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Dynamic coupling of ferrihydrite transformation and associated arsenic desorption/redistribution mediated by sulfate-reducing bacteria

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Journal of Environmental Sciences 2024年第1期135卷 39-50页

作者： Wenjing Zhou Huiyan Zhu Shiwen Hu Bowei Zhang Kun Gao Zhi Dang Chongxuan Liu State Environmental Protection Key Laboratory of Integrated Surface Water-Groundwater Pollution Control School of Environmental Science and EngineeringSouthern University of Science and TechnologyShenzhen 518055China The Key Lab of Pollution Control and Ecosystem Restoration in Industry Clusters Ministry of EducationSouth China University of TechnologyGuangzhou 510006China

Sulfate-reducing bacteria play an important role in the geochemistry of iron(oxyhydr)oxide and arsenic(As)in natural environments;however,the associated reaction processes are yet to be fully *** this study,batch experiments coupled with geochemical,spectroscopic,microscopic,and thermodynamic analyses were conducted to investigate the dynamic coupling of ferrihydrite transformation and the associated As desorption/redistribution mediated by Desulfovibrio vulgaris(***).The results indicated that *** could induce ferrihydrite transformation via S^(2-)-driven and direct reduction *** the absence of SO_(4)^(2-),*** directly reduced ferrihydrite,and As desorption and re-sorption occurred simultaneously during the partial transformation of ferrihydrite to *** increase in SO_(4)^(2-)loading promoted the S^(2-)-driven reduction of ferrihydrite and accelerated the subsequent mineralogical *** the low and medium SO_(4)^(2-)treatments,ferrihydrite was completely transformed to a mixture of magnetite and mackinawite,which increased the fraction of As in the residual phase and stabilized *** the high SO_(4)^(2-)treatment,although the replacement of ferrihydrite by only mackinawite also increased the fraction of As in the residual phase,22.1%of the total As was released into the solution due to the poor adsorption affinity of As to mackinawite and the conversion of As^(5+)to As^(3+).The mechanisms of ferrihydrite reduction,mineralogy transformation,and As mobilization and redistribution mediated by sulfate-reducing bacteria are closely related to the surrounding SO_(4)^(2-)*** results advance our understanding of the biogeochemical behavior of Fe,S,and As,and are helpful for the risk assessment and remediation of As contamination.

关键词： Sulfate-reducing bacteria Arsenic Ferrihydrite Transformation Redistribution

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Resilience-Oriented Transmission Expansion Planning under Hurricane Impact Considering Vulnerable Line Identification and Hardening

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PROTECTION AND control OF MODERN POWER SYSTEMS 2025年第3期10卷 98-113页

作者： Zhou, Jing Zhang, Heng Cheng, Haozhong Zhang, Shenxi Wang, Zheng Zhang, Xiaohu Electrical Engineering Department Key Laboratory of Control of Power Transmission and Conversion Ministry of Education Shanghai Jiao Tong University Shanghai China East China Branch of State Grid Corporation Shanghai China

Resilient enhancement measures are crucial for increasing systems' capacities to deal with extreme natural disasters. However, in the pre-disaster prevention stage of hurricanes, research that simultaneously considers load importance, vulnerable lines, and multiple resilience enhancement measures is lacking. To address this issue, a novel resilience-oriented transmission expansion planning (ROTEP) model is proposed that incorporates two resilience assessment indices: the combined loss of loads (CLL) and the vulnerable line survival proportion (VLSP). In addition, the novel function of the proposed model meets the requirements of normal and hurricane damage scenarios based on the collaborative implementation of three resilience enhancement measures (expansion planning, hardening, and unit commitment). The proposed ROTEP model is structured in two stages. The first-stage model aims to meet the load growth demand while minimizing the total planning cost of transmission lines, the operating cost of generators, and the penalty cost of wind power and load shedding across several normal scenarios. Based on the scheme obtained from the first-stage model, damage scenarios are constructed, and a fault chain set is formulated using a hurricane simulation model. Then, a cascading fault graph is constructed to identify vulnerable lines. The second-stage model further enhances the CLL and VLSP (if necessary) under several damage scenarios by hardening the highest-contributing or most vulnerable line. Finally, the efficacy of the proposed ROTEP model for enhancing resilience is validated with a modified IEEE RTS-24 system and a two-area IEEE RTS-1996 system.

关键词： Vulnerable line identification resilience enhancement measures hardening unit commitment transmission expansion planning

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A self-cleaning window for high-efficiency photodegradation of indoor formaldehyde

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Chinese Chemical Letters 2024年第9期35卷 340-345页

作者： Changzhu Huang Wei Dai Shimao Deng Yixin Tian Xiaolin Liu Jia Lin Hong Chen Department of Physics Shanghai Key Laboratory of Materials Protection and Advanced Materials in Electric PowerShanghai University of Electric PowerShanghai 200090China Shenzhen Key Laboratory of Interfacial Science and Engineering of Materials State Environmental Protection Key Laboratory of Integrated Surface Water-Groundwater Pollution ControlGuangdong Provincial Key Laboratory of Soil and Groundwater Pollution ControlSchool of Environmental Science and EngineeringSouthern University of Science and TechnologyShenzhen 518055China Eastern Institute for Advanced Study Eastern Institute of TechnologyNingbo 315200China

Formaldehyde(HCHO)as an indoor air pollutant released by new furniture and decorative materials is of great *** a self-cleaning device to remove HCHO is an ideal way to improve indoor air *** this study,a self-cleaning window with a multilayered structure constructed from fluorinedoped tin oxide/bismuth tungstate/resorcinol-formaldehyde resin(FTO/Bi_(2)WO_(6)/RF)has been fabricated,which is capable of degrading HCHO in natural indoor *** as-fabricated device could utilize the natural room light and promote the generation and transfer of the photocatalytic carriers in Bi_(2)WO_(6),which subsequently delivers a good catalytic oxygen reduction efficiency in RF to produce hydrogen peroxide(H_(2)O_(2)).The as-synthesized H_(2)O_(2)could further split into hydroxyl radicals(•OH),then oxide the HCHO molecules in the *** present study demonstrates a novel and efficient strategy to fabricate a transparent multifunctional window for self-cleaning indoor gaseous pollutants,the concept is of great importance to be expanded in a broad range of indoor furniture for in-house air pollution control.

关键词： Bismuth tungstate Resorcinol-formaldehyde Photocatalysis Hydrogen peroxide HCHO degradation

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Adaptive Optimal Output Regulation of Interconnected Singularly Perturbed Systems With Application to Power Systems

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IEEE/CAA Journal of Automatica Sinica 2024年第3期11卷 595-607页

作者： Jianguo Zhao Chunyu Yang Weinan Gao Linna Zhou Xiaomin Liu the Engineering Research Center of Intelligent Control for Underground Space Ministry of EducationChina University of Mining and TechnologyXuzhou 221116 the School of Information and Control Engineering China University of Mining and TechnologyXuzhou 221116 IEEE the State Key Laboratory of Synthetical Automation for Process Industries Northeastern UniversityShenyang 110819China

This article studies the adaptive optimal output regulation problem for a class of interconnected singularly perturbed systems(SPSs) with unknown dynamics based on reinforcement learning(RL).Taking into account the slow and fast characteristics among system states,the interconnected SPS is decomposed into the slow time-scale dynamics and the fast timescale dynamics through singular perturbation *** the fast time-scale dynamics with interconnections,we devise a decentralized optimal control strategy by selecting appropriate weight matrices in the cost *** the slow time-scale dynamics with unknown system parameters,an off-policy RL algorithm with convergence guarantee is given to learn the optimal control strategy in terms of measurement *** combining the slow and fast controllers,we establish the composite decentralized adaptive optimal output regulator,and rigorously analyze the stability and optimality of the closed-loop *** proposed decomposition design not only bypasses the numerical stiffness but also alleviates the *** efficacy of the proposed methodology is validated by a load-frequency control application of a two-area power system.

关键词： Adaptive optimal control decentralized control output regulation reinforcement learning(RL) singularly perturbed systems(SPSs)

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Enhancing the terrain adaptability of a multirobot cooperative transportation system via novel connectors and optimized cooperative strategies

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Frontiers of Mechanical engineering 2023年第3期18卷 79-97页

作者： Quan LIU Zhao GONG Zhenguo NIE Xin-Jun LIU State Key Laboratory of Tribology in Advanced Equipment&Institute of Manufacturing Engineering Department of Mechanical EngineeringTsinghuaUniversityBeijing 100084China Beijing Key Laboratory of Precision/Ultra-precision Manufacturing Equipments and Control Tsinghua UniversityBejing 100084China

Given limited terrain adaptability,most existing multirobot cooperative transportation systems(MRCTSs)mainly work on flat pavements,restricting their outdoor *** connectors'finite deformation capability and the control strategies'limitations are primarily responsible for this *** study proposes a novel MRCTS based on tracked mobile robots(TMRs)to improve terrain adaptability and expand the application scenarios of *** structure design,we develop a novel 6-degree-of-freedom passive adaptive connector to link multiple TMRs and the transported object(the communal payload).In addition,the connector is set with sensors to measure the position and orientation of the robot with respect to the object for feedback *** the control strategy,we present a virtual leader-physical follower collaborative *** leader robot is imaginary to describe the movement of the entire system and manage the follower *** the TMRs in the system act as follower robots to transport the object *** divided the whole control structure into the leader robot level and the follower robot level,we convert the motion control of the two kinds of robots to trajectory tracking control problems and propose a novel double closed-loop kinematics control ***,a control law satisfying saturation constraints is derived to ensure transportation *** adaptive control algorithm processes the wheelbase uncertainty of the ***,we develop a prototype of the TMR-based MRCTS for *** the trajectory tracking experiment,the developed MRCTS with the proposed control scheme can converge to the reference trajectory in the presence of initial tracking errors in a finite *** the outdoor experiment,the proposed MRCTS consisting of four TMRs can successfully transport a payload weighing 60 kg on an uneven road with the single TMR's maximum load limited to 15 *** experimental results demonstrate the effectiveness of

关键词： multirobot system cooperative transportation terain adaptability trajectory tracking collaborative paradigm uneven road

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In-situ construction of abundant active centers on hierarchically porous carbon electrode toward high-performance phosphate electrosorption: Synergistic effect of electric field and capture sites

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Green Energy & Environment 2024年第1期9卷 126-137页

作者： Peng Zhang Fukuan Li Mingming He Silu Huo Xueli Zhang Benqiang Cen Dezhi Fang Kexun Li Hao Wang College of Environmental Science and Engineering Nankai UniversityTianjin300350China MOE Key Laboratory of Pollution Processes and Environmental Criteria Tianjin Key Laboratory of Environmental Remediation and Pollution ControlTianjin Key Laboratory of Environmental Technology for Complex Trans-Media PollutionNankai UniversityTianjin300350China State Key Laboratory of Simulation and Regulation of Water Cycles in River Basins China Institute of Water Resources and Hydropower ResearchBeijing100038China

Phosphate removal is crucial for eutrophication control and water quality ***-assisted adsorption,an eco-friendly elec-trosorption process,exhibited a promising potential for wastewater ***,there are few works focused on phosphate electro-sorption,and reported electrodes cannot attach satisfactory removal capacities and ***,electro-assisted adsorption of phosphate via in-situ construction of La active centers on hierarchically porous carbon(LaPC)has been originally *** resulted LaPC composite not only possessed a hierarchically porous structure with uniformly dispersed La active sites,but also provided good conductivity for interfacial electron *** LaPC electrode achieved an ultrahigh phosphate electrosorption capability of 462.01 mg g^(-1) at 1 V,outperforming most existing *** superior phosphate removal performance originates from abundant active centers formed by the coupling of electricﬁeld and capture ***,the stability and selectivity toward phosphate capture were maintained well even under comprehensive ***,a series of kinetics and isotherms models were employed to validate the electrosorption *** work demonstrates a deep understanding and promotes a new level of phosphate electrosorption.

关键词： Electro-assisted adsorption Electrosorption Phosphate removal Active centers MOF-derived carbon

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Getting insights into gas-phase sulfation effect on catalytic performance of praseodymium oxides in NH_(3)-SCR of NO

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Journal of Rare Earths 2023年第6期41卷 952-958,I0005页

作者： Yandi Cai Peng Yang Qinglong Liu Kaili Ma Wenxin Ma Wang Song Qiuhui Qian Fei Gao Wei Tan Lin Dong State Key Laboratory of Pollution Control and Resource Reuse School of EnvironmentJiangsu Key Laboratory of Vehicle Emissions ControlCenter of Modern AnalysisKey Laboratory of Mesoscopic Chemistry of MOESchool of Chemistry and Chemical EngineeringNanjing UniversityNanjing 210023China Analysis and Testing Center Southeast UniversityNanjing 211189China National and Local Joint Engineering Laboratory of Municipal Sewage Resource Utilization Technology School of Environmental Science and EngineeringSuzhou University of Science and TechnologySuzhou 215009China

Sulfation treatment has been widely used to promote the catalytic performance of ceria(CeO_(2))based catalysts for the selective catalytic reduction of NO by NH_(3)(NH_(3)-SCR of NO).Praseodymium oxide(PrO_(x)),another commonly used rare earth material with similar structural properties as CeO_(2),also shows satistactory redox properties due to the facile redox cycle of Pr^(3+)■Pr^(4+).In this work,gas phase sulfation treatment with varied duration was performed on PrO_(x) at 200℃,and the NH_(3)-SCR activity of sulfated PrO_(x) was *** on the results of systematic characterizations(e.g.,N_(2)-physisorption,NH_(3) oxidation,NO oxidation,in situ diffuse Fourier transform infrared spectroscopy),it is revealed that the catalytic performance of sulfated PrO_(x)is highly dependent on the sulfation time(or the amount of sulfate species deposited on PrO_(x)),which has a significant impact on the competitive reaction between NH_(3) oxidation and NH_(3)-SCR of NO,thus determining the NH_(3)-SCR activity of PrO_(x).This work provides new insight into tuning the interaction between PrO_(x) surface and reactants(NO,NH_(3))via sulfation treatment,which cam guide the design and application of PrO_(x)based catalysts for NH_(3)-SCR of NO in the future.

关键词： NH_(3)-SCR Praseodymium oxides Sulfation treatment Surface acidity NH_(3)oxidation Rare earths

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Functional analysis of SDR112C1 associated with fenpropathrin tolerance in Tetranychus cinnabarinus(Boisduval)

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Insect Science 2025年第2期32卷 585-599页

作者： Jinhang Li Jialu Liu Lishu Peng Jingui Liu Lin Xu Junfeng He Longjiang Sun Guangmao Shen Lin He Key Laboratory of Entomology and Pest Control Engineering College of Plant ProtectionSouthwest UniversityChongqingChina Key Laboratory of Agricultural Biosafety and Green Production of Upper Yangtze River Ministry of EducationChongqingChina National Citrus Engineering Research Center Southwest UniversityChongqingChina Key Scientific Research Base of Pest and Mold Control of Heritage Collection(Chongqing China Three Gorges Museum) State Administration of Cultural HeritageChongqingChina

Short-chain dehydrogenases/reductases(SDRs)are ubiquitously distributed across diverse organisms and play pivotal roles in the growth,as well as endogenous and exogenous metabolism of various substances,including *** expression levels of SDR genes are reportedly upregulated in the fenpropathrin(FEN)-resistant(FeR)strain of Tetranychus ***,the functions of these SDR genes in acaricide tolerance remain *** this study,the activity of SDRs was found to be significantly higher(2.26-fold)in the FeR strain compared to the susceptible strain(SS)of ***.A specific upregulated SDR gene,named SDR112C1,exhibited significant overexpression(3.13-fold)in the FeR population compared with that in the SS ***,the expression of SDR112C1 showed a significant increase in the response to FEN ***,knockdown of the SDR112C1 gene resulted in decreased SDR activity and reduced mite viability against ***,heterologous expression and in vitro incubation assays confirmed that recombinant SDR112C1 could effectively deplete ***,the overexpression of the SDR112C1 gene in Drosophila melanogaster significantly decreased the toxicity of FEN to transgenic fruit *** findings suggest that the overexpression of SDR SDR112C1 is a crucial factor contributing to FEN tolerance in *** discovery not only enhances our understanding of SDR-mediated acaricide tolerance but also introduces a new family of detoxification enzymes to consider in practice,beyond cytochrome P450s,carboxyl/choline esterases and glutathione S-transferases.

关键词： fenpropathrin tolerance heterologous expression polyphagous mite shortchain dehydrogenase transgenic fruit fly

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Exploring reservoir computing:Implementation via double stochastic nanowire networks

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Chinese Physics B 2024年第3期33卷 572-582页

作者：唐健峰夏磊李广隶付军段书凯王丽丹 College of Artificial Intelligence Southwest UniversityChongqing 400715China Brain-inspired Computing & Intelligent Control of Chongqing Key Laboratory Chongqing 400715China National & Local Joint Engineering Laboratory of Intelligent Transmission and Control Technology Chongqing 400715China Chongqing Brain Science Collaborative Innovation Center Chongqing 400715China Key Laboratory of Luminescence Analysis and Molecular Sensing Ministry of EducationSouthwest UniversityChongqing 400715China State Key Laboratory of Intelligent Vehicle Safety Technology Chongqing 400715China

Neuromorphic computing,inspired by the human brain,uses memristor devices for complex *** studies show that self-organizing random nanowires can implement neuromorphic information processing,enabling data *** paper presents a model based on these nanowire networks,with an improved conductance variation *** suggest using these networks for temporal information processing via a reservoir computing scheme and propose an efficient data encoding method using voltage *** nanowire network layer generates dynamic behaviors for pulse voltages,allowing time series prediction *** experiment uses a double stochastic nanowire network architecture for processing multiple input signals,outperforming traditional reservoir computing in terms of fewer nodes,enriched dynamics and improved prediction *** results confirm the high accuracy of this architecture on multiple real-time series datasets,making neuromorphic nanowire networks promising for physical implementation of reservoir computing.

关键词： double-layer stochastic(DS)nanowire network architecture neuromorphic computation nanowire network reservoir computing time series prediction

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Interactions Among Food Systems,Climate Change,and Air Pollution:A Review

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工程（英文） 2025年第1期44卷 215-233页

作者： Chaopeng Hong Rui Zhong Mengyao Xu Peidong He Huibin Mo Yue Qin Danna Shi Xinlei Chen Kebin He Qiang Zhang Shenzhen Key Laboratory of Ecological Remediation and Carbon Sequestration Institute of Environment and EcologyShenzhen International Graduate SchoolTsinghua UniversityShenzhen 518055China State Environmental Protection Key Laboratory of Sources and Control of Air Pollution Complex Beijing 100084China Shenzhen Key Laboratory of Ecological Remediation and Carbon Sequestration Institute of Environment and EcologyShenzhen International Graduate SchoolTsinghua UniversityShenzhen 518055China College of Environmental Sciences and Engineering Peking UniversityBeijing 100871China Institute of Data and Information Shenzhen International Graduate SchoolTsinghua UniversityShenzhen 518055China State Environmental Protection Key Laboratory of Sources and Control of Air Pollution Complex Beijing 100084China State Key Joint Laboratory of Environment Simulation and Pollution Control School of EnvironmentTsinghua UniversityBeijing 100084China Ministry of Education Key Laboratory for Earth System Modeling Department of Earth System ScienceTsinghua UniversityBeijing 100084China

Food systems are deeply affected by climate change and air pollution,while being key contributors to these environmental *** the complex interactions among food systems,climate change,and air pollution is crucial for mitigating climate change,improving air quality,and promoting the sustainable development of food ***,the literature lacks a comprehensive review of these interactions,particularly in the current phase of rapid development in the *** address this gap,this study systematically reviews recent research on the impacts of climate change and air pollution on food systems,as well as the greenhouse gas and air pollutant emissions from agri-food systems and their contribution to global climate change and air *** addition,this study summarizes various strategies for mitigation and adaptation,including adjustments in agricultural practices and food supply *** changes in food systems are urgently needed to enhance adaptability and reduce *** review offers a critical overview of current research on the interactions among food systems,climate change,and air pollution and highlights future research directions to support the transition to sustainable food systems.

关键词： Food systems Climate change Air pollution Interactions Systematic review

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