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Characterizing the catalyst fluidization with field synergy to improve the amine absorption for CO2 capture

Chinese Journal of Chemical engineering 2019年第7期27卷 1608-1617页

作者： Yunsong Yu Chen Zhang Zaoxiao Zhang Geoff Wang School of Chemical Engineering and Technology Xi’an Jiaotong UniversityXi’an 710049China State Key Laboratory of Multiphase Flow in Power Engineering Xi’an Jiaotong UniversityXi’an 710049China School of Chemical Engineering The University of QueenslandSt LuciaQLD 4072Australia

There are great interests to capture the CO2 to control the greenhouse gas *** absorption of CO2 is being taken as an effective way to capture CO2 in ***,the amine absorption of CO2 is cost-ineffective due to great energy consumption and solution *** order to reduce the capture cost,catalyst fluidization is proposed here to intensify the mass transfer and heat *** fluidization with field synergy and DFT model is developed by incorporating the effects of catalyst reaction kinetics,drag force and multi-field into the mass transfer,heat transfer,fluid flow and catalyst *** with an improved distributor are performed well to validate the *** reaction kinetics is determined by the DFT simulation and *** mass transfer coefficient in the fluidized reactor is identified as 17%higher than the conventional packed *** the field synergy of catalyst fluidization,the energy consumption for CO2 desorption is reduced by 9%.Stepwise operation and inclination reactor are used to improve catalyst fluidization process.

关键词： CO2 capture Catalyst fluidization Mass transfer DFT Energy consumption Field synergy

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A Hydrodynamic Modei for Slug Frequency in Horizontal Gas-Liquid Two-Phase flow

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Chinese Journal of Chemical engineering 2003年第5期11卷 508-514页

作者：刘磊孙贺东胡志华周芳德 State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong University Xi'an 710049 China

The prediction of slug frequency has important significance on gas-liquid two-phase flow. A hydrody-namic modei was put forward to evaluate slug frequency for horizontal two-phase flow, based on the dependence of slug frequency on the frequency of unstable interfacial wave. Using air and water, experimental verification of the modei was carried out in a large range of flow parameters. Six electrical probes were installed at different positions of a horizontal plexiglass pipe to detect slug frequency development. The pipe is 30m long and its inner diameter is 24 mm. It is observed experimentally that the interfacial wave frequency at the inlet is about l to 3 times the frequency of stable slug. The slug frequencies predicted by the modei fit well with Tronconi (1990) modei and the experimental data. The combination of the hydrodynamic modei and the experimental data results in a conclusion that the frequency of equilibrium liquid slug is approximately half the miniraum frequency of interfacial wave.

关键词： gas-liquid flow two-phase flow interfacial wave hydrodynamic model slug frequency

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MIXED DISCONTINUOUS GALERKIN METHOD FOR QUASI-NEWTONIAN STOKES flowS

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Journal of Computational Mathematics 2024年第3期42卷 885-910页

作者： Yanxia Qian Fei Wang Wenjing Yan School of Mathematics and Statistics Xi'an Jiaotong UniversityXi'an 710049China School of Mathematics and Statistics&State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong UniversityXi'an 710049China

In this paper,we introduce and analyze an augmented mixed discontinuous Galerkin(MDG)method for a class of quasi-Newtonian Stokes *** the mixed formulation,the unknowns are strain rate,stress and velocity,which are approximated by a discontinuous piecewise polynomial triplet ■for k≥***,the discontinuous piecewise polynomial function spaces for the field of strain rate and the stress field are designed to be *** addition,the pressure is easily recovered through simple *** the benefit of the analysis,we enrich the MDG scheme with the constitutive equation relating the stress and the strain rate,so that the well-posedness of the augmented formulation is obtained by a nonlinear functional *** k≥0,we get the optimal convergence order for the stress in broken ■(div)-norm and velocity in L^(2)-***,the error estimates of the strain rate and the stress in-norm,and the pressure in L^(2)-norm are optimal under certain ***,several numerical examples are given to show the performance of the augmented MDG method and verify the theoretical *** evidence is provided to show that the orders of convergence are sharp.

关键词： Quasi-Newtonian fows Mixed discontinuous Galerkin method Symmetric strain rate Symmetric stress Optimal convergence orders

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Shock tube study on auto-ignition characteristics of kerosene/air mixtures

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Chinese Science Bulletin 2011年第13期56卷 1399-1406页

作者： ZHANG YingJia HUANG ZuoHua WANG JinHua XU ShengLi State Key Laboratory of Multiphase Flow in Power Engineering Xi' an Jiaotong University Xi' an 710049 China Department of Modern Mechanics University of Science and Technology of China Hefei 230026 China

Ignition delay times are obtained for kerosene/air mixtures behind the reflected shock waves at temperatures between 1445 and 1650 K,at a pressure of 0.11 MPa and an equivalence ratio of 1.0.A nebulization device with Laval nozzle is used to nebulize kerosene and form an aerosol phase,which evaporates and diffuses rapidly behind the incident shock *** auto-ignite behind the reflected shock *** ICCD is used to visualize the kerosene/air mixture's ignition *** mixture's ignition intensity increases with increase in initial *** and irregular flames exist below 1515 K while plane and discontinuous flames exist over 1560 *** delay times decrease with increase in initial *** data shows good agreement with results reported previously in the literature.A new surrogate (consisting of 10% toluene,10% ethylbenzene and 80% n-decane) is proposed for *** et al.'s mechanism is used to simulate the ignition of kerosene with calculations agreeing well with the experimental *** sensitivity of reaction H+O2 <=>OH+O,which shows the highest sensitivity to the ignition delay time,increases with an increase in *** chain breaching reaction of CH3 with O2 accelerates the total reaction rate and the H-atom abstraction of n-decane controls the total reaction *** rate of production and instantaneous heat production indicate that two reactions,H+O2 <=>OH+O and O+H2 <=>OH+H,are the key reactions to the formation of OH radicals,as well as the main endothermic ***,the reaction of R3 is the main heat release reaction during *** structure analysis shows that initial pressure is increased slightly as CO and H2O will appear before main ignition.

关键词：空气混合物煤油自燃特性点火延迟时间冲击管反应速率初始温度数据显示

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Numerical study of heat transfer characteristics in the solar receiver tube combined with MCRT method

Numerical study of heat transfer characteristics in the sola...

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2009 US-EU-China Thermophysics Conference - Renewable Energy, UECTC'09

作者： Cheng, Z.D. He, Y.L. Xiao, J. Tao, Y.B. Xu, R.J. State Key Laboratory of Multiphase Flow in Power Engineering School of Energy and Power Engineering Xi'an Jiaotong University Xi'an Shaan xi China

ISBN: (纸本)9780791802908

The solar energy flux distribution on the outer wall of the inner absorber tube of parabolic solar collector receiver is calculated successfully by a homemade code adopting Monte Carlo Ray-Trace Method (MCRT Method). It is revealed that the non-uniformity of the solar energy flux distribution is very large. Three-dimensional numerical simulation of coupled heat transfer characteristics in the receiver tube is calculated and analyzed by combining the MCRT Method and the FLUENT software, in which the heat transfer fluid and physical model are Syltherm 800 liquid oil and LS2 parabolic solar collector from the testing experiment of Dudley et al., respectively. Temperature- dependent properties of the oil and thermal radiation between the inner absorber tube and the outer glass cover tube are also taken into account. Then three typical testing conditions are chosen from the experiment to validate the reliability of the simulation code. Numerical results show that the predicted results agree well with the experimental data, the average relative error is within 2%. And then the mechanism of the coupled heat transfer in the receiver tube is further studied. Copyright © 2009 by ASME.

关键词： Numerical methods

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TiO_(2) nanorods based self-supported electrode of 1T/2H MoS_(2) nanosheets decorated by Ag nano-particles for efficient hydrogen evolution reaction

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Chinese Chemical Letters 2023年第11期34卷 355-359页

作者： Changzheng Lin Yunpeng Liu Yaxing Sun Zhenyu Wang Hao Xu Mingtao Li Jiangtao Feng Bo Hou Wei Yan Department of Environmental Science&Engineering Xi’an Jiaotong UniversityXi’an 710049China School of Physics and Astronomy Cardiff UniversityThe ParadeCardiffCF243AAWalesUnited Kingdom State Key Laboratory of Multiphase Flow in Power Engineering Xi’an Jiaotong UniversityXi’an 710049China International Research Center for Renewable Energy(IRCRE) State Key Laboratory of Multiphase Flow in Power Engineering(MFPE)Xi’an Jiaotong UniversityXi’an 710049China

Molybdenum disulfide(MoS_(2))has shown significant promise as an economic hydrogen evolution reaction(HER)catalyst for hydrogen generation,but its catalytic performance is still lower than noble metalbased ***,a silver nanoparticles(Ag NPs)-decorated 1T/2H phase layered MoS_(2) electrocatalyst grown on titanium dioxide nanorod arrays(Ag NPs/1T(2H)MoS_(2)/TNRs)was prepared through acid-tunable ammonium ion *** advantage of MoS_(2) layered structure and crystal phase controllability,as-prepared Ag NPs/1T(2H)MoS_(2)/TNRs exhibited ultrahigh HER ***-proposed strategy combines facile hydrogen desorption(Ag NPs)with efficient hydrogen adsorption(1T/2H MoS_(2))effectively circumventes the kinetic limitation of hydrogen desorption by 1T/2H MoS_(2).The as-prepared Ag NPs/1T(2H)MoS_(2)/TNRs electrocatalyst exhibited excellent HER activity in 0.5 mol/L H2SO4 with low overpotential(118 mV *** hydrogen electrode(RHE))and small Tafel slope(38.61 mV/dec).The overpotential exhibts no obvious attenuation after 10 h of constant current ***-principles calculation demonstrates that as-prepared 1T/2H MoS_(2) exhibit a large capacity to store *** protons can be subsequently transferred to Ag NPs,which significantly increases the hydrogen coverage on the surface of Ag NPs in HER process and thus change the rate-determining step of HER on Ag NPs from water dissociation to hydrogen *** study provides a unique strategy to improve the catalytic activity and stability for MoS_(2)-based electrocatalyst.

关键词： Molybdenum disulfide Silver nanoparticles Hydrogen evolution reaction Density functional theory Hydrogen spillover

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Numerical study on the coupled heat transfer performance of the parabolic solar absorber tube

Numerical study on the coupled heat transfer performance of ...

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2009 US-EU-China Thermophysics Conference - Renewable Energy, UECTC'09

作者： Tao, Y.B. He, Y.L. State Key Laboratory of Multiphase Flow in Power Engineering School of Energy and Power Engineering Xi'an Jiaotong University Xi'an Shaanxi 710049 China

ISBN: (纸本)9780791802908

In present paper, a two-dimensional numerical model for the coupled heat transfer process in the solar collector tube was developed and the unified dimensionless governing equations were derived. The full field computation method was adopted to deal with the fluid-solid conjugated heat transfer problem. The effects of Ra numbers and tube diameter ratio on the heat transfer and fluid flow performance were numerically analyzed under the constant heat flux conditions. The distributions of flow field, temperature field, local Nu and local temperature gradient were examined. The results show that when Ra is larger than 105, the effects of nature convection must be taken into account. Due to the effect of the nature convection, along the θ direction, the temperature in the cross-section decreases and the temperature gradient on the inner tube surface increases at first. When θ is near to π, the temperature and temperature gradients would present a converse variation. The local Nu on the inner tube surface increases along θ direction until it reaches a maximum then it decreases again. Due to the existing of the nature convection vortexes, the temperature distributions in some cross-sections present fluctuations along the r direction. Copyright © 2009 by ASME.

关键词： Heat flux

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Effect of anolyte pH and cathode Pt loading on electricity and hydrogen co-production performance of the bio-electrochemical system

Effect of anolyte pH and cathode Pt loading on electricity a...

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作者： Liu, Ya-Peng Wang, Yun-Hai Wang, Bai-Shi Chen, Qing-Yun Department of Environmental Engineering State Key Laboratory of Multiphase Flow in Power Engineering Xi'An Jiaotong University Xi'an 710049 China

In a novel bio-electrochemical system (BES) for hydrogen and electricity co-production with acetate substrate, the anolyte pH and cathode Pt loading effects are investigated to improve the cell performance for hydrogen and electricity co-production and reduce the cost. The optimized anolyte pH is 9. The maximum hydrogen production rate of 0.55 m3 m-3 d -1 and COD removal of 76% are obtained under optimal anolyte pH in the present BES. Over high or over low anolyte pH decreases the hydrogen production rate and COD removal. In addition, the experiments show that there is no considerable difference for the power density output and steady state current when the Pt catalyst loading is above 0.1 mg cm-2. But when the Pt catalyst loading is lower than 0.1 mg cm-2, the power density output and current decreases significantly. About 1.7 W m-3 power density output can be obtained by using 0.1 mg cm-2 Pt catalyst in the present research. © 2014, Hydrogen Energy Publications, LLC. Published by Elsevier Ltd. All rights reserved.

关键词： Hydrogen production

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Life Cycle Assessment Analysis and Comparison of 1000 MW S-CO_(2)Coal Fired power Plant and 1000 MW USC Water-Steam Coal-Fired power Plant

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Journal of Thermal Science 2022年第2期31卷 463-484页

作者： LI Mingjia WANG Ge XU Jinliang NI Jingwei SUN Enhui Key Laboratory of Thermo-Fluid Science and Engineering of Ministry of Education School of Energy&Power EngineeringXi’an Jiaotong UniversityXi’an 710049China Beijing Key Laboratory of Multiphase Flow and Heat Transfer for Low Grade Energy Utilization North China Electric Power UniversityBeijing 102206China

The objective of this paper is to understand the benefits that one can achieve for large-scale supercritical CO_(2)(S-CO_(2))coal-fired power *** aspects of energy environment and economy of 1000 MW S-CO_(2)coal-fired power generation system and 1000 MW ultra-supercritical(USC)water-steam Rankine cycle coal-fired power generation system are analyzed and compared at the similar main vapor parameters,by adopting the neural network genetic algorithm and life cycle assessment(LCA)***-objective optimization of the 1000 MW S-CO_(2)coal-fired power generation system is further carried *** power generation efficiency,environmental impact load,and investment recovery period are adopted as the objective *** main vapor parameters of temperature and pressure are set as the decision *** results are concluded as ***,the total energy consumption of the S-CO_(2)coal-fired power generation system is 10.48 MJ/k Wh and the energy payback ratio is 34.37%.The performance is superior to the USC coal-fired power generation ***,the resource depletion index of the S-CO_(2)coal-fired power generation system is 4.38μPRchina,90,which is lower than that of the USC coal-fired power generation system,and the resource consumption is ***,the environmental impact load of the S-CO_(2)coal-fired power generation system is 0.742 m PEchina,90,which is less than that of the USC coal-fired power generation system,0.783 m PEchina,*** all environmental impact types,human toxicity potential HTP and global warming potential GWP account for the most environmental ***,the investment cost of the S-CO_(2)coal-fired power generation system is generally less than that of the USC coal-fired power generation system because the cost of the S-CO_(2)turbine is only half of the cost of the steam *** optimal turbine inlet temperature T_(5)becomes smaller,and the optimal turbine inlet pressure is unchanged at 622.082°C/30 MPa.

关键词： S-CO_(2)power plant ultra-supercritical water-steam Rankine cycle power plant life cycle assessment energy efficiency environment impact economic performance

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Experimental study of nitrogen oxide emissions in a circulating fluidized bed

Experimental study of nitrogen oxide emissions in a circulat...

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20th International Conference on Fluidized Bed Combustion

作者： Liu, R.W. Zhou, Q.L. Hui, S.E. Xu, T.M. State Key Laboratory of Power Engineering Multiphase Flow Department of Energy and Power Engineering Xi'an Jiaotong University Xi'an Shaanxi 710049 China

The experimental study was carried out on the emission characteristics of nitrogen oxide in a 0.3MW circulating fluidized bed as well as analysis of the formation and destruction mechanism of nitrogen oxide. Several variables associated with the combustion system were investigated in the experiment, which include bed temperature, excess air, primary-to-secondary air ratio, and coal species. It is found that the NOx emissions decrease along the height of the furnace, while the N2O emissions increase continuously. More NOx emissions and less N2O emissions are generated as the bed temperature increases. It is also illustrated that an increase of air stoichiometry leads to a significant NOx increase and an obvious N2O increase. And air staging is proved to be an effective way to control the nitrogen oxide emissions in the fluid bed. Besides, it is also shown in the experiment that the concentration of NOx and N2O is higher during the combustion of anthracite than that during the combustion of bituminous.

关键词： Nitrogen oxides

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