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Synthesis of Co3o4@C/Ti3c2tx Mxene-Type Composites for Enhanced Electromagnetic Wave Absorption

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SSRN 2024年

作者： Hou, Yunxi Jia, Zhen Zheng, Hanli Hu, Zewei Shen, Lu Liu, Dongyu Li, Lu Liu, Shiwei Liu, Yue Yu, Shitao Key Laboratory of Multiphase Flow Reaction and Separation Engineering of Shandong Province State Key Laboratory Base of Eco-chemical Engineering College of Chemical Engineering Qingdao University of Science and Technology Qingdao266042 China A VIC Research Institute for Special Structures of Aeronautical Composites 19 Jiqi Road Jinan250000 China

Highly efficient microwave absorbing materials have attracted widespread attention due to the harmful effects of electromagnetic pollution on the human body and electronic equipment. In this paper, Co3O4@C composites with core-shell structure were prepared by hydrothermal method using a simple strategy, and then Ti3C2Tx was assembled with core-shell Co3O4@C by electrostatic self-assembly method, which resulted in the successful attachment of Co3O4@C to the lamellar structure of Ti3C2Tx and the formation of MXene-based composite wave-absorbing Co3O4@C/Ti3C2Tx material. The composites exhibit strong electromagnetic wave absorption when the mass ratio of Co3O4@C to Ti3C2Tx was 1:2, with a minimum reflection loss of -35.2 dB at a matched thickness of only 4.5 mm. Excellent electromagnetic wave absorption performance Co3O4@C/Ti3C2Tx composite material was mainly attributed to the synergistic effect of the multiple reflection absorption of the core-shell structure and the high conductivity and large specific surface area of MXene material. These results indicate that Co3O4@C/Ti3C2Tx composites were promising candidates for electromagnetic absorption and provide new ideas for the design of MXene-based magnetic absorption materials. © 2024, The Authors. All rights reserved.

关键词： Composite materials

Ab initio investigation of defect formation at ZrO2-CeO2 interfaces

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Physical Review B 2012年第8期86卷 085407-085407页

作者： Marco Fronzi Silvia Cereda Yoshitaka Tateyama Alessandro De Vita Enrico Traversa International Center for Materials Nanoarchitectonics (MANA) National Institute for Materials Science (NIMS) Tsukuba Japan Physics Department King's College London Strand London United Kingdom International Research Center for Renewable Energy State Key Laboratory of Multiphase Flow in Power Engineering Xian Jiaotong University Xian Shaanxi China

The structural and electronic properties of low index (100) and (111) ZrO2-CeO2 interfaces are analyzed on the basis of density functional theory calculations. The formation energy and relative stability of substitutional defects, oxygen vacancies, and vacancy-dopant complexes are investigated for the (100) orientation. By comparing these results with the ones obtained in bulk structures, we provide a possible explanation for the higher experimental ionic conductivity measured at the interface.

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Curvature Adaptive Voxel-Based Monte Carlo Method with Application for Customized Retinal Laser Surgery

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SSRN 2024年

作者： Zhang, Hao Li, Dong Chen, Bin Zhang, Hanfeng Liang, Yao Zheng, Yuping Wang, Guoxiang State Key Laboratory of Multiphase Flow in Power Engineering Xi’an Jiaotong University Xi’an710049 China Department of Ophthalmology 2nd affiliated hospital Medical School Xi’an Jiaotong University Xi’an710049 China Department of Mechanical Engineering The University of Akron AkronOH44325 United States

Accurate prediction of light propagation and energy deposition in biological tissues is crucial for the success of laser-based medical treatments. We propose a novel Curvature Adaptive Voxel-based Monte Carlo method (CAVMC) to correct for light reflection and refraction at curved interfaces by introducing coordinate transformation with an artificial surface parallel to the curved interface. This approach achieves an optimal balance between simulation accuracy and efficiency. Our study demonstrates that for small optical mismatches, the relative error can be reduced significantly, with the energy deposition error dropping from 34.7% to 6.6%. For large optical mismatches, CAVMC substantially improves accuracy, reducing computational errors by more than 50%. We validated CAVMC in a customized retinal laser therapy scenario for diabetic retinopathy, demonstrating its ability to accurately predict laser energy deposition and thermal effects, which is crucial for avoiding tissue damage during treatments. The efficiency and accuracy of the CAVMC method make it valuable for personalized retinal laser surgery and potentially other medical applications. Overall, CAVMC offers a robust tool for simulating light propagation in heterogeneous biological tissues, enhancing the precision and safety of medical treatments. © 2024, The Authors. All rights reserved.

关键词： Laser surgery

Study on the Flame Structure and flow Field of Hydrogen-Enriched Combustion in Array Micro-Tube

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SSRN 2024年

作者： Tian, Liang Feng, Wenbin Han, Xiao Liu, Yuzhi Liu, Hongfang Cai, Xiao School of Energy and Environmental Engineering Hebei University of Technology Tianjin300401 China National Key Laboratory of Science and Technology on Aero-Engine Aero thermodynamics Research Institute of Aero-Engine Collaborative Innovation Center for Advanced Aero-Engine Beihang University Beijing100191 China State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong University Xi’an710049 China

Addressing climate change and reducing greenhouse gas emissions are critical priorities. Utilizing hydrogen-rich methane or pure hydrogen as fuels within gas turbines, facilitated by array micro-tube premixed combustion technology, is anticipated to markedly accelerate the decarbonization process of the energy sector. In this study, the flame structure of the array micro-tube premixed burner under various fuel compositions was examined using OH-Planar Laser-Induced Fluorescence (OH-PLIF) and Particle Image Velocimetry (PIV) measurement techniques. The effects of the equivalence ratio (φ) and the hydrogen power ratio (HPR) on the characteristics of the flame front, including its curvature, density, volume, and the associated flow field properties, were discussed. As φ and HPR increase, the wrinkled structure of the flame front is significantly enhanced, with a more pronounced effect on smaller scales. This enhancement leads to the separation of the unburned pockets from the main flame. Concurrently, both the flame length and flame area decrease with the augmentation of φ and HPR, indicating a more concentrated combustion process and increased combustion intensity under hydrogen-enriched and pure hydrogen conditions. The study also observed a slight increase in both the negative and positive curvatures of the flame front, with a more notable increase in negative curvature. The increased negative curvature results in an elevated degree of wrinkling and a higher value of Σ (flame surface density), reaching a maximum of 0.876 mm-1 under the conditions where φ is 0.8 and (mean progress variable) is 0.5, resulting in the smallest observed flame volume of 100.6 mm3. Upon coupling the flame with the flow field, it was discovered that the exit flow field of the array micro-tube exhibits symmetry and a characteristic conical flame shape. The burning velocity of the side flame brushes increases, and the velocity peak shifts upstream. The above findings confirms that the additio

关键词： flow fields

Numerical Simulations on Hybrid Thermal Management of Mini-Channel Cold Plate and Pcm for Lithium-Ion Batteries

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SSRN 2024年

作者： Liu, Yang Zhou, Zhifu Wu, Wei-Tao Wei, Lei Li, Yang Liu, Xinyu Huang, Heng Li, Yubai Song, Yongchen Key Laboratory of Ocean Energy Utilization and Energy Conservation of Ministry of Education Dalian University of Technology Dalian116024 China State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong University Xi’an710049 China School of Mechanical Engineering Nanjing University of Science and Technology Nanjing210094 China Department of Mechanical and Energy Engineering Southern University of Science and Technology Shenzhen518055 China

In this study, a novel battery thermal management system (BTMS), combining phase change material (PCM) and mini-channel cold plates (MCPs), was modeled and analyzed. First, the effects on single cell cooling using MCPs and PCM alone are investigated at different coolant rates, temperatures, and PCM thicknesses. Then, the hybrid thermal management system (HTMS) is developed with the aim of reducing the cooling load of the PCM through hybridization with MCPs and the optimal combination of them is investigated. At the end of this work, the thermal performance of a battery pack with a hybrid thermal management structure has been analyzed, where the cold plate can take away the heat from the PCM to restore its thermal storage capacity. The results show that the combination of 3 channel and 10 mm PCM with 0.1 m/s coolant velocity and 20°C coolant temperature is the quit suitable regarding the cooling performance. Under 2C discharging rate, this design reduces the maximum battery temperature to 40°C, which is 32.5% lower, and the average temperature to 35℃, which is 41% lower than it without cooling. The study's findings offer potential new strategies and predictions for hybrid thermal management that utilize MCPs and PCM. © 2024, The Authors. All rights reserved.

关键词： Lithium-ion batteries

A mixed discontinuous Galerkin method with symmetric stress for Brinkman problem based on the velocity-pseudostress formulation

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arXiv

arXiv 2019年

作者： Qian, Yanxia Wu, Shuonan Wang, Fei Wang, Fei School of Mathematics and Statistics Xi'An Jiaotong University Xi'an Shaanxi710049 China School of Mathematical Sciences Peking University Beijing100871 China School of Mathematics and Statistics State Key Laboratory of Multiphase Flow in Power Engineering Xi'An Jiaotong University Xi'an Shaanxi710049 China

The Brinkman equations can be regarded as a combination of the Stokes and Darcy equations which model transitions between the fast flow in channels (governed by Stokes equations) and the slow flow in porous media (governed by Darcy?fs law). The numerical challenge for this model is the designing of a numerical scheme which is stable for both the Stokes-dominated (high permeability) and the Darcy-dominated (low permeability) equations. In this paper, we solve the Brinkman model in n dimensions (n = 2, 3) by using the mixed discontinuous Galerkin (MDG) method, which meets this challenge. This MDG method is based on the pseudostress-velocity formulation and uses a discontinuous piecewise polynomial pair PSk+1-Pk(k ≥ 0), where the stress field is symmetric. The main unknowns are the pseudostress and the velocity, whereas the pressure is easily recovered through a simple postprocessing. A key step in the analysis is to establish the parameter-robust inf-sup stability through specific parameter-dependent norms at both continuous and discrete levels. Therefore, the stability results presented here are uniform with respect to the permeability. Thanks to the parameter-robust stability analysis, we obtain optimal error estimates for the stress in broken H(div)-norm and velocity in L2-norm. Furthermore, the optimal L2 error estimate for pseudostress is derived under certain conditions. Finally, numerical experiments are provided to support the theoretical results and to show the robustness, accuracy, and flexibility of the MDG method. Copyright © 2019, The Authors. All rights reserved.

关键词： Stability

Numerical Simulations for Comparison of Cold Plate Cooling and Hfe-7000 Immersion Cooling in Lithium-Ion Battery Thermal Management

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SSRN 2024年

作者： Liu, Xinyu Zhou, Zhifu Wu, Wei-Tao Wei, Lei Hu, Chengzhi Li, Yang Huang, Heng Li, Yubai Song, Yongchen Key Laboratory of Ocean Energy Utilization and Energy Conservation of Ministry of Education Dalian University of Technology Dalian116024 China State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong University Xi’an710049 China School of Mechanical Engineering Nanjing University of Science and Technology Nanjing210094 China Department of Mechanical and Energy Engineering Southern University of Science and Technology Shenzhen518055 China

In this work, fluorinated liquids can be used as a new immersion coolant for effective battery thermal management (BTM) because of their insulating and non-flammable inert characteristics. In this research, the liquid chosen for immersion cooling is HFE-7000, characterized by a boiling point of 34°C. The analysis of bubble kinetics is employed to investigate the heat transfer mechanism in two-phase immersion cooling by examining the behavior of bubbles during the boiling process. The square ternary Li-ion batteries are subjected under loads of 2C and 3C cooled by immersion cooling and a mini-channel cold plate as a comparison. It turns out that immersion liquid cooling modules offer superior thermal performance. Under constant current (CC), the peak temperature is reduced by 4.89°C and 9.31°C compared with the mini-channel cold plate cooling (CPC). Under dynamic load conditions, the maximum temperature rise of the battery is reduced by 29.89% and 43.89% compared to CPC. As a passive heat dissipation method, two-phase immersion cooling reduces the design requirements for active control. Also, it delivers an efficient battery thermal management system (BTMS) designed for upcoming electric vehicles (EVs). © 2024, The Authors. All rights reserved.

关键词： Lithium-ion batteries

Zero-Energy Nonlinear Temperature Control of Lithium-Ion Battery Based on a Shape Memory Alloy

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SSRN 2024年

作者： Li, Yang Bai, Minli Zhou, Zhifu Wu, Wei-Tao Wei, Lei Hu, Chengzhi Liu, Xinyu Gao, Shuai Li, Yubai Song, Yongchen Key Laboratory of Ocean Energy Utilization and Energy Conservation of Ministry of Education Dalian University of Technology Dalian116023 China State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong University Xi'An710049 China School of Mechanical Engineering Nanjing University of Science and Technology Nanjing210094 China Department of Mechanical and Energy Engineering Southern University of Science and Technology Shenzhen518055 China

Improving the poor performance of lithium-ion battery (LIB) in extreme temperatures is essential to promoting electric vehicles (EVs) into wider application. The most severe challenge for the existing battery thermal management systems (BTMSs) is to overcome the contradiction between excellent heat dissipation at high temperatures and effective insulation at low temperatures. Here, we propose a zero-energy nonlinear temperature control strategy based on thermal regulator. The designed thermal regulator based on shape memory alloy (SMA) can switch the heat flux on the battery surface according to its temperature without any power supply or logic control and provide the desirable thermal functions. This thermal regulator increases the battery capacity by 55.44% in the cold environment of -20℃ compared to the baseline BTMS with superior heat dissipation. Simultaneously, it can limit the battery peak temperature to near the FS49 boiling point (49℃) in the hot environment of 45℃ to ensure safety. Furthermore, we demonstrate that the thermal regulator enables thermal runaway to be effectively suppressed inside the battery, reducing the emission of combustible or toxic gases by 72.26%, which is reported for the first time. Finally, we simplify the design of the thermal regulator from the perspective of system integration and demonstrate the feasibility of the thermal regulator at the battery pack level. © 2024, The Authors. All rights reserved.

关键词： Lithium-ion batteries

Thermal Management for the Prismatic Lithium-Ion Battery Pack by Immersion Cooling with Fluorinated Liquid

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SSRN 2024年

In this study, a novel FS49-based battery thermal management system (BTMS) was proposed and tested for cooling the prismatic lithium-ion battery (LIB) module. The boiling of dielectric refrigerant occurred at the battery surface, which provided strong and uniform cooling for each battery cell. The results show that the peak temperature difference of liquid immersion cooling (LIC) module during 1C rate discharging and charging was reduced by 91.3% and 94.44%, respectively, compared to the natural convection (NC) module. The reduction of temperature nonuniformity greatly reduced the state of charge (SOC) inhomogeneity of different cells within the module. Moreover, the energy density of LIC module can be optimized by reducing the cell spacing and liquid filling ratio. Comparing with 100% filling rate, the module maximum temperature corresponding to 25% filling rate (with wick) during 2C rate discharging is only increased by 1.6°C, however, the module peak temperature difference is reduced by 53.3%, and the energy density is increased by 13.14%. In addition, Equivalent circuit model (ECM) and volume of fluid (VOF) model were used to simulate the LIC module, and the numerical results are in good agreement with the experimental data. This study provides a systematic design plan and numerical method for the engineering application of LIC in the field of BTMS. © 2024, The Authors. All rights reserved.

关键词： Lithium-ion batteries