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14th IEEE Global Reliability and Prognostics and Health Management Conference, PHM-Hangzhou 2023

作者： Xu, Xiaokang Yang, Yi Wang, Jiangfeng Lou, Juwei Chen, Liangqi State Key Laboratory of Multiphase Flow in Power Engineering School of Energy and Power Engineering Xi'an Jiaotong University Xi'an China Laboratory of Science and Technology on Integrated Logistics Support College of Intelligence Science and Technology National University of Defense Technology Changsha China

ISBN: (纸本)9798350301359

The rotor system plays a very important role in supercritical carbon dioxide Brayton cycle system, and its dynamic problem will directly affect the motion stability and safety of the whole unit. In this paper, the rotor dynamic model of supercritical CO2 coaxial unit is established by finite element method, and the critical speed, modal shape and unbalance response of the rotor are studied. The first seven critical speed of the rotor and the first seven natural frequency of the rotor at the working speed are calculated. The bending modal of the rotor and the position where the rotor amplitude is the largest are analyzed, which can provide reference for the optimization design of the rotor stability. The influences of mass unbalances at the operational speed of rotor are analyzed. The research can provide some suggestions for the optimal design and actual operation of the supercritical CO2 coaxial integrated unit. © 2023 IEEE.

关键词： critical speed unbalance response vibration analysis

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engineering of Fe d-band center in Fe_(3)O_(4)/CeO_(2)hetero-nanoparticles via orbital coupling for high-efficiency oxygen reduction electrocatalysis

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Nano Research 2025年第1期18卷 129-139页

作者： Jiayi Liu Jingwen Yin Yingzi Lin Mingxin Pang Huan Pang Songtao Zhang Lin Xu Jun Yang Yawen Tang Jiangsu Key Laboratory of New Power Batteries Jiangsu Collaborative Innovation Center of Biomedical Functional MaterialsSchool of Chemistry and Materials ScienceNanjing Normal UniversityNanjing 210023Chin a 2 State Key Laboratory of Multiphase Complex Systems Center of MesoscienceInstitute of Process EngineeringChinese Academy of SciencesBeijing 100190China School of Chemistry and Chemical Engineering Yangzhou UniversityYangzhou 225009China Testing Center Yangzhou UniversityYangzhou 225009China

The deliberate engineering of the d-band center of metal site represents an effective strategy to boost the intrinsic electrocatalytic performance toward the oxygen reduction reaction(ORR).Herein,following a heterointerfaceinduced orbital coupling rationale,we report a judicious design of an efficient ORR electrocatalyst consisting of Fe_(3)O_(4)/CeO_(2)hetero-nanoparticles in-situ encased into N-doped carbon nanofibers(abbreviated as Fe_(3)O_(4)/CeO_(2)@N-CNFs hereafter).The theoretic calculations uncover that the Fe_(3)O_(4)/CeO_(2)heterointerface-triggered orbital coupling can cause the down shift of the d-band center positions of Fe sites,which leads to the weakened chemisorption of oxygenated groups and lowered energy barrier for the potential-determining step,ultimately dramatically boosting the ORR intrinsic *** a consequence,the well-designed Fe_(3)O_(4)/CeO_(2)@N-CNFs display admirable ORR activity with a half-wave potential of 0.84 V and outstanding structural/electrochemical stability in an alkaline electrolyte,surpassing the commercial Pt/C benchmark and a majority of recently reported Fe_(3)O_(4)-based *** encouragingly,the Fe_(3)O_(4)/CeO_(2)@N-CNFsincorporated Zn-air battery outperforms the Pt/C-assembled counterpart with higher power density,larger energy density,and excellent cycling stability,serving as a competent candidate for ORR-involved renewable energy *** study offers an innovative approach for the rational manipulation of the d-band center and interfacial electron behavior of active sites toward the optimization of electrocatalytic performance.

关键词： hetero-nanoparticles electrospinning interfacial engineering orbital coupling oxygen reduction reaction

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Progress of vanadium phosphorous oxide catalyst for n-butane selective oxidation

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Chinese Journal of Chemical engineering 2022年第3期35卷 297-315页

作者： Muhammad Faizan Yingwei Li Ruirui Zhang Xingsheng Wang Piao Song Ruixia Liu Beijing Key Laboratory of Ionic Liquids Clean Process State Key Laboratory of Multiphase Complex SystemInstitute of Process Engineering Chinese Academy of SciencesBeijing 100190China University of Chinese Academy of Sciences Beijing 100049China

The utilization of lighter alkanes into useful chemical products is essential for modern chemistry and reducing the CO_(2)***,n-butane has gained special attention across the globe due to the abundant production of maleic anhydride(MA).Vanadium phosphorous oxide(VPO)is the most effective catalyst for selective oxidation of n-butane to MA so ***,the VPO complex exists in more or less fifteen different structures,each one having distinct phase composition and exclusive surface morphology and physiochemical properties such as valence state,lattice oxygen,acidity etc.,which relies on precursor preparation method and the activation conditions of *** catalytic performance of VPO catalyst is improved by adding different promoters or co-catalyst such as various metals dopants,or either introducing template or structural-directing ***,new preparation strategies such as electrospinning,ball milling,hydrothermal,barothermal,ultrasound,microwave irradiation,calcination,sol-gel method and solvothermal synthesis are also employed for introducing improvement in catalytic *** in above-mentioned different aspects will be ascribed in current review in addition to summarizing overall catalysis activity and final *** analyze the performance of the catalytic precursor,the reaction mechanism and reaction kinetics both are discussed in this review to help clarify the key issues such as strong exothermic reaction,phosphorus supplement,water supplement,deactivation,and air/n-butane pretreatment *** to the various industrial applications of VPO.

关键词： N-butane selective oxidation Oxidation of light alkanes Vanadium phosphorus oxide(VPO) Maleic anhydride

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Porous Metal-Organic Framework-Polymer Composites Using High Internal Phase Emulsion Templates: A Review

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Chinese Journal of Structural Chemistry 2022年第12期41卷 60-69页

作者： Yue Qiu Jin-Jin Li Ling Zhao Zhenhao Xi Weikang Yuan State Key Laboratory of Chemical Engineering School of Chemical EngineeringEast China University of Science and TechnologyShanghai 200237China Shanghai Key Laboratory of Multiphase Materials Chemical Engineering East China University of Science and TechnologyShanghai 200237China

As promising engineering materials for green and sustainable processes, porous metalorganic framework(MOF)-polymer composites show great potential in applications, including adsorption, separation, catalysis, and bioengineering. Owing to the mild and scalable operation, porous polymeric materials derived from high internal phase emulsion templates(polyHIPE) have received great interests in recent decades. In this contribution, research progress of the preparation of porous MOF@polyHIPE composites and their applications are reviewed, highlighting how can MOF particles be shaped by HIPE templates, in particular the polymerizable ones. Four different emulsion templates stabilized by MOFs and the applications of corresponding MOF@polyHIPE are included. Hopefully,both the state-of-art and future directions present herein can give rise to the development of highperformance porous MOF@polyHIPEs.

关键词： high internal phase emulsion(HIPE) metal-organic frameworks(MOFs) adsorption and separation heterogeneous catalysis bioengineering

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Surface display of CadR protein on Rhodopseudomonas palustris CGA009 for enhanced heavy metal bioremediation

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Journal of Hazardous Materials 2025年 494卷 138592页

作者： Wang, Minmin Gao, Zixuan Jiang, Qiushi Mu, Xuefang Jiang, Youmin Li, Yanjing Zhang, Sihu Cao, Wen Guo, Liejin State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong University Xianning West Road Xi'an710049 China

Heavy metal pollution poses significant ecological and public health risks, and surface display engineering shows promise for bioremediation in this area. Although anoxygenic photosynthetic purple nonsulfur bacteria (PNSB) have been effectively applied to degrade pollutants due to their metabolic versatility, the use of surface display technology in PNSB remains very limited. In this study, we constructed a surface display system using Rhodopseudomonas palustris CGA009 as the host. The metal-binding protein CadR was fused with outer membrane protein A (OmpA) and expressed in CGA009. SDS-PAGE and immunofluorescence analysis identified the successful expression of the fusion protein on the cell surface. In addition, we used flow cytometry to explore the enhancement effects of linker peptides and different promoters on surface display efficiency under different light intensities. The surface display system enhanced the heavy metal resistance of the host bacteria, and the maximum removal rate of Cd2 + reached 95.6 %. By means of Langmuir isotherm analysis, the maximum biosorption capacity of the system for Cd2+ is 101.11 mg/g. The system demonstrates feasibility for application in complex real-world environmental samples. The presence of various metal ions does not interfere with the system's specific adsorption of Cd²⁺. It can stably maintain an adsorption efficiency of over 80 % under conditions of pH 6–8, temperatures of 20–35°C, and light intensity of 1000–6000 lux. Additionally, the system achieves a removal efficiency of 94.3 % in Cd wastewater. In summary, this study provides a reference for the development of photosynthetic bacterial surface display systems and provides an advanced bioremediation strategy for heavy metal contaminated wastewater. © 2025 Elsevier B.V.

关键词： Bioremediation

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engineering practice and economic analysis of ozone oxidation wet denitrification technology

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Chinese Journal of Chemical engineering 2021年第1期34卷 401-408页

作者： Yang Li Defu Che Chenglong Yang Mingyu Yao Tingwen Zhao Kangli Fu Hanchen Zhao Xi’an Thermal Power Research Institute Co LtdXi’an 710032China State Key Laboratory of Multiphase Flow for Power Engineering Xi’an Jiaotong UniversityXi’an 710049China

SO_(2)and NO emitted from coal-fired power plants have caused serious air pollution in *** this study,a test system for NO oxidation using O_(3)is *** basic characteristics of NO oxidation and products forms are studied.A separate test system for the combined removal of SO_(2)and NO_(x)is also established,and the absorption characteristics of NO_(x)are *** characteristics of NO oxidation and NO_(x)absorption were verified in a 35 t·h^(-1)industrial boiler wet combined desulfurization and denitrification *** operating economy of ozone oxidation wet denitrification technology is *** results show that O_(3)has a high rate and strong selectivity for NO *** O_(3)is insufficient,the primary oxidation product is NO_(2).When O_(3)is present in excess,NO_(2)continues to get oxidized to N_(2)O_(5)or NO_(3).The removal efficiency of NO_(2)in alkaline absorption system is low(only about 15%).NOx removal efficiency can be improved by oxidizing NO_(x)to N_(2)O_(5)or NO_(3)by increasing ozone *** the molar ratio of O_(3)/NO is 1.77,the NOx removal efficiency reaches 90.3%,while the operating cost of removing NO_(x)per kilogram is 6.06 USD(NO_(2)).

关键词： Ozone Denitrification Wet process engineering practice

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PROCESS MODELING AND ECONOMIC VIABILITY ANALYSIS OF A POWER-TO-H2-TO-POWER SYSTEM: CASE STUDY IN CHINA 37

PROCESS MODELING AND ECONOMIC VIABILITY ANALYSIS OF A POWER-...

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37th International Conference on Efficiency, Cost, Optimization, Simulation and Environmental Impact of Energy Systems, ECOS 2024

作者： Li, Yanxin Dai, Yanbing Han, Xiaoqu Guo, Xuanhua Karellas, Sotirios Yan, Junjie State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong University Xi'an China Qingdao Huaru Energy Technology Company Limited Qingdao China Laboratory of Steam Boilers and Thermal Plants National Technical University of Athens 9 Heroon Polytechniou str. Zografou Greece

ISBN: (纸本)9798331307660

The power sector generates the most significant greenhouse gas emissions in many countries, while renewable energy penetration faces a bottleneck due to its ***, it is imperative to make substantial efforts to promote the penetration of renewable energy sources into the power *** process of hydrogen production with renewable energy sources is becoming increasingly economical as the cost of renewable energy sources, particularly onshore wind, has fallen *** the present work, a power-to-H2-to-power system (PHPS) combining onshore wind power was proposed as a solution for high penetration of renewable energy, which incorporates a large-scale alkaline water electrolyzer, and a gas turbine.A techno-economic study based on NOVO PRO© and GT PRO was carried out and applied to cases in Shaanxi, *** performance and operational characteristics of two types of PHPS with different hydrogen storage methods, PHPS/Tank and PHPS/Cavern, were *** is indicated that when 30% of the fuel of the gas turbine was replaced by hydrogen, the levelized cost of energy (LCOE) of the PHPS/Cavern was 0.0498 €/kWh with an internal rate of return (IRR) of 6.41%, therefore, PHPS/Cavern was economically feasible in ***, the renewable energy utilization and carbon reduction benefits of the PHPS were *** surplus electricity (curtailed electricity) and carbon emissions of the PHPS/Cavern can be decreased by 52% and 12%, respectively, compared to those of PHPS without hydrogen as the energy *** performance of PHPS with different hydrogen substitution ratios was *** analysis was further conducted to investigate the influence of key parameters on the system performance, including wind modules investment, electrolyzer investment, transport distance, and electricity ***, under the future scenarios in China in 2050, the LCOE of PHPS/Cavern can be reduced by 15% as well as the IRR increased by 66%.The result

关键词： Hydrogen storage

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Experimental study on the thermochemical reduction of supercritical CO2 by guaiacol

Experimental study on the thermochemical reduction of superc...

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International Multidisciplinary Conference on Computer and Energy Science (SpliTech)

作者： Yimeng Wei Jiadela Kuanibieke Hui Jin State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong University China

The continuous growth of CO 2 emissions is one of the global problems facing humanity, and how to convert and exploit the stock of CO 2 has become an urgent issue. Biomass as an activity of CO 2 thermal reduction medium has become the focus of human attention in general. Supercritical CO 2 (SCCO 2 ) has the advantages of near-liquid density and high solubility, which can further strengthen the reduction process (T≥31.26℃, P≥72.9 atm). This paper described a SCCO 2 reduction method of guaiacol on an intermittent Kettle Reactor to investigate the effects of reaction temperature (400-700℃), residence time (5-20 min) and reactant concentration (4 wt%-16wt%) on the three-phase products. The experimental results indicated that the carbon gasification efficiency (CE) and hydrogen gasification efficiency (HE) were 43.7% and 56.7%, respectively, when the carbon dioxide consumption reached 16.15 mol/kg. As the temperature increased, the consumption of carbon dioxide increased and the concentration of reactants increased with opposite results.

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Homojunction photocatalysts for water splitting

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Nano Research 2022年第12期15卷 10171-10184页

作者： Xiangjiu Guan Shichao Zong Shaohua Shen International Research Center for Renewable Energy State Key Laboratory of Multiphase Flow in Power EngineeringXi’an Jiaotong UniversityXi’an710049China Suzhou Academy of Xi’an Jiaotong University Suzhou215123China Key Laboratory of Subsurface Hydrology and Ecological Effects in Arid Region Ministry of EducationSchool of Water and EnvironmentChang’an UniversityXi’an710064China

Charge-carrier separation is regarded as one of the critical issues of photocatalytic water splitting and could be accelerated by constructing microscopic junctions in *** photocatalysts consisting of different forms of semiconductor with identical compositions could inherit the advantages of heterojunction-based photocatalysts in charge separation due to the built-in electric field,while omitting the potential drawbacks of interfacial lattice distortion by providing continuous band ***,homojunction-based photocatalysts have recently drawn growing attention in water *** this review,the synthetic approaches to preparing photocatalysts with various homojunction structures including p-n junction,phase junction,and facet junction were introduced,together with a comprehensive analysis and discussion on the latest progress in the application of photocatalytic water *** review work is expected to inspire more related work with promoted research on designing efficient homojunction-based photocatalytic systems for water splitting.

关键词： photocatalytic water splitting homojunction charge separation

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Exploration on the stability conditions in bubble columns by noncooperative game theory

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Chinese Journal of Chemical engineering 2022年第10期50卷 75-84页

作者： Jiachen Liu Xiaoping Guan Ning Yang State Key Laboratory of Multiphase Complex Systems Institute of Process EngineeringChinese Academy of SciencesBeijing 100190China School of Chemical Engineering University of Chinese Academy of SciencesBeijing 100049China

The energy-minimization multiscale(EMMS)model,originally proposed for gas-solid fluidization,features a stability condition to close the simplified conservation *** was put forward to physically reflect the compromise of two dominant mechanisms,i.e.,the particle-dominated with minimal potential energy of particles,and the gas-dominated with the least resistance for gas to penetrate through the particle *** stability condition was then formulated as the minimization of the ratio of these two physical ***,the EMMS approach was later extended to the gas-liquid flow in bubble columns,termed dual-bubble-size *** considers the compromise of two dominant mechanisms,i.e.,the liquid-dominated regime with small bubbles,and the gas-dominated regime with large *** stability condition was then formulated as the minimization of the sum of these two physical ***,the two stability conditions were expressed in different manner,though gas-solid and gas-liquid systems bear some *** addition,both the conditions transform the original multiobjective variational problem into a single-objective *** mathematical formulation of stability condition remains therefore an open *** study utilizes noncooperative game theory and noninferior solutions to directly solve the multi-objective variational problem,aiming to explo re the different pathways of compromise of dominant *** results show that only keeping the single dominant mechanism cannot capture the jump change of gas holdup,which is associated with flow regime *** of dominant mechanisms,noninferior solutions and noncooperative game theory can predict the flow regime ***,the game between the two mechanisms makes the two-bubble structure degenerate and reduce to the single-bubble *** game of the three mechanisms restores the two-bubble *** exploration on the formulation of stability conditions may

关键词： Bubble column flow regimes Mesoscale Noncooperative gametheory

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