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Experimental Study on Cohesiveness Characteristics of Raw Cement Ash at Moderate Temperature

Energy Procedia 2017年 105卷 4674-4679页

作者： Tao Han Chang’an Wang Qi Cao Wufeng Chen Defu Che State Key Laboratory of Multiphase Flow in Power Engineering School of Energy and Power Engineering Xi’an Jiaotong University Xi’an 710049 China

Raw cement ash deposition in SP boilers gives rise to serious operation problems. In the present, mechanism of raw cement ash deposition is still unclear because the ash components, gas atmosphere and gas temperature are quite different from existing studies. The characteristics of cohesiveness of raw cement ash in moderate temperature were investigated in a lab-scale electric furnace. Three typical raw cement ashes were selected as samples, three base plates, including rough steel plate, smooth steel plate, organic glass plate were studied. Ball-impacting method was adopted to evaluate the cohesiveness of ash. Experimental results show that, the ash cohesiveness is mainly dependent on the components of ash, and the material property of base plate, while it exhibits little relationship with the roughness of the plate surface. Low-melting substances appear during ash deposition on steel plate. The results reveal that ferrum possibly has catalytic to some low-melting substances forming.

关键词： deposition cohesiveness roughness low-melting sunbstances

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Excess thermodynamic properties and FTIR studies of binary of 1, 3-dichlorobenzene with alkyl acetates (C1–C5) at different temperatures

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Chemical Data Collections 2020年 29卷

作者： R. Raju S. Ravikumar R. Gerald Arokiaraj S. Karlapudi K. Sivakumar V. Pandiyan Department of Physics Nehru Memorial College (Autonoums) Puthanampatti 621 007Tamil Nadu India. State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong University Shaanxi 710049 P. R. China. Department of Chemistry S.V.Arts Degree & P.G.College (T.T.D'S) Tirupati 517502 A.P India

Densities ( ρ ) and speed of sound ( u ) have been reported for the binary mixtures containing 1, 3- dichlorobenzene (1, 3-DCB) with methyl acetate, ethyl acetate, propyl acetate, butyl acetate and pentyl acetate at four different temperatures ( T = 303.15, 308.15, 313.15 and 318.15 K) and at atmospheric pressure. The experimental data of densities and speeds of sound has been further utilized to calculate excess molar volume ( V m E ) and excess isentropic compressibility ( κ S E ) the excess properties have been fitted to Redlich-Kister equation. Further, V m E results have also been discussed by using Prigogine–Flory–Patterson (PFP). The experimental speeds of sound data in the present investigated mixtures were compared with various theoretical models like collision factor theory (CFT) and free length theory (FLT) to check their relative merits of pure component properties. Moreover, the experimental excess functions were correlated in terms of FTIR spectral analysis.

关键词： Binary mixtures Densities Ester Halogenated benzene Speed of sound FTIR

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Ash Deposition and Alkali Metal Migration during Zhundong High-alkali Coal Gasification

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Energy Procedia 2017年 105卷 1350-1355页

作者： Guangyu Li Chang’an Wang Pengqian Wang Yongbo Du Xuan Liu Wufeng Chen Defu Che State Key Laboratory of Multiphase Flow in Power Engineering School of Energy and Power Engineering Xi’an Jiaotong University Xi’an 710049 China

Ash deposition is particularly serious during Zhundong coal combustion/gasification due to its high alkali metal content, which causes great troubles and limits its utilization. This paper focuses on the ash deposition characteristics and migration disciplinarian of akali metal during Zhundong coal gasification varing with different conditions, such as ash deposition temperature, gasification temperature, O 2 /coal, steam/coal, and deposition time. Experimental result indicates that gasification conditions play a significant role on ash deposition. The root cause of severe fouling is the high content of Na in Zhundong coal, most of which is water-soluble. Besides, the contents of Na, Fe, S, Cl in ash are obviously changed with flue gas temperature increasing, indicating these elements have great influence on ash deposition, and the migration of Na, Fe and Cl presents similar variation during deposition. In addition, Na deposits mainly above 873 K, and Fe gains enrichment in ash at various temperatures. With the increase of gasification temperature, the content of Na in the ash is increased, which could exacerbate ash deposition. Both O 2 /coal and steam/coal have a certain influence on migration of elements, and the increases of O 2 /coal and steam/coal can relieve the ash fouling phenomena. Deposited ash on heating surface will react with Na in flue gas at high temperature, leading to the increase of content of Na in the ash with deposition time increasing.

关键词： Coal gasification Zhundong coal alkali metal ash Deposition

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Effect of prompt dissociation of formyl radicals on 1,3,5-trioxane laminar flame speeds at high pressure 55

Effect of prompt dissociation of formyl radicals on 1,3,5-tr...

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55th AIAA Aerospace Sciences Meeting

作者： Zhao, Hao Fu, Jiapeng Ju, Yiguang Department of Mechanical and Aerospace Engineering Princeton University Engineering Quad Olden Street PrincetonNJ08544 United States Department of Power Engineering State Key Laboratory of Multiphase Flow in Power Engineering Xi’an Jiaotong University Xi’an710049 China

ISBN: (纸本)9781624104473

Flame speeds of all hydrocarbon fuels are very sensitive to the reactions of formaldehyde (CH2O) and formyl radical (HCO). In this paper, we studied the prompt dissociation effect of HCO on the flame speeds of trioxane and formaldehyde up to 9 atm. The effects of prompt HCO dissociation were examined at high pressure. Different kinetic models were compared against the experimental results. The results showed there was a significant effect of the HCO prompt reaction on the flame speed in a broad range of pressure and equivalence ratio. At higher pressure, it was observed that the prompt effect was reduced due to the third-body collision effect. However, with the increase of O2mole fraction, the prompt effect was enhanced. Comparison showed that HP Mech with the inclusion of the prompt reactions had a better prediction at lean and ultra-lean conditions than other mechanisms. The improved prediction of the flame speed indicated that the prompt effect needed to be considered in the model development of hydrocarbon and oxygenated fuel combustion. © 2017 by Hao Zhao, Jiapeng Fu, and Yiguang Ju.

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Ordered mesoporous Cu-Ca-Zr:A superior catalyst for direct synthesis of methyl formate from syngas

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Carbon Resources Conversion 2018年第2期1卷 174-182页

作者： Jiahao Zhuang Bin Lu Fangna Gu Ziyi Zhong Fabing Su State Key Laboratory of Multiphase Complex Systems Institute of Process EngineeringChinese Academy of SciencesBeijing 100190China University of Chinese Academy of Sciences Beijing 100049China Zhongke Langfang Institute of Process Engineering Fenghua Road No.1Langfang Economic&Technical Development ZoneHebei Province 065001China Institute of Chemical and Engineering Sciences Agency for ScienceTechnology and Research(A*STAR)1 Pesek RoadJurong IslandSingapore 627833Singapore Institute of Industrial Chemistry and Energy Technology Shenyang University of Chemical TechnologyShenyang 110142China

It is still a big challenge to obtain both highly active and stable Cu-based catalysts for direct synthesis of methyl formate(MF)from *** address the issue,we have designed and synthesized a series of ternary Cu-Ca-Zr catalysts,namely,the ordered mesoporous Cu-Ca-Zr catalyst prepared by one-pot evaporation-induced self-assembly(EISA)method,and the supported CuO/CaO-ZrO_(2)catalysts by impregnating with copper precursor or by immobilizing copper *** the latter two catalysts,the ordered mesoporous CaO-ZrO_(2)support was also prepared by the EISA *** catalysts were characterized by techniques such as ICP,XRD,TEM,N2 isotherm adsorption-desorption,XPS and H2-TPR,and used for direct synthesis of *** results indicated that the catalyst prepared by onepot EISA method,in which the CuO species are highly dispersed in frame of CaO-ZrO_(2),exhibits much better activity and stability as compared with the other two catalysts with most of CuO located on the outer surface of the CaO-ZrO_(2)support,because the former has a higher specific surface area,enhanced synergistic effect and stronger interaction between the CaO-ZrO_(2)support and CuO active constituent.

关键词： Methyl formate Direct synthesis Cu-based catalyst Ordered mesoporous Activity

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Release and Transformation of Potassium during Combustion of Biomass

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Energy Procedia 2017年 142卷 401-406页

作者： Lei Deng Jiaming Ye Xi Jin Tao Zhu Defu Che State Key Laboratory of Multiphase Flow in Power Engineering School of Energy and Power Engineering Xi’an Jiaotong University Xi’an 710049 China

To investigate the release and transformation of fuel K during combustion of biomass, wheat straw and corn stalk are burnt in a fixed-bed reactor system during 400−1000 °C, and weight measurement, elemental composition analysis, and chemical fractionation analysis are performed. The influences of fuel type, combustion temperature, and water washing pretreatment are discussed. The results show that wheat straw has a higher K release ratio than corn stalk, especially when combustion temperature is above 500 °C. For both biomass fuels, the released K is far less than the water-soluble K. For wheat straw, some of the other occurrence modes of K turn into the insoluble K gradually. For corn stalk, the water-soluble and ion-exchangeable K turn into HCl-soluble and insoluble K. Water washing removes all the water-soluble K of corn stalk and reduces the K release from 3.26 to 0.27 mg g -1 at 1000 °C.

关键词： Potassium release Transformation Biomass combustion Water washing

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Toward Greener and Smarter Process Industries

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engineering 2017年第2期3卷 152-153页

作者： Wei Ge State Key Laboratory of Multiphase Complex Systems. Institute of Process Engineering. Chinese Academy of Sciences Beijing 100190. China University of Chinese Academy of Sdences Beifing 100049 China

The main mission of the process industries is to process resourc-es and energies into a form that can be utilized in other industriesand throughout society. In this sense, process industries cover a vastterritory, encompassing the chemical/biochemical, material, mining,metallurgical, power, food, and even pharmaceutical industries; inaddition, they are closely related to mechanical, civil, electrical, andelectronic industries, as well as to emerging fields such as biotech-nology, nanotechnology, and information technologies.

关键词：期刊编辑工作规范写作方法

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Laser-induced Morphology Change and Photo-thermolysis of Gold Nano Particles with Application in Laser Dermatology

Laser-induced Morphology Change and Photo-thermolysis of Gol...

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2017第六届国际新材料大会

作者： Bin Chen State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong University China

Based on the principle of selective photothermolysis,laser photothermal therapy is regarded as the most effective treatment methodology for port-wine stain（PWS）,which is a congenital vascular malformation caused by the expansion of capillaries in the dermis.1064 nm Nd:YAG laser has great potential for the treatment of deeper and larger ***,the clinical effectiveness is limited because of the weak absorption of blood to Nd:YAG *** order to enhance the blood absorption,spherical gold nanoparticles were prepared by Sodium citrate reduction method with average size of 16.7 nm and absorbance peak at 522 *** nanorods were prepared by Seeded growth method and modified by PEG with average length and width of 79.1 nm and 13.5 *** this aspect ratio of 5.89,a strong absorption band at050 nm in the near-infrared range is *** can inject spherical gold particles into the bloodstream to enhance the light absorption of blood in visible range,while using gold nanorod to increase absorbance of blood to Nd:YAG Laser for improving the cure rate of laser treatment of vascular *** absorption was increased by 1.25 times for 581 nm（PDL laser） and 3.71 times for 1064 nm（Nd:YAG laser）.To investigate the morphology change and photothermolysis of gold NRs induced by Nd:YAG laser and obtain the optimal irradiation conditions for effectively destroying the vascular lesions,tissue-like phantoms were prepared and exposed to Nd:YAG laser with various laser parameters to investigate the photothermolysis of gold *** obtained the optimal photothermolysis of gold NRs for destroying the blood vessel as follows:When the concentration of gold NRs is 26.67 g/mL,the Nd:YAG laser energy density should be 40 J/cm2,with long laser pulse width of 0.3 ms for ten pulses.

关键词： Laser-induced Morphology Change and Photo-thermolysis of Gold Nano Particles with Application in Laser Dermatology

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Numerical Investigation on the Performance of Different Primary Nozzle Structures in the Supersonic Ejector

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Energy Procedia 2017年 105卷 4997-5004页

作者： Kangkang Xue Kaihua Li Weixiong Chen Daotong Chong Junjie Yan State Key Laboratory of Multiphase Flow in Power Engineering Xi’an JiaotongUniversity Xi’an Shaanxi 710049 P.R. China

Computational fluid dynamics (CFD) technique is employed to investigate the effect of primary nozzle structures on the supersonic ejector performance. The performance of the supersonic ejectors with three different nozzle structures, including conical nozzle, petalage nozzle and crenation nozzle, have been compared under the same conditions. Compared with the ejector equipped with the conical nozzle, the entrainment ratio of petalage nozzle is slightly smaller, while the critical back pressure increases by 5.2%. Just the opposite, the entrainment ratio of crenation nozzle is slightly higher, and the critical back pressure would decrease by 2.1%. In addition, the effects of primary/induced fluid pressure on the flow field (pressure and Mach number along the ejector centerline) are observed and analyzed to explain the mixing process occurring inside the ejector. It finds out that the shape of the mixing layer in the supersonic ejector with different nozzles is different.

关键词： Supersonic ejector CFD Primary nozzle Entrainment ratio Critical back pressure

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Changes in relative permeability curves for natural gas hydrate decomposition due to particle migration

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Journal of Natural Gas Science and engineering 2020年 84卷

作者： Yushu Wang Yongfei Yang Ke Wang Liu Tao Jie Liu Chenchen Wang Jun Yao Kai Zhang Wenhui Song Key Laboratory of Unconventional Oil & Gas Development (China University of Petroleum (East China)) Ministry of Education Qingdao 266580 PR China Research Center of Multiphase Flow in Porous Media School of Petroleum Engineering China University of Petroleum (East China) Qingdao 266580 PR China Hubei Cooperative Innovation Center of Unconventional Oil and Gas Yangtze University Wuhan 430100 China

It is very important to study the fluid flow in a natural gas hydrate (NGH) reservoir for hydrate exploitation. During the decomposition of NGH, some particles fall off and flow with the fluid as a result of poor cementation , which usually leads to sand production in the hydrate mining process. In this study, a three-dimensional pore network model (PNM) was established to simulate the three-phase flow of the gas phase (CH 4 ), water phase, and solid phase (particles). Relevant parameters were set considering the deposition, blockage, and flow in the process of particle migration. Then, the gas–water relative permeability curves under different hydrate saturations, particle diameters, and particle numbers were obtained, considering the influence of the change in the pore-throat space during the hydrate decomposition process . The results showed that the gas–water relative permeability equal points (isotonic points) first turned toward the left and then to the right. The analysis results showed that particle deposition and blockage mainly influenced the relative permeability curves during the early period of the hydrate decomposition process. An increase in the pore-throat space was the main factor affecting the relative permeability curves in the late period of the hydrate decomposition process. Moreover, increasing the particle diameter and number of particles caused the isosmotic points of the relative permeability curves moving to the left as a whole because the pore-throat space decreased. Increasing the number of particles first affected the fluid flow in the hydrate reservoir when the temperature was 280 K, pressure was 5.76 MPa, and hydrate saturation was 0.48. In the actual hydrate mining process, this could cause sudden changes in the relative permeability and production. Thus, this condition needs to be avoided. It has important significance in reference to the process of hydrate mining with sand production.

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