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5th International Energy Conversion engineering Conference

作者： Qinming, Zhang Shuzhong, Wang Liang, Wang Donghai, Xu Lingling, Lu State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong University Xi'an 710049 China Department of Thermal Engineering Xi'an Jiaotong University AIAA

ISBN: (纸本)1563479028

Gasification of high moisture content biomass in supercritical water has been identified as a promising alternative system for producing renewable hydrogen. Supercritical water partial oxidation is the process by which an oxidant appears during the reaction. The key advantage of this process is the rapid heating of the gasification medium, resulting in less char formation and improved hydrogen yield. Many researchers have studied the supercritical water gasification of model compounds. However, real biomass which is of importance for large production of hydrogen has yet to be thoroughly examined. In this paper, gasification of high moisture content municipal sludge was studied in a continuous reactor employing hydrogen peroxide as an oxygen source. The reaction was tested across temperatures and pressures in the range of 673 to 873 K and 24 to 30 MPa, and across various residence times ranging from 3 to 15 minutes. We found that sludge at low concentrations can be completely gasified with no observable char or tar formation. The improvement of gasification efficiency by partial oxidation was accompanied with a high yield of hydrogen and carbon monoxide. Through this, we evaluated the energy efficiency of sludge gasification. Our thermodynamic calculations show that the energy efficiency reaches 50% when considering hydrogen, carbon monoxide, and methane as the valuable gases in the ideal case. Taking into account the energy recovery from the hot water at 30 MPa and 873 K and assuming the ideal scenario of no external heat loss, the overall energy yield potentially reaches 85%. Our results show that the key mechanism of the gasification process is energy recovery, as the chemical reaction is endothermic and requires high temperatures.

关键词： Hydrogen production

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A universal charge-compensating strategy for high-energy-density pseudocapacitors

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Journal of Energy Chemistry 2023年第3期78卷 333-339,I0010页

作者： Baoyi Yin Jiaqi Zhang Yuanhui Su Yu Huan Liang Hao Chen Wang Xun Hu Tao Wei School of Material Science and Engineering University of Jinan336 Nanxinzhuang West RoadJinan 250022ShandongChina School of Microelectronics Dalian University of TechnologyDalian 116024LiaoningChina Shanghai Key Laboratory of Multiphase Flow and Heat Transfer in Power Engineering School of Energy and Power EngineeringUniversity of Shanghai for Science and TechnologyShanghai 200093China State Key Laboratory of ASIC and Systems School of MicroelectronicsFudan UniversityShanghai 200433China

For pseudocapacitive electrode materials(PseEMs),despite much progress having been made in achieving both high power density and high energy density,a general strategy to guide the enhancement of intrinsic capacitive properties of PseEMs remains ***,we demonstrate a universal chargecompensating strategy to improve the charge-storage capability of PseEMs intrinsically:ⅰ) in the electrolyte with anion as charge carriers(such as OH-),reducing the multivalent cations of PseEMs into lower valences could create more reversible low-to-high valence redox cou ples to promote the intercalation of the anions;ⅱ) in the electrolytes with cation as charge carriers(such as H^(+),Li^(+),Na^(+)),oxidizing the multivalent cations of PseEMs into higher valences could introduce more reversible high-to-low valence redox couples to promote the intercalation of the *** we demonstrated that the improved intrinsic charge-storage capability for PseEMs originates from the increased Faradaic charge storage sites.

关键词： Supercapacitors Universal charge-compensating strategy Changed valence state Increased Faradaic charge storage sites

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Experimental Investigation on flow Pattern and Bubble Behavior during Subcooled flow Boiling of R1233zd(E)in Parallel Channels

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Journal of Thermal Science 2023年第6期32卷 2374-2385页

作者： FANG Yidong ZHANG Zhao XU Dan WANG Yuchen YANG Huinan HUANG Yuqi School of Energy and Power Engineering University of Shanghai for Science and TechnologyShanghai200093China Shanghai Key Laboratory of Multiphase Flow and Heat Transfer in Power Engineering Shanghai200093China Key Laboratory of Clean Energy and Carbon Neutrality of Zhejiang Province Jiaxing Research InstituteZhejiang UniversityJiaxing314031China Key Laboratory of Smart Thermal Management Science&Technology for Vehicles of Zhejiang Province Taizhou317200China

In this study,the flow pattern and bubble behavior of R1233zd(E)during subcooled flow boiling in parallel channels are experimentally investigated with visualization and thermal *** test section is composed of 21 rectangular mini channels with the hydraulic diameter of 1.5 mm and the length of 140 *** flow,slug flow,churn flow and wavy-annular flow occur in sequence with the increase of vapor quality,while transient flow pattern transition process involving multiple flow patterns are also *** distribution of flow pattern is non-synchronized and axial-asymmetric,with earlier flow pattern transitions observed in peripheral channels away from the center *** initial nucleate site in each channel also show a random and axial-asymmetric distribution,while faster bubble growth can be noted in some channel under the comprehensive effects of liquid evaporation and bubble *** variation of heat transfer coefficient is correspondence to the flow pattern transition,showing different trends along the flow *** increase of mass flux can lead to delayed flow pattern transition and variation of heat transfer *** addition,higher heat transfer coefficient can be noted in channels away from the center axis.

关键词： flow boiling flow pattern bubble behavior parallel channel visualization

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Hydrogen production by biomass gasification in supercriticor subcritical water with Raney-Ni and other catalysts

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中国高等学校学术文摘·能源与动力工程 2009年第4期3卷 456-464页

作者： Aixia PEI Lisheng ZHANG Bizheng JIANG Liejin GUO Ximin ZHANG Youjun LV Hui JIN Zhongyuan Petroleum Company Puguang Natural Gas Treating Plant Sinopec Dazhou 636156 China State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong University Xi'an 710049 China

Gasification of peanut shell, sawdust and straw in supercritical or subcritical water has been studied in a batch reactor with the presence of a series of Raney-Ni and its mixture with ZnCl2 or Ca(OH)2. The main gas products were hydrogen, methane, carbon dioxide, and a small amount of carbon monoxide. Different types of Raney-Ni, containing different metal components such as Fe, Mo or Cr, have different influences on the gasification yield and hydrogen selectivity. The catalysis effect can be improved obviously by adding ZnCl2 or Ca(OH)2 Increasing the reaction temperature or adding ZnCl2 and Ca(OH)2 could improve the mass of H2 in gas products and reduce the mass of CH4 and CO2 at the same time. The possible mechanism is that ZnCl2 can decompose the biomass particle by accelerating cellulose hydrolyzation in high-temperature water, increasing more specific surface to admit catalysts, while Ca(OH)2 can absorb CO2 to produce CaCO3 deposit, which can drop out from the reactant system, and which will drive the reaction to get more hydrogen. With respect to the biomass conversion to gas product and selectivity of H2 at low temperature, the series of Raney-Ni has shown many advantages over other catalysts; thus, this kind of catalyst has great potential to be utilized in the hydrogen industry for the gasification of biomass.

关键词： biomass catalyst gasification Raney-Ni supercritical water hydrogen

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Dryout point prediction model for bilaterally heated vertical narrow annuli under low flow conditions

Dryout point prediction model for bilaterally heated vertica...

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25th Annual CNS Conference - Nuclear Energy: Meeting the Challenges

作者： Myint, Aye Tian, Wenxi Li, Zhihui Hao, Li Jia, Dounan State Key Laboratory of Multiphase Flow in Power Engineering School of Energy and Power Engineering Xi'an Jiaotong University No.28 Xianning West Road Xi'an City 710049 China

ISBN: (纸本)0919784798

Prediction of dryout point was experimentally investigated with deionized water upflowing through narrow annular channel with 1.0 mm and 1.5 mm gap respectively. The annular with narrow gap was bilaterally heated by AC current power supply. The experimental conditions covered a range of pressure from 0.8 to 3.5 MPa, mass flux of 60.39 to 135.6 kg/m2 and heat flux of 5 to 50 kW/m2 This paper presents a new analytical model for the prediction of dryout point for steam- water flow in narrow annular gap and bilaterally and uniformly heated tubes. The prediction of dryout point for bilaterally heated annuli was based on the droplet-diffusion model for internally heated annuli by Kirillov and Smogalev (1969, 1972). The dryout model prediction values are compared with a experimental data, showing a good agreement in accuracy for the above mentioned parametric range.

关键词： Nuclear power plants

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The role of rotary liquid-solid two-phase flow in the synergistic behavior between sand erosion and electrochemical corrosion of Ni 2 FeCrMo 0.2 alloy in marine environment

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Process Safety and Environmental Protection 2025年

作者： Xingqi Luo Qipeng Xu Kai Wang Jianjun Feng Yanhui Li Yan Liu Xiya Zhang State Key Laboratory of Water Engineering Ecology and Environment in Arid Area Xi’an University of Technology No.5 Jinhua South Road Xi’an 710048 China State Key Laboratory of Multiphase Flow in Power Engineering Xi’an Jiaotong University No.28 Xianning West Road Xi’an 710049 China Qinghai Salt Lake Industry Co. Ltd. No.28 Huanghe Road Golmud 816000 China

The erosion-corrosion behavior poses a significant threat to marine equipment, driven by complex multi-physics processes such as sand movement, surface erosion, electrochemical reactions, and corrosive ion transport. Aiming at the widely used rotating liquid-solid two-phase flow system in a marine environment, this study investigates the role of flow velocity in the erosion-corrosion behavior of Ni 2 FeCrMo 0.2 alloy. The coupling analysis of multi-component weight loss, electrochemical kinetics, and microstructure characterization clarifies the interactions between fluid flow, sand migration, ion transfer, and damage morphology, revealing the synergistic erosion-corrosion mechanism. The results show that the erosion-corrosion mechanism transfers with flow velocity. At low velocities, the erosion effect on the harder metal matrix is weak due to insufficient kinetic energy of the sand particles. However, the sand-surface impingement on the softer corrosion products and the mass transfer of corrosive ions lead to erosion-enhanced corrosion, which dominates the material damage process. In contrast, at higher velocities, the impact kinetic energy and frequency of sand particles rise, causing the erosion rate to increase exponentially, which surpasses corrosion, making erosion as the dominant damage mechanism at high velocities. Thses results highlight the critical role of flow velocity in controlling the erosion-corrosion synergy behavior.

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Experimental study on loop heat pipe with flat evaporator at different tilt angles

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Hsi-An Chiao Tung Ta Hsueh/Journal of Xi'an Jiaotong University 2013年第5期47卷 38-43页

作者： Long, Yan Wei, Jinjia Lü, Xiao State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong University Xi'an 710049 China

To realize highly efficient heat dissipation of electronics, a loop heat pipe (LHP) with a flat evaporator was designed to study its operation characteristics at the tilt angles of 0°, 30°, 45°, 60°, 90° with an improved evaporator structure and a well arranged pipes which can reduce heat loss due to back conduction and improve inner flow performance. The results show that the LHP with inclination has a lower power to start up than the horizontal one, and at the same heat load, the operation temperature of the evaporator is much lower and the system is easier to reach a steady state with less temperature oscillations. However, there is slight difference in operating performance for the LHP at different title angles. The thermal resistance decreases with an increase in the heat load and a steady state occurs at last. The thermal resistance is larger for the horizontal case than that for the inclination case at the same heat load. The thermal resistances are very different at different tilt angles at low heat load, but the difference is small at high heat load.

关键词： Thermal load

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Anti-K salt poisoning of MnO x catalyst via X (X = Ce, Sm and Er) oxides for low-temperature NH 3 -SCR of NO and oxidating CO

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Journal of Environmental Chemical engineering 2025年第3期13卷

作者： Liang Wang Shan Ren Xiaodi Li Chi He Chunli Zheng Xinzhe Li Shouning Chai Kejiang Li Chunbao Charles Xu College of Materials Science and Engineering Chongqing University Chongqing 400044 PR China State Key Laboratory of Multiphase Flow in Power Engineering School of Energy and Power Engineering Xi’an Jiaotong University Xi’an Shaanxi 710049 PR China School of Metallurgical and Ecological Engineering University of Science and Technology Beijing Beijing 100083 PR China School of Energy and Environment City University of Hong Kong Kowloon Hong Kong

Manganese oxide (MnO x ) serves as an effective catalyst for the simultaneous elimination of NO and CO pollutants in low-temperature flue gas. However, potassium salts present in industrial flue gas severely compromise the catalytic performance by altering surface physicochemical properties, leading to deactivation and reduced pollutant removal efficiency. To address this limitation, several rare earth (Ce, Sm and Er) oxides were incorporated into MnO x catalyst to enhance active site under potassium (K) exposure in this work. Catalytic activities of NO and CO removal both followed the order of K-Sm/MA > K-Er/MA > K-Ce/MA > K/MA. Especially, Sm/MA enhanced the considerable conversion of NO and CO at 175°C. Characterization revealed that Sm optimized the ration of Mn 4 + and O α , which showed higher active sites than other rare earth oxides modification. Moreover, in situ DRIFTS analysis confirmed the enhanced fast SCR process and the stronger interaction between CO and active sites on K-Sm/MA catalyst, which contributed to its superior K resistance and improved the removal efficiency. The K-Sm/MA catalyst accumulated more nitrate species and exhibited good reactivity, sustaining continuous NO conversion through the Langmuir-Hinshelwood (L-H) mechanism. Finally, a pathway model of Sm oxide on MnO x catalyst for the simultaneous NH 3 -SCR coupling CO oxidation at K poisoned situation.

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Single electron loss in the collisions of Ca+ and atomic hydrogen

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中国物理B（英文版） 2010年第9期19卷 344-348页

作者： Liu Hui-Ping Ouyang Xiao-Ping Hu Hua-Si Su Guang-Hui State Key Laboratory of Multiphase Flow in Power Engineering Department of Nuclear Science and TechnologyXi'anjiaotong UniversityXi'an 710049China

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Measurement and control system in process of carbon dioxide capture based on sparse support vector machine

Measurement and control system in process of carbon dioxide ...

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Global Congress on Intelligent Systems

作者： Yan, Liwei Lu, Hongfang Yu, Yunsong Zhang, Xu Li, Yun Zhang, Zaoxiao State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong University Xi'an 710049 China School of Energy and Power Engineering Xi'an Jiaotong University Xi'an 710049 China

ISBN: (纸本)9780769543048

Capturing CO2 from the flue gas of a power plant based on chemical absorption method is an effective way to cut down the emission of CO2. However, the principal components in the solvent are very difficult to be measured online. Therefore an online measurement and control system was designed for the process of capturing CO2 by MEA chemical absorption. The feature selection was done according to Bayesian networks. Furthermore based on the principle of a new sparse support vector machine (SLS-SVM), the measurement of ionic species distribution in the absorption solution was predicted, and the results agreed well with the data obtained by Nuclear Magnetic Resonance (NMR) measurement. The mean square error is 3.8645×10-7. The measurement of solution species distribution was carried out online by using infrared sensors and NMR technology. Meanwhile the sampling system and NMR unit were linked for the online analysis based on variable-temperature and variable-pressure NMR technology. Finally a measurement and control platform was constructed based on VI technology. It shows that the performance of traditional equipment can be improved by the novel system, which will provide a more effective method for CO2 capture process. © 2010 IEEE.

关键词： Bayesian networks

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