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SSRN 2025年

作者： Liu, Yunlian Liu, Mingkai Shen, Yuanhui Li, Yang Gai, Zhongrui Zhang, Ruqi Pan, Ying Jin, Hongguang Institute of Engineering Thermophysics Chinese Academy of Sciences Beijing100190 China University of Chinese Academy of Sciences Beijing100049 China State Key Laboratory of Multiphase Flow in Power Engineering Xi’an Jiaotong University Xi’an710049 China

The integrated CO2 capture and conversion (ICCC) has emerged as a promising and cost-effective pathway for achieving carbon neutrality. However, limited energy-efficient pathways and durable materials for ICCC systems remains challenging. This study proposes a novel approach that synergistically integrates CO2 capture and conversion through a unified chemical framework. The method employs Li-based sorbents for CO2 capture, coupled with CH4-driven sorbent regeneration that is seamlessly integrated with chemical looping dry reforming of methane (CLDRM), enabling in-situ CO2 conversion. By coupling sorbent regeneration with CLDRM, this system enhances decarbonation kinetics through Le Chatelier's principle via continuous CO2 conversion. One-step calcination synthesized Li-based sorbents particles exhibit stable CO2 capture capacity of 5.25 mmol·g-1 within 15 min per cycle, maintaining 7.5-15% operational efficiency over 40 cycles at 600 ℃. In CLDRM, hydrogen radicals from CH4 dissociation promote the conversion of CO2 to intermediates, lowering the apparent activation energy of sorbents regeneration by 29.2%. Through systematic optimization in a fixed-bed reactor, we achieved 90% CO2 uptake and 85% CH4 conversion, with syngas production rates reaching 13.71 mL·min-1·g-1. Notably, the H2/CO molar ratio in syngas stabilizes ~1.6, aligns with iron-based Fischer-Tropsch and methanol synthesis to produce valuable fuels. This integrated system maintains >80% syngas purity with © 2025, The Authors. All rights reserved.

关键词： Activation energy

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Experimental study on heat transfer deterioration and critical heat flux of DNB type in helically coiled tubes

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International Journal of Thermal Sciences 2025年 215卷

作者： Chang, Fucheng Lou, Jiacheng Wu, Xiaoyi Li, Shuai Yang, Jiaqi Li, Xi Li, Huixiong National Key Lab of Aerospace Power System and Plasma Technology School of Mechanical Engineering Xi'an Jiaotong University Xi'an710049 China State Key Laboratory of Multiphase Flow in Power Engineering School of Energy and Power Engineering Xi'an Jiaotong University Xi'an710049 China

Helically coiled tubes (HCTs) are extensively utilized in numerous engineering fields due to their exceptional heat transfer and structural capabilities. The thermal safety within HCTs is crucial for the long-term stable operation of heat transfer systems. The heat transfer deterioration and critical heat flux (CHF) of departure from nucleate boiling (DNB) type in the HCTs at subcritical pressure were experimentally studied in this paper. The special circumferential wall temperature distribution was obtained and the effects of inlet cooling, pressure, mass velocity and HCT orientation on CHF were investigated. As the inlet subcooling increased, the CHF increased almost linearly. As the mass velocity increased, the turbulence degree in the HCT increases significantly, bubbles were less likely to merge and accumulate, and the CHF increased substantially. It was found that the CHF in the vertical HCT was higher than that in the horizontal HCT under the same working conditions because of the combined action of gravity and centrifugal force. The CHFv/CHFh exhibits a reduction with elevated inlet subcooling and pressure, and the influence of mass velocity on CHFv/CHFh is related to the pressure. New orientation-specific CHF correlations for vertical and horizontal HCTs are developed, achieving high prediction accuracy across pressures of 16–20 MPa and mass fluxes of 320–560 kg m−2 s−1. These findings can provide theoretical support for the optimization design and safe operation of the HCT heat transfer systems. © 2025

关键词： Thermal engineering

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A study on free radical behaviors and reactions in supercritical water using quantum chemical simulation

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Journal of Molecular Liquids 2025年 419卷

作者： Ding, Weijing Takahashi, Osamu Wang, Junying Jin, Hui School of Transportation and Vehicle Engineering Shandong University of Technology Shandong Zi'bo255000 China State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong University Shaanxi Xi'an710049 China of Advanced Science and Engineering Hiroshima University Higashi-Hiroshima739-8526 Japan

Supercritical water (SCW) gasification is one of clean and efficient utilization way of biomass, other organic matters or coal for hydrogen production, in which radical reactions studies in SCW are limited but crucial. Density-functional tight-binding (DFTB) molecular simulation is one of efficient and convenient approaches to investigate these microscopic processes. Therefore, free radical reactions in severe SCW environment were investigated via DFTB calculations in this work. The results showed that the order of the free radicals containing bond cleavages reacted in SCW environment was ·OH, ·CH, ·CH2, ·HO2, ·CH3 and ·C6H5 under the same conditions. The reaction processes of different radicals in SCW were obtained. ·H was the most active free radical of reactions. This work is expected to understand the properties of free radicals in SCW better and explore intrinsic reaction mechanisms, which may provide a theoretical support for accomplishing efficient and low-carbon complete SCW gasification for hydrogen production. © 2024 Elsevier B.V.

关键词： Free radical Gasification Hydrogen production Reaction Supercritical Water (SCW)

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Preparation, improvement, and application of metal–organic framework-based sensing materials for gas leakage and emission: A review

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Nano Materials Science 2025年

作者： Liu, Manyi Wang, Liang Ren, Shan Bai, Bofeng Chai, Shouning He, Chi Zheng, Chunli Yin, Xitao Li, Fengguang College of Materials Science and Engineering Chongqing University Chongqing400044 China State Key Laboratory of Multiphase Flow in Power Engineering School of Energy and Power Engineering Xi'an Jiaotong University Xi'an710049 China School of Physics and Optoelectronic Engineering Ludong University Yantai264000 China School of Materials Science and Engineering Hubei University of Automotive Technology Shiyan442002 China

Industrial gas leaks and flue gas emissions pose significant threats to the safety of industrial operations and the atmospheric ecological environment. Traditional gas sensing materials often struggle to meet the challenges posed by complex industrial environments. Recently, metal-organic framework (MOF)-based gas sensing materials have garnered significant attention in industrial gas detection due to their high sensitivity, selectivity, and tunable properties. The exponential increase in related publications highlights the growing research interest in this field. This paper presents a comprehensive review of the advantages of various types of metal-organic frameworks and their derivatives for detecting industrial gas leaks and flue gas emissions, alongside an introduction of representative MOF synthesis methods. Furthermore, the primary sensing mechanisms of MOF-based gas sensing materials and strategies for enhancing the sensing performance are summarized. The current state of MOF-based gas sensing materials in industrial gas detection is also discussed. Finally, the potential limitations, existing challenges, and future directions of MOF-based industrial gas sensing materials are systematically analyzed, with suggestions for addressing these challenges to advance industrial gas detection technologies. © 2025 Chongqing University

关键词： Application Improvement Industrial gas detection MOF-Based sensing materials Preparation

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Numerical Study of Multi-Factor Coupling Effects on Energy Conversion Performance of Nanofluidic Reverse Electrodialysis

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Frontiers in Heat and Mass Transfer 2025年第2期23卷 507-528页

作者： Hao Li Cunlu Zhao Jinhui Zhou Jun Zhang Hui Wang Yanmei Jiao Yugang Zhao School of Physical and Mathematical Sciences Nanjing Tech University Nanjing 211816 China MOE Key Laboratory of Thermo-Fluid Science and Engineering Xi’an Jiaotong University Xi’an 710049 China Key Laboratory of Unsteady Aerodynamics and Flow Control Ministry of Industry and Information Technology Nanjing University of Aeronautics and Astronautics Nanjing 210016 China Shanghai Key Laboratory of Multiphase Flow and Heat Transfer in Power Engineering School of Energy and Power Engineering University of Shanghai for Science and Technology Shanghai 200093 China Key Laboratory of Icing and Anti/De-icing China Aerodynamics Research and Development Center Mianyang 621000 China

Based on the rapid advancements in nanomaterials and nanotechnology, the Nanofluidic Reverse Electrodialysis (NRED) has attracted significant attention as an innovative and promising energy conversion strategy for extracting sustainable and clean energy from the salinity gradient energy. However, the scarcity of research investigating the intricate multi-factor coupling effects on the energy conversion performance, especially the trade-offs between ion selectivity and mass transfer in nanochannels, of NRED poses a great challenge to achieving breakthroughs in energy conversion processes. This numerical study innovatively investigates the multi-factor coupling effect of three critical operational factors, including the nanochannel configuration, the temperature field, and the concentration difference, on the energy conversion processes of NRED. In this work, a dimensionless amplitude parameter s is introduced to emulate the randomly varied wall configuration of nanochannels that inherently occur in practical applications, thereby enhancing the realism and applicability of our analysis. Numerical results reveal that the application of a temperature gradient, which is oriented in opposition to the concentration gradient, enhances the ion transportation and selectivity simultaneously, leading to an enhancement in both output power and energy conversion efficiency. Additionally, the increased fluctuation of the nanochannel wall from s = 0 to s = 0.08 improves ion selectivity yet raises ion transport resistance, resulting in an enhancement in output power and energy conversion efficiency but a slight reduction in current. Furthermore, with increasing the concentration ratio c H / c L from 10 to 1000, either within a fixed temperature field or at a constant dimensionless amplitude, the maximum power consistently attains its optimal value at a concentration ratio of 100 but the cation transfer number experiences a monotonic decrease across this entire range of concentration

关键词： Salinity gradient energy nanofluidic reverse electrodialysis energy conversion nanochannel configuration multi-factor coupling effect

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Large eddy simulation on the wake characteristics of linearly stratified flow past a sphere

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Scientific Reports 2025年第1期15卷 1-13页

作者： Xia, Tianci Wei, Na Shi, Liuliu School of Energy and Power Engineering University of Shanghai for Science and Technology Shanghai 200093 China Shanghai Key Laboratory of Multiphase Flow and Heat Transfer in Power Engineering Shanghai 200093 China Key Laboratory of Power Machinery and Engineering of Ministry of Education Shanghai Jiao Tong University Shanghai 200240 China

In this study, Large Eddy Simulation (LES) has been employed to examine the influence of the Froude number (Fr) on the linearly stratified wake and internal waves behind a sphere at a subcritical Reynolds number of Re = 3700. Six distinct sets of models with varying Fr (Fr = 0.05, 0.25, 0.5, 1, 2, ∞) have been chosen to establish density linear stratification through the use of a User Defined Function (UDF). The analysis focuses on the impact of stratification on wake characteristics, velocity distribution, and the structure of internal waves within stratified flow. It is evident that density stratification plays a pivotal role in shaping wake structure. Notably, in stratified flows, wakes exhibit unique characteristics including the generation of internal waves, suppression of vertical velocity, and the emergence of oscillating wake patterns. The study reveals that a decrease in the Froude number leads to heightened vertical suppression of the wake and increased anisotropy of the velocity distribution. Furthermore, as the Froude number ascends from 0.05 to 2, the wake undergoes a transition from quasi-two-dimensional vortex shedding to three-dimensional turbulence. © The Author(s) 2025.

关键词： Froude number Internal wave Linearly stratified flow Wake

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Effect of surface roughness on corrosion behaviour of stainless steel in supercritical CO 2

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Journal of Materials Research and Technology 2025年 36卷 4946-4954页

作者： Liyong Cao Wenyan Zhang Chongjun Jiang Hui Wang Hong An Chao Ye Jiyun Ren Xiaole Huang Lei Deng China University of Xihua Chengdu 610039 China State Key Laboratory of Multiphase Flow in Power Engineering School of Energy and Power Engineering Xi'an Jiaotong University Xi'an 710049 China China University of Petroleum-Beijing Beijing 102249 China PipeChina Gansu Branch Lanzhou 730070 China Zhengzhou Yutong Group Co. Ltd. Zhengzhou 450000 China

To study the effect of surface roughness on the corrosion behavior of austenitic steels in supercritical CO 2 , the corrosion experiments were conducted on 304 and 310S stainless steels at 550 °C and 15 MPa. The corroded samples were characterized using XRD and SEM-EDS. The results demonstrate that surface roughness significantly affects the morphology and structure of the oxide films formed on 310S stainless steel. Samples prepared with varying surface roughness (grounded using from 200# to 1000# metallographic abrasive papers) showed that rougher surfaces tend to develop denser oxide layers, whereas smoother surfaces exhibit relatively loose and porous oxide films. Despite these differences in oxide structure, the overall corrosion weight gain remained largely unaffected, indicating minimal oxide shedding from 310S steel. The oxidation product is mainly Cr 2 O 3 . For 304 stainless steel, surface roughness was found to influence the composition of surface oxides. Both 200# and 1000# samples formed loose, porous oxide films prone to spallation, with the primary constituents being Fe 3 O 4 , (Fe, Cr) 3 O 4 and Fe 2 O 3 . Because the content of (Fe, Cr) 3 O 4 and Fe 3 O 4 of the former is higher, more voids appear in the oxide film, leading to spallation within the first 100 h of exposure. The rougher surface showed a more pronounced loss of oxide. But for the 600# sample, the main component is Fe 2 O 3 . Carburization was observed to intensify with increasing surface roughness in both materials. Notably, the 200# sample of 310S stainless steel exhibited more severe carburization compared to the 1000# sample of 304 stainless steel.

关键词： Supercritical CO 2 Corrosion Austenitic stainless steels Surface roughness Oxidation

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Prediction of acoustic agglomeration enhanced by solid seed particles using the DSMC method

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Advanced Powder Technology 2025年第6期36卷

作者： Su, Junxu Wu, Zhihao Fan, Fengxian Hu, Xiaohong Su, Mingxu School of Energy and Power Engineering University of Shanghai for Science and Technology Shanghai200093 China Shanghai Key Laboratory of Multiphase Flow and Heat Transfer in Power Engineering University of Shanghai for Science and Technology Shanghai200093 China

Acoustic agglomeration enhanced by large-sized solid seed particles is investigated using the direct simulation Monte Carlo (DSMC) method. The process of acoustic agglomeration is revealed in terms of temporal evolution of velocities, diameters, and number weights of simulated particles, as well as normalized concentration and average diameter of small particles. Furthermore, the enhancement of acoustic agglomeration by the solid seed particles is evaluated at varying parameters. The results show that the agglomeration performance is enhanced within a shorter residence time when the solid seed particles are present. Increasing acoustic intensity or solid seed particle concentration leads to more efficient acoustic agglomeration, while the acoustic frequency, particularly beyond 2 kHz, has little effect on agglomeration performance. Moreover, a noticeable increase in agglomeration efficiency is observed when the seed particle diameter increases from 20 to 40 µm. However, once it exceeds 40 µm, the increase in agglomeration efficiency diminishes. © 2025 The Society of Powder Technology Japan.

关键词： Agglomeration

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Development of a two-phase flow solver with two-fluid model based on OpenFOAM: Validation against two-phase boiling flow

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Annals of Nuclear Energy 2025年 220卷

作者： Wu, Wenqiang Huang, Tao Du, Peng Feng, Zhenyu Zhang, Dalin Zhou, Lei Song, Gongle Deng, Jian Qiu, Zhifang Tian, Wenxi Qiu, Suizheng Su, Guanghui State Key Laboratory of Multiphase Flow in Power Engineering Shaanxi Key Laboratory of Advanced Nuclear Energy and Technology School of Nuclear Science and Technology Xi'an Jiaotong University Shaanxi Xi'an710049 China Nuclear Power Institute of China 328 Changshun Avenue Chengdu610213 China

The continuous advancement in computer technology and mathematical-physical models has significantly propelled the development of numerical reactor technology. There is a growing focus on high-fidelity, multi-scale, and multi-physics coupling within a unified framework. OpenFOAM, based on the finite volume method, has emerged as a promising tool for addressing this challenge. This study explores its capabilities in system-level scales, successfully developing a two-fluid, six-equation solver. The realistic closure models cover flow and heat transfer scenarios within vertical channels under pre-CHF conditions. A virtual thermal structure accounts for conjugate heat transfer between the fluid and the solid. Furthermore, the solver adheres to the discretization and solution principles within the OpenFOAM framework. The developed solver has been extensively validated against experimental data for two-phase boiling flow, with results showing good agreement, thereby demonstrating the solver's success. This work builds upon previous efforts involving the drift-flux solver and indicates that OpenFOAM can effectively handle one-dimensional or system-level scale calculations. It provides robust support for future endeavors in multi-scale and multi-physics coupling technologies. © 2025 Elsevier Ltd

关键词： Finite volume method

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Research on flow characteristics of dual-outlet centrifugal disk blood pumps

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Shengwu Yixue Gongchengxue Zazhi/Journal of Biomedical engineering 2025年第2期42卷 374-381页

作者： Lian, Qilong Xiao, Yuan Xiao, Yiping Cao, Zhanshuo Cui, Guomin Shanghai Key Laboratory of Multiphase Flow and Heat Transfer in Power Engineering School of Energy and Power Engineering University of Shanghai for Science and Technology Shanghai200093 China

Tesla blood pumps demonstrate a reduced propensity for hemolysis and thrombosis compared with vane blood pumps. Considering the restricted driving force within the secondary flow channel of vane blood pumps, along with the low hydraulic efficiency of conventional Tesla blood pumps and their internal flow characteristics that significantly contribute to hemolysis and thrombosis, this study introduces a set of vanes atop the rotor of the Tesla blood pump. This forms a dual-fluid domain rotor, and an axial dual-outlet volute shell structure is adopted to realize the separation of the fluid domains. Through numerical simulations of the new structure, a comparative analysis was conducted in this study on the internal flow characteristics of double-outlet and single-outlet volute shells, and symmetric and asymmetric cross-sections of the same rotor. The results indicate that the flow field distribution is more uniform under the double-outlet volute shell structure, and overall energy dissipation is decreased. After implementing the double-outlet design, in the asymmetric cross-section, compared with the symmetric cross-section, the fluid velocity gradient and turbulent kinetic energy at the tongue of the septum are reduced, and the fluid velocity gradient at the convergence of the diffuser tube outlets are also decreased. The maximum scalar stress is lower, and the decline in head and efficiency is mitigated. Moreover, compared with the single-outlet volute shell, the hemolysis index in the asymmetric cross-section is reduced. In summary, this paper proposes a novel dual-outlet centrifugal disk blood pumps, which can provide a reference for the structural design and performance optimization of magnetically levitated centrifugal blood pumps. © 2025 West China Hospital, Sichuan Institute of Biomedical engineering. All rights reserved.

关键词： Shells (structures)

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