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20th International Conference on Fluidized Bed Combustion

作者： Liu, R.W. Zhou, Q.L. Hui, S.E. Xu, T.M. State Key Laboratory of Power Engineering Multiphase Flow Department of Energy and Power Engineering Xi'an Jiaotong University Xi'an Shaanxi 710049 China

The experimental study was carried out on the emission characteristics of nitrogen oxide in a 0.3MW circulating fluidized bed as well as analysis of the formation and destruction mechanism of nitrogen oxide. Several variables associated with the combustion system were investigated in the experiment, which include bed temperature, excess air, primary-to-secondary air ratio, and coal species. It is found that the NOx emissions decrease along the height of the furnace, while the N2O emissions increase continuously. More NOx emissions and less N2O emissions are generated as the bed temperature increases. It is also illustrated that an increase of air stoichiometry leads to a significant NOx increase and an obvious N2O increase. And air staging is proved to be an effective way to control the nitrogen oxide emissions in the fluid bed. Besides, it is also shown in the experiment that the concentration of NOx and N2O is higher during the combustion of anthracite than that during the combustion of bituminous.

关键词： Nitrogen oxides

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Vapor-liquid equilibrium of H2/CO2and H2/N2/CO2mixture, the liquefaction technology related to the supercritical water gasification products 8

Vapor-liquid equilibrium of H2/CO2and H2/N2/CO2mixture, the ...

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8th International Conference on Smart and Sustainable Technologies, SpliTech 2023

作者： Wu, Hongtu Jin, Hui Xi'an Jiaotong University State Key Laboratory of Multiphase Flow in Power Engineering School of Energy and Power Engineering Shaanxi Xi'an710049 China

ISBN: (纸本)9789532901283

In this paper, the dew point and liquid phase composition of H2/CO2 and H2/CO2/N2 mixtures at phase equilibrium calculated by PR-BM equation and Van Der Waal mixing rule with commercial MATLAB software are introduced, it is of theoretical significance for the wide application of the products of supercritical water gasification. First, the results obtained by the self-programming code are verified with the experimental data, the experimental data and simulation results of two kinds of CO2/H2 mixtures and two kinds of CO2/N2/H2 mixtures were compared. The average percentage deviation was 2.69%, 4.05%, 2.22%, 1.20%, respectively. Thus the absolute deviations of the mixtures are within the acceptable range, therefore, the model proposed in this paper can well predict the dew point of the mixtures composed of H2/CO2 or H2/CO2/***, the dew point and the CO2 content in the liquid phase of common H2/CO2 and H2/CO2/N2 vapor mixtures in supercritical water gasification products were predicted, and a series of analysis and discussion were conducted on the predicted results finally. © 2023 University of Split, FESB.

关键词： Carbon dioxide

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Reconstruction of particle distribution for tomographic particle image velocimetry based on unsupervised learning method

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Particuology 2024年第10期93卷 349-363页

作者： Duanyu Zhang Haoqin Huang Wu Zhou Mingjun Feng Dapeng Zhang Limin Gao School of Energy and Power Engineering University of Shanghai for Science and TechnologyShanghai200093China Shanghai Key Laboratory of Multiphase Flow and Heat Transfer for Power Engineering University of Shanghai for Science and TechnologyShanghai200093China National Key Laboratory of Aerodynamic Design and Research Northwestern Polytechnical UniversityXi'an710072China

The development of deep learning has inspired some new methods to solve the 3D reconstruction problem for Tomographic Particle Image Velocimetry (Tomo-PIV). However, the supervised learning method requires a large number of data with ground truth as training information, which is very difficult to gather from experiments. Although synthetic datasets can be used as alternatives, they are still not exactly the same with the real-world experimental data. In this paper, an Unsupervised Reconstruction Technique based on U-net (UnRTU) is proposed to reconstruct volume particle distribution explicitly. Instead of using ground truth data, a projection function is used as an unsupervised loss function for network training to reconstruct particle distribution. The UnRTU was compared with some traditional algebraic reconstruction algorithms and supervised learning method using synthetic data under different particle density and noise level. The results indicate that UnRTU outperforms these traditional approaches in both reconstruction quality and noise robustness, and is comparable to the supervised learning methods AI-PR. For experimental tests, particles dispersed in cured epoxy resin are moved by an electric rail with a certain speed to obtain the ground truth data of particle velocity. Compared with other algorithms, the reconstructed particle distribution by UnRTU has the best reconstruction fidelity. And the accuracy of the 3D velocity field estimated by UnRTU is 12.9% higher than that from the traditional MLOS-MART algorithm. It demonstrates significant potential and advantages for UnRTU in 3D reconstruction of particle distribution. Finally, UnRTU was successfully applied to the high-speed planar cascade airflow field, demonstrating its applicability for measuring complex fluid flow fields at higher particle density.

关键词： Tomographic particle image velocimetry 3D reconstruction Unsupervised learning Convolutional neural network

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Atomically Dispersed Co Sites on BiOCl Nanosheets for Efficient CO 2 Photoreduction

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Green Energy & Environment 2025年

作者： Ting Peng Yiduo Wang Ke Wang Kaini Zhang Yiqing Wang Yufei Xu Qingqing Guan Guofu Wang Wenjie Zhang Binglan Wu Shaohua Shen International Research Center for Renewable Energy State Key Laboratory of Multiphase Flow in Power Engineering Xi’an Jiaotong University Xi’an 710049 China College of Chemical and Biological Engineering Zhejiang University Hangzhou 310058 China Institute of Zhejiang University-Quzhou Quzhou 324000 China

Efficient CO 2 photoreduction to produce fuel remains a great challenge, due to the fast recombination of photogenerated charge carriers and the lack of effective reactive sites in the developed photocatalysts. Herein, single Co atoms (Co SA ) were highly dispersed on hydrothermally synthesized BiOCl nanosheets (BOC) by a facile two-step electrostatic self-assembly and pyrolysis method. The obtained Co SA -BOC could be performed for efficient CO 2 photoreduction to stoichiometrically produce CO and O 2 at the ratio of 2:1, with the CO evolution rate reaching 45.93 μmol g –1 h –1 , ∼4 times that of the pristine BOC. This distinctly improved photocatalytic performance for Co SA -BOC should be benefited from the introduction of atomically dispersed Co-O 4 coordination structures, which could accelerate the migration of photogenerated charge carriers to surface by creating an impurity energy level in the forbidden band, and act as the reactive sites to deliver the photogenerated electrons to activate CO 2 molecules for CO production. This work provides a facile and reliable strategy to highly disperse single atoms on low-dimensional semiconductors for efficient CO 2 photoreduction to selectively produce CO.

关键词： photocatalysis CO 2 reduction BiOCl nanosheets single Co atoms

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Study on the heat and mass transfer characteristics of wet air in metal foam in the space station environment

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Applied Thermal engineering 2025年

作者： Guowei Zhu Liang Zhang Yujuan Xia Hantao Zhou School of Energy and Power Engineering University of Shanghai for Science and Technology Shanghai 200093 China Key Laboratory of Multiphase Flow and Heat Transfer in Shanghai Power Engineering University of Shanghai for Science and Technology Shanghai 200093 China China National Institute of Standardization Beijing 100191 China

This paper has developed a novel dehumidification device for space station environment, which uses foam copper as the core, with a Stirling refrigerator providing cooling, heat pipes assisting in heat conduction and a siphon water guidance system employed to remove condensate. Experiments on dehumidifying wet air within the foam copper were then carried out under simulated microgravity dehumidification conditions. The experimental conditions included different inlet air temperatures, humidities, air velocities, and cold end temperatures of the Stirling refrigerator. The experimental research indicates that as the inlet air temperature rises from 20 °C to 30 °C, the mass transfer coefficient increases by 57.06 %, and the sensible heat coefficient rises by 10.62 %. When the air velocity increases from 0.4 m·s −1 to 1.4 m·s −1 , these two coefficients increase by 111.79 % and 170.83 %, respectively. In contrast, increasing the relative humidity from 50 % to 80 % results in a 34.09 % decrease in the sensible heat coefficient, while the mass transfer coefficient increases by 11.4 %. When the cold-end temperature rises from 8 °C to 13 °C, the sensible heat transfer and mass transfer coefficients increase by 9.63 % and 4.06 %, respectively. Based on this, a sensitivity analysis was conducted using the experimental data, and heat and mass transfer correlations were fitted. The mean standard deviations of the heat and mass transfer correlations are 3.74 % and 6.30 %, respectively, indicating a high degree of fitting accuracy. This work provides a new humidity control solution for future space station thermal management systems.

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Evaporation and drying characteristics of the sessile ferrofluid droplet under a horizontal magnetic field

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Fundamental Research 2022年第2期2卷 222-229页

作者： Zhaonan Liu Jiandong Zhou Yang Li Xin Zhuo Xiujuan Shi Dengwei Jing State Key Laboratory of Multiphase Flow in Power Engineering and International Research Center for Renewable Energy X^an Jiaotong UniversityXi'an 710049China

In this study,the evaporation characteristics and drying patterns of various sessile ferrofluid droplets on certain substrate under horizontal magnetic fields of controlled intensities are *** effects of droplet concentration and magnetic field intensity on the duration of each evaporation stage and drying patterns of droplets have been systematically *** turned out that a plateau appears at the initial stage of evaporation in the absence of magnetic field and it was found that the plateau value is positively correlated with the concentration of ferrofluid *** the external magnetic field,the evaporation time of droplets decreases,the stage of contact line retreat extends,the stage of late pinning mode shortens,and the deposition area of ferrofluid droplet decreases compared to that of without magnetics *** deposition area increases gradually and becomes more uniform with the increase of magnetic *** decrease of friction force which is due to the decrease of the number of nanoparticles at the contact line under external magnetic field is the main reason for the observed *** found that the coffee ring and the uniform deposition inside the droplet will be destroyed when the magnetic field intensity is higher than a critical *** work has a significant reference value for the evaporation of sessile magnetic fluid droplets under the applied magnetic field,especially when the drying pattern needs to be precisely controlled,such as in spray or biomedicine.

关键词： Ferrofluid Droplet Drying pattern Evaporation characteristics Magnetic field

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Intra-Ring Bridging:A Strategy for Molecular Design of Highly Energetic Nitramines

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Chinese Journal of Chemistry 2021年第10期39卷 2857-2864页

作者： Linyuan Wen Tao Yu Weipeng Lai Jinwen Shi Maochang Liu Yingzhe Liu Bozhou Wang State Key Laboratory of Fluorine&Nitrogen Chemicals Xi'an Modern Chemistry Research InstituteXi'anShaanxi710065 China International Research Center for Renewable Energy State Key Laboratory of Multiphase Flow in Power EngineeringXi'an Jiaotong UniversityXi'anShaanxi 710049China

Main observation and conclusion Important progress has been made in the development of energetic molecules with high performance by computer-aided molecular design in recent years,but structural novelty of organic scaffolds is *** this work,we propose an intra-ring bridging strategy inspired by the known energetic nitramines to design novel polycyclic and cage energetic *** than 100 energetic structures were designed by introducing the C—C bridges and increasing the ring *** synthesis difficulty is considered besides the two most concerned properties of EMs,energy and *** a comprehensive estimation,a symmetric cage molecule labeled as 8U-30 was finally selected because of its relatively high detonation performance,and comparable impact sensitivity as well as synthetic accessibility with ***,the proposed strategy could be utilized in further molecular design to gain various scaffolds,especially cage structures,for different demands.

关键词： Molecular modeling Energetic materials Cage compounds Computational chemistry Nitramines

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Photocatalytic water splitting on BiVO_(4):Balanced charge-carrier consumption and selective redox reaction

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Nano Research 2023年第4期16卷 4568-4573页

作者： Xiangjiu Guan Li Tian Yazhou Zhang Jinwen Shi Shaohua Shen International Research Center for Renewable Energy State Key Laboratory of Multiphase Flow in Power EngineeringXi’an Jiaotong UniversityXi’an 710049China Suzhou Academy of Xi’an Jiaotong University Suzhou 215123China State Key Laboratory for Physical Chemistry of Solid Surfaces College of Chemistry and Chemical EngineeringXiamen UniversityXiamen 361005China

Surficial redox reactions play an essential role in photocatalytic water splitting,and are closely related to the surface properties of a specific *** this work,using monoclinic BiVO_(4)decahedral single crystals as a model photocatalyst,we report on the interrelationship between the photocatalytic activity and the surficial reaction sites for charge-carrier *** controlled hydrothermal synthesis,the ratio of{010}to{110}facets on BiVO_(4),which respectively serve as reductive and oxidative sites,is carefully *** results show that superior photocatalytic water oxidation could be obtained on BiVO_(4)decahedrons with a medium ratio of reductive/oxidative sites and that efficient overall water splitting could be achieved via further modification of appropriate cocatalysts in Z-scheme *** excellent photocatalytic performance is attributed to the accelerated selective redox reactions by realizing balanced charge-carrier consumption,which provides insightful guidance for prospering photocatalytic reactions in energy conversion.

关键词： BiVO_(4) photocatalytic water splitting reactive site

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Thermodynamic, life cycle, and techno-economic assessment of an autothermal supercritical water gasification system for direct processing raw pig manure: Hydrogen generation and ammonia recovery

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Energy 2025年 330卷

作者： Mingming Du Fan Liu Haoran Yuan Yu-nan Chen Jing Gu Guangzhou Institute of Energy Conversion Chinese Academy of Sciences (CAS) Guangzhou 510640 PR China State Key Laboratory of Multiphase Flow in Power Engineering (SKLMF) Xi'an Jiaotong University Xi'an Shaanxi 710049 PR China Guangdong Provincial Key Laboratory of Renewable Energy Guangzhou 510640 PR China

Supercritical water gasification (SCWG) exhibits an excellent potential for the conversion from pig manure (PM) to H 2 . However, the low solid content characteristic of raw PM and ammonia discharge significantly constrain the thermodynamic efficiency of SCWG. To address these limitations, a novel SCWG system was designed for simultaneous autothermal H 2 production and ammonia recovery from raw PM. Thermodynamic analysis, life cycle, and techno-economic were carried out to assess system performance. Results indicated that the novel system exhibited exceptional adaptability to variations in concentration and mass flow of raw PM, with autothermal H 2 production achieved even at low concentration of 10 %. Raw PM was converted into high-concentration slurries through pulping operations, thereby reducing exergy losses of gasification, heat exchange, and cooling units. Further, the system implemented an efficient ammonia recovery utilizing steam generated during the pulping stage. Under a typical scenario, energy efficiency, exergy efficiency, GWPs, and EP of the novel system reached 50.34 %, 45.99 %, 0.005 kgCO 2 -eq/kgH 2 , and 0.07 kgNO 3 - -eq/kg H 2 , respectively. The levelized hydrogen cost of the new system was 15.81 CNY/kg. This study provides a valuable solution for autothermal SCWG of low-solid-content and high-nitrogen-content feedstocks to produce H 2 and recover ammonia.

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A novel mid-temperature chemical looping system with near-zero carbon emissions for hydrogen and power coproduction

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Energy 2025年 329卷

作者： Yang Li Yu Fang Mingkai Liu Kai Liu Zhongrui Gai Yuanhui Shen Ruqi Zhang Ying Pan Hongguang Jin Institute of Engineering Thermophysics Chinese Academy of Sciences Beijing 100190 China University of Chinese Academy of Sciences Beijing 100049 China International Research Center for Renewable Energy & State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong University Xi'an 710049 China

Designing an efficient system for conversion of fossil fuel to hydrogen with lower environmental impact represents a promising strategy to meet the demands of a low-carbon future society. This study introduces an integrated chemical looping system combining hydrogen production and combustion for low-carbon fossil fuel conversion. The system achieves hydrogen production at 600 °C, significantly lower than conventional steam methane reforming (850 °C). Moreover, chemical looping combustion is employed to enable efficient CO 2 capture. The proposed system is investigated from key reactions, system performance, and economic feasibility aspects. Experimental results show 80 % methane conversion, a hydrogen yield of 2.6 in the hydrogen production process, and nearly 100 % CO 2 purity from purge gas combustion. Thermodynamic analysis reveals the energy and exergy efficiencies of 74.3 % and 68.9 %, surpassing the reference system by 3.6 % and 4.1 %, respectively. Economic assessment indicates a 10 % reduction in the levelized cost of hydrogen compared to the reference system. 1000 consecutive cycles confirm the outstanding stability of the oxygen carrier particles for the system. This study demonstrates the system's feasibility, cost-effectiveness, and potential for sustainable hydrogen production with minimal environmental impact, introducing a promising method for the efficient utilization of fossil fuels.

关键词： Differential thermal analysis

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