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Electronic regulation to achieve efficient anaerobic digestion of organic fraction of municipal solid waste(OFMSW):strategies,challenges and potential solutions

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Frontiers of environmental Science & Engineering 2024年第4期18卷 159-165页

作者： Yongdong Chen Hong Wang Parisa Ghofrani-Isfahani Li Gu Xiaoguang Liu Xiaohu Dai State Key Laboratory of Pollution Control and Resources Reuse College of Environmental Science and EngineeringTongji UniversityShanghai 200092China Shanghai Institute of Pollution Control and Ecological Security Tongji UniversityShanghai 200092China Department of Chemical and Biochemical Engineering Technical University of DenmarkKgs Lyngby DK-2800Denmark College of Environment and Ecology Chongqing UniversityChongqing 400045China

Anaerobic digestion(AD)of organic fraction of municipal solid waste(OFMSW)is prone to system breakdown under high organic loading rates(OLRs)condition,which subsequently reduces the efficiency of digestion process and results in substantial economic *** this perspective paper,the substances metabolisms,electrons flow,as well as microbial interaction mechanisms within AD process are comprehensively discussed,and the underlying bottleneck that causes inefficient methane production is identified,which is“electrons surplus”.Systems encountering severe electron surplus are at risk of process failure,making it crucial to proactively prevent this phenomenon through appropriate *** this basis,the present perspective proposes three potential electronic regulation strategies to prevent electrons surplus,namely,electron shunt,accelerating electron transfer and regulating methanogenic metabolism pathway,and presents specific methodologies for each ***,the potential solutions to challenges that may occur during the electronic regulation process are also presented in this *** perspective aims to provide innovative approaches to achieve the efficient and stable operation of OFMSW anaerobic digestion,especially under high OLRs condition.

关键词： Anaerobic digestion Electrons surplus Electronic regulation Electrons shunt Electron transfer Methanogenic metabolism pathway

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Nano-sized alumina supported palladium catalysts for methane combustion with excellent thermal stability

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Journal of environmental Sciences 2023年第4期126卷 333-347页

作者： Wei Shi Guangyan Xu Xuewang Han Yingjie Wang Zhi Liu Sen Xue Nannan Sun Xiaoyan Shi Yunbo Yu Hong He State Key Joint Laboratory of Environment Simulation and Pollution Control Research Center for Eco-Environmental SciencesChinese Academy of SciencesBeijing 100085China University of Chinese Academy of Sciences Beijing 100049China Weichai Power Co. Ltd.Weifang 261061China Center for Excellence in Regional Atmospheric Environment Institute of Urban EnvironmentChinese Academy of SciencesXiamen 361021China

Pd/Al_(2)O_(3)catalysts supported on Al_(2)O_(3)of different particle sizes were synthesized and applied in methane *** catalysts were systematically characterized by Brunauer-Emmett-Teller (BET),X-ray diffraction (XRD),high resolution-transmission electron microscopy (HR-TEM),high-angle annular dark?eld-scanning transmission electron microscopy (HAADF-STEM),H_(2)-temperature-programmed reduction (H_(2)-TPR),O_(2)-temperature-programmed oxidation (O_(2)-TPO),X-ray photoelectron spectroscopy (XPS),and X-ray absorption?ne structure (XAFS).The characterization results indicated that nanosized Al_(2)O_(3)enabled the uniform dispersion of palladium nanoparticles,thus contributing to the excellent catalytic performance of these nano-sized Pd/Al_(2)O_(3)*** them,Pd/Al_(2)O_(3)-nano-10 (Pd/Al_(2)O_(3)supported by alumina with an average particle size of 10 nm)showed superior catalytic activity and stability for methane oxidation under harsh practical *** maintained excellent catalytic performance for methane oxidation for50 hr and remained stable even after harsh hydrothermal aging in 10 vol.%steam at 800℃ for 16 *** results revealed that the strong metal-support interactions and physical barriers provided by Al_(2)O_(3)-nano-10 suppressed the coalescence ripening of palladium species,and thus contributed to the superior sintering resistance of the Pd/Al_(2)O_(3)-nano-10 catalyst.

关键词： Methane combustion Pd/Al_(2)O_(3) Hydrothermal stability Metal-support interaction Physical barriers

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Identification of high oxygen-consuming substances in stormwater drainage systems illicitly connected with sewage system

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Journal of environmental Sciences 2024年第4期138卷 132-140页

作者： Chen Xu Zuxin Xu Wenhai Chu Shanshan Wu Rong Xiao Lei Su State Key Laboratory of Pollution Control and Resource Reuse College of Environmental Science and EngineeringTongji UniversityShanghai 200092China Ministry of Education Key Laboratory of Yangtze River Water Environment Tongji UniversityShanghai 200092China Guangzhou Resource Environmental Protection Technology Co. Ltd.Guangzhou 510030China

The dissolved oxygen content in water is an important indicator for assessing the quality of the water environment,and maintaining a certain amount of dissolved oxygen is essential for the healthy development of the ecological *** a water body is anoxic,the activity of anaerobic microorganisms increases and organic matter is decomposed to produce a large number of blackening and odorizing substances,resulting in black and odorous water bodies,which is a very common and typical phenomenon in ***,there is still a relatively universal occurrence of illicitly connected stormwater and sewage pipes in the urban drainage pipe network in China,which makes oxygen-consuming substances be directly discharged into rivers through stormwater pipes and consume the dissolved oxygen in the water bodies,resulting in an oxygen deficiency of the *** induces seasonal or year-round black and stink phenomena in urban ***,identifying high oxygen-consuming substances,which lays the foundation for the subsequent removal of oxygen-consuming substances,is *** a series of comparisons of water quality indicators and analysis of organic characteristics,it was found that the oxygen consumption capacity of domestic sewage was higher than that of industrial wastewater in the selected area of this study,and the oxygen-consuming substances of domestic sewage were small molecular amino *** comparing 20 conventional free amino acids,it was found that seven of them consumed oxygen easily,and compared with chemical oxygen consumption,biological oxygen consumption was in a leading position.

关键词： Urban drainage system Oxygen-consuming substances Domestic sewage Amino acid

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Development of a random-forest-copula-factorial analysis(RFCFA)method for predicting propagation between meteorological and hydrological drought

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National Science Open 2024年第1期3卷 6-27页

作者： Hao Wang Yongping Li Guohe Huang Quan Zhang Yuan Ma Yangfeng Li State Key Joint Laboratory of Environmental Simulation and Pollution Control School of EnvironmentBeijing Normal UniversityBeijing 100875China Institute for Energy Environment and Sustainable CommunitiesUniversity of ReginaRegina Sask S4S 0A2Canada

In the context of global climate warming,the propagation of meteorological drought(MD)may aggravate the devastating impact of hydrological drought(HD)on water security and sustainable *** are challenges in accurately predicting the propagation of drought and effectively quantifying the effects of uncertainty,especially in data-deficient *** this study,a novel method called RFCFA is developed through integrating random forest(RF),copula,and factorial analysis(FA)into a general framework as well as applied to the Aral Sea Basin(a typical arid and data-scarce basin in Central Asia)under considering the impact of climate *** findings can be summarized:(1)the projected future drought propagation probability of ASB is 39.2%,which is about 8%higher than historical level;(2)drought propagation is mainly affected by mean climate condition,catchment characteristics(i.e.,elevation,LUCC,and slope),and human activities(i.e.,irrigation and reservoir operation);(3)the lower propagation probability in spring is expected under SSP1-2.6 due to increased snow meltwater,and the drought propagation probability in autumn is the highest(reaching 45.4%)under the influence of reservoir operation;(4)the combined effects of meteorological conditions and agricultural irrigation can lead to a higher probability of future propagation in the upper river basin in *** are valuable for predicting drought propagation risk,revealing main factors and inherent uncertainties,as well as providing support for drought management and disaster prevention.

关键词： rought propagation random forest copula factorial analysis climate change Aral Sea Basin

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Characterization and prediction of tailpipe ammonia emissions from in-use China 5/6 light-duty gasoline vehicles

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Frontiers of environmental Science & Engineering 2024年第1期18卷 71-81页

作者： Lewei Zeng Fengbin Wang Shupei Xiao Xuan Zheng Xintong Li Qiyuan Xie Xiaoyang Yu Cheng Huang Qingyao Hu Yan You Ye Wu College of Chemistry and Environmental Engineering Shenzhen UniversityShenzhen 518060China State Key Laboratory of Engines Tianjin UniversityTianjin 300072China China Automotive Technology and Research Center Co.Ltd. Tianjin 300300China CATARC Automotive Test Center(Guangzhou)Co.Ltd. Guangzhou 511300China State Environmental Protection Key Laboratory of Cause and Prevention of Urban Air Pollution Complex Shanghai Academy of Environmental SciencesShanghai 200233China National Observation and Research Station of Coastal Ecological Environments in Macao Macao Environmental Research InstituteMacao University of Science and TechnologyMacao SAR 999078China School of Environment State Key Joint Laboratory of Environment Simulation and Pollution ControlTsinghua UniversityBeijing 100084China

On-road tailpipe ammonia (NH3) emissions contribute to urban secondary organic aerosol formation and have direct or indirect adverse impacts on the environment and human health. To understand the tailpipe NH3 emission characteristics, we performed comprehensive chassis dynamometer measurements of NH3 emission from two China 5 and two China 6 light-duty gasoline vehicles (LDGVs) equipped with three-way catalytic converters (TWCs). The results showed that the distance-based emission factors (EFs) were 12.72 ± 2.68 and 3.18 ± 1.37 mg/km for China 5 and China 6 LDGVs, respectively. Upgrades in emission standards were associated with a reduction in tailpipe NH3 emission. In addition, high NH3 EFs were observed during the engine warm-up period in cold-start cases owing to the intensive emissions of incomplete combustion products and suitable catalytic temperature in the TWCs. Notably, based on the instantaneous NH3 emission rate, distinct NH3–emitting events were detected under high/extra high velocity or rapid acceleration. Furthermore, NH3 emission rates correlated well with engine speed, vehicle specific power, and modified combustion efficiency, which were more easily accessible. These strong correlations were applied to reproduce NH3 emissions from China 5/6 LDGVs. The predicted NH3 EFs under different dynamometer and real-world cycles agreed well with existing measurement and prediction results, revealing that the NH3 EFs of LDGVs in urban routes were within 8.55–11.62 mg/km. The results presented here substantially contribute to improving the NH3 emission inventory for LDGVs and predicting on-road NH3 emissions in China.

关键词： NH3 instantaneous emissions Catalytic temperature Vehicle specific power Combustion efficiency Emission prediction

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La^(3+)@BC500-S_(2)O_(8)^(2−)system for removal of sulfonamide antibiotics in water

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Journal of environmental Sciences 2024年第12期146卷 140-148页

作者： Bing Wang Dongsu Bi Juan Wang Hengbo Qiao Yalei Zhang Zheng Shen School of Chemical and Environmental Engineering Shanghai Institute of TechnologyShanghai 201418China State Key Laboratory of Pollution Control and Resources Reuse Key Laboratory of Yangtze River Water Environment of MOENational Engineering Research Center of Protected AgricultureShanghai Engineering Research Center of Protected AgricultureTongji UniversityShanghai 200092China

Sulfonamide antibiotics(SAs)widely used have potentially negative effects on human beings and *** and advanced oxidation methods have been exten-sively applied in SAs wastewater *** this study,compared with Al^(3+)@BC500 and Fe^(3+)@BC500,La^(3+)@BC500 for activating persulfate(S2O82−)had the best effect removal per-formance of sulfadiazine(SDZ)and sulfamethoxazole(SMX).Morphology,acidity,oxygen-containing functional groups,and loading of La^(3+)@BC500 were analyzed by techniques,in-cluding EA,BET,XRD,XPS,*** results show that with the increase of La^(3+)loading,the surface characteristics of biochar gradually changed from CaCO_(3)to LaCO_(3)*** EPR technology,it is proved that LaCO_(3)OH on the surface of La^(3+)@BC500 can not only acti-vate S2O82−to generate SO_(4)^(−)•,but also to produce•*** the optimization experiment,the optimal dosage of La^(3+)is between 0.05 and 0.2(mol/L)/*** had a good removal effect at pH(5-9),but SMX had a good removal effect only at pH=*** potential also proves that the material is more stable under acidic *** removal process of SDZ is more in accord with pseudo-first-order kinetics(R^(2)=0.9869),while SMX is more in line with pseudo-second order kinetics(R^(2)=0.9926).

关键词： Sulfadiazine Sulfamethoxazole La^(3+)@BC500 Persulfate

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Inhibition of jarosite heterogeneous crystallization on anglesite via in-situ formation of competitive substrate

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Journal of environmental Sciences 2025年第3期149卷 394-405页

作者： Jiahui Wu Xu Yan Feiping Zhao Yong Ke Haiying Wang Wenchao Zhang Qingwei Wang Meiqing Shi Liyuan Chai School of Metallurgy and Environment Central South UniversityChangsha 410083China Chinese National Engineering Research Center for Control&Treatment of Heavy Metal Pollution Changsha 410083China State Key Laboratory of Advanced Metallurgy for Non-ferrous Metals Changsha 410083China

Heterogeneous crystallization is a common occurrence during the formation of *** leads to the encapsulation of valuable/hazardous metals within the primary phase,presenting significant challenges for waste treatment andmetal ***,we proposed a novel method involving the in-situ formation of a competitive substrate during the precipitation of jarosite waste,which is an essential process for removing iron in zinc *** observed that the in-situ-formed competitive substrate effectively inhibits the heterogeneous crystallization of jarosite on the surface of anglesite,a lead-rich phase present in the *** a result,the iron content on the anglesite surface decreases from34.8%to 1.65%.The competitive substrate was identified as schwertmannite,characterized by its loose structure and large surface ***,we have elucidated a novel mechanism underlying this inhibition of heterogeneous crystallization,which involves the local supersaturation of jarosite caused by the release of ferric and sulfate ions from the competitive *** local supersaturation promotes the preferential heterogeneous crystallization of jarosite on the competitive ***,during the formation of jarosite,the competitive substrate gradually vanished through a dissolution-recrystallization process following the Ostwald rule,where a metastable phase slowly transitions to a stable *** effectively precluded the introduction of impurities and reduced waste *** goal of this study is to provide fresh insights into the mechanism of heterogeneous crystallization control,and to offer practical crystallization strategies conducive to metal separation and recovery from solid waste in industries.

关键词： Heterogeneous crystallization Jarosite waste Competitive substrate Zinc hydrometallurgy

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Destructing surfactant network in nanoemulsions by positively charged magnetic nanorods to enhance oil-water separation

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Journal of environmental Sciences 2022年第8期34卷 112-121页

作者： Yongjiao Xiong Xiangfeng Huang Lexue Li Wanqi Liu Jialu Zhang Mengfan He Jia Liu Lijun Lu Kaiming Peng College of Environmental Science and Engineering State Key Laboratory of Pollution Control and Resource ReuseMinistry of Education Key Laboratory of Yangtze River Water EnvironmentTongji UniversityShanghai 200092China

The separation of ultrafine oil droplets from wasted nanoemulsions stabilized with high concentration of surfactants is precondition for oil reuse and the safe discharge of ***, the double barriers of the interfacial film and network structures formed by surfactants in nanoemulsions significantly impede the oil-water separation. To destroy these surfactant protective layers, we proposed a newly-developed polyethyleneimine micelle template approach to achieve simultaneous surface charge manipulation and morphology transformation of magnetic nanospheres to magnetic nanorods. The results revealed that positively charged magnetic nanospheres exhibited limited separation performance of nanoemulsions, with a maximum chemical oxygen demand(COD) removal of 50%, whereas magnetic nanorods achieved more than 95% COD removal in less than 30 s. The magnetic nanorods were also applicable to wasted nanoemulsions from different sources and exhibited excellent resistance to wide pH changes. Owing to their unique one-dimensional structure, the interfacial dispersion of magnetic nanorods was significantly promoted, leading to the efficient capture of surfactants and widespread destruction of both the interfacial film and network structure, which facilitated droplet merging into the oil phase. The easy-toprepare and easy-to-tune strategy in this study paves a feasible avenue to simultaneously tailor surface charge and morphology of magnetic nanoparticles, and reveals the huge potential of morphology manipulation for producing high-performance nanomaterials to be applied in complex interfacial interaction process. We believe that the newly-developed magnetic-nanorods significantly contribute to hazardous oily waste remediation and advances technology evolution toward problematic oil-pollution control.

关键词： Nanoemulsions Surface charge Magnetic nanorods Surfactant Interfacial film Oil-water separation

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Enhanced nitrous acid(HONO)formation via NO_(2)uptake and its potential contribution to heavy haze formation during wintertime

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Atmospheric and Oceanic Science Letters 2024年第6期17卷 15-20页

作者： Zirui Liu Rong Yang Jingyun Liu Keding Lu Guiqian Tang Yuepeng Pan Dongsheng Ji Yuesi Wang Bo Hu State Key Laboratory of Atmospheric Environment and Extreme Meteorology Institute of Atmospheric PhysicsChinese Academy of SciencesBeijingChina School of Atmospheric Sciences Chengdu University of Information TechnologyChengduChina College of Energy and Environmental Engineering Hebei Key Laboratory of Air Pollution Cause and ImpactHebei University of EngineeringHandanChina State Key Joint Laboratory or Environmental Simulation and Pollution Control College of Environmental Sciences and EngineeringPeking UniversityBeijingChina

full understanding of the sources of atmospheric nitrous acid(HONO)in the polluted urban atmosphere re-mains a *** this study,ambient HONO and relevant species were measured during January 2019 at an urban site in Beijing,China,and a budget analysis of HONO was conducted using a box model combined with field *** nighttime“missing sources”of HONO were identified on heavily polluted days based on traditional sources,which had a significant correlation with the relative humidity,ammonia(NH_(3)),and aerosol surface area,and the promotional effect of NH_(3)for nitrogen dioxide(NO_(2))uptake on the wet aerosol surface was ***,an updated parameterization scheme for quantifying the enhanced heterogeneous reactions of NO_(2)on aerosol surfaces is proposed,and the missing nighttime sources of HONO could be substantially com-pensated after the new scheme was *** evaluation on the contributions of HONO to hydroxyl radicals was conducted,and the authors found that the photolysis of HONO played a dominant role in the primary OH production on the polluted days(78%-90%).The study reveals great potential of an NH3-enhanced uptake coefficient of NO_(2)on the aerosol surface in the nocturnal HONO budget,and highlights the significance of HONO in the strong atmospheric oxidation capability during episodes with a heavily polluted atmosphere.

关键词： Nitrous acid Budget analysis Heterogeneous reactions of NO_(2) Heavy pollution episodes Atmospheric oxidation capacity

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Root exudate-driven rhizospheric recruitment of plant growth-promoting rhizobacteria

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Pedosphere 2025年第1期35卷 216-228页

作者： Hua LIN Caixing LAI Guo YU Geoffrey ISUNAHARA Liheng LIU Habib ULLAH Jie LIU College of Environmental Science and Engineering Guilin University of TechnologyGuilin 541004China Center for Water and Ecology State Key Joint Laboratory of Environment Simulation and Pollution ControlSchool of EnvironmentTsinghua UniversityBeijing 100084China Department of Natural Resource Sciences McGill UniversityMontreal H3A 0G4Canada Department of Environmental Science Zhejiang UniversityHangzhou 310058China

To promote growth,terrestrial plants release photosynthetic products into the rhizosphere in the form of root exudates through their root *** the attraction of root exudates,plant growth-promoting rhizobacteria(PGPR)colonize the rhizosphere to stimulate plant growth and/or suppress the growth of pathogenic *** rhizospheric recruitment of PGPR,as well as the establishment of root-microbe interactions,is initiated by chemotaxis towards root *** the past several decades,scientists have made notable strides in identifying representative chemoeffectors in root exudates,as well as the corresponding *** review here the most recent developments in rhizospheric chemotaxis,particularly the chemoeffectors in root exudates,the structural and functional characterization of methyl-accepting chemotaxis proteins of PGPR,and the impacts of rhizospheric chemotaxis on root colonization,biofilm formation,and other root-microbe interactions during ***,we propose several perspectives that aim to fully unlock the potential of PGPR as bioinoculants in sustainable agriculture.

关键词： biofilm formation chemoattractant chemoeffector methyl-accepting chemotaxis proteins rhizospheric colonization

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