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Epitaxial growth of borophene on graphene surface towards efficient and broadband photodetector

Nano Research 2024年第4期17卷 3053-3060页

作者： Zenghui Wu Chen Shifan Zitong Wu Yi Liu Wei Shao Xinchao Liang Chuang Hou Guoan Tai The State Key Laboratory of Mechanics and Control of Mechanical Structures and Laboratory of Intelligent Nano Materials and Devices of Ministry of Education College of Aerospace EngineeringNanjing University of Aeronautics and AstronauticsNanjing 210016China

In-situ integration of multiple materials with well-defined interfaces as heterostructures is of great interest due to their unique properties and potential for new device *** of its polymorphism and diverse bonding geometries,borophene is a promising candidate for two-dimensional heterostructures,but suitable synthesis conditions have limited its potential *** this end,we demonstrate the vertical borophene and graphene heterostructures which form by epitaxial growth of borophene onto multilayer graphene on Cu substrates via chemical vapor deposition,where hydrogen and NaBH_(4) are respectively used as the carrier gas and the boron *** lattice structure of the as-synthesized borophene well coincides with the predictedα′-boron *** borophene-based photodetector shows an excellent broadband photoresponse from the ultraviolet(255 nm)to the infrared(940 nm)wavelengths,with enhanced responsivity compared to pristine borophene or graphene *** work informs emerging efforts to integrate borophene into nanoelectronic applications for both fundamental investigations and technological applications.

关键词： borophene graphene heterostructure photodetector two-dimensional materials

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Release characteristics of arsenic from sediments and its source or sink competition with phosphorus:A case of a great lake with grass-algae alternation

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Journal of Environmental Sciences 2025年第3期149卷 278-287页

作者： Shuhang Wang Yongsheng Chang Wei Huang Dianhai Yang Feifei Che State Key Laboratory of Pollution Control and Resource Reuse College of Environmental Science and EngineeringTongji UniversityShanghai 200092China College of Environmental Science and Engineering Donghua UniversityShanghai 201620China National Engineering Laboratory for Lake Pollution Control and Ecological Restoration Chinese Research Academy of Environmental SciencesBeijing 100012China

The arsenic(As)release from sediments in great lakes is affected by various *** this study,the characteristics of As release fromsediments was investigated,and the As sources and sinks with the strengths in sediments from different areas(grass-type,algae-type,and grass-algae alternation areas)in great shallow lakes(Taihu Lake,China)were analyzed,and the influence of P competition in the process of As release was also *** results showed that changing trend of the values of equilibrium As concentration in sediments were consistent with the regional changes(0 to 28.12μg/L),and the sediments from algaetype areas had the higher *** sediments from western lake and northwest lake bay were a strong As and a weak P source,and the north lake bay had the opposite trend of these two *** P source competition with As from the sediments occurred in algae-type *** grass-type areas had strong As and P retention capacities,indicating a sink role of sediment with high As and P sorption *** degree of As and P saturation had similar trend in sediments,and the grass-type areas had the higher values,18.3%-21.4%and 15.31%-20.34%,*** analysis results showed that most of As release contribution was from the bottom(30-50 cm)sediments,and the surface(0-10 cm)sediments from algae-type areas contributed more to the overlying water than other region.

关键词： Arsenic Phosphorus Sediment Source and sink Contribution

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Technologies for pollutant removal and resource recovery from blackwater:a review

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Frontiers of Environmental Science & engineering 2023年第7期17卷 57-77页

作者： Wei Zhang Huaqiang Chu Libin Yang Xiaogang You Zhenjiang Yu Yalei Zhang Xuefei Zhou State Key Laboratory of Pollution Control and Resource Reuse College of Environmental Science and EngineeringTongji UniversityShanghai 200092China

Blackwater(BW),consisting of feces,urine,flushing water and toilet paper,makes up an important portion of domestic *** improper disposal of BW may lead to environmental pollution and disease transmission,threatening the sustainabie development of the *** in nutrients and organic matter,BW could be treated for resource recovery and reuse through various *** at providing guidance for the future development of BW treatment and resource recovery,this paper presented a literature review of BWs produced in different countries and types of toilets,including their physiochemical characteristics,and current treatment and resource recovery *** degradation and utilization of carbon(C),nitrogen(N)and phosphorus(P)within BW are *** performance of different systems was classified and *** all the treating systems,biological and ecological systems have been long and widely applied for BW treatment,showing their universality and operability in nutrients and energy recovery,but they are either slow or ineffective in removal of some refractory *** processes,especially advanced oxidation processes(AOPs),are becoming increasingly extensively studied in BW treatment because of their high efficiency,especially for the removal of micropollutants and *** review could serve as an instructive guidance for the design and optimization of BW treatment technologies,aiming to help in the fulfilment of sustainable human excreta management.

关键词： Blackwater Water-flushing toilet Sanitation Nutrientrecovery Waterreuse Sustainable development

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Nanogenerator-based bidirectional pressure sensor array and its demonstration in underwater invasive species detection

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Nano Research 2023年第9期16卷 11822-11831页

作者： Yunqi Cao Hongyang Shi Xiaobo Tan Nelson Sepúlveda State Key Laboratory of Industrial Control Technology College of Control Science and EngineeringZhejiang UniversityHangzhou 310027China Department of Electrical and Computer Engineering Michigan State UniversityEast LansingMichigan 48824USA

Lakes areas,which cause catastrophic damages in both commercial fishery and ecological ***,current assessment strategies may pose challenges for lake-wide abundance estimation and non-target anadromous species ***,we demonstrate an efficacious species-specific non-destructive sensing system based on porous ferroelectret nanogenerator for in-situ monitoring of lamprey spawning migration using their unique suction *** show that the porous structure enables a redistribution of surface charges under bidirectional deformations,which allows the detection of both positive and negative *** quasi-piezoelectric effect is further validated by quantitative analysis in a wide pressure range of−50 to 60 kPa,providing detailed insights into transduction working *** reliable lamprey detection,a 4×4-pixel sensor array is developed and integrated with a complementary metal-oxide-semiconductor(CMOS)based signal processing array thus constituting a sensing panel capable of recording oral suction patterns in an underwater environment.

关键词： bidirectional pressure sensing nanogenerators self-powered sensor array ferroelectret invasive species detection

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Characterizing molecular fingerprint of dissolved organic matter shaped by natural and anthropogenic factors in a large macrophytic shallow lake wetland

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Frontiers of Environmental Science & engineering 2025年第3期19卷 73-86页

作者： Shengwu Yuan Yiping Xu Pengfei Wang Ruili Xie Jiangbo Hu Zhenghui Fu Kun Wang Shuhang Wang Xia Jiang Kaifeng Rao Mei Ma Zijian Wang State Key Laboratory of Environmental Criteria and Risk Assessment National Engineering Laboratory for Lake Pollution Control and Ecological RestorationState Environment Protection Key Laboratory for Lake Pollution ControlState Environmental Protection Key Laboratory of Drinking Water Source ProtectionChinese Research Academy of Environmental ScienceBeijing 100012China Research Center for Eco-Environmental Sciences Chinese Academy of SciencesBeijing 100085China College of Resources and Environment University of Chinese Academy of SciencesBeijing 100049China

Dissolved organic matter(DOM)participates in and affects many biological processes in aquatic ecosystems,altering nutrient cycling,bioavailability and toxicity of *** water contains thousands of DOM molecules,which largely originate from natural sources and are greatly influenced by external inputs through anthropogenic *** elucidate the shaping mechanism of the DOM composition under complex habitat conditions and anthropogenic disturbances,the characteristic molecular fingerprint of DOM was determined based on chemodiversity information obtained via ultrahigh-resolution mass spectrometry for the Baiyangdian wetland(a typical large macrophytic shallow lake in North China).In the Baiyangdian wetland,the DOM composition exhibited high complexity and spatial heterogeneity,and more recalcitrant DOM molecules were identified in summer than in *** multiple natural factors(nutrient concentration,depth of water and quality of submerged macrophytes)and anthropogenic factors(different land uses and discharge of pollutants)were associated with the relative abundance of various DOM molecules,only the influences from the anthropogenic factors were statistically *** alpha diversity index of DOM could reflect variations in both the natural factors(total dissolved phosphorus)and the anthropogenic factors(discharge of nitrogen and phosphorus).Furthermore,the DOM composition in each group were clustered according to the ecological functions(natural reserves,tourism,breeding,and domestic supply functions),and exhibited molecular fingerprint *** study provides an effective approach to characterize the molecular fingerprint features of DOM and critical information to better understand the shaping mechanism of the DOM composition under complex habitat conditions and anthropogenic disturbances.

关键词： DOM FT-ICR-MS Chemodiversity Habitat Ecological function Baiyangdian wetland

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QTFN:A General End-to-End Time-Frequency Network to Reveal the Time-Varying Signatures of the Time Series

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Big Data Mining and Analytics 2024年第3期7卷 905-919页

作者： Tao Chen Yang Jiao Lei Xie Hongye Su State Key Laboratory of Industrial Control Technology Zhejiang UniversityHangzhou 310027China Shenzhen Key Laboratory of Intelligent Bioinformatics and College of Computer Science and Control EngineeringShenzhen Institute of Advanced TechnologyChinese Academy of SciencesShenzhen 518055China

Nonstationary time series are ubiquitous in almost all natural and engineering *** the time-varying signatures from nonstationary time series is still a challenging problem for data *** Time-Frequency Distribution(TFD)provides a powerful tool to analyze these ***,they suffer from Cross-Term(CT)issues that impair the readability of ***,to achieve high-resolution and CT-free TFDs,an end-to-end architecture termed Quadratic TF-Net(QTFN)is proposed in this *** by classic TFD theory,the design of this deep learning architecture is heuristic,which firstly generates various basis functions through ***,more comprehensive TF features can be extracted by these basis ***,to balance the results of various basis functions adaptively,the Efficient Channel Attention(ECA)block is also embedded into ***,a new structure called Muti-scale Residual Encoder-Decoder(MRED)is also proposed to improve the learning ability of the model by highly integrating the multi-scale learning and encoder-decoder ***,although the model is only trained by synthetic signals,both synthetic and real-world signals are tested to validate the generalization capability and superiority of the proposed QTFN.

关键词： Time-Frequency Analysis(TFA) Multi-scale Residual Encoder-Decoder(MRED) quadratic Time-Frequency Distribution(TFD)

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Fluid evolution and fragmentation characteristics under high pressure water jet impact on thermal rock

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International Journal of Mining Science and Technology 2025年第3期35卷 483-497页

作者： Jianming Shangguan Zhaolong Ge Qinglin Deng Yuhuai Cui Zhi Yao State Key Laboratory of Coal Mine Disaster Dynamics and Control Chongqing UniversityChongqing 400044China School of Resources and Safety Engineering Chongqing UniversityChongqing 400044China

In the application of high-pressure water jet assisted breaking of deep underground rock engineering,the influence mechanism of rock temperature on the rock fragmentation process under jet action is still ***,the fluid evolution characteristics and rock fracture behavior during jet impingement were *** results indicate that the breaking process of high-temperature rock by jet impact can be divided into four stages:initial fluid-solid contact stage,intense thermal exchange stage,perforation and fracturing stage,and crack propagation and penetration *** the increase of rock temperature,the jet reflection angles and the time required for complete cooling of the impact surface significantly decrease,while the number of cracks and crack propagation rate significantly increase,and the rock breaking critical time is shortened by up to 34.5%.Based on numerical simulation results,it was found that the center temperature of granite at 400℃ rapidly decreased from 390 to 260℃ within 0.7 s under jet *** addition,a critical temperature and critical heat flux prediction model considering the staged breaking of hot rocks was *** findings provide valuable insights to guide the water jet technology assisted deep ground hot rock excavation project.

关键词： Fluid evolution Fragmentation characteristics Fracture process Water jet Thermal rock

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Visualization and characterization of experimental hydraulic fractures interacting with karst fracture-cavity distributions

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Journal of Rock Mechanics and Geotechnical engineering 2024年第5期16卷 1667-1683页

作者： Hanzhi Yang Xin Chang Chunhe Yang Wuhao Guo Lei Wang Guokai Zhao Yintong Guo State Key Laboratory of Coal Mine Disaster Dynamics and Control Chongqing UniversityChongqing400044China State Key Laboratory of Geomechanics and Geotechnical Engineering Institute of Rock and Soil MechanicsChinese Academy of SciencesWuhan430071China

Karst fracture-cavity carbonate reservoirs,in which natural cavities are connected by natural fractures to form cavity clusters in many circumstances,have become significant fields of oil and gas exploration and *** fracturing is considered as the best method for exploiting carbonate reservoirs;however,previous studies primarily focused on the effects of individual types of geological formations,such as natural fractures or cavities,on fracture *** this study,true-triaxial physical simulation experiments were systematically performed under four types of stress difference conditions after the accurate prefabrication of four types of different fracture-cavity distributions in artificial ***,the interaction mechanism between the hydraulic fractures and fracture-cavity structures was systematically analyzed in combination with the stress distribution,cross-sectional morphology of the main propagation path,and three-dimensional visualization of the overall fracture *** was found that the propagation of hydraulic fractures near the cavity was inhibited by the stress concentration surrounding the *** contrast,a natural fracture with a smaller approach angle(0°and 30°)around the cavity can alleviate the stress concentration and significantly facilitate the connection with the *** addition,the hydraulic fracture crossed the natural fracture at the 45°approach angle and bypassed the cavity under higher stress difference conditions.A new stimulation effectiveness evaluation index was established based on the stimulated reservoir area(SRA),tortuosity of the hydraulic fractures(T),and connectivity index(CI)of the *** findings provide new insights into the fracturing design of carbonate reservoirs.

关键词： Karst fracture-cavity reservoir Fracturing experiment Fracture propagation Cross-sectional morphology Stimulation effectiveness

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Antibiotics-heavy metals combined pollution in agricultural soils: Sources, fate, risks, and countermeasures

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Green Energy and Environment 2025年第5期10卷 869-897页

作者： Shu, Yuanxiang Li, Donghao Xie, Tong Zhao, Ke Zhou, Lu Li, Fengxiang College of Environmental Science and Engineering Ministry of Education Key Laboratory of Pollution Processes and Environmental Criteria Remediation and Pollution Control for Urban Ecological Environmental Nankai University Tianjin300350 China College of Municipal and Environmental Engineering Ministry of Education Key Laboratory of Songliao Aquatic Environment Jilin Jianzhu University Changchun130118 China College of the Environment State Key Laboratory of Pollution Control and Resource Reuse Jiangsu Key Laboratory of Vehicle Emissions Control Nanjing University Nanjing210023 China

Agricultural soil is related to food security and human health, antibiotics and heavy metals (HMs), as two typical pollutants, possess a high coexistence rate in the environmental medium, which is extremely prone to inducing antibiotic-HMs combined pollution. Recently, frequent human activities have led to more prominent antibiotics-HMs combined contamination in agricultural soils, especially the production and spread of antibiotic resistance genes (ARGs), heavy metal resistance genes (MRGs), antibiotic resistant bacteria (ARB), and antibiotics-HMs complexes (AMCs), which seriously threaten soil ecology and human health. This review describes the main sources (Intrinsic and manmade sources), composite mechanisms (co-selective resistance, oxidative stress, and Joint toxicity mechanism), environmental fate and the potential risks (soil ecological and human health risks) of antibiotics and HMs in agricultural soils. Finally, the current effective source blocking, transmission control, and attenuation strategies are classified for discussion, such as the application of additives and barrier materials, as well as plant and animal remediation and bioremediation, etc., pointing out that future research should focus on the whole chain process of "source-process-terminal", intending to provide a theoretical basis and decision-making reference for future research. © 2024 Institute of Process engineering, Chinese Academy of Sciences

关键词： Bioremediation

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Feature-Aligned Stacked Autoencoder: A Novel Semisupervised Deep Learning Model for Pattern Classification of Industrial Faults

IEEE Transactions on Artificial Intelligence

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IEEE Transactions on Artificial Intelligence 2023年第4期4卷 592-601页

作者： Zhang, Xinmin Zhang, Hongyi Song, Zhihuan Zhejiang University College of Control Science and Engineering State Key Laboratory Industrial Control Technology Hangzhou310027 China

Autoencoder is a widely used deep learning method, which first extracts features from all data through unsupervised reconstruction, and then fine-tunes the network with labeled data. However, due to the limited number of labeled data samples, the network may lack sufficient generalization ability and is prone to overfitting. This article proposes a new semisupervised deep learning method called feature-aligned stacked autoencoder (FA-SAE). FA-SAE takes advantage of the unlabeled data during the fine-tuning process by aligning the feature of both labeled and unlabeled data. In FA-SAE, a new training loss function is designed by integrating the Sinkhorn distance measure of the difference between the features extracted from labeled and unlabeled data through the neural network into the cross-entropy classification loss. The effectiveness of the proposed FA-SAE is verified through its application to two industrial processes, and the application results demonstrated that the proposed FA-SAE has better generalization ability and higher fault classification accuracy as compared to the state-of-the-art methods. © 2020 IEEE.

关键词： Deep learning

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