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Design of Ultra-Stable Solid Amine Adsorbents and Mechanisms of Hydroxyl Group-Dependent Deactivation for Reversible CO2 Capture from Flue Gas

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Nano-Micro Letters 2025年第7期17卷 363-381页

作者： Meng Zhao Liang Huang Yanshan Gao Ziling Wang Shuyu Liang Xuancan Zhu Qiang Wang Hong He Dermot O'Hare College of Environmental Science and Engineering Beijing Forestry University State Key Laboratory of Efficient Production of Forest Resources Beijing Forestry University Research Center of Solar Power and Refrigeration Institute of Refrigeration and CryogenicsShanghai Jiao Tong University State Key Joint Laboratory of Environment Simulation and Pollution Control Research Centre for Eco-Environmental SciencesChinese Academy of Sciences Chemistry Research Laboratory Department of ChemistryUniversity of Oxford

Although supported solid amine adsorbents have attracted great attention for CO2capture,critical chemical deactivation problems including oxidative degradation and urea formation have severely restricted their practical applications for flue gas *** this work,we reveal that the nature of surface hydroxyl groups （metal hydroxyl Al–OH and nonmetal hydroxyl Si–OH） plays a key role in the deactivation *** polyethyleneimine （PEI） supported on Al–OH-containing substrates suffers from severe oxidative degradation during the CO2capture step due to the breakage of amine-support hydrogen bonding networks,but exhibits an excellent anti-urea formation feature by preventing dehydration of carbamate products under a pure CO2regeneration *** contrast,PEI supported on Si–OH-containing substrates exhibits excellent anti-oxidative stability under simulated flue gas conditions by forming a robust hydrogen bonding protective network with Si–OH,but suffers from obvi- ous urea formation during the pure CO2regeneration *** also reveal that the urea formation problem for PEI-SBA-15 can be avoided by the incorporation of an OH-containing PEG *** on the intrinsic understanding of degradation mechanisms,we successfully synthesized an adsorbent 40PEI-20PEG-SBA-15 that demonstrates outstanding stability and retention of a high CO2capacity of 2.45 mmol g-1over 1000 adsorption–desorption cycles,together with negligible capacity loss during aging in simulated flue gas （10%CO2+5%O2+3%H2O） for one month at60–70℃.We believe this work makes great contribution to the advancement in the field of ultra-stable solid amine-based CO2capture materials.

关键词： CO2 capture Long-term stability Oxidative degradation Solid amine adsorbent Urea formation

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A Noise-Excitation Generative Adversarial Network for Actuator Fault Diagnosis of Multi-legged Robot

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无人系统（英文） 2023年第2期11卷 159-173页

作者： Liling Ma Jian Guo Jiehao Li Junzheng Wang State Key Laboratory of Complex System Intelligent Control and Decision School of Automation Beijing Institute of TechnologyBeijing 100081P.R.China

This research provides a novel approach for detecting multi-legged robot actuator *** most significant concept is to design the Fault Diagnosis Generative Adversarial Network(FD-GAN)to fully adapt to the fault diagnosis problem with insufficient *** found that it is difficult for methods based on classification and prediction to learn failure patterns without enough data.A straightforward solution is to use massive amounts of normal data to drive the diagnostic *** introduce frequency-domain information and fuse multi-sensor data to increase the features and expand the difference between normal data and fault data.A GAN-based framework is designed to calculate the probability that the enhanced data belongs to the normal *** uses a generator network as a feature extractor,and uses a discriminator network as a fault probability evaluator,which creates a new use of GAN in the field of fault *** the many learning strategies of GAN,we find that a key point that can distinguish the two types of data is to use the hidden layer noise with appropriate discrimination as the *** also design a fault location method based on binary search,which greatly improves the search efficiency and engineering value of the entire *** have conducted a lot of experiments to prove the diagnostic effectiveness of our architecture in various road conditions and working *** compared FD-GAN with popular diagnostic *** results show that our method has the highest accuracy and recall rate.

关键词： Actuator fault diagnosis multi-legged robot generative adversarial network attention mechanism

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Characterizing permeability-porosity relationships of porous rocks using a stress sensitivity model in consideration of elastic-structural deformation and tortuosity sensitivity

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Journal of Rock Mechanics and Geotechnical Engineering 2024年第9期16卷 3437-3451页

作者： Ronghe Xu Liqin Wang Xiaoli Zhao Yuze Mao MIIT Key Laboratory of Aerospace Bearing Technology and Equipment Harbin Institute of TechnologyHarbin150001China State Key Laboratory of Robotics and System Harbin Institute of TechnologyHarbin150001China Shanghai Aerospace Control Technology Institute Shanghai201100China

Clarifying the relationship between stress sensitivities of permeability and porosity is of great significance in guiding underground resource *** and more studies focus on how to construct stress sensitivity models to describe the relationship and obtain a comprehensive stress sensitivity of porous ***,the limitations of elastic deformation calculation and incompleteness of considered tortuosity sensitivity lead to the fact that the existing stress sensitivity models are still unsatisfactory in terms of accuracy and ***,a more accurate and generic stress sensitivity model considering elastic-structural deformation of capillary cross-section and tortuosity sensitivity is proposed in this *** elastic deformation is derived from the fractal scaling model and Hooke's *** the effects of elastic-structural deformation on tortuosity sensitivity,an empirical formula is proposed,and the conditions for its applicability are *** predictive performance of the proposed model for the permeability-porosity relationships is validated in several sets of publicly available experimental *** experimental data are from different rocks under different pressure *** mean and standard deviation of relative errors of predicted stress sensitivity with respect to experimental data are 2.63%and 1.91%.Compared with other models,the proposed model has higher accuracy and better predictive generalization *** is also found that the porosity sensitivity exponent a,which can describe permeability-porosity relationships,is 2 when only elastic deformation is considered.a decreases from 2 when structural deformation is also *** addition,a may be greater than 3 due to the increase in tortuosity sensitivity when tortuosity sensitivity is considered even if the rock is not fractured.

关键词： Stress sensitivity model Permeability-porosity relationships Elastic-structural deformation Tortuosity stress sensitivity

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An S-scheme artificial photosynthetic system with H-TiO2/g-C3N4 heterojunction coupled with MXene boosts solar H2 evolution

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材料科学技术（英文版） 2025年第8期211卷 22-29页

作者： Depeng Meng Xiaowen Ruan Minghua Xu Dongxu Jiao Guozhen Fang Yu Qiu Yueyang Zhang Haiyan Zhang Sai Kishore Ravi Xiaoqiang Cui State Key Laboratory of Automotive Simulation and Control School of Materials Science and EngineeringKey Laboratory of Automobile Materials of MOEJilin Provincial International Cooperation Key Laboratory of High-Efficiency Clean Energy MaterialsJilin UniversityChangchun 130012China School of Energy and Environment City University of Hong KongTat Chee AvenueKowloonSARHong KongChina

Solar hydrogenproduction via water splitting is pivotal for solar energy harnessing,addressing key challenges in energy and environmental ***,two critical issues persist with single-component photocatalysts:suboptimal carrier transport and inadequate light *** heterojunction-based artificial photosynthetic systems like Z-scheme photocatalysts have been explored,their charge recombination and light harvesting efficiency are still unsatisfactory.S-scheme heterojunc-tions have gained attention in photocatalysis,owing to their pronounced built-in electric field and su-perior redox *** this study,we introduce a MXene-based S-scheme H-TiO2/g-C3N4/Ti3C2 het-erojunction(TCMX),synthesized through electrostatic *** as-prepared TCMX exhibited an excellent photocatalytic hydrogen evolution rate of 53.67 mmol g-1 h-1 surpassing the performance of commercial Rutile TiO2,H-TiO2,g-C3N4,and *** effectiveness of TCMX is largely due to the built-in electric field in the S-scheme heterojunction and the cocatalytic activity of MXene promoting rapid separation of photogenerated charges and resulting in well-separated electron and hole enriched *** study offers a new approach to enhance photocatalytic hydrogen evolution efficiency and paves the way for the future design of S-scheme heterojunctions.

关键词： S-scheme MXene Heterojunction Hydrogen Charge transfer

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Enhancing oxidation reaction over Pt-MnO_(2) catalyst by activation of surface oxygen

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Journal of Environmental Sciences 2023年第12期35卷 117-125页

作者： Ruoting Shan Zhenteng Sheng Shuo Hu Hongfei Xiao Yuhua Zhang Jianghao Zhang Li Wang Changbin Zhang Jinlin Li Key Laboratory of Catalysis and Energy Materials Chemistry of Ministry of Education&Hubei Key Laboratory of Catalysis and Materials Science South-Central Minzu UniversityWuhan 430074China State Key Joint Laboratory of Environment Simulation and Pollution Control Research Center for Eco-environmental SciencesChinese Academy of SciencesBeijing 100085China

Formaldehyde(HCHO) and carbon monoxide(CO) are both common air pollutants and hazardous to human body. It is imperative to develop the catalyst that is able to efficiently remove these pollutants. In this work, we activated Pt-MnO_(2)under different conditions for highly active oxidation of HCHO and CO, and the catalyst activated under CO displayed superior performance. A suite of complementary characterizations revealed that the catalyst activated with CO created the highly dispersed Pt nanoparticles to maintain a more positively charged state of Pt, which appropriately weakens the Mn-O bonding strength in the adjacent region of Pt for efficient supply of active oxygen during the reaction. Compared with other catalysts activated under different conditions, the CO-activated Pt-MnO_(2)displays much higher activity for oxidation of HCHO and CO. This research contributes to elucidating the mechanism for regulating the oxidation activity of Pt-based catalyst.

关键词： Pt/MnO_(2)catalysts HCHO abatement CO abatement Catalytic oxidation Activation of surface oxygen

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A Novel Directional Pilot Protection for Flexible DC Distribution Grid 9

A Novel Directional Pilot Protection for Flexible DC Distrib...

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9th Asia Conference on Power and Electrical Engineering, ACPEE 2024

作者： Wei, Xiuyan Zou, Guibin Shandong University Key Laboratory of Power System Intelligent Dispatch and Control of Ministry of Education Ji'nan250061 China Northeast Electric Power University Key Laboratory of Modern Power System Simulation and Control & Renewable Energy Technology Ministry of Education Jilin132012 China

ISBN: (纸本)9798350309638

The existing directional pilot protection (DPP) is susceptible to the line distributed capacitance and the fault resistance, and mostly rely on the current limiting reactance (CLR) at the line ends. To solve the above problems, the line-mode fault component power (LFCP) based DPP is proposed for flexible DC distribution grid (FDCDG). First, the characters of LFCP are discussed under different faults. The theoretical analysis show that the polarity of the LFCP under internal fault is same, while the polarity of the LFCP is opposite under external fault. Then, the LFCP is built as the directional criterion, and the corresponding protection scheme is constructed. The electromagnetic transient simulations of the PSCAD/EMTDC verify that the proposed DPP is less affected by the noise, and has low requirement on the sampling rate, strong engineering applicability. © 2024 IEEE.

关键词： Electric power distribution

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Harmonic state-Space Based AC-Side Impedance Model of MMC and High Frequency Oscillation Characteristics Analysis

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Energy Engineering 2023年第4期120卷 831-849页

作者： Hui Fang Jingsen Zhou Haozheng Wang Yanxu Wang Hongji Xiang Yechun Xin State Grid Chongqing Electric Power Company Research Institute Chongqing401120China Key Laboratory of Modern Power System Simulation and Control&Renewable Energy Technology(Northeast Electric Power University) Jilin132012China

Recently,high-frequency oscillation of themodularmultilevel converter(MMC)based high-voltage direct current(HVDC)projects has attracted great *** order to analyze the small-signal stability,this paper uses the harmonic state-space(HSS)method to establish a detailed frequency domain impedance model of the AC-side of the HVDC transmission system,which considers the internal dynamic *** addition,the suggested model is also used to assess the system’s high-frequency oscillationmechanism,and the effects of the MMC current inner loop control,feedforward voltage links,and control delay on the high-frequency impedance characteristics and the effect of higher harmonic ***,three oscillation suppression schemes are analyzed for the oscillation problems occurring in actual engineering,and a simplified impedance model considering only the highfrequency impedance characteristics is established to compare the suppression effect with the detailed impedance model to prove its reliability.

关键词： Modular multilevel converter impedance modeling small-signal stability suppression strategy

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A Study of Nanosecond Clock Synchronization Methods for Real-Time Transient simulation 6

A Study of Nanosecond Clock Synchronization Methods for Real...

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6th International Conference on Communications, Information system and Computer Engineering, CISCE 2024

作者： Guo, Qi Lu, Yuanhong Zhang, Jingyue Zhang, Jie Guo, Haiping Hu, Binjiang Electric Power Research Institute China Southern Power Grid State Key Laboratory of HVDC China Guangdong Provincial Key Laboratory of Intelligent Operation and Control for New Energy Power System China Electric Power Research Institute China Southern Power Grid Csg Key Laboratory for Power System Simulation Guangdong China

ISBN: (纸本)9798350353174

Conventional nanosecond clock synchronization protocols are generally target-type or content-type, the synchronization rate is low, which leads to the increasing of the mean value difference of synchronization, so we propose to study the design of nanosecond clock synchronization method for real-time transient simulation. Combined with the actual clock synchronization requirements, we first calculate the link congestion coefficient, adopt a multilevel approach to strengthen the synchronization rate, set up a multilevel clock synchronization protocol, based on which we determine the clock source quality coefficients and construct a nanosecond clock synchronization model for real-time transient simulation, and use redundancy processing to achieve clock synchronization. The test results show that compared with the high-efficiency phase-color clock synchronization method and the cross-clock synchronization method, the mean synchronization difference of the designed transient simulation nanosecond clock synchronization method is controlled to be less than 0.5, which indicates that the designed clock synchronization method is more efficient, stable, and targeted, and the synchronization effect is significantly improved. © 2024 IEEE.

关键词： Mechanical clocks

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A Mode-Switching Soot Load Observer for Automotive Particulate Filters 7

A Mode-Switching Soot Load Observer for Automotive Particula...

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7th CAA International Conference on Vehicular control and Intelligence, CVCI 2023

作者： Lin, Xiangxue Hu, Yunfeng Jiang, Linlin Gong, Xun Sun, Yao State Key Laboratory of Automotive Simulation and Control College of Telecommunications Engineering Jilin University Changchun China FAW-Volkswagen Technology Center Changchun China State Key Laboratory of Automotive Simulation and Control College of Artificial Intelligence Jilin University Changchun China State Key Laboratory of Automotive Simulation and Control College of Automotive Engineering Jilin University Changchun China

ISBN: (纸本)9798350340488

In automotive particulate filter applications, accurate real-time soot load is critical to filter regeneration, which significantly affects vehicle safety and economics. Based on the modified soot accumulation and filter pressure drop characteristics, equations of state and measurement have been deduced, and a corresponding novel Luenberger observer is developed. Due to the limitations of the differential pressure sensor, the deviation of its measurement value is small at small exhaust flow rates and can not reflect the soot load. To figure out this issue, a mode-switching strategy is proposed to schedule the correction gain according to the exhaust flow rate. A co-simulation platform has been built to validate the observer, which adopts GT-Power as the test vehicle. Compared with the open-loop observer under single and multiple NEDC cycles, the mode-switching observer shows some improvement, and the maximum deviation is reduced from 0.58g/L to 0.1g/L. Thus, by reducing the times of regenerations, fuel consumption can be saved about 8%. Finally, the proposed observer shows better robustness when a disturbance occurs, the maximum deviation still maintain a low level of about 0.25g/L. © 2023 IEEE.

关键词： Luenberger observer Mode-switching Particulate filter Soot accumulation and regeneration soot load Transient cycle validation

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control, Modeling and Stability Analysis of DRU-based Grid-forming Converter

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Chinese Journal of Electrical Engineering 2025年第1期11卷 83-92页

作者： Wencong Wu Minzhi Wang Liang Tu Haiqing Cai Guanglei Yan Xiaohui Qu Haohan Gu Wei Chen State Key Laboratory of HVDC China Southern Power GridGuangzhou 510663China National Energy Power Grid Technology R&D Center Guangzhou 510663China Guangdong Provincial Key Laboratory of Intelligent Operation and Control for New Energy Power Systems China Southern Power GridGuangzhou 510663China CSG Key Laboratory for Power System Simulation China Southern Power GridGuangzhou 510663China School of Electrical Engineering Southeast UniversityNanjing 210096China

Diode rectifier unit(DRU)-based high-voltage direct current(HVDC)transmissionsystems areeffectivein achieving the stableandeconomical operation of offshore *** theuncontrollable characteristicsof DRUs,a grid-forming(GFM)strategy forwind-turbine converters isnecessary to support offshore AC voltageand ***,the active power-synchronization control in traditional GFM converters is unsuitable for DRU-based GFM ***,the stability issue for DRU-based HVDC systems involving DRU-based GFM and grid-following(GFL)converters has not yet been *** solve these issues,this study begins with the characteristics of a DRU-based HVDC system and presents a control scheme for DRU-based GFM converters for power ***,the dq-frame impedance model of the DRU-based GFM converteris proposed for the stability analysis of the entire HVDC ***,a simulation platform is built to verify the model accuracy and system stability.

关键词： Diode rectifier unit offshore wind-powergeneration grid-forming converter impedance model stabilityanalysis

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