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14th International Conference on environmental Science and Technology, ICEST 2023

作者： Zhao, S.H. Li, J.W. Liu, J. Li, Y.P. Fujian Engineering and Research Center of Rural Sewage Treatment and Water Safety School of Environmental Science and Engineering Xiamen University of Technology Xiamen361024 China State Key Joint Laboratory of Environmental Simulation and Pollution Control School of Environment Beijing Normal University Beijing100875 China

ISBN: (纸本)9783031546839

Using low-carbon/zero-carbon energy sources and negative emission technologies, and economic policies have proven to be effective measures for electric power plants’ CO2 emission mitigation. This study constructs an interval fractional electric power system planning (IFES) model for minimizing CO2 emission intensity considering the interactions between the measures and other constraints under uncertainty. The model is applied to Fujian Province as a real-case study, which contains electricity mix improvement, three types of CO2 emission reduction technologies, one policy. It was found that: (i) System carbon emission intensity is [170, 213] g/RMB;(ii) The proportion of clean energy power generation in Fujian Province will reach [92.32, 93.13]% in the 2055–2060, with nuclear energy, wind power and photovoltaic power generation ranking the top three;(iii) The electricity mix improvement has made the greatest contribution to the carbon neutrality of the power system (74.62%), and the contributions of CCS, DAC, and ESC are (9.11, 5.25, 11.02%) respectively. The research results provide scientific planning solutions for carbon reduction in the power industry in Fujian Province. The developed IF-ESP model can also be used in other regions around the world. © The Author(s), under exclusive license to Springer Nature Switzerland AG 2024.

关键词： Electric power system planning

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Impact of anthropogenic heat emissions on meteorological parameters and air quality in Beijing using a high-resolution model simulation

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Frontiers of environmental Science & Engineering 2022年第4期16卷 47-57页

作者： Hengrui Tao Jia Xing Gaofeng Pan Jonathan Pleim Limei Ran Shuxiao Wang Xing Chang Guojing Li Fei Chen Junhua Li Aviation University of Air Force Changchun 130022China School of Environment and State Key Joint Laboratory of Environment Simulation and Pollution Control Tsinghua UniversityBeijing 100084China State Environmental Protection Key Laboratory of Sources and Control of Air Pollution Complex Beijing 100084China Research Triangle Park Environmental Protection AgencyNC 27711USA East Remote Sensing Laboratory United States Department of AgricultureNC 20250USA Unit No.96941 of Chinese People's Liberation Army Beijing 100041China Unit No.31010 of Chinese People's Liberation Army Beijing 100081China

Anthropogenic heat emissions(AHE)play an important role in modulating the atmospheric thermodynamic and kinetic properties within the urban planetary boundary layer,particularly in densely populated megacities like *** this study,we estimate the AHE by using a Large-scale Urban Consumption of energY(LUCY)model and further couple LUCY with a high-resolution regional chemical transport model to evaluate the impact of AHE on atmospheric environment in *** areas with high AHE,the 2-m temperature(T_(2))increased to varying degrees and showed distinct diurnal and seasonal variations with maxima in night and *** increase in 10-m wind speed(WS_(10))and planetary boundary layer height(PBLH)exhibited slight diurnal variations but showed significant seasonal ***,the systematic continuous precipitation increased by 2.1 mm due to the increase in PBLH and water vapor in upper *** contrast,the precipitation in local thermal convective showers increased little because of the limited water ***,the PM_(2.5) reduced in areas with high AHE because of the increase in WS_(10) and PBLH and continued to reduce as the pollution levels *** contrast,in areas where prevailing wind direction was opposite to that of thermal circulation caused by AHE,the WS_(10) reduced,leading to increased PM_(2.5).The changes of PM_(2.5) illustrated that a reasonable AHE scheme might be an effective means to improve the performance of PM_(2.5) ***,high AHE aggravated the O_(3) pollution in urban areas due to the reduction in NO_(x).

关键词： Anthropogenic heat emissions LUCY High-resolution Meteorological parameters Air quality

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Secondary organic aerosol formation from straw burning using an oxidation flow reactor

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Journal of environmental Sciences 2022年第4期34卷 249-258页

作者： Hui Wang Song Guo Zhijun Wu Kai Qiao Rongzhi Tang Ying Yu Weizhao Xu Wenfei Zhu Liwu Zeng Xiaofeng Huang Lingyan He Mattias Hallquist State Key Joint Laboratory of Environmental Simulation and Pollution Control International Joint Laboratory for Regional Pollution ControlMinistry of Education(IJRC)College of Environmental Sciences and EngineeringPeking UniversityBeijing 100871China Collaborative Innovation Center of Atmospheric Environment and Equipment Technology Nanjing University of Information Science&TechnologyNanjing 10044China Key Laboratory for Urban Habitat Environmental Science and Technology College of Environment and EnergyPeking University Shenzhen Graduate SchoolShenzhen 518055China Department of Chemistry and Molecular Biology Atmospheric ScienceUniversity of GothenburgSE-41296 GothenburgSweden

Herein,we use an oxidation flow reactor,Gothenburg:Potential Aerosol Mass(Go:PAM)reactor,to investigate the secondary organic aerosol(SOA)formation from wheat straw *** burning emissions are exposed to high concentrations of hydroxyl radicals(OH)to simulate processes equivalent to atmospheric oxidation of 0-2.55 *** volatile organic compounds(VOCs)were investigated,and particles were measured before and after the Go:PAM *** influence of water content(i.e.5%and 11%)in wheat straw was also *** burning stages,the flaming stage,and non-flaming stages,were *** particle emission factors(EFs)at a water content of 11%(~3.89 g/kg-fuel)are significantly higher than those at a water content of 5%(~2.26 g/kg-fuel)during the flaming ***,the water content showed no significant influence at the non-flaming *** of aromatics at a non-flaming stage(321.8±46.2 mg/kg-fuel)are larger than that at a flaming stage(130.9±37.1 mg/kg-fuel).The OA enhancement ratios increased with the increase in OH exposure at first and decreased with the additional increment of OH *** maximum OA enhancement ratio is~12 during the non-flaming stages,which is much higher than~1.7 during the flaming *** mass spectrum of the primary wheat burning organic aerosols closely resembles that of resolved biomass burning organic aerosols(BBOA)based on measurements in ambient *** results show that large gap(0%-90%)still remains to estimate biomass burning SOA if only the oxidation of VOCs were included.

关键词： Gothenburg:Potential Aerosol Mass(Go:PAM)reactor Wheat straw burning Flaming Non-flaming Secondary organic aerosol formation

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Arsenic release from microbial reduction of scorodite in the presence of electron shuttle in flooded soil

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Journal of environmental Sciences 2023年第4期126卷 113-122页

作者： Yujuan Fang Manjia Chen Chengshuai Liu Leheng Dong Jimei Zhou Xiu Yi Dongqing Ji Jiangtao Qiao Hui Tong School of Water and Environment Chang’an UniversityXi’an 710054China National-Regional Joint Engineering Research Center for Soil Pollution Control and Remediation in South China Guangdong Key Laboratory of Integrated Agro-environmental Pollution Control and ManagementInstitute of Eco-environmental and Soil SciencesGuangdong Academy of SciencesGuangzhou 510650China State Key Laboratory of Environmental Geochemistry Institute of GeochemistryChinese Academy of SciencesGuiyang 550081China College of Agriculture/Tree Peony Henan University of Science and TechnologyLuoyang 471023China

Scorodite (FeAsO_(4)·H_(2)O) is a common arsenic-bearing (As-bearing) iron mineral in nearsurface environments that could immobilize or store As in a bound *** flooded soils,microbe induced Fe(Ⅲ) or As(Ⅴ) reduction can increase the mobility and bioavailability of ***,humic substances can act as electron shuttles to promote this *** dynamics of As release and diversity of putative As(Ⅴ)-reducing bacteria during scorodite reduction have yet to be investigated in detail in flooded ***,the microbial reductive dissolution of scorodite was conducted in an flooded soil in the presence of anthraquinone-2,6-disulfonate (AQDS).Anaeromyxobacter,Dechloromonas,Geothrix,Geobacter,Ideonella,and Zoogloea were found to be the dominant indigenous bacteria during Fe(Ⅲ) and As(Ⅴ) *** increased the relative abundance of dominant species,but did not change the diversity and microbial community of the systems with *** these bacteria,Geobacter exhibited the greatest increase and was the dominant Fe(Ⅲ)-and As(Ⅴ)-reducing bacteria during the incubation with AQDS and *** promoted both Fe(Ⅲ) and As(Ⅴ) reduction,and over 80%of released As(Ⅴ) was microbially transformed to As(Ⅲ).The increases in the abundance of arrA gene and putative arrA sequences of Geobacter were higher with AQDS than without *** a result,the addition of AQDS promoted microbial Fe(Ⅲ) and As(Ⅴ) release and reduction from As-bearing iron minerals into the *** results contribute to exploration of the transformation of As from As-bearing iron minerals under anaerobic conditions,thus providing insights into the bioremediation of As-contaminated soil.

关键词： Scorodite Fe(III)reduction As(V)reduction Arsenate reductase gene(arrA) AQDS

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Micropollutant removal and disinfection byproduct control by sequential peroxymonosulfate-UV treatment in water: A case study with sulfamethoxazole

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Journal of environmental Sciences 2022年第7期34卷 141-150页

作者： Tian-Yang Zhang Yong-Shan Lu Zhen-Ning Luo Wen-Jun Sun Bin Xu Chen-Yan Hu Yu-Lin Tang Zheng-Yu Dong Xiao-Meng Ren State Key Laboratory of Pollution Control and Resource Reuse Key Laboratory of Yangtze Water EnvironmentMinistry of EducationCollege of Environmental Science and EngineeringTongji UniversityShanghai 200092China Shanghai Institute of Pollution Control and Ecological Security Shanghai 200092China School of Environment Tsinghua UniversityBeijing 100084China College of Environmental and Chemical Engineering Shanghai University of Electric PowerShanghai 200090China PLA Naval Medical Center Shanghai 200433China

UV/peroxymonosulfate(UV/PMS) advanced oxidation process has attracted significant attention for removal of micropollutants in water. However, during practical water treatment applications, the PMS treatment must be performed before the UV treatment to achieve full contact. In this study, sulfamethoxazole(SMX) was selected as the target micropollutant. Four different operational approaches, including UV alone, PMS alone, simultaneous UV/PMS and sequential PMS-UV, were compared for their differences in SMX removal and disinfection by-product(DBP) formation potentials during chlorine-driven disinfection. Among the four approaches, UV/PMS and PMS-UV achieved over 90% removal efficiencies for SMX without substantial differences. For raw water, the trichloronitromethane(TCNM) formation potential after treatment with PMS-UV was lower than that after UV/PMS treatment. The time interval over which the PMS-UV process was conducted had little effect on the final removal efficiency for SMX. However, a brief(5 min) pre-PMS treatment significantly reduced the TCNM formation potential and the genotoxicity from DBPs. The formation risk for TCNM during chlorination increased markedly with increasing PMS dosages, and the appropriate dosage under these experimental conditions was suggested to be 0.5–1.0 mmol/L. Under alkaline conditions, PMS-UV treatment can enhance SMX degradation as well as dramatically reduced the formation potentials for haloketones, haloacetonitriles and halonitromethanes. This study suggests that proper optimization of UV/PMS processes can remove SMX and reduce its DBP formation.

关键词： Peroxymonosulfate-UV(PMS-UV) Sulfamethoxazole(SMX) Disinfection by-products(DBPs) Operational approaches Water treatment

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Distribution,sources,and burial flux of black carbon in sediment of Daye lake,central China

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国际泥沙研究（英文版） 2024年第5期39卷 750-760页

作者： Changlin Zhan Yongming Han Jiaquan Zhang Shan Liu Hongxia Liu Wensheng Xiao Junji Cao School of Environmental Science and Engineering Hubei Key Laboratory of Mine Environmental Pollution Control and RemediationHubei Polytechnic UniversityHuangshi435003China Department of Agroecology Aarhus UniversityTjele8830Denmark State Key Laboratory of Loess Institute of Earth EnvironmentChinese Academy of SciencesXi'an710061China School of Human Settlements and Civil Engineering Xi'an Jiaotong UniversityXi'an710049China National Observation and Research Station of Regional Ecological Environment Change and Comprehensive Management in the Guanzhong Plain Xi'an710061China School of Environmental Science and Engineering Hubei Key Laboratory of Mine Environmental Pollution Control and RemediationHubei Polytechnic UniversityHuangshi435003China Institute of Atmospheric Physics Chinese Academy of SciencesBeijing100029China

Black carbon(BC),primarily originating from fossil fuel and biomass combustion,holds significance for global carbon cycling,climate change,and human *** a lake's role as a carbon sink,detailed information about BC sedimentary burial flux and sink in its sediment remains insufficiently *** current study investigates the distribution,sources,and burial flux of BC and its sub-types(char and soot)in the surface sediment of Daye Lake,the largest lake in Huangshi City,central *** concentrations in the sediment ranged from 0.10 to 3.60 mg/g,corresponding to 0.40％-17.02％of organic carbon(OC).Higher values of BC and BC/OC observed in the western region suggest direct terrestrial input via river discharge and surface runoff,influenced by anthropogenic *** contrast,variations in char/soot ratios reflect diverse combustion sources and hydrological dynamics in different *** indications from BC/OC and char/soot ratios imply that fossil fuel combustion is the predominant *** weak correlations between BC and OC suggest that they may come from different sources or undergo different processes that affect their distribution in the lake ***,a stronger correlation was observed between BC and soot,as well as between char and soot,indicating potential similarities in their input *** BC burial flux displays notable variations across the lake,ranging from 0.69 to 24.07 g/m2/yr,with elevated values observed in the western *** BC sink in the sediments of Daye Lake was estimated to be 0.635 Gg/*** locally small,it significantly contributes to the broader picture of BC burial in Chinese lakes and the global distribution of BC in lake ecosystems.

关键词： Black carbon Sediment source Burial flux Daye lake

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Influence of kaolinite and montmorillonite on benzo[a]pyrene biodegradation by Paracoccus aminovorans HPD-2 and the underlying interface interaction mechanisms

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Pedosphere 2022年第2期32卷 246-255页

作者： Xinhong GAN Ying TENG Jian XU Ning ZHANG Wenjie REN Ling ZHAO Peter CHRISTIE Yongming LUO Key Laboratory of Soil Environment and Pollution Remediation Institute of Soil ScienceChinese Academy of SciencesNanjing 210008China State Environmental Protection Key Laboratory of Soil Environmental Management and Pollution Control Nanjing Institute of Environmental ScienceMinistry of Ecology and Environment(MEE)of ChinaNanjing 210042China University of Chinese Academy of Sciences Beijing 100049China

Clay minerals play an important role in biogeochemical ***,kaolinite and montmorillonite,the two most abundant and widespread clay minerals with typical layered structures,were selected to investigate and compare their effects on the biodegradation of benzo[a]pyrene(BaP)by Paracoccus aminovorans HPD-2 and to investigate the underlying interface ***,the BaP degradation efficiency was significantly higher 7 d after montmorillonite addition,reaching 68.9%(P<0.05),when compared with that of the control without addition of clay minerals(CK,61.4%);however,the addition of kaolinite significantly reduced the BaP degradation efficiency to 45.8%.This suggests that kaolinite inhibits BaP degradation by inhibiting the growth of strain HPD-2,or its strong hydrophobicity and readily agglomerates in the degradation system,resulting in a decrease in the bio-accessibility of BaP to strain *** may buffer some unfavorable factors,and cells may be fixed on the surface of montmorillonite colloidal particles across energy ***,the adsorption of BaP on montmorillonite may be weakened after swelling,reducing the effect on the bio-accessibility of BaP,thus promoting the biodegradation of BaP by strain *** experimental results indicate that differential bacterial growth,BaP bio-accessibility,interface interaction,and the buffering effect may explain the differential effects of the different minerals on polycyclic aromatic hydrocarbon *** observations improve our understanding of the mechanisms by which clay minerals,organic pollutants,and degrading bacteria interact during the biodegradation process and provide a theoretical basis for increasing the biodegradation of soil pollutants by native microorganisms under field conditions.

关键词： bio-accessibility cell viability clay mineral degrading bacteria nano-scale secondary ion mass spectrometry polycyclic aromatic hydrocarbon

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Precise regulation of acid pretreatment for red mud SCR catalyst:Targeting on optimizing the acidity and reducibility

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Frontiers of environmental Science & Engineering 2022年第7期16卷 61-71页

作者： Xiang Zhang Yue Xuan Bin Wang Chuan Gao Shengli Niu Gaiju Zhao Dong Wang Junhua Li Chunmei Lu John C.Crittenden National Engineering Laboratory for Coal-Burning Pollutants Emission Reduction School of Energy and Power EngineeringShandong UniversityJinan250061China School of Civil and Environmental Engineering and the Brook Byers Institute for Sustainable Systems Georgia Institute of TechnologyAtlantaGA30332USA State Key Joint Laboratory of Environment Simulation and Pollution Control National Engineering Laboratory for Multi Flue Gas Pollution Control Technology and EquipmentSchool of EnvironmentTsinghua UniversityBeijing100084China Energy Institute Qilu University of Technology(Shandong Academy of Sciences)Jinan250013China

Red mud(RM),as an alkaline waste,was recently proved to be a promising substitute for the SCR *** could improve the acidity and reducibility of red mud,which were critical for SCR ***,the dealkalization effect depended on the reaction between acid solution and red *** this study,we realized the directional control of the chemical state of active sites through tuning the acid pretreatment(dealkalization)*** pretreatment endpoint was controlled at pH values of 3–5 with diluted nitric *** the pH values of red mud were 3 and 5(CRM-3 and CRM-5),activated catalysts showed NOx conversion above 90%at 275℃–475℃.The high initial reaction rate,Ce^(3+)/(Ce^(3+)+Ce^(4+))ratio,and surface acidity accounted for the excellent SCR performance of CRM-5 ***,more Fe^(3+) on the CRM-3 surface improved the NH_(3) *** was a strong interaction between Al and Fe in both CRM-5 and CRM-3 *** results showed that the adsorption capacity of the Al-O_(3)-Fe for NH_(3) and NO is stronger than that of Fe-O_(3)-Fe,which enhanced the NOx conversion of the ***,the almandine was formed in CRM-4,consumed part of Fe^(3+) and Al^(3+),and the interaction between Al and Fe was ***,deposited almandine on the catalyst surface covered the active sites,thus leading to lower NH_(3)-SCR activity.

关键词： Air pollution control Nitrogen oxides Selective catalytic reduction Red mud Solid waste utilization

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Facile low-temperature supercritical carbonization method to prepare high-loading nickel single atom catalysts for efficient photodegradation of tetracycline

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Journal of environmental Sciences 2024年第4期138卷 373-384页

作者： Han Qiao Lirong Zheng Shiwen Hu Gang Tang Hongri Suo Chongxuan Liu School of Environment Harbin Institute of TechnologyHarbin 150090China State Environmental Protection Key Laboratory of Integrated Surface Water-Groundwater Pollution Control School of Environmental Science and EngineeringSouthern University of Science and TechnologyShenzhen 518055China Beijing Synchrotron Radiation Facility(BSRF) Institute of High Energy PhysicsChinese Academy of SciencesBeijing 100049China

environmental photocatalysis is a promising technology for treating antibiotics in *** this study,a supercritical carbonization method was developed to synthesize a single-atom photocatalyst with a high loading of Ni(above 5 wt.%)anchored on a carbonnitrogen-silicate substrate for the efficient photodegradation of a ubiquitous environmental contaminant of tetracycline(TC).The photocatalyst was prepared from an easily obtained metal-biopolymer-inorganic supramolecular hydrogel,followed by supercritical drying and carbonization *** low-temperature(300℃)supercritical ethanol treatment prevents the excessive structural degradation of hydrogel and greatly reduces the metal clustering and aggregation,which contributed to the high Ni *** characterizations confirmed that Ni was present at isolated sites and stabilized by Ni-N and Ni-O bonds in a Ni-(N/O)_(6)-C/SiC configuration.A 5%Ni-C-Si catalyst,which performed the best among the studied catalysts,exhibited a wide visible light response with a narrow bandgap of 1.45 eV that could efficiently and repeatedly catalyze the oxidation of TC with a conversion rate of almost 100% within 40 *** reactive species trapping experiments and electron spin resonance(ESR)tests demonstrated that the h+,and·O_(2)-were mainly responsible for TC *** TC degradation mechanism and possible reaction pathways were provided ***,this study proposed a novel strategy to synthesize a high metal loading singleatom photocatalyst that can efficiently remove TC with high concentrations,and this strategy might be extended for synthesis of other carbon-based single-atom catalysts with valuable properties.

关键词： Carbon-based single-atom catalyst Nickel Photocatalytic degradation Tetracycline Visible light

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Hybrid energy harvesting systems for self-powered sustainable water purification by harnessing ambient energy

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Frontiers of environmental Science & Engineering 2023年第10期17卷 1-16页

作者： Zhengyang Huo Young Jun Kim Yuying Chen Tianyang Song Yang Yang Qingbin Yuan Sang Woo Kim School of Environment and Natural Resources Renmin University of ChinaBeijing 100872China School of Advanced Materials Science and Engineering Sungkyunkwan University(SKKU)Suwon 16419Republic of Korea State Key Laboratory of Pollution Control and Resource Reuse School of the EnvironmentNanjing UniversityNanjing 210023China Institute of Scientific and Technical Information of China Beijing 100038China

The development of self-powered water purification technologies for decentralized applications is crucial for ensuring the provision of drinking water in resource-limited regions. The elimination of the dependence on external energy inputs and the attainment of self-powered status significantly expands the applicability of the treatment system in real-world scenarios. Hybrid energy harvesters, which convert multiple ambient energies simultaneously, show the potential to drive self-powered water purification facilities under fluctuating actual conditions. Here, we propose recent advancements in hybrid energy systems that simultaneously harvest various ambient energies (e.g., photo irradiation, flow kinetic, thermal, and vibration) to drive water purification processes. The mechanisms of various energy harvesters and point-of-use water purification treatments are first outlined. Then we summarize the hybrid energy harvesters that can drive water purification treatment. These hybrid energy harvesters are based on the mechanisms of mechanical and photovoltaic, mechanical and thermal, and thermal and photovoltaic effects. This review provides a comprehensive understanding of the potential for advancing beyond the current state-of-the-art of hybrid energy harvester-driven water treatment processes. Future endeavors should focus on improving catalyst efficiency and developing sustainable hybrid energy harvesters to drive self-powered treatments under unstable conditions (e.g., fluctuating temperatures and humidity).

关键词： Piezocatalysis Solar energy Waste heat Decentralized water treatment Point-of-use Nanogenerator

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