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A state-of-the-art review on the utilization of biochar as renewable energy for the sustainable steel industry

Applied Energy 2025年 394卷

作者： Shan Ren Siyi Yang Hongsheng Chen Liang Wang Manyi Liu Guangwei Wang Chunbao Xu College of Materials Science and Engineering Chongqing University Chongqing 400044 China State Key Laboratory of Multiphase Flow in Power Engineering School of Energy and Power Engineering Xi'an Jiaotong University Xi'an 710049 China State Key Laboratory of Advanced Metallurgy University of Science & Tech. Beijing Beijing 100083 China School of Energy and Environment City University of Hong Kong Kowloon Hong Kong

The steel industry is a major contributor to global anthropogenic CO₂ emissions, accounting for nearly 10 % of the total. Within this sector, ironmaking processes, particularly those using the traditional blast furnace-basic oxygen furnace route, are responsible for almost 90 % of the industry's CO₂ emissions. Biochar, derived from renewable feedstocks, offers a sustainable and eco-friendly alternative to fossil fuels for ironmaking. This review examines the cutting-edge techniques for producing biochar and recent advancements in utilizing biochar across various ironmaking processes, including sintering/pelletizing, coke making, blast furnace injection, and direct reduction iron processes, with a focus on reducing CO₂ emissions. Despite demonstrated benefits such as reduced pollution, improved burden permeability, and enhanced gas utilization efficiency in pilot and industrial trials, large-scale biochar application remains limited by the varying quality requirements of different processes. Innovatively, a green hydrogen-metallurgical route that utilizes hydrogen-rich syngas derived from biomass and biochar is proposed in this work, serving as a comprehensive solution to address the challenges associated with the quality discrepancies of biochar produced by different carbonization methods and the diverse quality requirements for biochar in various ironmaking processes. This solution not only underscores its potential to significantly transform the iron and steel industry towards a more sustainable and low-carbon future, but also highlights the innovative contributions of this research to the fields of renewable energy, solid waste resources, metallurgical industry, and global climate change.

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Chemical looping based ammonia production--A promising pathway for production of the noncarbon fuel

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Science Bulletin 2022年第20期67卷 2124-2138,M0004页

作者： Qinghua Lai Tianyi Cai Shik Chi Edman Tsang Xia Chen Runping Ye Zhenghe Xu Morris D.Argyle Dong Ding Yongmei Chen Jianji Wang Armistead G.Russell Ye Wu Jian Liu Maohong Fan College of Engineering and Applied Science University of WyomingLaramie WY 82071USA School of Energy and Power Engineering Shanghai Key Laboratory of Multiphase Flow and Heat Transfer in Power EngineeringUniversity of Shanghai for Science and TechnologyShanghai 200093China Wolfson Catalysis Department of ChemistryUniversity of OxfordOxford Ox13QRUK College of Chemistry and Chemical Engineering Ocean University of ChinaQingdao 266100China State Key Laboratory of Catalysis Dalian Institute of Chemical PhysicsChinese Academy of SciencesDalian 116023China Department of Materials Science and Engineering Southern University of Science and TechnologyShenzhen 518055China Department of Chemical and Materials Engineering University of AlbertaEdmonton Alberta T6G1H9Canada Department of Chemical Engineering Brigham Young UniversityProvo UT 84602USA Idaho National Laboratory Idaho Falls ID83415USA College of Chemistry Beijing University of Chemical TechnologyBejing 100029China School of Chemistry and Environmental Science Henan Normal UniversityXinxiang 453007China School of Civil and Environmental Engineering Georgia Institute of TechnologyAtlanta GA 30332USA MIIT Key Laboratory of Thermal Control of Electronic Equipment School of Power EngineeringNanjing University of Science&TechnologyNanjing 210094China DICP-Surrey Joint Centre for Future Materials Department of Chemical and Process Engineeringand Advanced Technology InstituteUniversity of SurreyGuilford Surrey GU27XH UK

Ammonia, primarily made with Haber-Bosch process developed in 1909 and winning two Nobel prizes, is a promising noncarbon fuel for preventing global warming of 1.5 °C above pre-industrial levels. However,the undesired characteristics of the process, including high carbon footprint, necessitate alternative ammonia synthesis methods, and among them is chemical looping ammonia production(CLAP) that uses nitrogen carrier materials and operates at atmospheric pressure with high product selectivity and energy efficiency. To date, neither a systematic review nor a perspective in nitrogen carriers and CLAP has been reported in the critical area. Thus, this work not only assesses the previous results of CLAP but also provides perspectives towards the future of CLAP. It classifies, characterizes, and holistically analyzes the fundamentally different CLAP pathways and discusses the ways of further improving the CLAP performance with the assistance of plasma technology and artificial intelligence(AI).

关键词： Ammonia synthesis Chemical looping Nitrogen carrier Renewable fuels Energy carrier

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Beam dynamics induced by the quantum metric of exceptional rings

arXiv

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arXiv 2024年

作者： Zhang, Zhaoyang Septembre, Ismaël Liu, Zhenzhi Kokhanchik, Pavel Liang, Shun Liu, Fu Li, Changbiao Wang, Hongxing Liu, Maochang Zhang, Yanpeng Xiao, Min Malpuech, Guillaume Solnyshkov, Dmitry Key Laboratory for Physical Electronics and Devices The Ministry of Education Shaanxi Key Lab of Information Photonic Technique School of Electronic Science and Engineering Faculty of Electronics and Information Xi’an Jiaotong University Xi’an710049 China Institut Pascal PHOTON-N2 Université Clermont Auvergne CNRS Clermont INP Clermont-FerrandF-63000 France Naturwissenschaftlich-Technische Fakultät Universität Siegen Walter-Flex-Straße 3 Siegen57068 Germany International Research Center for Renewable Energy State Key Laboratory of Multiphase Flow in Power Engineering Xi’an Jiaotong University Xi’an710049 China Department of Physics University of Arkansas FayettevilleAR72701 United States Paris75231 France

Topological physics has broadened its scope from the study of topological insulating phases to include nodal phases containing band structure singularities. The geometry of the corresponding quantum states is described by the quantum metric which provides a theoretical framework for explaining phenomena that conventional approaches fail to address. The field has become even broader by encompassing non-Hermitian singularities: in addition to Dirac, Weyl nodes, or nodal lines, it is now common to encounter exceptional points, exceptional or Weyl rings, and even Weyl spheres. They give access to fascinating effects that cannot be reached within the Hermitian picture. However, the quantum geometry of non-Hermitian singularities is not a straightforward extension of the Hermitian one, remaining far less understood. Here, we study experimentally and theoretically the dynamics of wave packets at exceptional rings stemming from Dirac points in a photonic honeycomb lattice. First, we demonstrate a transition between conical diffraction and non-Hermitian broadening in real space. Next, we predict and demonstrate a new non-Hermitian effect in the reciprocal space, induced by the non-orthogonality of the eigenstates. We call it transverse non-Hermitian drift, and its description requires biorthogonal quantum metric. The non-Hermitian drift can be used for applications in beam steering. Copyright © 2024, The Authors. All rights reserved.

关键词： Topology

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Facile Synthesis of Bulk Au-Co-Coox-Ceox@Iron Ball and its Photocatalytic Application in 4-Nitrophenol Degradation

SSRN

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SSRN 2023年

作者： Sun, Li Qiao, Zhili Zhi, Yuan Zhang, Hua Dou, Binlin Shan, Yuejin Huang, Weijia School of Energy and Power Engineering University of Shanghai for Science and Technology Jun Gong Road 516 Shanghai200093 China R&D Department Shanghai Minrula Biotechnology Co.Ltd Building 15 Haji Sixth Road 218 Shanghai201306 China Department of Material and Environmental Chemistry Research Division of Functional Materials Design Utsunomiya University Yoto 7-1-2 Utsunomiya321-8585 Japan Shanghai Key Laboratory of Multiphase Flow and Heat Transfer in Power Engineering China

Bulk noble metal-semiconductor composites can be chosen as photocatalysts to carry out the continuous-flow (C-F) degradation of 4-nitrophenol (4-NP) whereas their preparation is complex and uncontrollable. Here, bulk Au/Co-CC@iron ball is designed and prepared by a facile and controllable route without any toxic chemical. The bulk Au/Co-CC@iron ball shows excellent photocatalytic activity and reusability for the 4-NP degradation, which can be ascribed to the synergistic action of active components and foliated iron ball surface. Furthermore, the highly active Au/Co-CC@iron ball is used as packing material to construct a new-type of packed reactor, by which the C-F degradation of 4-NP is successfully achieved. As-fabricated packed reactor and its tandem module exhibit superior photocatalytic performance for the C-F degradation of 4-NP. Noteworthy, based on the tandem module with six reactors, the removal rate of 4-NP can reach up to 2750 µmol/h. Meanwhile, the reactor and its module display satisfactory operational stability and reusability in the C-F degradation of 4-NP. Clearly, the provided route is effective for the preparation of bulk noble metal-semiconductor composites with exceptional performance, which can also be a prospective strategy to obtain bulk packing materials to serve for the C-F degradation. © 2023, The Authors. All rights reserved.

关键词： Precious metals

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Computational homogenization of thermomechanical properties for Fully Ceramic Microencapsulated fuel with 3D printed SiC matrix

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Annals of Nuclear Energy 2025年 222卷

作者： Chen, Yiwen Lu, Qi Liu, Changwen Li, Wei Zhang, Dalin Su, G.H. State Key Laboratory of Multiphase Flow in Power Engineering Shaanxi Key Laboratory of Advanced Nuclear Energy and Technology School of Nuclear Science and Technology Xi'an Jiaotong University Xi'an710049 China Science and Technology on Reactor System Design Technology Laboratory Nuclear Power Institute of China Chengdu61213 China State Key Laboratory for Strength and Vibration of Mechanical Structures Xi'an Jiaotong University Xi'an710049 China

Fully Ceramic Microencapsulated (FCM) fuel, fabricated using 3D printing technology, incorporates traditional Tristructural-Isotropic (TRISO) fuel particles embedded within a 3D-printed SiC matrix. This fuel type shows great potential for compact, high-temperature nuclear reactors. However, comprehensive performance analysis remains challenging due to the multilayered structure, complex material properties, and the irradiation behavior of numerous TRISO particles within the matrix. To address these challenges, this study aims to apply finite element (FE)-based computational homogenization to evaluate the fuel's thermomechanical properties. First, a detailed finite element analysis (FEA) of a single TRISO particle's performance was conducted, focusing primarily on the Buffer-IPyC gap size change during irradiation, a critical factor influencing the fuel's thermal performance. Second, the homogenization of a single TRISO particle was performed using FEA, accounting for the changes in the Buffer-IPyC gap size. Finally, homogenized TRISO particles were randomly distributed and perfectly bonded within a 3D-printed SiC matrix to form a Representative Volume Element (RVE). The FE homogenization of the RVE was then conducted to derive the effective thermomechanical properties of the FCM fuel. The packing fraction of TRISO particles in the matrix ranged from 10 % to 50 %, with temperature and burnup conditions spanning 800–1600 K and 0–16 % FIMA, respectively. Results show that irradiation significantly affects the effective properties of the fuel, though this impact diminishes as burnup increases. Additionally, the effective thermal conductivity of the FCM fuel decreases with increasing TRISO packing fraction, assuming the thermal conductivity of the SiC matrix exceeds that of TRISO particles. This study provides a valuable reference for the design and optimization of FCM fuel for future nuclear applications. © 2025 Elsevier Ltd

关键词： Thermal conductivity of solids

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Corrigendum to “Numerical simulation of an externally heated fixed bed reactor for coal pyrolysis based on porous media” [Chem. Eng. Res. Des. 211 (2024) 137–151]

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Chemical engineering Research and Design 2025年 218卷 454-454页

作者： Haoyue Li Yuanpei Luo Fei Dai Jun Sui Hongguang Jin Laboratory of Distributed Energy Systems and Renewable Energy Institute of Engineering Thermophysics Chinese Academy of Sciences Beijing 100190 China University of Chinese Academy of Sciences Beijing 100049 China State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong University Xi'an 710049 China

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Remote open-path laser-induced breakdown spectroscopy for the analysis of manganese in steel samples at high temperature

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Plasma Science and Technology 2019年第3期21卷 52-59页

作者： Minchao CUI Yoshihiro DEGUCHI Zhenzhen WANG Seiya TANAKA Min-Gyu JEON Yuki FUJITA Shengdun ZHAO School of Mechanical Engineering Xi'an Jiaotong University Graduate School of Advanced Technology and Science University of Tokushima State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong University Division of Mechanical Engineering Korea Maritime and Ocean University School of Mechanical Engineering Xi’an Jiaotong University

A remote open-path laser-induced breakdown spectroscopy(LIBS) system was designed and studied in the present work for the purpose of combining the LIBS technique with the steel production line. In this system, the relatively simple configuration and optics were employed to measure the steel samples at a remote distance and a hot sample temperature. The system has obtained a robustness for the deviation of the sample position because of the open-path and alloptical structure. The measurement was carried out at different sample temperatures by placing the samples in a muffle furnace with a window in the front door. The results show that the intensity of the spectral lines increased as the sample temperature increased. The influence of the sample temperature on the quantitative analysis of manganese in the steel samples was investigated by measuring ten standard steel samples at different temperatures. Three samples were selected as the test sample for the simulation measurement. The results show that, at the sample temperature of 500 ℃, the average relative error of prediction is 3.1% and the average relative standard deviation is 7.7%, respectively.

关键词： remote open-path LIBS steel manganese sample temperature quantitative analysis

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Strengthening Chlorobenzene Catalytic Degradation Rate and Selectivity Over Laxsr1-Xmno3±Δ by Anchoring Interfacial Oxygen Vacancy

SSRN

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SSRN 2022年

作者： Li, Lu Tao, Dan Zhao, Qi Fu, Shuangshuang Min, Xin Chen, Changwei Tian, Mingjiao Shi, Jianwen He, Chi State Key Laboratory of Electrical Insulation and Power Equipment Center of Nanomaterials for Renewable Energy School of Electrical Engineering Xi’an Jiaotong University Shaanxi Xi’an710049 China State Key Laboratory of Multiphase Flow in Power Engineering School of Energy and Power Engineering Xi’an Jiaotong University Shaanxi Xi’an710049 China College of Geology and Environment Xi’an University of Science and Technology Shaanxi Xi’an710054 China Faculty of Electronic and Information Engineering Xi’an Jiaotong University Shaanxi Xi’an710049 China School of Environmental and Municipal Engineering Xi’an University of Architecture and Technology Shaanxi Xi’an710055 China School of Environmental Science and Engineering Shanghai Jiao Tong University 800 Dongchuan Road Shanghai200240 China

Surficial lattice oxygen in perovskite compounds is a common participant during chloroaromatic catalytic destruction. Herein, we proposed a facile oxygen vacancy construction strategy for preparing high active LaxSr1-xMnO3±δ (LSMO) via NaBH4 treatment. Results reveal that LSMO composites are not only reduced by NaBH4 under mild condition, but trigger a significant Sr segregation effect, which plays a key role in oxygen vacancy formation accounting to the electron donation from Sr to Mn acceptor and subsequent lattice oxygen activation. Moreover, the concentration of interfacial active oxygen species can be regulated by taming the La-Sr interaction with different Sr substitution proportions. The anchored oxygen vacancies (OVs) take advantage of electron capture or transfer and induce molecule oxygen into active oxygen species to react with chlorobenzene molecules, resulting in a preferential catalytic oxidation capacity. Amongst, reduced La0.5Sr0.5MnO3±δ catalyst displays superior chlorobenzene destruction efficiency with 90% of which converted as low as 236 °C, which also exhibited a stable performance in long-time operation. However, the OVs would be refilled by water H2O molecules resulting in a weaker water resistance for OVs anchored catalyst. In summary, the annihilation of OVs is the most important factor for catalyst deactivation. The research offers a new avenue to construct interfacial oxygen species in perovskite oxides during the chlorobenzene deep oxidation process. © 2022, The Authors. All rights reserved.

关键词： Catalytic oxidation

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Full-core normal and preliminary transient analysis for SiC-based rod designs 14

Full-core normal and preliminary transient analysis for SiC-...

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14th International Nuclear Fuel Cycle Conference, GLOBAL 2019 and Light Water Reactor Fuel Performance Conference, TOP FUEL 2019

作者： He, Yanan Deng, Yangbin Wu, Yingwei Shirvan, Koroush Department of Nuclear Science and Engineering MIT CambridgeMA02139 United States State Key Laboratory of Multiphase Flow in Power Engineering Department of Nuclear Science and Technology Xi'an Jiaotong University Xi'an City710049 China College of Physics and Energy Shenzhen University Shenzhen518060 China

When introducing a new fuel concept in traditional light water reactors (LWRs), analyzing its performance under a variety of power histories while attempting to simulate its stress state as realistic as possible is desired. By having access to such capability, the fuel developer can assess the safety characteristics of the new fuel concept and optimize its design performance. SiC/SiC Ceramic Matrix Composite (CMC) with chemically vapor deposited (CVD) SiC, is an accident tolerant fuel (ATF) concept owing to its high mechanical strength and remarkably enhanced oxidation-resistance. The modeling of SiC cladding requires capability to simulate multilayers and capture the nonlinear response of SiC material under neutron radiation. In addition, considering its probabilistic failure characteristics, efficient running fuel performance tools are required to assess its initial safety performance and optimize its design. In this work, we added a multi-layer deformation model in FRAPCON-4.0 and FRAPTRAN-2.0, with the primary motivation to analyze the performance of SiC cladding for UO2, annular UO2 and U3Si2 fuels from a full core point-of-view. We then performed reactivity-initiated accident (RIA) and loss-of-coolant accident (LOCA) for the limiting rod. During normal conditions, the failure risk of SiC cladding is mainly determined by pellet-cladding mechanical interaction (PCMI) and U3Si2 is a more promising fuel compared to UO2. While promising performance was simulated during LOCA for all fuels, during RIA, U3Si2 performance was found to be likely more limiting compared to UO2. Results show that the full core simulation methods developed for this work are robust and computationally efficient and can be adopted for other ATF design analysis. Copyright © GLOBAL 2019 - International Nuclear Fuel Cycle Conference and TOP FUEL 2019 - Light Water Reactor Fuel Performance *** rights reserved.

关键词： Silicon carbide

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Performance of different flocculants for harvesting Chlorella vulgaris by dissolved air flotation and sedimentation

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Bioresource Technology 2025年 132743页

作者： X. Wei N.R.H. Rao S. Tyagi W. Thielemans W. Cao L.J. Guo K. Muylaert State Key Laboratory of Multiphase Flow in Power Engineering Xi’an Jiaotong University Xi’an 710049 Shaanxi China Laboratory of Aquatic Biology KU Leuven Campus Kulak Kortrijk 8500 Kortrijk Belgium Sustainable Materials Laboratory Department of Chemical Engineering KU Leuven Campus Kulak Kortrijk 8500 Kortrijk Belgium

This study systematically evaluated the performance of dissolved air flotation and sedimentation for harvesting Chlorella vulgaris using eight different flocculants. Significant variation was observed in both the maximum harvesting efficiency and the minimum effective flocculant dose across different flocculant-process combinations. Among the tested flocculants, pyridinium modified cellulose nanocrystals achieved the highest harvesting efficiency of 99 % in both dissolved air flotation and sedimentation, while chitosan required the lowest minimum flocculant dose (∼2 mg·g −1 ) to induce flocculation. The impact of floc size formed during the flocculation step on harvesting performance was also investigated, revealing that large flocs significantly favored sedimentation-based microalgae harvesting. A preliminary cost analysis highlighted the importance of integrating economic considerations into the selection of both flocculant and harvesting method. The findings suggest that optimal flocculant and process selection should be based not only on harvesting efficiency but also on cost-effectiveness for microalgal biomass recovery.

关键词： Cationic flocculants Dissolved air flotation optimization Floc size distribution Microalgal recovery Water treatment

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