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Advances in thermal-related analysis techniques for solid-state lithium batteries

InfoMat 2023年第4期5卷 77-116页

作者： Jianan Wang Kai Yang Shiyi Sun Qianyue Ma Gong Yi Xin Chen Ze Wang Wei Yan Xinhua Liu Qiong Cai Yunlong Zhao Department of Environmental Science and Engineering State Key Laboratory of Multiphase Flow in Power EngineeringSchool of Energy and Power EngineeringXi'an Jiaotong UniversityXi'anthe People's Republic of China Department of Chemical&Process Engineering Faculty of Engineering and Physical SciencesUniversity of SurreyGuildfordUK Advanced Technology Institute University of SurreyGuildfordUK School of Transportation Science and Engineering Beihang UniversityBeijingthe People's Republic of China

Solid-state lithium batteries(SSLBs)have been broadly accepted as a promising candidate for the next generation lithium-ion batteries(LIBs)with high energy density,long duration,and high *** intrinsic non-flammable nature and electrochemical/thermal/mechanical stability of solid electrolytes are expected to fundamentally solve the safety problems of conventional ***,thermal degradation and thermal runaway could also happen in *** example,the large interfacial resistance between solid electrolytes and electrodes could aggravate the joule heat generation;the anisotropic thermal diffusion could trigger the uneven temperature distribution and formation of hotspots further leading to lithium dendrite *** research efforts have been devoted to exploring solid electrolytes with outstanding performance and harmonizing interfacial incompatibility in the past *** have been fewer comprehensive reports investigating the thermal reaction process,thermal degradation,and thermal runaway of *** review seeks to highlight advanced thermal-related analysis techniques for SSLBs,by focusing particularly on multiscale and multidimensional thermal-related characterization,thermal monitoring techniques such as sensors,thermal experimental techniques imitating the abuse operating condition,and thermalrelated advanced *** perspectives are proposed to bridge fundamental studies to technological relevance for better understanding and performance optimization of SSLBs.

关键词： characterization monitoring simulation solid-state batteries thermal technique

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Numerical and experimental research of the characteristics of concentration solar cells

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Frontiers in Energy 2021年第2期15卷 279-291页

作者： Zilong WANG Hua ZHANG Binlin DOU Weidong WU Guanhua ZHANG Shanghai Key Laboratory of Multiphase Flow and Heat Transfer in Power Engineering School of Energy and Power EngineeringUniversity of Shanghai for Science and TechnologyShanghai 200093China

The development of automatic tracking solar concentrator photovoltaic systems is currently attracting growing *** concentration photovoltaic systems(HCPVs)combining triple-junction InGaP/lnGaAs/Ge solar cells with a concentrator provide high conversion *** mathematical model for triple-junction solar cells,having a higher efficiency and superior temperature characteristics,was established based on the one-diode equivalent circuit cell model.A paraboloidal concentrator with a secondary optic system and a concentration ratio in the range of 100X–150X along with a sun tracking system was developed in this *** GaInP/GalnAs/Ge triple-junction solar cell,produced by AZUR SPACE Solar Power,was also used in this *** solar cells produced by Shanghai Solar Youth Energy(SY)and Shenzhen Yinshengsheng Technology ***.(YXS)were used as comparison samples in a further comparative study at different concentration ratios(200X–1000X).A detailed analysis on the factors that influence the electrical output characteristics of the InGaP/lnGaAs/Ge solar cell was conducted with a dish-style concentrating photovoltaic *** results show that the short-circuit current(Isc)and the open-circuit voltage(Voc)of multi-junction solar cells increases with the increasing concentration ratio,while the cell efficiency(ηc)of the solar cells increases first and then decreases with increasing concentration *** increasing solar cell temperature,Isc increases,while Voc andηc decrease.A comparison of the experimental and simulation results indicate that the maximum root mean square error is less than 10%,which provides a certain theoretical basis for the study of the characteristics of triple-junction solar cell that can be applied in the analysis and discussion regarding the influence of the relevant parameters on the performance of high concentration photovoltaic systems.

关键词： concentration three-junction solar cell mathematical model electrical properties solar energy

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Chalcogen heteroatoms doped nickel-nitrogen-carbon single-atom catalysts with asymmetric coordination for efficient electrochemical CO_(2) reduction

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Chinese Journal of Catalysis 2024年第9期64卷 54-65页

作者： Jialin Wang Kaini Zhang Ta Thi Thuy Ng Yiqing Wang Yuchuan Shi Daixing Wei Chung-Li Dong Shaohua Shen International Research Center for Renewable Energy State Key Laboratory of Multiphase Flow in Power EngineeringXi'an Jiaotong UniversityXi'an 710049ShaanxiChina Department of Physics Tamkang UniversityNew Taipei City 25137TaiwanChina

The electronic configuration of central metal atoms in single-atom catalysts(SACs)is pivotal in electrochemical CO_(2) reduction reaction(eCO_(2)RR).Herein,chalcogen heteroatoms(e.g.,S,Se,and Te)were incorporated into the symmetric nickel-nitrogen-carbon(Ni-N_(4)-C)configuration to obtain Ni-X-N_(3)-C(X:S,Se,and Te)SACs with asymmetric coordination presented for central Ni *** these obtained Ni-X-N_(3)-C(X:S,Se,and Te)SACs,Ni-Se-N_(3)-C exhibited superior eCO_(2)RR activity,with CO selectivity reaching~98% at-0.70 V versus reversible hydrogen electrode(RHE).The Zn-CO_(2) battery integrated with Ni-Se-N_(3)-C as cathode and Zn foil as anode achieved a peak power density of 1.82 mW cm^(-2) and maintained remarkable rechargeable stability over 20 ***-situ spectral investigations and theoretical calculations demonstrated that the chalcogen heteroatoms doped into the Ni-N_(4)-C configuration would break coordination symmetry and trigger charge redistribution,and then regulate the intermediate behaviors and thermodynamic reaction pathways for eCO_(2)***,for Ni-Se-N_(3)-C,the introduced Se atoms could significantly raise the d-band center of central Ni atoms and thus remarkably lower the energy barrier for the rate-determining step of ^(*)COOH formation,contributing to the promising eCO_(2)RR performance for high selectivity CO production by competing with hydrogen evolution reaction.

关键词： Electrochemical CO_(2) reduction reaction Chalcogen heteroatoms Single-atom catalysts Asymmetric coordination CO production

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Experimental and modeling investigation of zero net liquid flow in hilly terrain pipeline

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Petroleum Science 2025年第5期22卷 2183-2202页

作者： Huang, Bo Xu, Qiang Chang, Ying-Jie Cao, Ye-Qi Yu, Hai-Yang Li, Yu-Wen Guo, Lie-Jin State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong University Shaanxi Xi'an710049 China College of Petroleum Engineering Xi'an Shiyou University Shaanxi 710065 China

Hilly terrain pipeline is a common form of pipeline in oil and gas storage and transportation industry. Due to the hilly terrain influence, the liquid at the elbow of the gathering pipeline is easy to flow back and accumulate to form slug flow, so it is necessary to remove the accumulated liquid by gas purging. In this paper, experiment is carried out in hilly terrain pipelines. Three flow patterns of stratified flow, slug flow and stratified entrained flow are observed. The process of gas purging accumulated liquid is divided into four stages, namely liquid accumulation, liquid rising;continuous outflow and tail outflow. At the same time, the flow pattern maps of each stage are drawn. The pressure drop signal is analyzed in time domain and frequency domain, and the contour map of pressure drop distribution is drawn. It is found that the ratio of range to average value can well distinguish the occurrence range of each flow pattern. Based on visualization, the transition process of slug flow to stratified flow and stratified entrained flow is studied, and the transition boundary prediction model is established. An image processing method is proposed to convert the image signal into a similarity curve, and PSD analysis is performed to calculate the slug frequency. The normal distribution is used to fit the slug frequency, and the predicted correlation is in good agreement with the experimental data. © 2025 The Authors

关键词： Optical flows

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Urchin-like Nb_(2)O_(5)hollow microspheres enabling efficient and selective photocatalytic C–C bond cleavage in lignin models under ambient conditions

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Chinese Chemical Letters 2022年第9期33卷 4357-4362页

作者： Huan Chen Donghui Hong Kun Wan Junjie Wang Bo Niu Yayun Zhang Donghui Long State Key Laboratory of Chemical Engineering East China University of Science and TechnologyShanghai 200237China Shanghai Key Laboratory of Multiphase Materials Chemical Engineering East China University of Science and TechnologyShanghai 200237China

Selective cleavage of robust C−C bonds to harvest value-added aromatic oxygenates is an intriguing but challenging task in lignin *** is a promising technology with the advantages of mild reaction conditions and strong ***,we show a novel urchin-like Nb_(2)O_(5)hollow microsphere(U-Nb_(2)O_(5)HM),prepared by one-pot hydrothermal method,are highly active and selective for C_(α)−C_(β)bond cleavage of ligninβ-O-4 model compounds under mild conditions,achieving 94%substrate conversion and 96%C−C bond cleavage *** experimental studies and density functional theory(DFT)calculations revealed that the superior performance of U-Nb_(2)O_(5)HMs arises from more exposed active sites,more efficient free charge separation and the active(001)facet,which facilitates the activation of Cβ−H bond of lignin models and generate key Cβradical intermediates by photogenerated holes,further inducing the C_(α)−C_(β)bond cleavage to produce aromatic *** work could provide some suggestions for the fabrication of hierarchical photocatalysts in the lignin depolymerization system.

关键词： Niobium oxide Urchin-like hierarchical structure Photocatalysis β-O-4 Lignin model C_(β)radical

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Multiblock poly(ether-b-amide)copolymers comprised of PA1212 and PPO-PEO-PPO with specific moisture-responsive and antistatic properties

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Chinese Journal of Chemical engineering 2023年第1期53卷 421-430页

作者： Jie Jiang Wei Cheng Qiuyu Tang Xun Pan Jinjin Li Ling Zhao Zhenhao Xi Weikang Yuan State Key Laboratory of Chemical Engineering School of Chemical EngineeringEast ChinaUniversity of Science and TechnologyShanghai 200237China Shanghai Key Laboratory of Multiphase Materials Chemical Engineering East China University of Science and TechnologyShanghai 200237China Flinders Institute for Nanoscale Science and Technology Flinders UniversitySA 5042Australia College of Chemistry and Chemical Engineering Xinjiang UniversityUrumqi 830046China

Functional multiblock poly(ether-b-amide)(PEBA)copolymers,comprised of PA1212(polyamide 1212)as hard segments and Jeffamine ED-2003 as soft segments,were successfully prepared via two-step melt polycondensation without any amidation ***,using diamino-terminated poly(propylene oxide)-poly(ethylene oxide)-poly(propylene oxide)(PPO-PEO-PPO),Jeffamine ED-2003,enhances the compatibility between polyamide oligomer and polyether,which is better than the traditional route using hydroxyl-terminated *** chemical structure of multiblock PEBAs,as well as the microphase separated structure with crystalline phase of polyamide and polyether,were confirmed by heteronuclear multiple-bond correlation spectrum,heteronuclear multiple quantum correlation spectrum,Fourier transform infrared spectroscopy(FT-IR),differential scanning calorimetry and dynamic mechanical *** hydrophilic PEBA copolymers showed water adsorption ranging from 87.3%to 17.1%depending on the polyether content,and specially showed moisture responsive behavior within seconds when exposed to *** corresponding mechanism was studied using time-resolved attenuated total reflectance FT-IR spectroscopy in the molecular level and the water diffusion coefficient was estimated to be 1.07×10^(–8)cm^(2)∙s^(-1).Two-dimensional correlation FT-IR spectra analysis was performed to confirm that the interaction between water and polyether phase was in preference to that between water and polyamide matrix,and water molecule only forms hydrogen bond with the polyether *** to the incorporation of PEO segments,the PEBAs have the surface resistivity varying from 5.6×10^(9)to 6.5×10^(10)Ω,which makes PEBA potential candidate as permanent antistatic agent.

关键词： Poly(ether-b-amide)s Moisture-responsive Antistatic In situ FT-IR 2D FT-IR analysis

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Numerical Simulation Study on Wet Gas flowmetering Overreading Characteristics of Venturi Tube under Low Pressure Conditions 3

Numerical Simulation Study on Wet Gas Flowmetering Overreadi...

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3rd International Conference on Testing Technology and Automation engineering, TTAE 2023

作者： Xing, Zhaokai Wu, Fang Hu, Rongyuan Xu, Guobin Xie, Hongjun Fan, Shaohua Wang, Shanshan Yang, Jinfeng Meng, Lin Liu, Qihang State Nuclear Electric Power Planning Design & Research Institute Co Ltd Beijing100095 China Shandong Nuclear Power Company Ltd Yantai265116 China Xi'an Jiaotong University State Key Laboratory of Multiphase Flow in Power Engineering Xi'an710049 China

ISBN: (纸本)9781510674769

A numerical simulation study of Venturi overreading characteristics is carried out with Mixture model and Realizable k-e model, and a prediction model of Venturi overreading under low pressure conditions is proposed. Compared with the existing experimental data, it demonstrates that the numerical simulation results have high accuracy, the results indicate that the quality is the main factor affecting the Venturi overreading Meanwhile, the model in this paper is compared with with ten classical overreading prediction models such as homogeneous model. It shows that the average prediction deviation of the model in this paper is 3.2%, ranking second, and the maximum prediction deviation is 7.3%. This study can provide reference for the study of Venturi wet gas flowmetering overreading model, and also provide a theoretical basis and options for flowmetering technology. © 2024 SPIE.

关键词： Forecasting

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Rotor dynamic analysis of supercritical carbon dioxide Bryton cycle coaxial integrated unit 14

Rotor dynamic analysis of supercritical carbon dioxide Bryto...

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14th IEEE Global Reliability and Prognostics and Health Management Conference, PHM-Hangzhou 2023

作者： Xu, Xiaokang Yang, Yi Wang, Jiangfeng Lou, Juwei Chen, Liangqi State Key Laboratory of Multiphase Flow in Power Engineering School of Energy and Power Engineering Xi'an Jiaotong University Xi'an China Laboratory of Science and Technology on Integrated Logistics Support College of Intelligence Science and Technology National University of Defense Technology Changsha China

ISBN: (纸本)9798350301359

The rotor system plays a very important role in supercritical carbon dioxide Brayton cycle system, and its dynamic problem will directly affect the motion stability and safety of the whole unit. In this paper, the rotor dynamic model of supercritical CO2 coaxial unit is established by finite element method, and the critical speed, modal shape and unbalance response of the rotor are studied. The first seven critical speed of the rotor and the first seven natural frequency of the rotor at the working speed are calculated. The bending modal of the rotor and the position where the rotor amplitude is the largest are analyzed, which can provide reference for the optimization design of the rotor stability. The influences of mass unbalances at the operational speed of rotor are analyzed. The research can provide some suggestions for the optimal design and actual operation of the supercritical CO2 coaxial integrated unit. © 2023 IEEE.

关键词： critical speed unbalance response vibration analysis

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engineering of Fe d-band center in Fe_(3)O_(4)/CeO_(2)hetero-nanoparticles via orbital coupling for high-efficiency oxygen reduction electrocatalysis

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Nano Research 2025年第1期18卷 129-139页

作者： Jiayi Liu Jingwen Yin Yingzi Lin Mingxin Pang Huan Pang Songtao Zhang Lin Xu Jun Yang Yawen Tang Jiangsu Key Laboratory of New Power Batteries Jiangsu Collaborative Innovation Center of Biomedical Functional MaterialsSchool of Chemistry and Materials ScienceNanjing Normal UniversityNanjing 210023Chin a 2 State Key Laboratory of Multiphase Complex Systems Center of MesoscienceInstitute of Process EngineeringChinese Academy of SciencesBeijing 100190China School of Chemistry and Chemical Engineering Yangzhou UniversityYangzhou 225009China Testing Center Yangzhou UniversityYangzhou 225009China

The deliberate engineering of the d-band center of metal site represents an effective strategy to boost the intrinsic electrocatalytic performance toward the oxygen reduction reaction(ORR).Herein,following a heterointerfaceinduced orbital coupling rationale,we report a judicious design of an efficient ORR electrocatalyst consisting of Fe_(3)O_(4)/CeO_(2)hetero-nanoparticles in-situ encased into N-doped carbon nanofibers(abbreviated as Fe_(3)O_(4)/CeO_(2)@N-CNFs hereafter).The theoretic calculations uncover that the Fe_(3)O_(4)/CeO_(2)heterointerface-triggered orbital coupling can cause the down shift of the d-band center positions of Fe sites,which leads to the weakened chemisorption of oxygenated groups and lowered energy barrier for the potential-determining step,ultimately dramatically boosting the ORR intrinsic *** a consequence,the well-designed Fe_(3)O_(4)/CeO_(2)@N-CNFs display admirable ORR activity with a half-wave potential of 0.84 V and outstanding structural/electrochemical stability in an alkaline electrolyte,surpassing the commercial Pt/C benchmark and a majority of recently reported Fe_(3)O_(4)-based *** encouragingly,the Fe_(3)O_(4)/CeO_(2)@N-CNFsincorporated Zn-air battery outperforms the Pt/C-assembled counterpart with higher power density,larger energy density,and excellent cycling stability,serving as a competent candidate for ORR-involved renewable energy *** study offers an innovative approach for the rational manipulation of the d-band center and interfacial electron behavior of active sites toward the optimization of electrocatalytic performance.

关键词： hetero-nanoparticles electrospinning interfacial engineering orbital coupling oxygen reduction reaction

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Progress of vanadium phosphorous oxide catalyst for n-butane selective oxidation

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Chinese Journal of Chemical engineering 2022年第3期35卷 297-315页

作者： Muhammad Faizan Yingwei Li Ruirui Zhang Xingsheng Wang Piao Song Ruixia Liu Beijing Key Laboratory of Ionic Liquids Clean Process State Key Laboratory of Multiphase Complex SystemInstitute of Process Engineering Chinese Academy of SciencesBeijing 100190China University of Chinese Academy of Sciences Beijing 100049China

The utilization of lighter alkanes into useful chemical products is essential for modern chemistry and reducing the CO_(2)***,n-butane has gained special attention across the globe due to the abundant production of maleic anhydride(MA).Vanadium phosphorous oxide(VPO)is the most effective catalyst for selective oxidation of n-butane to MA so ***,the VPO complex exists in more or less fifteen different structures,each one having distinct phase composition and exclusive surface morphology and physiochemical properties such as valence state,lattice oxygen,acidity etc.,which relies on precursor preparation method and the activation conditions of *** catalytic performance of VPO catalyst is improved by adding different promoters or co-catalyst such as various metals dopants,or either introducing template or structural-directing ***,new preparation strategies such as electrospinning,ball milling,hydrothermal,barothermal,ultrasound,microwave irradiation,calcination,sol-gel method and solvothermal synthesis are also employed for introducing improvement in catalytic *** in above-mentioned different aspects will be ascribed in current review in addition to summarizing overall catalysis activity and final *** analyze the performance of the catalytic precursor,the reaction mechanism and reaction kinetics both are discussed in this review to help clarify the key issues such as strong exothermic reaction,phosphorus supplement,water supplement,deactivation,and air/n-butane pretreatment *** to the various industrial applications of VPO.

关键词： N-butane selective oxidation Oxidation of light alkanes Vanadium phosphorus oxide(VPO) Maleic anhydride

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