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Photochemical Systems for Solar‑to‑Fuel Production

Electrochemical Energy Reviews 2022年第3期5卷 137-177页

作者： Ya Liu Feng Wang Zihao Jiao Shengjie Bai Haoran Qiu Liejin Guo International Research Center for Renewable Energy State Key Laboratory of Multiphase Flow in Power EngineeringXi’an Jiaotong UniversityXi’an 710049ShaanxiChina

The photochemical system,which utilizes only solar energy and H_(2)O/CO_(2) to produce hydrogen/carbon-based fuels,is considered a promising approach to reduce CO_(2) emissions and achieve the goal of carbon *** date,numerous photochemical systems have been developed to obtain a viable solar-to-fuel production system with sufficient energy ***,more effort is still needed to meet the requirements of industrial *** this review,we systematically discuss a typical photochemical system for solar-to-fuel production,from classical theories and fundamental mechanisms to raw material selection,reaction condition optimization,and unit device/system advancement,from the viewpoint of ordered energy ***-of-the-art photochemical systems,including photocatalytic,photovoltaic-electrochemical,photoelectrochemical,solar thermochemical,and other emerging systems,are *** highlight the existing bottlenecks and discuss the developing trend of this ***,optimization strategies and new opportunities are proposed to enhance photochemical systems with higher energy efficiency.

关键词： Solar energy Photochemical Hydrogen Carbon-based fuels

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Study on Thermo-Conductive Plastic Finned TubeRadiators

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Journal of Thermal Science 1997年第1期6卷 21-26页

作者： Yang Jiehui Cheng Lixin(Chemical engineering School, state key laboratory of multiphase flow in Power engineering, Xi’anJiaotong University, Xi’an 710049, China) Chemical Engineering School State Key Laboratory of Multiphase Flow in Power Engineering Xi’an Jiaotong University Xi’an China

This paper discusses thermo-conductive plastic finned tube radiators used in water saving type powerstations. First, the development of thermo-conductive plastics is introduced. Second, in order todetermine the rational geometric dimensions of thermo-conductive plastic finned tubes, an objectivefunction which takes the minimum volume of the consumed material for making finned tubes as an ob-ject is introduced. On the basis of the function, the economy comparison between thermaxonductiveplastic finned tubes and metal finned tubes is conducted.

关键词： air-cooling radiator thermo-conductive plastic finned tube optimum geometric parameters economy comparison

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Effect of Particle Orientation on Heat Transfer in Arrays of Prolate Particles

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Computer Modeling in engineering & Sciences 2023年第8期136卷 1509-1526页

作者： Romana Basit Xinyang Li Zheqing Huang Qiang Zhou School of Chemical Engineering and Technology Xi’an Jiaotong UniversityXi’anChina State Key Laboratory of Multiphase Flow in Power Engineering Xi’an Jiaotong UniversityXi’anChina

Direct Numerical Simulations have been carried out to study the forced convection heat transfer of flow through fixed prolate particles for a variety of aspect ratios ar={5/4,5/3,5/1}with Reynolds number(Re)up to *** variations of the solid volume fraction c={0.1,0.2,0.3}with four Hermans orientation factors S={−0.5,0,0.5,1}are *** has been found that changes in S cause prominent variations in the Nusselt *** general,Nusselt number increases with the decrease of *** all three aspect ratios,the Nusselt number remains a linear function of S at different c and ***,it is concluded that,for heat transfer from prolate muti-particle system,the effects of orientations cannot be ignored.A new correlation for Nusselt number has been developed for arrays of prolate particles using the simulation data as a function of Re,c,S and ar.

关键词： Direct Numerical Simulation heat transfer lattice Boltzmann method particle orientations prolate particles

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Resource utilization of solid waste carbide slag:a brief review of application technologies in various scenes

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Waste Disposal and Sustainable Energy 2022年第1期4卷 1-16页

作者： Hongxia Wang Wanyi Xu Maimoona Sharif Guangxu Cheng Zaoxiao Zhang State Key Laboratory of Multiphase Flow in Power Engineering School of Chemical Engineering and TechnologyXi’an Jiaotong UniversityXi’an 710049ShaanxiChina

China is the largest producer and consumer of calcium carbide in the *** calcium carbide industry is an indispensable industry to support the basic life of *** huge production capacity of calcium carbide is accompanied by a large number of solid waste carbide *** to the immature treatment technology of carbide slag,a large number of carbide slag are stacked on-site,resulting in land occupation,air-drying,easy take-off ash,and pollution of the environment and water *** China,calcium carbide is mainly used to produce acetylene and further utilized,80%of which is used to produce polyvinyl chloride(PVC).A large amount of carbide slag is not used,while only a small part is used in the traditional building materials industry,flue gas desulfurization,sewage treatment,etc.,however,the economic benefits are ***,converting the solid waste carbide slag produced by the calcium carbide industry into high value-added CaCO3,CaCl2,CaSO4 whiskers,*** become a potential way to expand the development field of the calcium carbide industry and is environmentally *** paper focuses on summarizing the traditional and emerging high value-added utiliza-tion technologies of carbide slag,and then introduces the application research of carbide slag in carbon emission ***,the defects of these technologies are summarized and further research directions are *** study provides basic guidance for the diversified development of efficient resource utilization of carbide *** abstract Diversified development of calcium carbide industry,resource utilization of solid waste carbide slag and its application of carbon emission reduction have been fully reviewed.

关键词： Calcium carbide Carbide slag Application research High added value Carbon emission reduction

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One-step preparation of efficient cuprous chloride catalyst for direct synthesis of trimethoxysilane

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Chinese Journal of Chemical engineering 2024年第7期71卷 161-171页

作者： Jiaxin Zhang Lu Wang Zhiqiang Ma Chuanjun Di Guanghui Chen Jipeng Dong Jianlong Li Fei Gao Key Laboratory of Multiphase Flow Reaction and Separation Engineering of Shandong Province College of Chemical EngineeringQingdao University of Science and TechnologyQingdao 266042China

CuCl-based catalysts are the most commonly used catalysts for the“direct synthesis”of trimethoxysilane(M3).CuCl species are sensitive to air and water,and are prone to oxidation *** CuCl is directly used as a catalyst,it needs to be purified before the utilization,and the operating conditions for the catalyst preparation are relatively harsh,requiring the inert gas *** a high-temperature activation step required for CuCl-based catalysts used for catalyzing synthesis of M3 to form active phase Cu–Si alloys(Cu_(x)Si)with Si powder,in this work,a series of catalysts for the“direct synthesis”of M3 were obtained by a one-step high-temperature activation of the mixture of stable CuCl_(2) precursors,activated carbon-reducing agent,and Si powder,simultaneously achieving the reduction of CuCl_(2) to CuCl and the formation of active phase Cu_(x)Si alloys of CuCl with Si *** prepared samples were characterized through various characterization techniques,and investigated for the catalytic performance for the“direct synthesis”of ***,the operation conditions were optimized,including the activation temperature,catalyst dosage,Si powder particle size,and reaction *** characterization results indicate that during the one-step activation process,the CuCl_(2) precursor is reduced to CuCl,and the resulting CuCl simultaneously reacts with Si powder to form active phases Cu3Si and Cu15Si4 *** optimal catalyst Sacm(250,0.8:10)exhibits a good catalytic activity with selectivity of 95%and yield of 77%for M3,and shows a good universality for various alcohol ***,the catalytic mechanism of the prepared catalyst for the“direct synthesis”of M3 was discussed.

关键词： Trimethoxysilane Cuprous chloride Catalysis Catalyst activation Reduction Active phase formation

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Thermo-economic analysis and optimization of a novel self-condensing transcritical CO 2 power cycle with ejector refrigeration

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Process Safety and Environmental Protection 2025年 199卷

作者： Jiaxi Xia Jingjing Hou Jiangfeng Wang Juwei Lou Yumin Guo School of mechanical and Electrical Engineering Henan Agricultural University Zhengzhou 450002 China State Key Laboratory of Multiphase Flow in Power Engineering School of Energy and Power Engineering Xi’an Jiaotong University Xi’an 710049 China

The transcritical CO 2 power cycle stands out as a promising approach for the utilization of waste heat and renewable energy, but its practical application is restricted by the condensation challenges of working fluid. To tackle this issue, a novel self-condensing transcritical CO 2 power cycle (SC-TCO 2 PC), which integrates the transcritical CO 2 power cycle with an ejector refrigeration cycle, is proposed. Detailed mathematical models are formulated, and parametric study is carried out to illustrate the correlations between the crucial parameters and system performance from both thermodynamic and economic viewpoints. Then a multi-objective optimization is applied to explore the potential for performance enhancement. Furthermore, the comparative analysis of the SC-TCO 2 PC and the recuperative supercritical CO 2 Brayton cycle (SCO 2 BC) are conducted under optimized conditions. The results demonstrated that the enhanced turbine inlet pressure and temperature positively influence the thermal-economic performance of the SC-TCO 2 PC. Furthermore, the maximum thermal efficiency of 43.90 %, exergy efficiency of 72.97 % and minimum cost per unit of electricity of 0.0372$/kWh are attainable for the SC-TCO 2 PC, reflecting the improvements of 4.88 %pt for maximum thermal efficiency, 6.60 %pt for maximum exergy efficiency and a 8.87 % reduction for minimum unit power cost in comparison to the recuperative SCO 2 BC. In optimum conditions, the SC-TCO 2 PC is capable of achieving a thermal efficiency of 42.11 % and an exergy efficiency of 70.54 % with the cost per unit of electricity of 0.0440$/kWh.

关键词： Brayton cycle

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Particle convective heat transfer near the wall in a supercritical water fluidized bed by single particle model coupled with CFD-DEM

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Particuology 2023年第2期73卷 47-58页

作者： Tianning Zhang Zhen Wan Youjun Lu State Key Laboratory of Multiphase Flow in Power Engineering(SKLMFPE) Xi'an Jiaotong UniversityXi'an710049ShaanxiChina Xi'an Electronic Engineering Research Institute Xi'an710100ShaanxiChina

Supercritical water fluidized bed(SCWFB)is a promising reactor to gasify biomass or *** optimization design is closely related to wall-to-bed heat transfer,where particle convective heat transfer plays an important *** paper evaluates the particle convective heat transfer coefficient(h_(pc))at the wall in SCWFB using the single particle *** critical parameters in the single particle model which is difficult to get experimentally are obtained by the computational fluid dynamics-discrete element method(CFD-DEM).The contact statistics related to particle-to-wall heat transfer,such as contact number and contact distance,are also *** results show that particle residence time(τ),as the key parameter to evaluate h_(pc),is found to decrease with rising velocity,while increase with larger thermal boundary layer thickness.τfollows a gamma function initially adopted in the gas-solid fluidized bed,making it possible to evaluate h_(pc) in SCWFB by a simplified single particle *** theoretical predicted h_(pc) tends to increase with rising thermal gradient thickness at a lower velocity(1.5 U_(mf)),while first decreases and then increases at higher velocity(1.75 and 2 U_(mf)).h_(pc) occupies 30%-57%of the overall wall-to-bed heat transfer coefficient for a particle diameter of 0.25 *** results are helpful to predict the overall wall-to-bed heat transfer coefficient in SCWFB combined with a reasonable fluid convective heat transfer model from a theoretical perspective.

关键词： Supercritical water Fluidized bed Particle residence time Discrete element method Single particle model

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Numerical simulation of strongly swirling turbulent flows in a liquid-liquid hydrocyclone using the Reynolds stress transport equation model

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Science China(Technological Sciences) 2000年第1期43卷 86-96页

作者：陆耀军周力行沈熊 State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong University Xi'an 710049 China Department of Engineering Mechanics Tsinghua University Beijing 100084 China

The Reynolds stress transport equation model (DSM) is used to predict the strongly swirling turbulent flows in a liquid-liquid hydrocyclone, and the predictions are compared with LDV measurements . Predictions properly give the flow behavior observed in experiments, such as the Rankine-vortex structure and double peaks near the inlet region in tangential velocity profile, the downward flow near the wall and upward flow near the core in axial velocity profiles. In the inlet or upstream region of the hydrocyclone, the reverse flow near the axis is well predicted, but in the region with smaller cone angle and cylindrical section, there are some discrepancies between the model predictions and the LDV measurements. Predictions show that the pressure is small in the near-axis region and increases to the maximum near the wall. Both predictions and measurements indicate that the turbulence in hydrocy-clones is inhomogeneous and anisotropic.

关键词： strongly swirling flows numerical simulation hydrocyclone

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Error Analysis of Liquid Holdup Measurement in Gas-Liquid Annular flow Through Circular Pipes Using High-Speed Camera Method

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Journal of Shanghai Jiaotong university(Science) 2018年第S1期23卷 34-40页

作者： LIU Li BAI Bofeng School of Nuclear Science and Engineering Shanghai Jiao Tong University State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong University

Accurate measurement of gas-liquid phase fraction is essential for the proper modelling of the pressure drop, heat transfer coefficient, mass transfer rate and interfacial area in two-phase flows. In this paper, taking the issue of optical distortion into account, an analytical model was proposed to estimate and correct the liquid holdup in gas-liquid annular flow through a circular pipe using high-speed camera method. The error in the liquid holdup measurement generated from different refractive indices among transparent circular pipe, liquid film and air core was firstly theoretically analyzed based on the geometric optics. Experimental tests were then carried out to identify the difference as well as to validate the proposed model. Results indicated that the prediction of the liquid holdup has a good performance with the experimental data(i.e., mean relative error is 4.1%) and the measured liquid holdup is larger than the real one. It was found that the measured liquid holdup is larger than the real one. Generally, when the real liquid holdup gets smaller, the discrepancy between the measured liquid holdup by image and the real liquid holdup becomes more significant. Thus, after measuring the liquid holdup from the images, the value of the measured liquid holdup must be corrected by the present model in order to obtain the real liquid holdup.

关键词： gas-liquid annular flow liquid holdup optical refraction analytical correction

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Experimental Study on Condensation Heat Transfer Characteristics inside an Inclined Wave-Finned Flat Tube of Direct Air-Cooling System

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Journal of Thermal Science 2021年第2期30卷 432-440页

作者： WANG Haitao TAO Tao MEI Xuesong WANG Haijun GU Hongfang State Key Laboratory for Manufacturing Systems Engineering Xi'an Jiaotong UniversityXi'an 710049China Shaanxi Key Laboratory of Intelligent Robots School of Mechanical EngineeringXi'an Jiaotong UniversityXi'an 710049China State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong UniversityXi'an 710049China

In this paper,the condensation heat transfer characteristics of parallel flow and counter flow inside an inclined wave-finned flat tube is investigated *** condensation heat transfer coefficients are analyzed based on the experimental *** of experiments show that condensation heat transfer coefficient decreases as the temperature difference Δt=ts-tw increases and mass flow rate *** parallel flow has a similar development with the counter flow,and the condensation heat transfer coefficient of counter flow is less than that of parallel flow under the same air cooling *** addition,condensation heat transfer coefficient correlations are also obtained under experimental *** calculations agree well with the measured data and the agreement is seen to be within ±4% for the parallel flow and ±5% for the counter flow.

关键词： condensation heat transfer wave-finned fiat tube modified model parallel flow counter flow

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