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Noble-metal free plasmonic nanomaterials for enhanced photocatalytic applications—A review

Nano Research 2022年第12期15卷 10268-10291页

作者： Jinghua Li Yiming Zhang Yalong Huang Bing Luo Li Jing Dengwei Jing International Research Center for Renewable Energy&State Key Laboratory of Multiphase Flow in Power Engineering Xi’an Jiaotong UniversityXi’an710049China School of Chemical Engineering and Technology Xi’an Jiaotong UniversityXi’an710049China

Plasmonic nanomaterial catalysis is currently at the frontier of photocatalysis,overcoming the limitations of wide bandgap semiconductors for light *** localized surface plasmon resonance(LSPR)properties allow broad ultraviolet-visible-near infrared ray(UV-vis-NIR)absorption,making it an ideal material for solar energy *** plasmonic nanostructures rely on precious *** noble metal plasmonic nanomaterials have proven to be one of the strategies for enhancing photocatalytic activity,their expensive cost and limitations in light absorption range have hindered their practical *** a result,noble-metal free plasmonic nanomaterials have risen to the top of the research priority ***,this paper reviews the fundamental principles and classification of the LSPR effect of noble-metal free plasmonic nanomaterials in photocatalytic and their recent applications in hydrogen generation,carbon dioxide reduction,and pollutant *** cases elucidate the possible working mechanism of enhanced photocatalysis by noble-metal free plasmonic ***,the challenges and future opportunities for noble-metal free plasmonic nanomaterials in energy conversion and storage are discussed and envisioned.

关键词： localized surface plasmon resonance(LSPR) noble-metal free plasmonic nanomaterials photocatalysis

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Technological innovations on direct carbon mitigation by ordered energy conversion and full resource utilization

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Carbon Neutrality 2022年第1期1卷 598-619页

作者： Liejin Guo Zhisong Ou Ya Liu Zhiwei Ge Hui Jin Guobiao Ou Mengmeng Song Zihao Jiao Wenhao Jing State Key Laboratory of Multiphase Flow in Power Engineering Xi’an Jiaotong UniversityNo.28Xianning West RoadXi’an 710049People’s Republic of China

Coal consumption leads to over 15 billion tons of global CO_(2) emissions annually,which will continue at a considerable intensity in the foreseeable *** remove the huge amount of CO_(2),a practically feasible way of direct carbon mitigation,instead of capturing that from dilute tail gases,should be developed;as intended,we developed two innovative supporting technologies,of which the status,strengths,applications,and perspective are discussed in this *** is supercritical water gasification-based coal/biomass utilization technology,which orderly converts chemical energy of coal and low-grade heat into hydrogen energy,and can achieve poly-generation of steam,heat,hydrogen,power,pure CO_(2),and *** other one is the renewables-powered CO_(2) reduction techniques,which uses CO_(2) as the resource for carbon-based fuel *** combining the above two technical loops,one can achieve a full resource utilization and zero CO_(2) emission,making it a practically feasible way for China and global countries to achieve carbon neutrality while creating substantial domestic benefits of economic growth,competitiveness,well-beings,and new industries.

关键词： Carbon neutrality Coal utilization Direct carbon mitigation Supercritical water gasification Renewable energy CO_(2)reduction

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Simulation of the dynamic behavior of droplet impact on the microstructure surface 1

Simulation of the dynamic behavior of droplet impact on the ...

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1st International Conference on Fluid Dynamics and Computational Science, FDCS 2022

作者： Yang, Jianhua Gao, Ming Sun, Hailin Liu, Zhennan Zhang, Kaiyuan Shanghai Key Laboratory of Multiphase Flow and Heat Transfer in Power Engineering School of Energy and Power Engineering The University of Shanghai for Science and Technology Shanghai200093 China

The problem of droplets impacting rough wall has always been a hot spot in the engineering field. In this paper, the single-component multiphase lattice Boltzmann method is used to construct the wall microstructure, and the dynamic behavior characteristics of droplets impacting rough walls are simulated. The results show that the final state of a droplet impacting rectangular microstructure shows that the hydrophilic surface is more hydrophilic and the hydrophobic surface is more hydrophobic, and compared with the smooth surface, the microstructure surface hinders the rebound of the droplet, and the application of microstructure on the wall can promote the spreading of a droplet on the wall. © 2023 Institute of Physics Publishing. All rights reserved.

关键词： Drops

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A New Structure of Cooling Wall Tube for Supercritical CO_(2)Coal-Fired power Plants

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Journal of Thermal Science 2023年第3期32卷 1239-1250页

作者： WANG Yanjuan GAO Shuo JIANG Qiongqiong LI Yi LIU Qibin XU Jinliang The Beijing Key Laboratory of Multiphase Flow and Heat Transfer North China Electric Power UniversityBeijing 102206China Institute of Engineering Thermophysics Chinese Academy of SciencesBeijing 100190China University of Chinese Academy of Sciences Beijing 100049China

In terms of developing supercritical CO_(2)(sCO_(2))coal-fired power plants,enhancing cooling wall performance is one of significant factors to improve system *** this paper,a new cooling wall tube structure is proposed to match the non-uniform heat flux(NUH)with the thermal resistance by changing the cooling wall tube eccentricity.A three-dimensional multi-physical coupling model of cooling wall is constructed to compare the novel structure to the conventional *** properties of fluid dynamics,thermal stress,coupled heat transfer and cooling wall deformation are *** contrast to the traditional structure,the maximum temperature and circumferential temperature difference(CTD)of the proposed structure can be reduced by 2%and 27.4%,*** essential working parameters related to the performances of the cooling wall tube are *** maximum temperature of the new structure is reduced by 8-13 K and the maximum thermal stress is reduced by about 10%-15%under all the simulated working conditions when the eccentricity changes from 0 to *** proposed structure can effectively reduce the maximum temperature and circumferential temperature gradient under ***,a novel insight is put out for the design and optimization of the cooling wall tube in coal-fired power plants.

关键词： supercritical carbon dioxide cooling wall tube thermal-hydraulic structural coupling supereritical heat transfer

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氧化铁光阳极界面内建电场调控强化光生电荷空间分离

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Science China Materials 2023年第2期66卷 603-613页

作者：卯连连邓豪李明涛沈少华 International Research Center for Renewable Energy State Key Laboratory of Multiphase Flow in Power EngineeringXi’an Jiaotong UniversityXi’an 710049China

为了缓解氧化铁光阳极内部和表面的电荷复合,本文引入了一种界面电荷调控策略,利用界面内建电场(IEF)促进电荷的空间分离.水热生长的钛掺杂氧化铁(Hem)纳米棒通过简单的两步浸渍涂层过程,以石墨相氮化碳(g-C_(3)N_(4))和小的三氧化钼(Mo... 详细信息

为了缓解氧化铁光阳极内部和表面的电荷复合,本文引入了一种界面电荷调控策略,利用界面内建电场(IEF)促进电荷的空间分离.水热生长的钛掺杂氧化铁(Hem)纳米棒通过简单的两步浸渍涂层过程,以石墨相氮化碳(g-C_(3)N_(4))和小的三氧化钼(MoO_(3))团簇进行修饰.与原始的Hem相比,得到的Hem/C_(3)N_(4)/MoO_(3)表现出显著增强的光电化学分解水性能,相对于可逆氢电极,在1.23 V时,光阳极电流密度从0.3 mA cm^(-2)显著提高到1.6 mA cm^(-2),入射光子-电流转换效率在300 nm时达到18.4%.结果表明,在Hem/C_(3)N_(4)/MoO_(3)异质结中引入IEF是通过调控界面电荷特性实现的,此界面电荷特性是由Hem/C_(3)N_(4)界面的TypeⅡ能带排列和光阳极表面增强的能带弯曲所引起的,IEF能显著促进电荷的空间分离.研究这一界面电荷调控过程能为基于氧化铁的光阳极和其他半导体器件提供一种简单有效的策略,通过缓解载流子传输动力学的瓶颈,促进电荷的空间分离,实现高效的太阳能转换.

关键词：太阳能转换阳极电流密度半导体器件能带弯曲入射光子石墨相氮化碳载流子传输氢电极

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On the spreading behavior of a droplet on a circular cylinder using the lattice Boltzmann method

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Chinese Physics B 2024年第6期33卷 434-443页

作者：杨帆金虎戴梦瑶 School of Energy and Power Engineering University of Shanghai for Science and TechnologyShanghai 200093China Shanghai Key Laboratory of Multiphase Flow and Heat Transfer in Power Engineering Shanghai 200093China

The study of a droplet spreading on a circular cylinder under gravity was carried out using the pseudo-potential lattice Boltzmann high-density ratios multiphase model with a non-ideal Peng–Robinson equation of state. The calculation results indicate that the motion of the droplet on the cylinder can be divided into three stages: spreading, sliding, and *** contact length and contact time of a droplet on a cylindrical surface can be affected by factors such as the wettability gradient of the cylindrical wall, the Bond number, and droplet size. Furthermore, phase diagrams showing the relationship between Bond number, cylinder wall wettability gradient, and contact time as well as maximum contact length for three different droplet sizes are given. A theoretical foundation for additional research into the heat and mass transfer process between the droplet and the cylinder can be established by comprehending the variable rules of maximum contact length and contact time.

关键词： lattice Boltzmann methods droplet circular cylinder wettability gradient

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Thermodynamic performance optimization of two-stage hydraulic-driven piston hydrogen compressors based on variable speed control method

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International Journal of Hydrogen Energy 2025年 145卷 205-214页

作者： Qiang Qi Shengdong Ren Chengqian Wang Ziying Chen Xiaohan Jia Xueyuan Peng School of Energy and Power Engineering Xi'an Jiaotong University China State Key Laboratory of Multiphase Flow in Power Engineering Xi’an Jiaotong University China

The two-stage hydraulic driven piston compressor is increasingly used in 70 MPa hydrogen refueling stations. Due to variable suction pressures as hydrogen is drawn from trailer into the compressor, unbalanced distribution of pressure ratios, and hereby power consumption and discharge temperatures may occur between two stages, consequently resulting in excessively large power and high discharge temperature for a single stage. This paper proposes a scheme of equalizing pressure ratios of the two stages at any varied suction pressures by regulating the oil supply rate of the hydraulic cylinder of each stage separately. Thermodynamic simulations at varied suction pressures were conducted for the compressor with constant speed and variable speed, respectively, and a test rig was built up to validate the simulated results. The results indicate that almost identical pressure ratios between two stages were achieved by regulating the speed of each stage. As a result, the difference in power between the two stages was reduced from 35.8 kW to 11.9 kW, while the temperature deviation between the two stages was decreased from 200.8 K to 5.6 K. Furthermore, the highest discharge temperature of the two stages compressors dropped from 603.9 K to 501.1 K.

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Thermo-Hydraulic Characteristics of Non-Isothermal Batch Transportation Pipeline System with Different Inlet Oil Temperature

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Journal of Thermal Science 2023年第3期32卷 965-981页

作者： CHEN Zhimin YUAN Qing JIANG Weixin LI Zongze YU Bo School of Mechanical Engineering Beijing Institute of Petrochemical TechnologyBeijing 102617China School of Chemical Engineering and Technology Xi'an Jiaotong UniversityXi'an 710049China Faculty of Environment and Life Beijing University of TechnologyBeijing 100124China State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong UniversityXi'an 710049China

The batch transportation process of several kinds of crude oil is accomplished by an entire coupled pipeline system,which exhibits complex thermo-hydraulic *** on the coupled characteristics among soil,pipelines and devices(including pumps,heating furnaces and valves),a coupled simulation model of batch transportation for the crude oil pipeline system is established,and a novel coupled simulation algorithm is *** simulation results are in good agreement with the field data of an actual crude oil pipeline *** addition,based on the numerical simulation,thermo-hydraulic characteristics of pipeline system are investigated,and some new thermo-hydraulic characteristics are *** the batch transportation process with constant flowrate,the change trends of temperature at the outlet of each pipeline segment are hysteretic and the change ranges of temperature become small along *** the adjustment of devices influences thermohydraulic characteristics to some *** the batch transportation process with variable flowrate,the complex thermo-hydraulic characteristics are exhibited,which are induced by the comprehensive influence of the changes of oil type,flowrate and absorbed/released *** with the transportation process with constant flowrate,the high-viscosity oil exhibits similar minimum temperature and lower maximum pressure in the transportation process with variable flowrate,which means that the higher transportation safety of pipeline system is *** study can provide a scientific reference for making the safer batch transportation scheme of crude oil pipeline system.

关键词： crude oil pipeline system batch transportation coupled simulation variable flowrate thermo-hydraulic characteristics

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利用三元合金保护和催化的硅光阳极与廉价硅太阳能电池相结合实现12.0%的太阳能制氢效率

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engineering 2023年第6期25卷 128-137,M0006页

作者：何凌云洪欣王亦清邢众航耿嘉峰郭鹏慧苏进展沈少华 International Research Center for Renewable Energy State Key Laboratory of Multiphase Flow in Power EngineeringXi’an Jiaotong UniversityXi’an 710049China

n型硅(n-Si)表面在水溶液中容易被氧化和钝化,导致其在光电化学(PEC)分解水的析氧反应(OER)动力学缓慢。本工作通过欠电位沉积成功地在p^(+)n-Si基底上电沉积了三金属Ni_(0.9)Fe_(0.05)Co_(0.05)保护层。制备的Ni_(0.9)Fe_(0.05)Co_(0.0... 详细信息

n型硅(n-Si)表面在水溶液中容易被氧化和钝化,导致其在光电化学(PEC)分解水的析氧反应(OER)动力学缓慢。本工作通过欠电位沉积成功地在p^(+)n-Si基底上电沉积了三金属Ni_(0.9)Fe_(0.05)Co_(0.05)保护层。制备的Ni_(0.9)Fe_(0.05)Co_(0.05)/p^(+)n-Si光阳极具有优异的稳定性和PEC水氧化活性,具有相对低的OER起始电位(相对于可逆氢电极电势(RHE)仅为0.938 V),并且在1.23 V ***电位时具有较高的光电流密度(33.1 m A·cm^(-2)),显著优于Ni/p^(+)n-Si光阳极。工作证明了Fe在Ni层的掺杂会在Ni_(0.9)Fe_(0.05)Co_(0.05)/p^(+)n-Si界面处产生较大的能带弯曲,促进界面电荷分离。此外,Co的加入会产生丰富的Ni^(3+)和氧空位(Ov),作为活性位点可以加速OER动力学过程,协同促进PEC过程中的水氧化的活性。令人鼓舞的是,通过将Ni_(0.9)Fe_(0.05)Co_(0.05)/p^(+)n-Si光阳极连接到廉价的硅太阳能电池上,所制备的集成光伏/PEC(PV/PEC)器件实现了无偏压下高达12.0%的太阳制氢能量转换效率。这项工作提供了一种简单的方法来设计高效、稳定的n-Si基光阳极,并对其构效关系有了深刻的理解;这种方法制备的材料在集成低成本PV/PEC器件用于无辅助太阳能驱动水分解方面具有巨大的潜力。

关键词：欠电位沉积电极电势阳极连接硅太阳能电池能量转换效率太阳能制氢能带弯曲光阳极

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Influence of active and passive equipment for advanced pressurized water reactor on thermal hydraulic and source term behavior in severe accidents

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Energy Storage and Saving 2023年第1期2卷 392-402页

作者： Jishen Li Bin Zhang School of Nuclear Science and Technology Xi’an Jiaotong UniversityXi’an710049China State Key Laboratory of Multiphase Flow in Power Engineering Xi’an Jiaotong UniversityXi’an710049China

Extensive studies have been carried out on the behavior of core degradation and fission products of common pressurized water reactors(PWRs).However,few of them have investigated the relationship between thermal hydraulic and fission product behavior in advanced passive *** to the impact of thermal hydraulic be-haviors in different accident sequences on the release and transportation of fission products,an integrated severe accident analysis(ISAA)code with highly coupled thermal hydraulic and source term calculations is required to simultaneously analyze thermal hydraulic and source term *** advanced passive PWRs,important safety systems that may affect the behavior of the core and fission products should be *** is therefore necessary to simulate the thermal hydraulic and fission product behavior of advanced passive *** this study,the ISAA code is adopted to simulate the occurrence of a hypothetical double ended cold leg LBLOCA of HPR1000 in three scenarios of equipment *** results show that the high-temperature fuel rods and cladding ma-terials exhibit delayed failure at the lower position of the active core,whereas earlier failure at higher position during the *** and passive equipment affects fuel temperature,the oxidation conditions of the fuel,the interaction of fission products and structural materials,and the state of the fuel,thereby affecting the release of fission products in the ***1000 only relies on passive equipment to relieve the core degradation in severe accidents,realize the in-vessel retention of melt,and eliminate the ex-vessel release possibility of fission *** is hoped that the results can provide references for HPR1000 to formulate the severe accident management guidelines(SAMG).

关键词： Nuclear safety LBLOCA Severe accident Source term HPR1000 Active and passive equipment

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