung cancer by increasing the activity of 6-phosphogluconate dehydrogenase(6PGD)and a-enolase(ENO1).Furthermore,PRMT6 methylated R324 of 6PGD to enhancing its activity;while methylation at R9 and R372 of ENO1 promotes formation of active ENO1 dimers and 2-phosphoglycerate(2-PG)binding to ENO1,***,targeting PRMT6 blocked the oxidative PPP flux,glycolysis pathway,and tumor growth,as well as enhanced the antitumor effects of cisplatin in lung ***,this study demonstrates that PRMT6 acts as a posttranslational modification(PTM)regulator of glucose metabolism,which leads to the pathogenesis of lung *** was proven that the PRMT6-6PGD/ENO1 regulatory axis is an important determinant of carcinogenesis and may become a promising cancer therapeutic strategy.

关键词： Lung cancer Metabolic reprogramming Post-translational modification PRMT6 Pentose phosphate pathway flux Glycolysis 6-Phospho-gluconate dehydrogenase a-enolase ENO1

Immobilizing ultrafine bimetallic PtAg alloy onto uniform MnO_(2) microsphere as a highly active catalyst for CO oxidation

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Chinese Chemical Letters 2021年第6期32卷 2057-2060页

作者： Shengpeng Mo Peng Peng Yinchang Pei Taiming Shen Qinglin Xie Mingli Fu Yunfa Chen Daiqi Ye College of Environment Science and Engineering Guilin University of TechnologyGuilin 541004China School of Environment and Energy South China University of TechnologyGuangzhou 510006China Guangxi Key Laboratory of Theory and Technology for Environmental Pollution Control Guilin University of TechnologyGuilin 541004China State Key Laboratory of Multi-Phase Complex Systems Institute of Process EngineeringChinese Academy of SciencesBeijing 100190China

Herein,a facile glycol reduction route is successful employed to synthesize bimetallic Pt Ag alloys with homogeneous distribution of sizes and *** studies reveal that the ultrafine Pt Ag alloys with well-defined sizes from around 3.3 nm to 5.8 nm are immobilized onto MnO_(2)microsphere,which remarkably enhances the catalytic performances for CO ***,quasi in-situ X-ray photoelectron spectroscopy(XPS)result reveals that both Mn and Pt ions on the surface of catalysts would realize alternating reduction-oxidation by CO and O_(2)molecules,and the oxygen vacancy sites could be replenished and excited by gas-phase O_(2).

关键词： Bimetallic alloys PtAg NPs MnO_(2) Quasi in-situ XPS CO oxidation

Unraveling the Effect of Sorbitol on Cu-Based Catalysts for the Continuous Hydrogenation of Co2-Derived Ethylene Carbonate to Methanol and Ethylene Glycol

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SSRN 2025年

作者： Song, Tong-Yang Zhang, Ji-Zheng Chen, Xian-Lang Huang, Xin-Yuan Jia, Ai-Ping Li, Xiaohong Li, Rong-Rong Lu, Ji-Qing Key Laboratory of the Ministry of Education for Advanced Catalysis Materials Zhejiang Key Laboratory for Reactive Chemistry on Solid Surfaces Institute of Physical Chemistry Zhejiang Normal University Jinhua321004 China Engineering Research Center of Recycling & Comprehensive Utilization of Pharmaceutical and Chemical Waste of Zhejiang Province School of Pharmaceutical and Chemical Engineering Taizhou University Zhejiang Taizhou318000 China State Key Laboratory of Petroleum Molecular & Process Engineering Shanghai Key Laboratory of Green Chemistry and Chemical Processes ECNU Engineering Center for Sustainable Carbon School of Chemistry and Molecular Engineering East China Normal University Shanghai200062 China Zhejiang Normal University China

The hydrogenation of ethylene carbonate (EC) is a crucial step in the indirect transformation of CO2 into methanol (MeOH) and ethylene glycol (EG) over Cu-based catalysts. In this work, a series of sorbitol-modified Cu/SiO2 catalyst were prepared and tested for continuous hydrogenation of EC. As a result, the MeOH selectivity displayed a volcano-like trend with the sorbitol/Cu molar ratios. The optimized Cu@0.04Cs/SiO2 catalyst exhibited excellent MeOH selectivity (91.4%) and EG selectivity (99.6%) at an EC conversion of 99.9%. The results showed that copper-sorbitol complexes were preferentially formed, which could restrict the formation of copper phyllosilicate. However, a strong electronic interaction between copper and carbon, as confirmed by multiple characterizations, which may lead to possible formation of Cu-O-C bond located on the periphery of copper and carbon interface. This interfacial effect not only reduces the activation energy but also effectively enhances the Cu+/(Cu0 + Cu+) ratios, and thus improves the selectivity to MeOH. Furthermore, according to DFT calculation and kinetic study results, the interface between copper and carbon serves as active sites to facilitate the adsorption of H2 and EC, resulting in reduced activation energy. © 2025, The Authors. All rights reserved.

关键词： Activation energy