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SSRN 2024年

作者： Nie, Xiongfei Qiu, Xinjie Zhang, Ruina Ke, Quanli Liu, Huayan Zhang, Xiangping Lu, Hanfeng Cui, Guokai Zhang, Suojiang Innovation Team of Air Pollution Control Institute of Catalytic Reaction Engineering State Key Laboratory Breeding Base of Green Chemistry Synthesis Technology College of Chemical Engineering Zhejiang University of Technology Hangzhou310014 China Beijing Key Laboratory of Ionic Liquids Clean Process CAS Key Laboratory of Green Process and Engineering State Key Laboratory of Multiphase Complex Systems Institute of Process Engineering Chinese Academy of Sciences Beijing100190 China

Developing advanced sorbents for efficient aromatic VOCs sorption from humid conditions are highly desired. In this work, a series of tunable and functional ionic liquids embedded hyper-crosslinked polymers (ILHCPs) containing different structures of anion-functional ionic liquids (ILs) with 1,4-dichloroxylene (DCX) as the crosslinker were designed and prepared for highly efficient gaseous toluene adsorption under humidity. These ILHCPs could achieve high surface area (600~900 m2 g−1), high micropore volume (0.1~0.3 cm3 g−1), small average pore size (4~5 nm), and large water contact angle (up to 110°) through tuning the anion structures and the initial IL:DCX molar ratio. Gaseous toluene adsorption isotherms on typical ILHCPs were tested under 298, 308, and 318 K, and a dual-site Langmuir-Freundlich (DSLF) model was used for well describing adsorption isotherms, which can be divided into two contributions for site I and site II. The isosteric heats of gaseous toluene adsorption were calculated. Furthermore, toluene adsorption under different humidity conditions were also tested. Compared with DCX-based self-condensed HCP, toluene adsorption capacity of ILHCPs remained steadily (270 mg g−1) even under 80% humidity. To our best knowledge, this is the first example of tuning functional ILHCPs for efficient H2O-tolerant gaseous toluene adsorption. The method may also open a door to achieving high adsorption efficiency of other volatile organic compounds by functional IL-based porous materials. © 2024, The Authors. All rights reserved.

关键词： Gas adsorption

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Electrochemical CO_(2) reduction with ionic liquids: review and evaluation

Industrial Chemistry & Materials

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Industrial Chemistry & Materials 2023年第3期1卷 410-430页

作者： Yangshuo Li Fangfang Li Aatto Laaksonen Chuan Wang Paul Cobden Per Boden Yanrong Liu Xiangping Zhang Xiaoyan Ji Energy Engineering Division of Energy ScienceLulea University of TechnologyLuleå97187Sweden Department of Materials and Environmental Chemistry Arrhenius LaboratoryStockholm University10691 StockholmSweden Centre of Advanced Research in Bionanoconjugates and Biopolymers Petru Poni Institute of Macromolecular ChemistryAleea Grigore Ghica-Voda41A700487 IasiRomania State Key Laboratory of Materials-Oriented and Chemical Engineering Nanjing Tech UniversityNanjing210009P.R.China University of Cagliari Department of Chemical and Geological SciencesCampus MonserratoSS 554 bivio per Sestu09042MonserratoItaly Metallurgy Department Swerim AB97125LuleåSweden SMA Mineral AB 68227FilipstadSweden CAS Key Laboratory of Green Process and Engineering Beijing Key Laboratory of Ionic Liquids Clean ProcessState Key Laboratory of Multiphase Complex SystemsInstitute of Process EngineeringChinese Academy of SciencesBeijing 100190China

The increasing CO_(2) emission,as the chief culprit causing numerous environmental problems,could be addressed by the electrochemical CO_(2) reduction(CO_(2)R)to the added-value carbon-based *** liquids(ILs)as electrolytes and co-catalysts have been widely studied to promote CO_(2)R owing to their unique *** the potential products of CO_(2)R,those only containing one carbon atom,named C1 products,including CO,CH_(3)OH,CH_(4),and syngas,are easier to achieve than *** this study,we first summarized the research status on CO_(2)R to these C1 products,and then,the state-of-theart experimental results were used to evaluate the economic potential and environmental *** the rapid development in CO_(2)R,future scenarios with better CO_(2)R performances were reasonably assumed to predict the future business for each *** the studied C1 products,the research focuses on CO,where satisfactory results have been *** evaluation shows that producing CO via CO_(2)R is the only profitable route at ***3OH and syngas of H2/CO(1:1)as the targeted products can become profitable in the foreseen *** addition,the life cycle assessment(LCA)was used to evaluate the environmental impact,showing that CO_(2)R to CH4 is the most environmentally friendly pathway,followed by the syngas of H_(2)/CO(2:1)and CO,and the further improvement of the CO_(2)R performance can make all the studied C1 products more environmentally ***,CO is the most promising product from both economic and environmental impact aspects.

关键词： Electrochemical-CO_(2)-reduction Ionic-liquids C1-product Economic-evaluation Environmental-impact

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Exact Algorithm for Batch Scheduling with Many-to-Many Job-Tool Matching and Job Release Time Constraints

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IEEE Transactions on Automation Science and engineering 2025年 22卷 16499-16511页

作者： Li, Shengchao Liu, Shixin Zhao, Ziyan Zhou, Mengchu Northeastern University State Key Laboratory of Synthetical Automation for Process Industries College of Information Science and Engineering Shenyang 110819 China Northeastern University at Qinhuangdao Hebei Key Laboratory of Industrial Software for Advanced Planning and Scheduling of Complex Industrial Processes School of Control Engineering Qinhuangdao 066004 China New Jersey Institute of Technology Department of Electrical and Computer Engineering Newark 07102 NJ United States

Job-dependent tool switching is necessary in many batch processing systems (BPSs). Heterogeneous tool demand and extra time consumption for tool switch bring great challenge for high-performance production scheduling in BPSs. In this study, we present a novel batch scheduling problem derived from a satellite vibration test system. Different from basic scheduling problems in BPSs with tool switching, it has complications caused by many-to-many task-tool matching and job release time constraints. Specifically, each job has predetermined candidate tools. One of them should be selected and equipped to process a given job. Unlike sequence-dependent setup time that is only related to two adjacent jobs, tool switching time is additionally dependent on the tools selected by both jobs from their respective candidate tools. Both job sequence and tool selections need to be determined to minimize makespan. Mixed-integer linear programming (MILP) and constraint programming (CP) models are developed for formulating the problem. We prove that the problem is NP hard. To obtain exact solutions, we propose a novel branch-and-bound algorithm (B&B) based on the analysis and extraction of problem properties. It integrates a domain reduction mechanism, branching strategies, and dominance rules. Among them, the domain reduction mechanism reduces the number of jobs to be scheduled;the branching strategies accelerate solving speed;and the dominance rules save the memory consumption. Ablation studies and key influencing factor experiments are performed. The results show that the proposed B&B can optimally solve much larger instances than state-of-the-art methods (including some heuristics). It can optimally solve industrial-size problems in a short time, implying that it can well satisfy the performance demand of a satellite vibration test system and thus advancing the filed of optimal scheduling for BPSs. © 2004-2012 IEEE.

关键词： Batch scheduling branch-and-bound algorithm heterogenerous tool demand mixed-integer linear programming satellite vibration test system

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Stimuli-Responsive lonic Liquids and the Regulation of Aggrega-tion Structure and Phase Behavior

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Chinese Journal of Chemistry 2021年第3期39卷 729-744页

作者： Xiao-Qing Yuan Ya-Qin Zhang Zhi-Yong Li Feng Huo Yi-Hui Dong Hong-Yan He Beijing Key Laboratory of lonic Liquids Clean Process CAS Key Laboratory of Green Process and EngineeringState Key Laboratory of Multiphase Complex SystemsInstitute of Process EngineeringChinese Academy of SciencesBejling 100190China Dalian National Laboratory for Clean Energy DalianLiaoning 116023China Collaborative Innovation Center of Henan Province for Green Manufacturing of Fine Chemicals Key Laboratory of Green Chermical Media and ReactionsMinistry of EducationSchool of Chemistry and Chemical EngineeringHenan Normal UniversityXinxiangHenan 453007China

lonic liquids with stimuli-responsive characteristics are an essential branch in the comprehensive ionic liquids'family,which can meet the controllable and reversible needs in practical applications with different stimulation *** this review,we summarize the recent research progress of these stimuli-responsive ionic liquids,mainly focusing on their chemical structures,properties,responsive mechanism,aggregation structures,and phase behaviors,which were driven by external stimuli,such as CO2,magnetism,light,temperature,redox,and ***,the particular or potential applications of stimuli-responsive ionic liquids are expounded in various fields of science,including catalytic reaction,extraction,separation,nano-material preparation,and gas *** the end,the challenges and strategies of the subject are briefly *** is expected that this review will contribute to the rational design and applications of stimu-liresponsive ionic liquids in the future.

关键词： lonic liquids Stimuli Responsive Aggregation Phase behavior

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Versatility of π-d Conjugated Coordination Nickel Metal-Organic Frameworks as Electrode Materials of Metal-Ion Batteries

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Energy Material Advances 2024年第1期5卷 120-132页

作者： Zaohong Zhang Kaihui Xu Jing Yang Zhuoyu Ji Yunchen Ge Zhicong Shi Yongwei Zhang Kai Zhang Chuan Wu Jia Hong Pan State Key Laboratory of Featured Metal Materials and Life-Cycle Safety for Composite Structures School of ResourcesEnvironments and MaterialsGuangxi UniversityNanning 530004China Low Carbon Energy Process Intensification Research Institute and MOE Key Laboratory of Resources and Environmental Systems Optimization North China Electric Power UniversityBeijing 102206China Institute of High Performance Computing Agency for ScienceTechnology and Research(A*STAR)Singapore 138632Singapore Guangxi Key Laboratory of Manufacturing Systems and Advanced Manufacturing Technology Guilin University of Electronic TechnologyGuilin 541004China School of Materials Science and Engineering Beijing Institute of TechnologyBeijing 100081China Beijing Key Laboratory of Environmental Science and Engineering School of Materials Science and EngineeringBeijing Institute of TechnologyBeijing 100081China Yangtze Delta Region Academy of Beijing Institute of Technology Jiaxing 314019China

Metal-organic frameworks have emerged as promising electrode materials for metal-ion batteries due to their superior structural ***,they face challenges such as poor reversibility and easy degradation during electrochemical redox ***,we report the synthesis ofπ-d conjugated coordination polymers through NH_(3)-vapor-assisted self-polymerization of NiCl_(2)·6H_(2)O with 1,2,4,5-benzenetetramine tetrahydrochloride(namely,Ni-BTA).The synthesized Ni-BTA exhibits an open lattice structure that enhances the capacity for metal-ion diffusion,ensuring prolonged electrochemical cycling ***,electrochemical characterizations reveal that Ni-BTA functions as a bifunctional material,serving as both cathode and anode materials for lithium-ion batteries(LIBs).After 1,000 cycles at 1.0 A g^(−1),the cathode and anode show high discharge capacities of 199.7 and 338.4 mAh g^(−1),***,symmetrical all-organic batteries constructed with Ni-BTA exhibit a high specific capacity of 30.6 mAh g-1 and an ultrastable coulombic efficiency of approximately≈100%after 6,000 cycles at 1.0 A g^(−1).Furthermore,Ni-BTA exhibits versatility as a robust cathode for aluminum ion batteries(AIBs),delivering a discharge capacity of 18.7 mAh g^(−1) after 10,000 cycles at 1.0 A g^(−1).These findings highlight the potential of Ni-BTA as a versatile and durable electrode materials for both LIBs and AIBs.

关键词： d conjugation electrochemical stability open lattice stru metal ion batteries electrochemical redox processesherewe lithium ion batteries coordination polymers electrode materials

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Efficient fluidization intensification process to fabricate in-situ dispersed(SiO+G)/CNTs composites for high-performance lithium-ion battery anode applications

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Particuology 2021年第3期19卷 84-90页

作者： Hebang Shi He Zhang Chaoquan Hu Shaofu Li Maoqiao Xiang Pengpeng Lv Qingshan Zhu State key Laboratory of Multiphase Complex Systems Institute of Process EngineeringChinese Academy of SciencesBeijing 100190China University of Chinese Academy of Science Beijing 100049China College of Materials and Metallurgy Guizhou UniversityGuiyang 550025China Nanjing IPE Institute of Green Manufacturing Industry Nanjing 211135China

An efficient fluidization process intensification method was proposed to prepare carbon nanotube(CNT)-enhanced high-performance SiO anodes for lithium-ion *** introduction of graphite particles decreased bonding among SiO particles,inhibiting agglomerate growth and enhancing ***(SiO+G)/CNTs composites were synthesized by fluidized bed chemical vapor deposition with the CNTs grown in-situ,which ensured uniform dispersion and superior anchoring of the *** in-situ-grown CNTs and stacked graphite ensured excellent structural stability and *** synthesized(SiO+G)/CNTs delivered a stable reversible capacity of 466 mAh g^(−1) after 125 cycles and a capacity of∼200 mAh g^(−1) at 2 A g^(−1).The charging results indicated that the 3D network structure comprising CNTs and graphite not only effectively buffered the electrode expansion but also greatly improved mechanical flexibility.

关键词： process intensification Fluidized bed chemical vapor deposition Carbon nanotubes Silicon suboxide anode

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Advances in thermal-related analysis techniques for solid-state lithium batteries

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InfoMat 2023年第4期5卷 77-116页

作者： Jianan Wang Kai Yang Shiyi Sun Qianyue Ma Gong Yi Xin Chen Ze Wang Wei Yan Xinhua Liu Qiong Cai Yunlong Zhao Department of Environmental Science and Engineering State Key Laboratory of Multiphase Flow in Power EngineeringSchool of Energy and Power EngineeringXi'an Jiaotong UniversityXi'anthe People's Republic of China Department of Chemical&Process Engineering Faculty of Engineering and Physical SciencesUniversity of SurreyGuildfordUK Advanced Technology Institute University of SurreyGuildfordUK School of Transportation Science and Engineering Beihang UniversityBeijingthe People's Republic of China

Solid-state lithium batteries(SSLBs)have been broadly accepted as a promising candidate for the next generation lithium-ion batteries(LIBs)with high energy density,long duration,and high *** intrinsic non-flammable nature and electrochemical/thermal/mechanical stability of solid electrolytes are expected to fundamentally solve the safety problems of conventional ***,thermal degradation and thermal runaway could also happen in *** example,the large interfacial resistance between solid electrolytes and electrodes could aggravate the joule heat generation;the anisotropic thermal diffusion could trigger the uneven temperature distribution and formation of hotspots further leading to lithium dendrite *** research efforts have been devoted to exploring solid electrolytes with outstanding performance and harmonizing interfacial incompatibility in the past *** have been fewer comprehensive reports investigating the thermal reaction process,thermal degradation,and thermal runaway of *** review seeks to highlight advanced thermal-related analysis techniques for SSLBs,by focusing particularly on multiscale and multidimensional thermal-related characterization,thermal monitoring techniques such as sensors,thermal experimental techniques imitating the abuse operating condition,and thermalrelated advanced *** perspectives are proposed to bridge fundamental studies to technological relevance for better understanding and performance optimization of SSLBs.

关键词： characterization monitoring simulation solid-state batteries thermal technique

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Mesoscale structures and mechanisms in ionic liquids

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Particuology 2020年第1期18卷 55-64页

作者： Xiaomin Liu Xiaoqian Yao Yanlei Wang Suojiang Zhang School of Chemistry and Chemical Engineering Qingdao UniversityQingdao 266071ShandongChina Beijing Key Laboratory of Ionic Liquids Clean Process State Key Laboratory of Multiphase Complex SystemsKey Laboratory of Green Process and EngineeringInstitute of process EngineeringChinese Academy of SciencesBeijing 100190China

Ionic liquids(ILs)have attracted intensive attention and have been used widely in many applications because of their diversified properties,which are caused by the special structure of the *** clusters are one of the typical structures that exist widely in the IL *** are stable under certain conditions and change under other *** clusters are a typical mesoscale phenomenon in *** this review,we summarize our recent progress related to ionic clusters,including the ionic-cluster structure,changing mechanisms,and their effect on the physicochemical *** cluster investigation based on mesoscience is very important,will provide new insight into the structures and properties of ILs,and will boost further exploration of IL applications.

关键词： Ionic liquid Mesoscale structure Ionic cluster

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Ionic liquids/deep eutectic solvents for CO_(2) capture:Reviewing and evaluating

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Green Energy & Environment 2021年第3期6卷 314-328页

作者： Yanrong Liu Zhengxing Dai Zhibo Zhang Shaojuan Zeng Fangfang Li Xiangping Zhang Yi Nie Lei Zhang Suojiang Zhang Xiaoyan Ji Energy Engineering Division of Energy ScienceLuleåUniversity of TechnologyLuleåSweden Swerim AB Box 812SE-97125LuleåSweden State Key Laboratory of Material-Oriented Chemical Engineering Nanjing Tech UniversityNanjingChina CAS Key Laboratory of Green Process and Engineering Beijing Key Laboratory of Ionic Liquids Clean ProcessState Key Laboratory of Multiphase Complex SystemsInstitute of Process EngineeringChinese Academy of SciencesBeijingChina Zhengzhou Institute of Emerging Industrial Technology ZhengzhouChina College of Materials Science and Engineering Fujian University of TechnologyFuzhouFujian350118China School of Chemical Engineering University of Chinese Academy of SciencesBeijingChina

The CO_(2)solubilities(including CO_(2)Henry’s constant)in physical-and chemical-based ILs/DESs and the COSMO-RS models describing these properties were comprehensively collected and *** summarized results indicate that chemical-based ILs/DESs are superior to physical-based ILs/DESs for CO_(2)capture,especially those ILs have functionalized cation and anion,and superbase DESs;some of the superbase DESs have higher CO_(2)solubilities than those of ILs;the best physical-and chemical-based ILs,as well as physical-and chemicalbased DESs are[BMIM][BF4](4.20 mol kg^(-1)),[DETAH][Im](11.91 mol kg^(-1)),[L-Arg]-Gly 1:6(4.92 mol kg^(-1))and TBD-EG 1:4(12.90 mol kg^(-1)),*** the original COSMO-RS mainly providing qualitative predictions,six corrected COSMO-RS models have been proposed to improve the prediction performance based on the experimental data,but only one model is with universal *** newly determined experimental results were further used to verify the perditions of original and corrected COSMO-RS *** comparison indicates that the original COSMO-RS qualitatively predicts CO_(2)solubility for some but not all ILs/DESs,while the quantitative prediction is incapable at *** original COSMO-RS is capable to predict CO_(2)Henry’s constant qualitatively for both physical-based ILs and DESs,and quantitative prediction is only available for *** the corrected COSMO-RS models,only the model with universal parameters provides quantitative predictions for CO_(2)solubility in physical-based DESs,while other corrected models always show large deviations(>83%)compared with the experimental CO_(2)Henry’s constants.

关键词： Ionic liquid Deep eutectic solvent CO_(2)solubility Henry’s constant COSMO-RS

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Nanomaterials for co‐immobilization of multiple enzymes

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BMEMat(BioMedical engineering Materials) 2025年第1期3卷 92-115页

作者： Jingyu Zhang Jonathan F.Lovell Jiafu Shi Yumiao Zhang School of Chemical Engineering and Technology Key Laboratory of Systems Bioengineering(Ministry of Education)Frontiers Science Center for Synthetic Biology(Ministry of Education)Tianjin UniversityTianjinChina Department of Biomedical Engineering The State University of New York at BuffaloBuffaloUSA School of Environmental Science and Engineering Collaborative Innovation Center of Chemical Science and Engineering(Tianjin)TianjinChina State Key Laboratory of Biochemical Engineering Institute of Process EngineeringChinese Academy of SciencesBeijingChina

In order to co‐immobilize multiple enzymes,a wide range of nanomaterials has been designed to achieve synergistic enzyme activity and enhance catalytic ***,as carriers for enzyme co‐immobilization,possess various advantages such as tunable morphology and size,high specific surface area,and abundant chemically active *** can significantly enhance enzyme stability,activity,and catalytic *** overview the commonly used methods and strategies of enzyme co‐*** review further summarizes the latest research advances in nanomaterials for enzyme coimmobilization applications over the past 5 ***,the advantages and challenges of these nanomaterials used for enzyme co‐immobilization as well as some potential future directions are also discussed.

关键词： cascade enzymatic reactions co‐immobilization enzyme immobilization nanoparticles

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