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Mixing regime shapes the community assembly process,microbial interaction and proliferation of cyanobacterial species Planktothrix in a stratified lake

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Journal of environmental Sciences 2022年第5期34卷 103-113页

作者： Junwen Chen Huacong Liu Yaohui Bai Jing Qi Weixiao Qi Huijuan Liu Jianfeng Peng Jiuhui Qu Center for Water and Ecology State Key Joint Laboratory of Environment Simulation and Pollution ControlSchool of EnvironmentTsinghua UniversityBeijing 100084China Key Laboratory of Drinking Water Science and Technology Research Center for Eco-Environmental SciencesChinese Academy of SciencesBeijing 100085China

Lake mixing influences aquatic chemical properties and microbial community composition,and thus,we hypothesized that it would alter microbial community assembly and *** clarify this issue,we explored the community assembly processes and cooccurrence networks in four seasons at two depths(epilimnion and hypolimnion)in a mesotrophic and stratified lake(Chenghai Lake),which formed stratification in the summer and turnover in the *** the stratification period,the epilimnion and hypolimnion went through contrary assembly processes but converged to similar assembly patterns in the mixing *** a highly homogeneous selection environment,species with low niche breadth were filtered,resulting in decreased species *** mixing in the winter homogenized the environment,resulting in a simpler microbial cooccurrence ***,we observed a high abundance of the cyanobacterial genus Planktothrix in the winter,proba-bly due to nutrient redistribution and Planktothrix adaptivity to the winter environment in which mixing played important *** study provides deeper fundamental insights into how environmental factors influence microbial community structure through community assembly processes.

关键词： Stratified lake Water mixing Microbial community assembly Microbial interaction Planktothrix

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Cu-clusters nodes of 2D metal-organic frameworks as a cost-effective noble-metal-free cocatalyst with high atom-utilization efficiency for efficient photocatalytic hydrogen evolution

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Chinese Chemical Letters 2022年第6期33卷 3049-3052页

作者： Guangmei Jiang Xingyan Liu Huilong Jian Peng Lu Jinwu Bai Guizhi Zhang Wen Yun Siqi Li Youzhou He Chongqing Key Laboratory of Catalysis and New Environmental Materials College of Environment and ResourcesChongqing Technology and Business UniversityChongqing 400067China State Key Joint Laboratory of Environment Simulation and Pollution Control School of EnvironmentTsinghua UniversityBeijing 100084China

Several 2D nanosheets of porphyrin MOFs with various transition-metal clusters as metal nodes were prepared via a simple solvothermal method to apply in the photocatalytic hydrogen evolution,in which the hydrogen production rate of the optimal NS-Cu was as high as 15.39 mmol g^(-1)h^(-1).A series of experimental technologies especially cyclic voltammetry(CV)and Mott-Schottky(M-S)had been adopted to investigate the charge-transfer property of photo-generated electron-hole pairs,it was found that the uniformly dispersed Cu-clusters nodes in the original 2D MOFs played a key role in the electron transfer process,that was,the photo-generated electron transferred from excited state eosin-Y to the Cu-clusters nodes for the efficient hydrogen *** excellent photocatalytic performance could be attributed to the reversible oxidation-–reduction process of Cu^(Ⅱ)/Cu^(Ⅰ),which had excellent electron-receiving and electron-outputting *** results provided a novel avenue to adapt the uniformly dispersed metal nodes in the original MOFs as cost-effective noble-metal-free cocatalysts with very high atomutilization efficiency to improve the photocatalytic hydrogen evolution performance in dye-sensitized system.

关键词： 2D nanosheets Photocatalytic hydrogen production Cu-clusters nodes Cu^(Ⅱ)/Cu^(Ⅰ) Cocatalysts

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Disinfection Byproducts and Their Precursors in Drinking Water Sources:Origins,Influencing Factors,and environmental Insights

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Engineering 2024年第5期36卷 36-50页

作者： Rong Xiao Yang Deng Zuxin Xu Wenhai Chu State Key Laboratory of Pollution Control and Resource Reuse College of Environmental Science and EngineeringTongji UniversityShanghai 200092China Ministry of Education Key Laboratory of the Yangtze River Water Environment Tongji UniversityShanghai 200092China Department of Earth and Environmental Studies Montclair State UniversityMontclairNJ 07043USA

Tracing the contamination origins in water sources and identifying the impacts of natural and human processes are essential for ecological safety and public ***,current analysis approaches are not ideal,as they tend to be laborious,time-consuming,or technically *** byproducts(DBPs)are a family of well-known secondary pollutants formed by the reactions of chemical disinfectants with DBP precursors during water disinfection *** DBP precursors have various origins(e.g.,natural,domestic,industrial,and agricultural sources),and since the formation of DBPs from different precursors in the presence of specific disinfectants is distinctive,we argue that DBPs and DBP precursors can serve as alternative indicators to assess the contamination in water sources and identify pollution *** providing a retrospective of the origins of DBPs and DBP precursors,as well as the specific formation patterns of DBPs from different precursors,this article presents an overview of the impacts of various natural and anthropogenic factors on DBPs and DBP precursors in drinking water *** practice,the DBPs(i.e.,their concentration and speciation)originally present in source water and the DBP precursors determined using DBP formation potential tests—in which water samples are dosed with a stoichiometric excess of specific disinfectants in order to maximize DBP formation under certain reaction conditions—can be considered as alternative *** jointly used with other water quality parameters(e.g.,dissolved organic carbon,dissolved organic nitrogen,fluorescence,and molecular weight distribution)and specific contaminants of emerging concern(e.g.,certain pharmaceuticals and personal care products),DBPs and DBP precursors in drinking water sources can provide a more comprehensive picture of water pollution for better managing water resources and ensuring human health.

关键词： Disinfection byproducts Disinfection byproduct precursors Drinking water sources Contamination indicator Natural factors Human factors

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Particle-bound polycyclic aromatic hydrocarbons in typical urban of Yunnan-Guizhou Plateau:Characterization,sources and risk assessment

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Frontiers of environmental Science & Engineering 2022年第9期16卷 25-38页

作者： Yaoqian Zhong Bingxin Xia Jianwu Shi Ping Ning Chaoneng Zhang Xinyu Han Jiming Hao Faculty of Environmental Science and Engineering Kunming University of Science and TechnologyKunming 650500China State Key Joint Laboratory of Environmental Simulation and Pollution Control School of EnvironmentTsinghua UniversityBeijing 100084China

Monthly particle-phase ambient samples collected at six sampling locations in Yuxi,a high-altitude city on the edge of Southeast Asia,were measured for particle-associated *** trace substances,polycyclic aromatic hydrocarbons(PAHs)are susceptible to the influences of meteorological conditions,emissions,and gas-particulate partitioning and it is challenging job to precise quantify the source and define the transmission *** daily concentrations of total PM_(2.5)-bound PAHs ranged from 0.65 to 80.76 ng/m^(3),with an annual mean of 11.94 ng/m^(3).Here,we found that the concentration of PM_(2.5)-bound PAHs in winter was significantly higher than that in summer,which was mainly due to source and meteorology *** increase of fossil combustion and biomass burning in cold season became the main contributors of PAHs,while precipitation and low temperature exacerbated this *** to the concentration variation trend of PM_(2.5)-bound PAHs and their relationship with meteorological conditions,a new grouping of PAHs is applied,which suggested that PAHs have different environmental fates and migration paths.A combination of source analysis and trajectory model supported local sources from combustion of fossil fuel and vehicle exhaust contributed to the major portion on PAHs in particle,but on the Indochina Peninsula the large number of pollutants emitted by biomass burning during the fire season would affect the composition of PAHs through long-range *** assessment in spatial and temporal variability suggested that citizens living in industrial areas were higher health risk caused by exposure the PM_(2.5)-bound PAHs than that in other regions,and the risk in winter was three times than in summer.

关键词： Particle-associated PAHs Fine particle Source appointment Group analysis Risk assessment Biomass burning

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Effect of different reduction methods on Pd/Al_(2)O_(3) for o-xylene oxidation at low temperature

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Journal of environmental Sciences 2023年第3期125卷 95-100页

作者： Mingyu Fan Yafei Wang Jianghao Zhang Changbin Zhang Xue Han Beijing Institute of Petrochemical Technology Beijing 102617China State Key Joint Laboratory of Environment Simulation and Pollution Control Research Center for Eco-environmental SciencesChinese Academy of SciencesBeijing 100085China General Research Institute for Non-Ferrous Metals Beijing 100088China

Pd/Al_(2)O_(3)was pretreated by CO,H_(2)and NaBH_(4)reduction,*** reduced catalysts were tested for o-xylene oxidation and characterized by power X-ray diffraction(XRD),transmission electron microscopy (TEM),X-ray photoelectron spectroscopy (XPS) and temperature-programmed decomposition of palladium hydride (TPDH).The characterizations indicate the pretreatments lead to distinct Pd particle sizes and amount of surface activated oxygen species,which are responsible for the catalytic *** with H_(2)and NaBH_(4)reduction methods,CO reduction shows a strong interaction between Pd and Al_(2)O_(3)with smaller Pd particle size and more surface activated *** exhibited excellent catalytic performance,complete oxidation of 50 ppmV o-xylene at 85℃with a WHSV of 60,000 mL/(g·hr).

关键词： Pd Reduction method Catalytic oxidation o-Xylene

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Current research status on the distribution and transport of micro(nano)plastics in hyporheic zones and groundwater

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Journal of environmental Sciences 2025年第5期151卷 387-409页

作者： Dongming Zhang Qiqing Chen Ting Xu Daqiang Yin Key Laboratory of Yangtze River Water Environment Ministry of EducationCollege of Environmental Science and EngineeringTongji UniversityShanghai 200092China Shanghai Institute of Pollution Control and Ecological Security Shanghai 200092China State Key Laboratory of Estuarine and Coastal Research East China Normal UniversityShanghai 200241China

Micro(nano)plastics,as an emerging environmental pollutant,are gradually discovered in hyporheic zones and *** studies have focused on the origin and spatial/temporal distribution of micro(nano)plastics in regional groundwater,together with the influence of their properties and effects of environmental factors on their ***,the transport of micro(nano)plastics in the whole hyporheic zone-groundwater system and the behavior of co-existing substances still lack a complete theoretical *** provide systematic theoretical support for that,this review summarizes the current pollution status of micro(nano)plastics in the hyporheic zone-groundwater system,provides a comprehensive introduction of their sources and fate,and classifies the transport mechanisms into mechanical transport,physicochemical transport and biological processes assisted transport fromthe perspectives ofmechanical stress,physicochemical reactions,and bioturbation,***,this review proposes to advance the understanding of the multi-dimensional hydrosphere transport of micro(nano)plastics centered on groundwater,themicroorganisms-mediated synergistic transformation and co-transport involving the intertidal ***,this review systematically dissects the presence and transport cycles of micro(nano)plastics within the hyporheic zone-groundwater system and proposes prospects for future studies based on the limitations of current studies.

关键词： Micro(nano)plastics Groundwater Hyporheic zone Transport mechanisms Abundance

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Phosphate removal by a La(OH)_(3) loaded magnetic MAPTAC-based cationic hydrogel:Enhanced surface charge density and Donnan membrane effect

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Journal of environmental Sciences 2022年第3期34卷 26-39页

作者： Yanqing Zhou Yili Wang Shuoxun Dong Haotian Hao Junyi Li Chenyang Liu Xiaolin Li Yao Tong College of Environmental Science and Engineering Beijing Key Lab for Source Control Technology of Water PollutionBeijing Forestry UniversityBeijing 100083China Center for Water and Ecology State Key Joint Laboratory of Environment Simulation and Pollution ControlSchool of EnvironmentTsinghua UniversityBeijing 100083China State Key Laboratory of Environmental Aquatic Chemistry Research Center for Eco-Environmental SciencesChinese Academy of SciencesBeijing 100085China

Cationic hydrogels have received great attention to control eutrophication and recycle *** this study,a type of La(OH)_(3) loaded magnetic MAPTAC-based cationic hydrogel(La(OH)_(3)@MMCH)was developed as a potential adsorbent for enhanced phosphate removal from aqueous ***(OH)_(3)@MMCH exhibited high adsorption capacity of 105.72±5.99 mg P/g,and reached equilibrium within 2 ***(OH)_(3)@MMCH could perform effectively in a wide pH range from 3.0 to 9.0 and in the presence of coexisting ions(including SO_(4)^(2-),Cl^(-),NO_(3)^(-),HCO_(3)^(-),SiO_(4)^(4-) and HA).The adsorption-desorption experiment indicated that La(OH)_(3)@MMCH could be easily regenerated by using NaOH-NaCl as the desorption agent,and 73.3%adsorption capacity remained after five ***,La(OH)_(3)@MMCH was employed to treat surface water with phosphate concentration of 1.90 mg/L and showed great removal efficiency of 95.21%.Actually,MMCH showed high surface charge density of 34.38-59.38 meq/kg in the pH range from 3.0 to 11.0 and great swelling ratio of 3014.57%within 24 h,indicating that MMCH could produce the enhanced Donnan membrane effect to pre-permeate ***,the bifunctional structure of La(OH)_(3)@MMCH enabled it to capture phosphate through electrostatic attraction and ligand *** the results prove that La(OH)_(3)@MMCH is a promising adsorbent for eutrophication control and phosphate recovery.

关键词： Cationic hydrogel La(0H)_(3) Phosphate adsorption Enhanced Donnan membrane effect

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Enhancing comprehension of water vapor on adsorption performance of VOC on porous carbon materials and its application challenge

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Frontiers of environmental Science & Engineering 2024年第9期18卷 51-66页

作者： Xiaolong Yao Kuan Wan Wenxin Yu Zheng Liu School of Ecology and Environment Beijing Technology and Business UniversityBeijing 100048China State Environmental Protection Key Laboratory of Food Chain Pollution Control Beijing Technology and Business UniversityBeijing 100048China School of Resources Environment and MaterialsGuangxi UniversityNanning 530004China

Volatile organic compounds(VOC)have been proven to cause considerable harm to both the ecological environment and human *** VOC emissions are primarily generated by the industrial *** utilization of porous carbon as an adsorbent has emerged as an effective method for the efficient removal of VOC from industrial ***,during the actual production processes,VOC exhaust gases are often mixed with water vapor,which poses challenges for adsorption *** review provides a comprehensive overview of the remarkable advancements in various carbon materials in terms of their ability to adsorb both VOC and water ***,it systematically summarizes the influence of surface groups on adsorbents and the molecular properties of VOC on their adsorption by carbon ***,this review introduces the mechanism underlying adsorption-adsorbent interactions and discusses the construction of models for adsorbing water vapor and *** challenges associated with the application of carbon materials for VOC adsorption in humid environments are also *** review aims to offer theoretical and technical guidance for the effective purification of moist VOC waste gases emitted from industrial sources,thereby achieving precise control of VOC emissions.

关键词： Adsorption Water vapor Carbon-based adsorbents Surface functional groups VOC properties

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Urban sprawl and its effects on water competition between building industry and residents: Evidence from 31 provinces in China

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Water-Energy Nexus 2024年第1期7卷 26-38页

作者： Ding, Yu Jia, Ling Wang, Chenglong Wang, Peng Faculty of Civil Engineering and Mechanics Jiangsu University Zhenjiang212013 China State Key Laboratory of Pollution Control and Resource Reuse School of the Environment Nanjing University Nanjing210023 China

With accelerated urban sprawl, water scarcity and increased water stress have become global issues. Water of building industry and domestic water are two major contributors to total water consumption that cannot be ignored. This paper seeks to emphasize the effects of urban sprawl on water competition between building industry and residents. To achieve this objective, a framework for quantifying the water usage of the life cycle of the building was first constructed. Additionally, the degree of urban sprawl and water competition between domestic and building industry was computed. This study characterized the evolution path of urban sprawl and water competition using standard deviation ellipse. Spatial econometric models were used to determine the impact of urban sprawl on water competition. The results indicate that there is a high spatial correlation between urban sprawl and water competition. The center of gravity of China's urban sprawl is consistent with the north-to-south movement of water competition. As economic sprawl increases by 1%, water competition will rise by 0.440%. As the population expands by 1%, the water competition index shifts by 0.018%. Moreover, 0.017% more water was used for every 1% increase in land sprawl. © 2023

关键词： Competition

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Tuning SMSI to stabilize metallic Pd species:A case study on Pd/TiO_(2) for HCHO oxidation

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Chinese Chemical Letters 2024年第3期35卷 162-166页

作者： Chunying Wang Xiaofeng Liu Jingyi Wang Yaobin Li Shaohua Xie Fudong Liu Changbin Zhang Yuming Zheng Wenpo Shan Hong He Center for Excellence in Regional Atmospheric Environment Key Laboratory of Urban Pollutant ConversionInstitute of Urban EnvironmentChinese Academy of SciencesXiamen 361021China Zhejiang Key Laboratory of Urban Environmental Processes and Pollution Control Ningbo Urban Environment Observation and Research StationChinese Academy of SciencesNingbo 315800China Department of Civil Environmentaland Construction Engineering(CECE)Catalysis Cluster for Renewable Energy and Chemical Transformations(REACT)Nano Science Technology Center(NSTC)University of Central FloridaOrlandoFL 32816USA State Key Joint Laboratory of Environment Simulation and Pollution Control Research Center for Eco-environmental SciencesChinese Academy of SciencesBeijing 100085China

Pretreatment of the carrier for supported catalysts can effectively improve the strong metal-support interaction(SMSI)and increase the dispersion of precious metals,which are critical to many important catalytic *** this work,we tuned SMSI on Pd/TiO_(2)catalysts through inducing surface defects of TiO_(2)by pretreated with different atmospheres(H_(2)/N_(2),N_(2),O_(2)/N_(2))at the high temperature(800℃).Multiple characterization results illustrated that surface defects anchored Pd species and thus enhanced their *** reduction,Ti^(3+)species formed and transferred onto the metallic Pd species and then induced SMSI,which effectively stabilize Pd species in the metallic *** stronger MSI,the more stability of Pd *** a case,Pd/TiO_(2)–800H_(2),with strongest MSI,displayed the best HCHO oxidation performance at low temperature(10℃).

关键词： Pd/TiO_(2) Surface defects SMSI Formaldehyde Stability of Pd species

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