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SSRN 2024年

作者： Wang, Cui Jin, Hui School of Water and Environment Chang'an University Xi’an710054 China Key Laboratory of Subsurface Hydrology and Ecological Effect in Arid Region of the Ministry of Education Chang'an University Xi’an710054 China Key Laboratory of Eco-hydrology and Water Security in Arid and Semi-arid Regions of Ministry of Water Resources Chang’an University Xi’an710054 China State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong University Xi’an710049 China Ministry of Education of China Chongqing University Chongqing400044 China

Biomass energy is renewable and rich in the world, providing a solution for the shortage in fossil fuel and serious environmental pollution. Proposing efficient utilization method of biomass waste demands urgent attention. Supercritical water gasification (SCWG) process is a potential technology. In this work, a poly-generation system based on SCWG was developed to convert biomass waste to gas, biochar, heat and electricity. Firstly, mass, energy, and exergy flow were calculated at the typical condition. Subsequently, impact of various operating parameters on the hydrogen-rich syngas yield, generated electricity, thermodynamic performance was investigated. The result demonstrated that the exergy loss primarily occurred on cooler, reactor, heat exchanger and preheater, accounting for more than 90% of total exergy loss, arising from irreversible reaction, heat transfer and heat dissipation. Higher temperature, biomass concentration and preheated water exerted a positive effect for hydrogen-rich gas production and supplied heat energy, while these parameters were disadvantageous to exergy efficiency. Biochar energy was affected by biomass concentration. Energy efficiency increased with preheated water quantity and biomass concentration rising, and impact of biomass concentration was more significant. Conversely, evaluated gasification temperature displayed an adverse effect on energy efficiency. The maximal exergy efficiency reached 58.3% at 550℃, 33%, 900 kg·h-1. © 2024, The Authors. All rights reserved.

关键词： Biomass

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Investigation of Droplet Dynamic Behavior in Pemfcs Gas Diffusion Layer and Gas Channel with Micro-Ct and Lattice Boltzmann Method

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SSRN 2024年

作者： Lv, Xuecheng Zhou, Zhifu Wu, Wei-Tao Wei, Lei Gao, Linsong Lyu, Jizu Hu, Chengzhi Li, Yang Li, Yubai Song, Yongchen Key Laboratory of Ocean Energy Utilization and Energy Conservation of Ministry of Education Dalian University of Technology Dalian116024 China State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong University Xi'An710049 China School of Mechanical Engineering Nanjing University of Science and Technology Nanjing210094 China Department of Mechanical and Energy Engineering Southern University of Science and Technology Shenzhen518055 China School of Mechanical Engineering and Mechanics Xiangtan University Xiangtan411105 China School of Mechanical Engineering Guangdong Ocean University Zhanjiang524088 China

This study reconstructed the 3D structure for the gas diffusion layer (GDL) of proton exchange membrane fuel cells (PEMFCs) using the micro-CT technique and investigated the dynamic behavior of droplets inside the multi-scale space of GDL and gas channel (GC) using the lattice Boltzmann method (LBM). The prediction model for droplet detachment at the GDL-GC interface was developed. The results indicate that there is a significant difference between the breakage location of the liquid bridge and the trajectory of the liquid droplet after detaching from the GDL-GC interface in the multi-scale space of GC and GDL, compared to the single-scale GC space where GDL is ignored. The increase in gas velocity and internal contact angle of the GDL contribute to reducing the droplet detachment volume and increasing the droplet detachment frequency. At the internal contact angle of 120º-140º, GDL exhibited the most efficient removal of liquid water. A contact angle smaller than this range would hinder the detachment of droplets in the GC, while a contact angle larger than this range would lead to the accumulation of liquid water in the GDL. The surface force generated by the connection of liquid bridges in the analytical model for critical droplet detachment forms an angle with the gas flow direction, with the characteristic length determining this force being the minimum diameter at the necking of the liquid bridge. © 2024, The Authors. All rights reserved.

关键词： Contact angle

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TiO2-SnO2:F interfacial electronic structure investigated by soft x-ray absorption spectroscopy

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Physical Review B 2012年第12期85卷 125109-125109页

作者： Coleman X. Kronawitter Mukes Kapilashrami Jonathan R. Bakke Stacey F. Bent Cheng-Hao Chuang Way-Faung Pong Jinghua Guo Lionel Vayssieres Samuel S. Mao Department of Mechanical Engineering University of California at Berkeley Berkeley California 94720 USA Environmental Energy Technologies Division Lawrence Berkeley National Laboratory Berkeley California 94720 USA Advanced Light Source Lawrence Berkeley National Laboratory Berkeley California 94720 USA Department of Chemical Engineering Stanford University Stanford California 94305 USA Department of Physics Tamkang University Tamsui Taiwan Republic of China International Research Center for Renewable Energy State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong University Shaanxi 710049 People's Republic of China

The electronic structure of the titanium dioxide (TiO2)-fluorine-doped tin dioxide (SnO2:F) interface is investigated by soft x-ray absorption spectroscopy using synchrotron radiation. The measurements probe the site- and symmetry-selected unoccupied density of states and reflect the interaction between an early transition-metal-oxide (d0) semiconductor and a post-transition-metal-oxide (d10) degenerate semiconductor. The distinct interfacial electronic structure of TiO2-SnO2:F is established by contrasting spectra with those for anatase and rutile TiO2, SnO2:F, and ZnO-SnO2:F and CdO-SnO2:F interfaces. Oxygen 1s absorption spectra, which relate to the O 2p partial density of states of the conduction band, indicate that the interface is associated with a reduction in Ti d-O p orbital hybridization and an alteration of the TiO2 crystal field. These observations are consistent with measured titanium 2p absorption spectra, which in addition provide evidence for distortion of long-range order around the cation site in the interfacial TiO2. The TiO2-SnO2:F interface is a functional component of a number of optoelectronic devices, perhaps most notably within the anode structure of solar cell architectures. In nonequilibrium conditions, such as those found in operating solar cells, interfacial electronic structure directly influences performance by modifying, for instance, the quasi-Fermi level electrons and the potential distribution at the transparent electrode.

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Research on a Poly-Generation System for Gas-Biochar-Heat-Electricity by Supercritical Water Gasification of Biomass Waste

SSRN

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SSRN 2024年

Biomass energy is renewable and rich in the world, providing a solution for the shortage in fossil fuel and serious environmental pollution. Proposing efficient utilization method of biomass waste demands urgent attention. Supercritical water gasification (SCWG) process is a potential technology. In this work, a poly-generation system based on SCWG was developed to convert biomass waste to gas, biochar, heat and electricity. Firstly, mass, energy, and exergy flow were calculated at the typical condition. Subsequently, impact of various operating parameters, including gasification temperature, mass flowrate of preheated water, biomass concentration, on the hydrogen-rich syngas yield, generated electricity, thermodynamic performance of the system was investigated. The result demonstrated that the exergy loss primarily occurred on cooler, reactor, heat exchanger and preheater, accounting for more than 90% of total exergy loss under different conditions, arising from irreversible reaction, heat transfer and heat dissipation. Higher temperature, higher biomass concentration and more preheated water exerted a positive effect for hydrogen-rich gas production and supplied heat energy, while these parameters were disadvantageous to exergy efficiency. Biochar energy was primarily affected by biomass concentration. Energy efficiency increased with preheated water quantity and biomass concentration rising, and impact of biomass concentration was more significant. Conversely, evaluated gasification temperature displayed an adverse effect on energy efficiency. The maximal exergy efficiency reached about 58.3% at 550°C, biomass concentration of 33%, preheated water mass flowrate of 900 kg·h-1 © 2024, The Authors. All rights reserved.

关键词： Biomass

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Flocculation of suspended cohesive particles in homogeneous isotropic turbulence

arXiv

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arXiv 2021年

作者： Zhao, K. Pomes, F. Vowinckel, Bernhard Hsu, T.-J. Bai, B. Meiburg, E. Department of Mechanical Engineering UC Santa Barbara Santa BarbaraCA93106 United States State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong University Xi'an710049 China Leichtweiß-Institute for Hydraulic Engineering and Water Resources Technische Universität Braunschweig Braunschweig38106 Germany Center for Applied Coastal Research Department of Civil & Environmental Engineering University of Delaware NewarkDE19716 United States

We investigate the dynamics of cohesive particles in homogeneous isotropic turbulence, based on one-way coupled simulations that include Stokes drag, lubrication, cohesive and direct contact forces. We observe a transient flocculation phase characterized by a growing average floc size, followed by a statistically steady equilibrium phase. We analyze the temporal evolution of floc size and shape due to aggregation, breakage, and deformation. Larger turbulent shear and weaker cohesive forces yield elongated flocs that are smaller in size. Flocculation proceeds most rapidly when the fluid and particle time scales are balanced and a suitably defined Stokes number is O(1). During the transient stage, cohesive forces of intermediate strength produce flocs of the largest size, as they are strong enough to cause aggregation, but not so strong as to pull the floc into a compact shape. Small Stokes numbers and weak turbulence delay the onset of the equilibrium stage. During equilibrium, stronger cohesive forces yield flocs of larger size. The equilibrium floc size distribution exhibits a preferred size that depends on the cohesive number. We observe that flocs are generally elongated by turbulent stresses before breakage. Flocs of size close to the Kolmogorov length scale preferentially align themselves with the intermediate strain direction and the vorticity vector. Flocs of smaller size tend to align themselves with the extensional strain direction. More generally, flocs are aligned with the strongest Lagrangian stretching direction. The Kolmogorov scale is seen to limit floc growth. We propose a new flocculation model with a variable fractal dimension that predicts the temporal evolution of the floc size and shape. © 2021, CC BY.

关键词： Flocculation

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Realization of Multilocal Gradient-Doping Pcn by Alkali Metal Ion Sustained Release Capsules for Enhanced Photocatalytic Water Splitting

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SSRN 2023年

作者： Yan, Jiawei Fang, Fenjian Wei, Zhidong Chi, Jiasheng Chen, Mingxia Jiang, Zhi Jiang, Kun Shen, Shaohua Shangguan, Wenfeng Research Center for Combustion and Environment Technology Shanghai Jiao Tong University Shanghai200240 China College of Smart Energy Shanghai Jiao Tong University Shanghai200240 China College of Electrical Energy and Power Engineering Institute of Fuel Cells Shanghai Jiao Tong University Shanghai200240 China International Research Center for Renewable Energy State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong University Xi’an710049 China

The gradient-doping technique has been widely applied to induce an oriented built-in electric-field. However, it is still not efficient enough for charge mobility especially for particulate semiconductors, as the field is primarily in one direction from inner to surface. Here, we propose a multilocal gradient-doping technique that a nano-capsule is designed to store dopants and then release them into semiconductors nonuniformly. As an illustration, scattered pyrochlore-type K2Ta2O6 nanoparticles have been validated the capability of storing and releasing K+, which subsequently diffuse into the substrate PCN. Multi point-radiative gradient in K+ concentration, confined within the K2Ta2O6’s vicinity, will construct several 3D potential wells which can not only accelerate the carrier separation but also offer more migration channels for both photo-induced electrons and holes to the surface. Consequently, the multilocal K+ gradient-doping PCN shows the longest carriers’ lifetime and highest AQY (~21.8% at 400 nm) compared with the other uniformly doping techniques. © 2023, The Authors. All rights reserved.

关键词： Charge transfer

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Corrigendum to “Multi-scale coupling analysis of the flow blockage accident in the typical LFR” [Int. J. Therm. Sci., 195, January 2024, 108615]

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International Journal of Thermal Sciences 2024年 204卷

作者： Hanrui Qiu Mingjun Wang Jing Zhang Wenxi Tian G.H. Su State Key Laboratory of Multiphase Flow in Power Engineering School of Nuclear Science and Technology Xi'an Jiaotong University Xi'an 710049 China

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Research on droplets growth of Marangoni condensation during the time-series process

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Journal of Physics: Conference Series 2017年第1期925卷

作者： Y Li J Wang K Xia N Chen J Yan State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong University Xi'lan 710049 P.R. China

In this paper, the condensate droplets growth of Marangoni condensation during the time-series process was experimentally studied. The photographs taken in the experiments were handled by image processing method. The droplets coverage ratio was introduced to analyse the growth process. As the time-series process went on, the condensate droplets coverage ratio increased fast at first, and then increased slowly until reaching a stable state. The droplets coverage ratio increased with the increase in the vapor-to-surface temperature difference and decreased with the increase in the ethanol vapor concentration.

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Fluoride-Salt-Cooled High-Temperature Reactor: An Integrated Nuclear-Based Energy Production and Conversion System

SSRN

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SSRN 2023年

作者： Zhang, Dalin Li, Xinyu Jiang, Dianqiang Zhou, Xingguang Lv, Xindi Yun, Shichang Wu, Wenqiang He, Xuanang Li, Haoyang Min, Xin Chen, Kailong Tian, Wenxi Qiu, Suizheng Su, Guanghui Zhao, Quanbin Fu, Yao Tang, Chuntao Zhuo, Wenbin Li, Jinggang Zuo, Jiaxu State Key Laboratory of Multiphase Flow in Power Engineering Shaanxi Key Laboratory of Advanced Nuclear Energy and Technology School of Nuclear Science and Technology Xi’an Jiaotong University Xi’an710049 China Shanghai Institute of Applied Physics Chinese Academy of Sciences Shanghai201800 China Shanghai Nuclear Engineering Research & Design Institute Co. Ltd. Shanghai200233 China CNNC Key Laboratory on Nuclear Reactor Thermal Hydraulics Technology Nuclear Power Institute of China Chengdu610213 China China Nuclear Power Technology Research Institute Guangdong Shenzhen518000 China Nuclear and Radiation Safety Center Ministry of Ecology and Environment Beijing100082 China

Based on the analysis of energy structure and the development trends of advanced nuclear energy technology, combining the complementary advantages of nuclear energy and other energy sources in China, the Fluoride-salt-cooled High-temperature Reactor(FuSTAR) system has been proposed. FuSTAR system is designed to address production capacity issues in areas with energy shortages or resource concentration and can be combined with high-temperature process heat to achieve high-value-added processes such as hydrogen production. In this paper, the design and optimization processes of FuSTAR are described from three aspects: the neutronic and thermal-hydraulic system, the thermal transport system, and the power cycle system. Tri-structural isotropic fuel combined with helical cruciform elements has been studied in detail on the neutron physics and thermal-hydraulic properties, and the flow and heat transfer experiment is carried out for the first time. The multilayer nonlinear programming method has been applied to the design of thermal transport systems and the passive residual heat removal system and proved to be fast and efficient. Then the optimal parameters and configuration of the thermoelectric conversion system are obtained directly by using the superstructure optimization method, which saves computing resources greatly. Based on the above design and parameters, the inherent safety of FuSTAR is demonstrated through deterministic safety analysis. In addition, the iodine-sulfur cycle technology is also designed and analyzed, and the characteristics of tritium production in FuSTAR are calculated. The research provides important guidance for the detailed design and operation of FuSTAR. Moreover, this study highlights the significant potential of integrating nuclear energy with other energy sources in an optimized energy-production system. Based on the current research findings, prospects for future research directions are also suggested. © 2023, The Authors. All rights r

关键词： High temperature reactors

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Comparison of Chemical Composition and Acidity of Size-Resolved Inorganic Aerosols at the Top and Foot of Mt. Hua, Northwest China: The Role of the Gas-Particle Distribution of Ammonia

SSRN

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SSRN 2023年

作者： Li, Jianjun Feng, Qiao Liu, Haijiao Dai, Wenting Cao, Yue Shen, Minxia Liu, Yali Qi, Weining Chen, Yukun Guo, Xiao Zhang, Yifan Li, Lu Zhou, Bianhong State Key Laboratory of Loess and Quaternary Geology Key Lab of Aerosol Chemistry and Physics Institute of Earth Environment Chinese Academy of Sciences Xi’an710061 China College of Geography and Environment Baoji University of Arts and Sciences Shaanxi Key Laboratory of Disaster Monitoring and Mechanism Simulation Baoji721013 China Xi’an Institute for Innovative Earth Environment Research Xi’an710061 China National Observation and Research Station of Regional Ecological Environment Change and Comprehensive Management in the Guanzhong Plain Shaanxi China State Key Laboratory of Multiphase Flow in Power Engineering Xi’an Jiaotong University Xi’an710049 China

Aerosol pH is not only a diagnostic indicator of secondary aerosol formation, but also a key factor in the specific chemical reaction routes that produce sulfates and nitrates. To understand the characteristics of aerosol acidity in the Mt. Hua, the chemical fractions of water-soluble inorganic ions in the atmospheric PM2.5 and size-resolved particle at the top and foot of Mt. Hua in summer 2020 were studied. The results showed the mass concentrations of PM2.5 and water-soluble ions at the foot were 2.0-2.6 times higher than those at the top. The secondary inorganic ions, i.e. SO42-, NO3-, and NH4+ (SNA) were 56%-61% higher by day than by night. SO42- was mainly distributed in the fine particles (Dp 2.1 µm) was mainly attributed to the gaseous HNO3 volatilized from fine particles reacting with cations in coarse particles to form non-volatile salts (such as Ca(NO3)2). The pH values of PM2.5 were 2.7 ± 1.3 and 3.3 ± 0.42 at the top and foot, respectively. NH4+/NH3(g) plays a decisive role in stabilising aerosol acidity. In addition, the increase of the liquid water content (LWC) at the foot facilitates the gas-particle conversion of NH3, while the H+ concentration was diluted, resulting in a decrease in acidity at the foot. NH4+/NH3 had good linear correlations with SO42−, NO3－, and LWC during the daytime at both sites, indicating that SO42−, NO3－, and LWC together affect the gas-particle distribution of ammonia by day: however, the effect of LWC at night was not evident. © 2023, The Authors. All rights reserved.

关键词： Ammonia

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