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SSRN 2023年

作者： Li, Naixu Xu, Lei Ren, Yuqi Liu, Maochang Zhu, Fengfan Cheng, Miao Zhou, Jiancheng Chen, Wenshuai Wang, Ke Wang, Nan School of Chemistry and Chemical Engineering Southeast University No.2 Dongnandaxue Road Jiangsu Nanjing211189 China International Research Center for Renewable Energy State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong University No.28 Xianning West Road Shaanxi Xi'An710049 China Key Laboratory of Bio-Based Material Science and Technology Ministry of Education Northeast Forestry University No. 26 Hexing Road Harbin150040 China

This study is dedicated to solving the problems of low energy utilization and low yield in the conventional photocatalytic CO2 reduction process. In this work, a novel concentrated solar (light) reactor was established to improve solar energy utilization efficiency and CO2 conversion rate by concentrating light and heat (that is, by converting light into heat). The TF@TNT/0.4CoOx-0.1CuO monolithic photocatalyst based on titanium foam was designed and prepared. The results showed that the light intensity increased by ~10.6 times (from 400 mW/cm2 to 4266 mW/cm2) while the yield of CH4, the product of CO2 reduction driven by photo-thermal coupling effect, increased by ~220 times (from 0.53 µmol/cm2 to 116.4 µmol/cm2) in the concentrated solar (light) reactor. The results of CH4 yield, electrochemical measurement, and apparent activation energy calculation were investigated in the concentrator reactor under the conditions of concentrated and non-concentrated irradiation of simulated sunlight in different wavelength ranges. It can be found that the concentrated light and the induced photo-thermal coupling effect can significantly reduce the reaction barrier (from 41.62 to 31.51 kJ/mol) and improve the conversion efficiency of solar energy to chemical energy by ~15 times. This provides a potentially feasible method for efficient and green utilization of CO2 driven by solar energy. © 2023, The Authors. All rights reserved.

关键词： Solar energy

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Determination of mass diffusion coefficients of oxygenated fuel additives in air using digital real-time holographic interferometry

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Journal of Physics: Conference Series 2009年第1期147卷

作者： Maogang He Ying Guo Qiu Zhong Ying Zhang State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong University Xi'an 710049 People's Republic of China

In this work, an experimental system based on digital real-time holographic interferometry for measuring the mass diffusion coefficients of fluid is introduced. The method of processing interference fringe hologram is also introduced thoroughly. By uncertainties analysis and experimental verification, the accuracy of this system is validated. The experimental uncertainties in temperature and mass diffusion coefficient are estimated to be no greater than ± 0.16 K and ± 0.2 %, respectively. On this basis, the mass diffusion coefficients of three fuel additives, diethyl 1,6-hexanedioate (diethyl adipate, DEA), dimethyl carbonate (DMC) and diethyl carbonate (DEC) in air were measured at T = (278.15 to 338.15) K under atmospheric pressure, and polynomial was fitted by the experimental data.

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Strengthening Chlorobenzene Catalytic Degradation Rate and Selectivity Over Laxsr1-Xmno3±Δ by Anchoring Interfacial Oxygen Vacancy

SSRN

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SSRN 2022年

作者： Li, Lu Tao, Dan Zhao, Qi Fu, Shuangshuang Min, Xin Chen, Changwei Tian, Mingjiao Shi, Jianwen He, Chi State Key Laboratory of Electrical Insulation and Power Equipment Center of Nanomaterials for Renewable Energy School of Electrical Engineering Xi’an Jiaotong University Shaanxi Xi’an710049 China State Key Laboratory of Multiphase Flow in Power Engineering School of Energy and Power Engineering Xi’an Jiaotong University Shaanxi Xi’an710049 China College of Geology and Environment Xi’an University of Science and Technology Shaanxi Xi’an710054 China Faculty of Electronic and Information Engineering Xi’an Jiaotong University Shaanxi Xi’an710049 China School of Environmental and Municipal Engineering Xi’an University of Architecture and Technology Shaanxi Xi’an710055 China School of Environmental Science and Engineering Shanghai Jiao Tong University 800 Dongchuan Road Shanghai200240 China

Surficial lattice oxygen in perovskite compounds is a common participant during chloroaromatic catalytic destruction. Herein, we proposed a facile oxygen vacancy construction strategy for preparing high active LaxSr1-xMnO3±δ (LSMO) via NaBH4 treatment. Results reveal that LSMO composites are not only reduced by NaBH4 under mild condition, but trigger a significant Sr segregation effect, which plays a key role in oxygen vacancy formation accounting to the electron donation from Sr to Mn acceptor and subsequent lattice oxygen activation. Moreover, the concentration of interfacial active oxygen species can be regulated by taming the La-Sr interaction with different Sr substitution proportions. The anchored oxygen vacancies (OVs) take advantage of electron capture or transfer and induce molecule oxygen into active oxygen species to react with chlorobenzene molecules, resulting in a preferential catalytic oxidation capacity. Amongst, reduced La0.5Sr0.5MnO3±δ catalyst displays superior chlorobenzene destruction efficiency with 90% of which converted as low as 236 °C, which also exhibited a stable performance in long-time operation. However, the OVs would be refilled by water H2O molecules resulting in a weaker water resistance for OVs anchored catalyst. In summary, the annihilation of OVs is the most important factor for catalyst deactivation. The research offers a new avenue to construct interfacial oxygen species in perovskite oxides during the chlorobenzene deep oxidation process. © 2022, The Authors. All rights reserved.

关键词： Catalytic oxidation

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Research on a Poly-Generation System for Gas-Biochar-Heat-Electricity by Supercritical Water Gasification of Biomass Waste

SSRN

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SSRN 2024年

作者： Wang, Cui Jin, Hui School of Water and Environment Chang'an University Xi’an710054 China Key Laboratory of Subsurface Hydrology and Ecological Effect in Arid Region of the Ministry of Education Chang'an University Xi’an710054 China Key Laboratory of Eco-hydrology and Water Security in Arid and Semi-arid Regions of Ministry of Water Resources Chang’an University Xi’an710054 China State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong University Xi’an710049 China Ministry of Education of China Chongqing University Chongqing400044 China

Biomass energy is renewable and rich in the world, providing a solution for the shortage in fossil fuel and serious environmental pollution. Proposing efficient utilization method of biomass waste demands urgent attention. Supercritical water gasification (SCWG) process is a potential technology. In this work, a poly-generation system based on SCWG was developed to convert biomass waste to gas, biochar, heat and electricity. Firstly, mass, energy, and exergy flow were calculated at the typical condition. Subsequently, impact of various operating parameters, including gasification temperature, mass flowrate of preheated water, biomass concentration, on the hydrogen-rich syngas yield, generated electricity, thermodynamic performance of the system was investigated. The result demonstrated that the exergy loss primarily occurred on cooler, reactor, heat exchanger and preheater, accounting for more than 90% of total exergy loss under different conditions, arising from irreversible reaction, heat transfer and heat dissipation. Higher temperature, higher biomass concentration and more preheated water exerted a positive effect for hydrogen-rich gas production and supplied heat energy, while these parameters were disadvantageous to exergy efficiency. Biochar energy was primarily affected by biomass concentration. Energy efficiency increased with preheated water quantity and biomass concentration rising, and impact of biomass concentration was more significant. Conversely, evaluated gasification temperature displayed an adverse effect on energy efficiency. The maximal exergy efficiency reached about 58.3% at 550℃, biomass concentration of 33%, preheated water mass flowrate of 900 kg·h-1 © 2024, The Authors. All rights reserved.

关键词： Biomass

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A Piv Measurement and Numerical Simulation of Gas‐Liquid Two‐Phrase flow in An Aeration Tank

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AIP Conference Proceedings 2007年第1期914卷 453-457页

作者： Wen Cheng Chun‐Di Yang Yuichi Murai Fujio Yamamoto 1State Key Laboratory of Multiphase Flow in Power Engineerig Xi’ann Jiaotong University Xi’an 710049 China 2Environment Research Institute Xian University of Technology Xian 710048 China 3Div. of Mec. Science Graduate School of Engineering Hokkaido University Japan 4Graduate School of Engineering University of Fukui Bunkyo 3‐9‐1 Fukui 910‐8507 Japan

Aeration plays an important role in the treatment of activated sludge. The aeration performance is deeply affected by the movement law of bubble liquid flow in aeration tank. In order to discuss the influence of gas‐phase, liquid‐phase motions in an aeration tank on the sewage disposal, three kinds of boundaries and initial conditions were applied in the experiment to study the law of two‐phase flow. A developed two‐equation turbulence model was employed in this paper. Results obtained by experiment are compared with those from the mathematical model. It is found that the results of measurement and simulation agree with each other.

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Measurement of falling film thickness around a horizontal tube using laser-induced fluorescence technique

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Journal of Physics: Conference Series 2009年第1期147卷

作者： Xiaofei Wang Maogang He Hualiang Fan Ying Zhang State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong University Xi'an 710049 People's Republic of China

An optical method for the non-intrusive measurement of falling film thickness on the perimeter of the horizontal tube is described. This non-intrusive measurement method is based on the visualization of the falling film flowing around the horizontal tube and uses the laser induced fluorescence and image processing techniques. The falling film thickness around a Turbo-CII horizontal tube and a plain horizontal tube was measured when water flushed the tube vertically with a stable velocity. The results for the Turbo-CII tube are compared with those for the plain tube, and show that the film thickness around the Turbo-CII tube varies with the same trend as that around the plain tube, and the minimal values of the film thickness tend to locate at different angular position of 95°-120° under different conditions. The film thickness around the enhanced tube changes within a smaller range with time than that around the plain tube. The corresponding effects on flow uniformity have also been discussed.

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Numerical study on the influence of plugging rate on the performance of adjustable steam ejector

International Journal of Fluid Engineering

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International Journal of Fluid engineering 2024年第2期1卷 50-60页

作者： Jianxiang Gao Zepeng Yuan Yuyan Hou Weixiong Chen State Key Laboratory of Multiphase Flow in Power Engineering Xi’an Jiaotong UniversityXi’an 710049People’s Republic of China

During the operation of thermal power plant systems, severe challenges to the quality and safety of the heat supply arise owing to the effects of peak regulation. Steam ejectors, widely employed in the district heating sector, often exhibit poorer performance under off-design conditions as a result of their fixed structure. This study analyzes the effects of varying plugging rate, primary pressure, and induced pressure on the performance of adjustable steam ejectors. As the plugging rate increases, the mass flow rate of the primary fluid decrease, potentially falling below 32%, and that of the induced fluid initially experiences a minor increase, followed by a rapid decrease. Concurrently, the critical back pressure also decreases with an increase in the plugging rate, potentially falling by up to 65%. By contrast, the entrainment ratio surges with increasing plugging rate, with the maximum increase reaching up to 4.75 times. Under the same primary steam pressure and induced steam pressure, there exists an optimal entrainment ratio. Furthermore, both the critical back pressure and the optimal entrainment ratio increase as the primary steam pressure and induced steam pressure increase.

关键词： performance steam optimal

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Novel Design of In-Situ Hydrogen Sorption/Storage Integrated Enhanced Hydrogen Production in Supercritical Co2 Gasification, Air Gasification, and Steam Gasification from Biomass

SSRN

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SSRN 2023年

作者： Yang, Tiebing Tie Dou, Binlin Zhang, Hua Wu, Kai Ning, Luo Chen, Haisheng Xu, Yujie Li, Wei Wu, Chunfei School of Energy and Power Engineering Shanghai Key Laboratory of Multiphase Flow and Heat Transfer in Power Engineering University of Shanghai for Science and Technology Shanghai200093 China Institute of Engineering Thermophysics Chinese Academy of Sciences Beijing100190 China Department of Energy Engineering Zhejiang University Hangzhou310027 China School of Chemistry and Chemical Engineering Queen's University Belfast BelfastBT7 1NN United Kingdom

Novel process on in-situ hydrogen sorption/storage during water gas shift (WGS) was proposed and the enhanced hydrogen production in supercritical CO2 gasification (CG), air gasification (AG), and steam gasification (SG) from biomass was integrated. The effects of temperature, pressure, steam-to-carbon (S/C) ratio, and adsorbent content for in-situ hydrogen sorption/storage on the enhanced hydrogen production were determined. The energy and exergy analysises under different thermodynamic conditions were calculated and compared. The results show that as the temperature increases, the hydrogen conversion and yield from water gas shift (WGS) reaction with in-situ hydrogen sorption/storage based on Mg-based sorbent were greatly increased, in which SG has the highest hydrogen yield and AG has the highest hydrogen conversion. The steam-to-carbon (S/C) ratio has a positive effect on the hydrogen production for all the processes, and also presents an effect on in-situ hydrogen sorption/storage during WGS. The methanation reaction was greatly inhibited by AG. The energy requirement order was SG> CG >AG, and the system energy can be supplied by in-situ hydrogen sorption/storage. © 2023, The Authors. All rights reserved.

关键词： Biomass

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An efficient cellular flow model for cohesive particle flocculation in turbulence

arXiv

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arXiv 2020年

作者： Zhao, K. Vowinckel, Bernhard Hsu, T.-J. Köllner, T. Bai, B. Meiburg, E. Department of Mechanical Engineering UC Santa Barbara CA93106 United States State Key Laboratory of Multiphase Flow in Power Engineering Xi’an Jiaotong University Xi’an710049 China Leichtweiß-Institut für Wasserbau Technische Universität Braunschweig Braunschweig38106 Germany Center for Applied Coastal Research Department of Civil & Environmental Engineering University of Delaware NewarkDE19716 United States

We propose a one-way coupled model that tracks individual primary particles in a conceptually simple cellular flow setup to predict flocculation in turbulence. This computationally efficient model accounts for Stokes drag, lubrication, cohesive and direct contact forces on the primary spherical particles, and allows for a systematic simulation campaign that yields the transient mean floc size as a function of the governing dimensionless parameters. The simulations reproduce the growth of the cohesive flocs with time, and the emergence of a log-normal equilibrium distribution governed by the balance of aggregation and breakage. Flocculation proceeds most rapidly when the Stokes number of the primary particles is O(1). Results from this simple computational model are consistent with experimental observations, thus allowing us to propose a new analytical flocculation model that yields improved agreement with experimental data, especially during the transient stages. Copyright © 2020, The Authors. All rights reserved.

关键词： Turbulence

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Adsorption of Dibenzofuran by Modified Biochar Derived from Microwave Gasification

SSRN

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SSRN 2024年

作者： Ren, Jiyun Zhang, Yong Wang, Hui Huang, Xiaoming Jin, Xiaoling Zhang, Kai Li, Ruiyu Yang, Kaixuan Yue, Yang Deng, Lei Che, Defu State Key Laboratory of Multiphase Flow in Power Engineering School of Energy and Power Engineering Xi’an Jiaotong University Xi’an710049 China Yantai Longyuan Power Technology Co. Ltd Yantai264000 China West Pipeline Company of PipeChina Urumchi830000 China Jinggangshan Power Plant Huaneng Power International Inc Jiangxi 343009 China Shunde Institute of Inspection Guangdong Institute of Special Equipment Inspection and Research Foshan528300 China Shanghai Power Equipment Research Institute Co. Ltd. Shanghai200240 China

Dioxins, emanating from the waste incineration, constitutes an organic pollutant that poses considerable risks to human health and environment. In this study, the corn straw char (CSC) and oak char (OC) derived from the electric heating and microwave gasification, and the coconut-shell activated carbon (AC) are employed as absorbents for the adsorption of dibenzofuran (DBF, dioxins model compound). Characterization techniques including BET, X-ray CT, SEM-EDS, FTIR, and XPS are performed to identify the DBF adsorption mechanism on biochar. The results show that the biochar prepared by the microwave gasification has a more well-developed pore structure than that of the electric heating gasification. Higher porosity (16.94%) and lower mineral content (1.75%) are responsible for the effective adsorption of DBF onto AC. The adsorption capacity of CSC is proportional to the modified concentration of KOH. It is mainly ascribed to the decrement of carboxyl and lactone groups and the enhancement of alkaline functional groups on the biochar surface, which augments the hydrophobicity and π–π electron donor–acceptor (EDA) interaction. Instead, DBF adsorption capacity on the biochar is adversely affected by HNO3 modification. For all biochar samples, the corresponding maximum adsorption ratios are AC (87.11%) > KOH-modified CSC (77.14%) > unmodified CSC (49.11%) > unmodified OC (39.70%) > HNO3-modified CSC (36.09%). The adsorption mechanisms of DBF on the gasified biochar encompass pore filling, hydrophobicity, and π–π EDA interaction. A desirable adsorption capacity of DBF on the biochar prepared by the microwave gasification is attainable through augmenting the specific surface area while diminishing the oxygen-containing groups of the surface simultaneously. © 2024, The Authors. All rights reserved.

关键词： Potassium hydroxide

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