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Supply-side drivers of phosphorus emissions from phosphorus supply chains in China

Ecosystem Health and Sustainability 2022年第1期8卷 523-533页

作者： Jing Zhang Qiumeng Zhong Yadong Yu Jetashree Xuechun Yang Cuiyang Feng Hui Li Sai Liang State Key Joint Laboratory of Environment Simulation and Pollution Control School of EnvironmentBeijing Normal UniversityBeijingChina Key Laboratory for City Cluster Environmental Safety and Green Development of the Ministry of Education School of EcologyEnvironment and ResourcesGuangdong University of TechnologyGuangzhouGuangdongChina School of Business East China University of Science and TechnologyShanghaiChina Institute of Circular Economy Beijing University of TechnologyBeijingChina School of Management China University of Mining&Technology(Beijing)BeijingChina

Human activities interfere with natural Phosphorus(P)cycles by introducing increased levels of P emissions to air,land,and water.A supply-side analysis of P supply chains and associated P emissions can provide insights into underlying economic activities and transitions responsible for human-induced P *** the China's Mainland as the case,this study constructs time-series physical input-output tables to describe P supply chains during ***,it identifies critical products and influencing factors of P supply chains enabling P emissions to the environment(including air,land,and water)from the supply *** results show that phosphate rock,an important initial supplier of P from natural environment to China’s P supply chain,was responsible for 86%of P emissions in ***,food crops and livestock are important initial suppliers of P from soil to China’s P supply chain,through cultivation and pasturing,*** 1949 to 2012,the change in primary input level was the largest driver of P emission increments,followed by changes in population,emission intensity,and primary input *** the contrary,changes in production structure reduced P *** findings could support supply-side policy decisions on P emission control.

关键词： Phosphorus input-output analysis structural decomposition analysis supply chain primary input

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Microeukaryotic plankton community dynamics under ecological water replenishment:Insights from eDNA metabarcoding

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environmental Science and Ecotechnology 2024年第4期20卷 278-290页

作者： Shuping Wang Songsong Gu Yaqun Zhang Ye Deng Wenhui Qiu Qianhang Sun Tianxu Zhang Pengyuan Wang Zhenguang Yan State Key Laboratory of Environmental Criteria and Risk Assessment Chinese Research Academy of Environmental SciencesBeijing100012China CAS Key Laboratory of Environmental Biotechnology Research Center for Eco-Environmental SciencesChinese Academy of SciencesBeijing100085China Key Laboratory of Aquatic Genomics Ministry of Agriculture and Rural AffairsBeijing Key Laboratory of Fishery BiotechnologyChinese Academy of Fishery SciencesBeijing100141China College of Resources and Environment University of Chinese Academy of SciencesBeijing100190China Guangdong Provincial Key Laboratory of Soil and Groundwater Pollution Control School of Environmental Science and EngineeringSouthern University of Science and TechnologyShenzhen518055China

Ecological water replenishment(EWR)is an important strategy for river restoration globally,but timely evaluation of its ecological effects at a large spatiotemporal scale to further adjust the EWR schemes is of great ***,we examine the impact of EWR on microeukaryotic plankton communities in three distinct river ecosystems through environmental DNA(eDNA)*** three ecosystems include a long-term cut-off river,a short-term connected river after EWR,and long-term connected *** analyzed community stability by investigating species composition,stochastic and deterministic dynamics interplay,and ecological network *** found that EWR markedly reduced the diversity and complexity of microeukaryotic plankton,altered their community dynamics,and lessened the variation within the ***,EWR disrupted the deterministic patterns of community organization,favoring dispersal constraints,and aligning with trends observed in naturally connected *** shift from an isolated to a temporarily connected river appeared to transition community structuring mechanisms from deterministic to stochastic dominance,whereas,in permanently connected rivers,both forces concurrently influenced community *** ecological network in temporarily connected rivers post-EWR demonstrated significantly greater stability and intricacy compared to other river *** shift markedly bolstered the resilience of the ecological *** eDNA metabarcoding insights offer a novel understanding of ecosystem resilience under EWR interventions,which could be critical in assessing the effects of river restoration projects throughout their life cycle.

关键词： Ecological water replenishment Community stability Succession Community assembly mechanism Ecological network

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Antibiotic resistome mostly relates to bacterial taxonomy along a suburban transmission chain

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Frontiers of environmental Science & Engineering 2022年第3期16卷 63-72页

作者： Ziyan Qin Qun Gao Qiang Dong Joy D.Van Nostrand Qi Qi Yifan Su Suo Liu Tianjiao Dai Jingmin Cheng Jizhong Zhou Yunfeng Yang State Key Joint Laboratory of Environment Simulation and Pollution Control School of EnvironmentTsinghua UniversityBeijing 100084China Institute of Chemical Defense Beijing 102205China Institute for Environmental Genomics and Department of Microbiology and Plant BiologyUniversity of OklahomaNormanOK 73019USA School of Civil Engineering and Environmental Sciences University of OklahomaNormanOK 73019USA Earth and Environmental Sciences Lawrence Berkeley National LaboratoryBerkeleyCA 94720USA

Antibiotic resistance genes comprising antibiotic resistome are of great concern due to their increase in the *** evidence of shared resistomes between soils and animal husbandry has imposed potential risks to human ***,the correlation between a given community’s resistome and bacterial taxonomic composition is ***,a transmission chain of resistomes from swine manure to compost and compost-amended soil were analyzed in five suburban areas of Beijing,China,with unamended agricultural soils as control *** resistomes and bacterial taxonomic compositions were distinct between(I)manure and compost;and(II)compost-amended and control *** manure,compost,and compost-amended soils,theβ-diversity of the resistome and bacterial taxonomic composition was significantly correlated,while no correlation was detected in control *** taxonomic composition explained 36.0%of total variations of the resistome composition,much higher than environmental ***,those results demonstrated that antibiotic resistome was closely related to bacterial taxonomic composition along the suburban transmission chain.

关键词： Antibiotic resistance genes Resistome Bacterial taxonomy Transmission chain

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Estimation for ammonia emissions at county level in China from 2013 to 2018

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Science China Earth Sciences 2022年第6期65卷 1116-1127页

作者： Wenling LIAO Mingxu LIU Xin HUANG Tiantian WANG Zhenying XU Fang SHANG Yu SONG Xuhui CAI Hongsheng ZHANG Ling KANG Tong ZHU State Key Joint Laboratory of Environmental Simulation and Pollution Control Department of Environmental SciencePeking UniversityBeijing 100871China Joint International Research Laboratory of Atmospheric and Earth System Sciences School of Atmospheric SciencesNanjing UniversityNanjing 210023China Laboratory for Atmosphere-Ocean Studies Department of Atmospheric and Oceanic ScienceSchool of PhysicsPeking UniversityBeijing 100871China

Ammonia (NH_(3)) can interact with other trace chemicals in the atmosphere,significantly impacting atmospheric chemistry and global climate *** is a largely agricultural country with high consumption of nitrogen fertilizer and large livestock herds,resulting in high NH_(3) *** this study,a comprehensive county-level inventory of Chinese NH_(3) emissions from 2013 to 2018 was *** on previous research,an estimate of NH_(3) emissions from household coal combustion was added to the *** estimation of emissions from open biomass burning was improved by using a method based on fire radiative energy (FRE).The total NH_(3) emissions in China increased from 2013 (9.64 Tg) to 2015 (9.75 Tg),and then decreased to 9.12 Tg in *** from fossil fuels reached a peak value in 2018,accounting for 8.4%of total emissions,while fertilizer application and livestock waste were responsible for fewer emissions than in previous years,accounting for 27.7%and 49.9%of the total from non-fossil fuel sources,*** highest emission rates were in central and southwestern ***,NH_(3) emissions peaked in spring and *** inventory had a 1-km spatial resolution and a monthly temporal resolution,which confirmed its suitability for global and regional air quality simulations.

关键词： Ammonia emission Seasonal variations Spatial distribution Policy Suggestions China

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Unneglectable Terrestrial Export of Dissolved Organic Carbon in China

SSRN

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SSRN 2024年

作者： Yu, Qian Li, Han Ge, Xiaodong Ma, Mingrui Zhao, Wenxin Yang, Jinya Mulder, Jan Zhang, Lei Zhao, Yu Duan, Lei State Key Laboratory of Pollution Control & Resource Reuse School of Environment Nanjing University Jiangsu Nanjing210023 China State Key Laboratory of Environmental Simulation and Pollution Control School of Environment Tsinghua University Beijing100084 China Faculty of Environmental Sciences and Natural Resource Management Norwegian University of Life Sciences Box 5003 Ås1432 Norway State Environmental Protection Key Laboratory of Sources and Control of Air Pollution Complex Tsinghua University Beijing100084 China China

Transport of dissolved organic carbon (DOC) from land to inland waters is a crucial yet usually overlooked component of carbon budget. Its magnitude and response to global change are poorly quantified due to limited direct observation, especially in China. Here we compiled a database from 462 headwaters across China, primary based on our own observation, and applied a generalized additive model (GAM) to quantify terrestrial DOC export from 2000 to 2020. Our results reveal substantial underestimations in current assessments relying on riverine data. Over this period, terrestrial DOC export averaged 13.4 ± 1.5 Tg C yr−1, accounting for approximately 10% of national net biome productivity (NBP). Projections under SSP2-4.5 and carbon-neutral scenarios suggest an increase to 17.1 Tg C yr−1 in 2060, driven by decreasing atmospheric deposition and rising temperatures. This highlights the importance of considering DOC export in terrestrial carbon sink assessments, particularly as global change continues to evolve. © 2024, The Authors. All rights reserved.

关键词： Carbon sequestration

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Alkaline hydrogen production promoted by small-molecule modification on flowerlike Co_(2)(OH)_(2)CO_(3)

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Journal of Energy Chemistry 2023年第9期84卷 73-80页

作者： Yue Liu Huan Zhang Chen Yang Ziyang Xu Yiyang Shi Xukun Zhu Xinde Duan Ling Qin Yachao Jin Li Song Mingdao Zhang Hegen Zheng Institute of Energy Supply Technology for High-end Equipment Jiangsu Key Laboratory of Atmospheric Environment Monitoring and Pollution ControlJiangsu Collaborative Innovation Center of Atmospheric Environment and Equipment TechnologySchool of Environmental Science and EngineeringNanjing University of Information Science&TechnologyNanjing 210044JiangsuChina State Key Laboratory of Coordination Chemistry School of Chemistry and Chemical EngineeringCollaborative Innovation Center of Advanced MicrostructuresNanjing UniversityNanjing 210023JiangsuChina School of Chemistry and Chemical Engineering Hefei University of TechnologyHefei 230009AnhuiChina

Developing a low-cost and high-efficiency nonprecious metal-based catalyst for hydrogen evolution reaction(HER) is of great significance for the utilization of hydrogen *** this work,we report a molecular-modification strategy to fabricate a self-supported hydrogen evolution electrode,specially by grafting the macrocyclic molecules(HHTP=2,3,6,7,10,11-hexahydroxytriphenylene) on the surface of a cobaltous dihydroxy carbonate(COC) seed *** HHTP-COC electrode is endowed with a rodlike structure,which provides favorable access for charge transportation and mass *** macrocyclic molecule structure in HHTP can be grafted on COC and improve the electrical conductivity,while the interaction between HHTP and COC induces the rearrangement of charge configuration on the *** to the combination effects of several aspects,the HHTP-COC electrode achieves astonishing HER activity,with a low overpotential of 61.0 mV(η_(10),at the current density of 10 mA cm^(-2)) and excellent stability in alkaline *** kind of interface engineering based on the organic molecules can be applied to the design and manufacture of electrocatalysts in the field of energy conversion and storage.

关键词： Interfacial interaction Hydrogen evolution Molecule modification DFT calculation

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Evidence on the causes of the rising levels of COD_(Mn) along the middle route of the South-to-North Diversion Project in China:The role of algal dissolved organic matter

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Journal of environmental Sciences 2022年第3期34卷 281-290页

作者： Chao Wang Hong Zhang Pei Lei Xiaokang Xin Aijing Zhang Wei Yin Changjiang Water Resources Protection Institute Wuhan 430051China State Key Laboratory of Environmental Aquatic Chemistry Research Center for Eco-Environmental SciencesChinese Academy of SciencesBeijing 100085China State Key Laboratory of Pollution Control and Resources Reuse School of the EnvironmentNanjing UniversityNanjing 210046China Construction and Administration Bureau of South-to-North Water Diversion Middle Route Project Beijing 100038China Key Laboratory cf Ecological Regulation ofNon-point Source Pollution in Lake and Reservoir Water Sources Wuhan 430051China

As the biggest inter-basin water transfer scheme in the world,the South-to-North Water Diversion Project(SNWD) was designed to alleviate the water crisis in North *** main channel of the middle route of the SNWD is of great concern in terms of the drinking water *** this study,we tested the hypothesis that the dissolved organic matter(DOM) derived from the planktonic algae causes the rising levels of COD_(Mn) along the middle route by monitoring data on water quality(2015-2019,monthly resolution).The results showed that algal density in the main channel increased along the channel and was significantly correlated with COD_(Mn)(p <0.01).Five fluorescent components of DOM,including tyrosine-like(14.85%),tryptophan-like(22.48%),microbial byproduct-like(26.34%),fulvic acid-like(11.41%),and humic acid-like(24.92%) components,were *** level of tyrosine-like components increased along the channel and was significantly correlated with algal density(p<0.01),indicating that algae significantly changed the level of DOM in the *** decomposition and metabolism were found to be the main mechanisms that drive the changes in COD_(Mn).Therefore,controlling algal density would be an important measure to prevent further increase in CODMn and for the guarantee of excellent water quality.

关键词： Dissolved organic matter(DOM)Algae COD_(Mn) South-to-North Diversion Project Danjiangkou reservoir Three-dimensional fluorescence excitation emission matrix spectroscopy(3D-EEMs)

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Steam disinfection releases micro(nano)plastics from silicone-rubber baby teats as examined by optical photothermal infrared microspectroscopy (vol 17, pg 76, 2022)

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NATURE NANOTECHNOLOGY 2022年第6期17卷 672-672页

作者： Su, Yu Hu, Xi Tang, Hongjie Lu, Kun Li, Huimin Liu, Sijin Xing, Baoshan Ji, Rong State Key Laboratory of Pollution Control and Resource Reuse School of the Environment Nanjing University Nanjing China Quantum Design (Beijing) Co. Ltd Beijing China State Key Laboratory of Environmental Chemistry and Ecotoxicology Research Center for Eco-Environmental Sciences Chinese Academy of Sciences Beijing China Stockbridge School of Agriculture University of Massachusetts Amherst MA USA

Silicone-rubber baby teats used to bottle-feed infants are frequently disinfected by moist heating. However, infant exposure to small microplastics (0.66 million elastomer-derived micro-sized plastics (MPs) (roughly 8... 详细信息

Silicone-rubber baby teats used to bottle-feed infants are frequently disinfected by moist heating. However, infant exposure to small microplastics (<10 μm) potentially released from the heated teats by hydrothermal decomposition has not been studied, owing to the limitations of conventional spectroscopy in visualizing microplastic formation and in characterizing the particles at the submicrometre scale. Here both the surfaces of silicone teats subjected to steam disinfection and the wash waters of the steamed teats were analysed using optical-photothermal infrared microspectroscopy. This new technique revealed submicrometre-resolved steam etching on and chemical modification of the teat surface. Numerous flake- or oil-film-shaped micro(nano)plastics (MNPs) (in the size range of 0.6–332 μm) presented in the wash waters, including cyclic and branched polysiloxanes or polyimides, which were generated by the steam-induced degradation of the base polydimethylsiloxane elastomer and the polyamide resin additive. The results indicated that by the age of one year, a baby could ingest >0.66 million elastomer-derived micro-sized plastics (MPs) (roughly 81% in 1.5–10 μm). Global MP emission from teat disinfection may be as high as 5.2 × 1013 particles per year. Our findings highlight an entry route for surface-active silicone-rubber-derived MNPs into both the human body and the environment. The health and environmental risks of the particles are as yet unknown.

关键词： environmental health and safety issues Imaging techniques Materials Science general Nanotechnology Nanotechnology and Microengineering

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Robust route to H_(2)O_(2)and H_(2)via intermediate water splitting enabled by capitalizing on minimum vanadium-doped piezocatalysts

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Nano Research 2022年第9期15卷 7986-7993页

作者： Yuekun Li Li Li Fangyan Liu Biao Wang Feng Gao Chuan Liu Jingyun Fang Feng Huang Zhang Lin Mengye Wang School of Materials Sun Yat-Sen UniversityShenzhen 518107.State Key Laboratory of Optoelectronic Materials and TechnologiesSun Yat-Sen UniversityGuangzhou 510275China School of Environment and Energy Guangdong Provincial Key Laboratory of Solid Wastes Pollution Control and RecyclingSouth China University of TechnologyGuangzhou 510006China School of Metallurgy and Environment Central South UniversityChangsha 410083China Guangdong Provincial Key Laboratory of Environmental Pollution Control and Remediation Technology School of Environmental Science and EngineeringSun Yat-Sen UniversityGuangzhou 510275China The Guangdong Province Key Laboratory of Display Material and Technology School of Electronics and Information TechnologySun Yat-Sen UniversityGuangzhou 510275China

H_(2)O_(2)is an environmentally friendly chemical for a wide range of water *** industrial production of H_(2)O_(2)is an anthraquinone oxidation process,which,however,consumes extensive energy and produces *** we report a green and sustainable piezocatalytic intermediate water splitting process to simultaneously obtain H_(2)O_(2)and H_(2)using single crystal vanadium(V)-doped NaNbO_(3)(V-NaNbO_(3))nanocubes as *** introduction of V improves the specific surface area and active sites of NaNbO_(3).Notably,V-NaNbO_(3)piezocatalysts of 10 mg exhibit 3.1-fold higher piezocatalytic efficiency than the same catalysts of 50 mg,as more piezocatalysts lead to higher probability of *** aggregation causes reducing active sites and decreased built-in electric field due to the neutralization between different ***,piezocatalytic H_(2)O_(2)and H_(2)production rates of V-NaNbO_(3)(10 mol%)nanocubes(102.6 and 346.2μmol·g^(−1)·h^(−1),respectively)are increased by 2.2 and 4.6 times compared to the as-prepared pristine NaNbO_(3)counterparts,*** improved catalytic efficiency is attributed to the promoted piezo-response and more active sites of NaNbO_(3)catalysts after V doping,as uncovered by piezoresponse force microscopy(PFM)and density functional theory(DFT)*** importantly,our DFT results illustrate that inducing V could reduce the dynamic barrier of water dissociation over NaNbO_(3),thus enhancing the yield of H_(2)O_(2)and H_(2).This facile yet robust piezocatalytic route using minimal amounts of catalysts to obtain H_(2)O_(2)and H_(2)may stand out as a promising candidate for environmental applications and water splitting.

关键词： water splitting H_(2)evolution H_(2)O_(2)production piezocatalysis vanadium-doped NaNbO_(3)

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Predicting Bioaccumulation of Nanomaterials:Modeling Approaches with Challenges

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environment & Health 2024年第4期2卷 189-201页

作者： Hang Zeng Zhuoyan Lv Xiaoyan Sun Yang Tong Wei Wu Shipeng Dong Liang Mao State Key Laboratory of Pollution Control and Resource Reuse School of the EnvironmentChemistry and Biomedicine Innovation CenterNanjing UniversityNanjing 210023China Nanjing Qixia District Hospital Nanjing 210023China High Tech Research and Development Center Ministry of Science and TechnologyBeijing 100044China

Understanding the bioaccumulation of nanomaterials(NMs)by organisms is essential in evaluating their potential ***,the experimental determination of bioaccumulation is substantially challenging,which spawned the development of prediction approaches via establishing models for various *** modeling approaches,such as the biotic ligand model(BLM),partition coefficients,accumulation factor models,and quantitative structure−activity relationship(QSAR)models,were initially used in the application of NMs,aiming to provide a reliable quantitative dose in a resource-saving *** methods,which are based on the uptake patterns of substances,probably lead to deviated results due to the different uptake behaviors of *** this study,currently developed models to evaluate the bioaccumulation of NMs are critically reviewed,with their feasibilities and limitations being *** addition,the recently developed machine learning amended models have taken great efforts in realizing biological behaviors of NMs in organisms by providing in silico *** this data-driven approach has limitations in mechanism exploration,it may give different insights into the bioaccumulation model establishment and critical feature identification.

关键词： Modeling Forecast Bioaccumulation Nanomaterials Machine learning

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