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Promoting effect of d-band center and in-situ precipitation strategy on sulfur evolution reaction

Journal of Energy Chemistry 2025年第5期104卷 740-748页

作者： Jun Pu Yun Tan Jiasen Yin Zihan Shen Shoujie Liu Kai Zhang Lei Zhou Yagang Yao Key Laboratory of Functional Molecular Solids Ministry of EducationAnhui Provincial Engineering Laboratory for New-Energy Vehicle Battery Energy-Storage MaterialsCollege of Chemistry and Materials ScienceAnhui Normal UniversityWuhu 241002AnhuiChina National Laboratory of Solid State Microstructures College of Engineering and Applied SciencesJiangsu Key Laboratory of Artificial Functional MaterialsCollaborative Innovation Center of Advanced MicrostructuresNanjing UniversityNanjing 210093JiangsuChina State Key Laboratory of Multiphase Complex Systems Institute of Process EngineeringChinese Academy of SciencesBeijing 100190China School of Materials Science and Engineering Anhui UniversityHefei 230601AnhuiChina School of Energy and Power Engineering Jiangsu UniversityZhenjiang 212013JiangsuChina Department of Electrical Engineering Eindhoven University of TechnologyEindhoven MB 5600the Netherlands

The slow conversion of polyphase in lithium-sulfur(Li-S)batteries not only intensifies the shuttle effect of lithium polysulfides(LiPSs),but also causes the continuous accumulation of inactive sulfur species,resulting in rapid capacity attenuation and sluggish dynamic ***,the promoting effect of atomic interface stress on sulfur reaction was investigated via CoFe-CoFe_(2)O_(4)heterogeneous nanosheets with a cavity *** strain force induced by the in-situ precipitation of Co Fe bimetallic alloy in oxide matrix increased the d-band center,which was conducive to the interaction between catalyst and Li *** sulfur cathode based on this two-dimensional(2D)nanosheet design showed an extremely high capacity of 751 mAh g^(-1)at 4 *** with a sulfur loading of 5.55 mg cm^(-2),its area capacity was still as high as 7.15 mAh cm^(-2).Meanwhile,the enhanced stability greatly improved the practical potential of Li-S batteries.

关键词： 2D nanosheets In-situ precipitation Strain effect D-band center Li-S batteries

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Experimental Study on Stable Jet Impact Process Under Simulated Pipeline Rupture 21

Experimental Study on Stable Jet Impact Process Under Simula...

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21st IEEE Student Conference on Research and Development, SCOReD 2023

作者： Tao, Zhang Qincheng, Bi Jinle, Zhao Teng, Wang Jingrong, Chen Fan, Feng Xi'an Jiaotong University State Key Lab Multiphase Flow Power Engn Shaanxi Xi'an China North China Electric Power University School of Energy Power and Mechanical Engineering Bao'ding Hebei China

ISBN: (纸本)9798350318821

In this study, an advanced experimental system was utilized that incorporated heating, jetting, recycling, and cooling capabilities to ensure the successful execution of stable jet impact experiment that simulating a pipeline complete rupture. High-temperature resistant tempered glass was employed in the experimental system to realize the visibility. During the experiment, 8mm pipes/nozzles of varying lengths were employed as the test sections, and jetting phenomena when the import status is single-phase cold water or two-phase mixture at 0-2MPa were obtained by high-resolution photos. Additionally, the shape of the jet cone and the impact force exerted on the target plate were meticulously analyzed after the working fluid under different state parameters jetting into an atmospheric pressure environment through pipes/nozzles. The research also focused on the variation trend in the magnitude of the jet-impact force, as a function of inlet pressure and temperature, target plate distances, and length-to-diameter ratios. The research findings revealed that cold water(below 100°C), sub-cooled water(above 100°C but not reaching saturation temperature), and two-phase steam-water mixture exhibited distinct jet cone shapes during the jetting process, resulting in varying distributions of the jet force. Furthermore, the distance from the spout to the target plate and the length-to-diameter ratio significantly influenced the magnitude of the jet impact force. © 2023 IEEE.

关键词： Pipelines

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Numerical Simulation of flow Distribution and Transient Thermal Stratification Characteristics of Passive Residual Heat Removal Heat Exchangers

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Yuanzineng Kexue Jishu/Atomic Energy Science and Technology 2025年第5期59卷 1006-1015页

作者： He, Shaopeng Wang, Mingjun Tian, Wenxi Qiu, Suizheng Su, Guanghui State Key Laboratory of Multiphase Flow in Power Engineering Xi’an Jiaotong University Xi’an710049 China Nuclear Thermal-hydraulic Laboratory Xi’an Jiaotong University Xi’an710049 China

The passive residual heat removal heat exchanger (PRHR HX) is a key component of the third-generation advanced pressurized water reactor (PWR) nuclear power plant’s passive safety systems. The PRHR HX has numerous heat transfer tubes with varying lengths and arrangements on the primary side, leading to different flow distributions and resistance characteristics. The secondary side experiences various physical processes, including natural convection, mixed convection, and boiling heat transfer, significantly impacting the heat exchanger’s natural circulation and residual heat removal capacity. Current numerical analysis methods for PRHR HX inadequately consider flow distribution and resistance characteristics on the primary side. A porous medium-pipe-level coupling calculation method was established, introducing a parallel C-shaped pipe-level flow distribution and resistance iterative solution model. A matching strategy for grid control volumes on both sides and physical field communication was proposed, and a mathematical-physical model suitable for natural circulation and two-phase boiling conditions was developed for the PRHR HX, enabling coupling analysis between the primary side’s pipe-level resolution physical field and the secondary side’s porous medium computational domain. Based on data from Japan’s ROSA test facility, program validation was conducted, comparing heat transfer amounts, primary side outlet temperatures, and temperature profiles under single-phase and two-phase conditions, with good agreement between calculated and experimental values. flow distribution and resistance characteristics on the primary side under coupled conditions of the AP1000 reactor’s PRHR HX was explored. The variation of secondary side thermal stratification with different operational parameters was analyzed. Results indicate that when the total flow rate on the primary side increases, the proportion of frictional pressure drop in the total pressure drop increases, diminishin

关键词： Natural convection

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Performance Analysis of Cooling Wall of Supercritical CO_(2) Coal-Fired Plants

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Journal of Thermal Science 2022年第6期31卷 1881-1890页

作者： WANG Yanjuan YU Binhui GAO Shuo LIU Qibin XU Jinliang The Beijing Key Laboratory of Multiphase Flow and Heat Transfer North China Electric Power UniversityBeijing 102206China Institute of Engineering Thermophysics Chinese Academy of SciencesBeijing 100190China University of Chinese Academy of Sciences Beijing 100049China

Using supercritical CO_(2)(S-CO_(2)) instead of water steam as heat transfer fluid for coal-fired power plants is another way to further improve the power generation efficiency. In this paper, a multi-field coupling model that integrates fluid flow, heat transfer and thermal stress is proposed to solve the complex problem. The effects of the key operating parameters on the performances of the cooling wall are numerically investigated. More details of the characteristics of fluid dynamics, thermal stress, pressure drop, coupled heat transfer and the whole flow and temperature fields in the S-CO_(2) cooling wall are revealed and discussed. A comparison study is made between the cooling wall tube and waterwall tube. Both temperature and thermal deformations of cooling wall tube are much higher than that of water. Numerical simulation results indicate that inclination angle has little effects on the temperature distribution, while increase of pressure drop is obvious as the inclination angle increases. Increasing tube diameter can effectively reduce both the pressure drop and the temperature of the cooling wall tube. As a result, a new insight is introduced for the design of S-CO_(2) power cycle.

关键词： supercritical CO_(2) cooling wall coal-fired power plant heat transfer

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PROCESS MODELING AND ECONOMIC VIABILITY ANALYSIS OF A power-TO-H2-TO-power SYSTEM: CASE STUDY IN CHINA 37

PROCESS MODELING AND ECONOMIC VIABILITY ANALYSIS OF A POWER-...

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37th International Conference on Efficiency, Cost, Optimization, Simulation and Environmental Impact of Energy Systems, ECOS 2024

作者： Li, Yanxin Dai, Yanbing Han, Xiaoqu Guo, Xuanhua Karellas, Sotirios Yan, Junjie State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong University Xi'an China Qingdao Huaru Energy Technology Company Limited Qingdao China Laboratory of Steam Boilers and Thermal Plants National Technical University of Athens 9 Heroon Polytechniou str. Zografou Greece

ISBN: (纸本)9798331307660

The power sector generates the most significant greenhouse gas emissions in many countries, while renewable energy penetration faces a bottleneck due to its ***, it is imperative to make substantial efforts to promote the penetration of renewable energy sources into the power *** process of hydrogen production with renewable energy sources is becoming increasingly economical as the cost of renewable energy sources, particularly onshore wind, has fallen *** the present work, a power-to-H2-to-power system (PHPS) combining onshore wind power was proposed as a solution for high penetration of renewable energy, which incorporates a large-scale alkaline water electrolyzer, and a gas turbine.A techno-economic study based on NOVO PRO© and GT PRO was carried out and applied to cases in Shaanxi, *** performance and operational characteristics of two types of PHPS with different hydrogen storage methods, PHPS/Tank and PHPS/Cavern, were *** is indicated that when 30% of the fuel of the gas turbine was replaced by hydrogen, the levelized cost of energy (LCOE) of the PHPS/Cavern was 0.0498 €/kWh with an internal rate of return (IRR) of 6.41%, therefore, PHPS/Cavern was economically feasible in ***, the renewable energy utilization and carbon reduction benefits of the PHPS were *** surplus electricity (curtailed electricity) and carbon emissions of the PHPS/Cavern can be decreased by 52% and 12%, respectively, compared to those of PHPS without hydrogen as the energy *** performance of PHPS with different hydrogen substitution ratios was *** analysis was further conducted to investigate the influence of key parameters on the system performance, including wind modules investment, electrolyzer investment, transport distance, and electricity ***, under the future scenarios in China in 2050, the LCOE of PHPS/Cavern can be reduced by 15% as well as the IRR increased by 66%.The result

关键词： Hydrogen storage

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Regulation on polymerization degree and surface feature in graphitic carbon nitride towards efficient photocatalytic H2 evolution under visible-light irradiation

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Journal of Materials Science & Technology 2022年第3期98卷 160-168页

作者： Cheng Cheng Chung-Li Dong Jinwen Shi Liuhao Mao Yu-Cheng Huang Xing Kang Shichao Zong Shaohua Shen International Research Center for Renewable Energy(IRCRE) State Key Laboratory of Multiphase Flow in Power Engineering(MFPE)Xi'an Jiaotong University(XJTU)28 West Xianning RoadXi’an 710049China Department of Physics Tamkang University151 Yingzhuan RoadTamsui 25137TaiwanChina

A kind of graphitic carbon nitride(TSC-550) with high polymerization degree and improved surface property was prepared by a new precursor of thiosemicarbazide. The sulfur motif and high nitrogen content in thiosemicarbazide promoted the polymerization of thiosemicarbazide to form graphitic carbon nitride framework with high degree of polymerization, which significantly influenced the electronic structure and surface chemical properties. TSC-550 possessed a narrow bandgap of 2.19 eV that facilitated the utilization of visible light, and possessed a less positive charge, acidic surface that resulted in enhanced hydrogen adsorption ability in water solution, which promoted the H;evolution kinetics. In addition, the extended π-conjugated electronic system promoted the separation and migration of photogenerated charge carries in plane of TSC-550 framework, as well as the increasing interlayer C–N interactions in TSC-550 created conductive paths across the layers to tunnel interlayers for rapid electron transportation. As a result, TSC-550 nanosheets showed excellent photocatalytic H;production activity,the AQY achieved 36.4% at 425 nm.

关键词： Degree of polymerization Graphitic carbon nitride Photocatalysis Solar energy Hydrogen

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Experimental Study on Condensation Heat Transfer Characteristics inside an Inclined Wave-Finned Flat Tube of Direct Air-Cooling System

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Journal of Thermal Science 2021年第2期30卷 432-440页

作者： WANG Haitao TAO Tao MEI Xuesong WANG Haijun GU Hongfang State Key Laboratory for Manufacturing Systems Engineering Xi'an Jiaotong UniversityXi'an 710049China Shaanxi Key Laboratory of Intelligent Robots School of Mechanical EngineeringXi'an Jiaotong UniversityXi'an 710049China State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong UniversityXi'an 710049China

In this paper,the condensation heat transfer characteristics of parallel flow and counter flow inside an inclined wave-finned flat tube is investigated *** condensation heat transfer coefficients are analyzed based on the experimental *** of experiments show that condensation heat transfer coefficient decreases as the temperature difference Δt=ts-tw increases and mass flow rate *** parallel flow has a similar development with the counter flow,and the condensation heat transfer coefficient of counter flow is less than that of parallel flow under the same air cooling *** addition,condensation heat transfer coefficient correlations are also obtained under experimental *** calculations agree well with the measured data and the agreement is seen to be within ±4% for the parallel flow and ±5% for the counter flow.

关键词： condensation heat transfer wave-finned fiat tube modified model parallel flow counter flow

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Study on boiling heat transfer mechanism based on microlayer evaporation theory 6

Study on boiling heat transfer mechanism based on microlayer...

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6th International Conference on Fluid Mechanics and Industrial Applications, FMIA 2022

作者： Dong, Wu-Han Gao, Ming Shen, Zhong-Xiang Zhang, Li-Xin Shanghai Key Laboratory of Multiphase Flow and Heat Transfer in Power Engineering School of Energy and Power Engineering University of Shanghai for Science and Technology Shanghai200093 China

Based on dynamic microlayer evaporation model. Heat transfer mechanism of nuclear boiling and microlayer thickness under single bubble on heated surface. It has a lot to do with the temperature of the wall. Therefore, this paper studies the mechanism of bubble microlayer and makes comparative analysis with its experiments. It is helpful to master nuclear boiling heat transfer more comprehensively. In the study of individual bubble microlayer thickness. The effects of time and radius on wall temperature are considered in this paper. The theoretical formula of initial thickness of microlayer is deduced. The theoretical formula is compared with the experimental data of microlayer evaporation under the nucleation bubble. It was found that the experimental data fell within ±25% of the formula range. It is consistent with the previous experimental research. © Published under licence by IOP Publishing Ltd.

关键词： Evaporation

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A n-Si/CoOx/Ni:CoOOH photoanode producing 600 mV photovoltage for efficient photoelectrochemical water splitting

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Science China Materials 2022年第12期65卷 3442-3451页

作者： Zhuocheng Yin Yuchuan Shi Shaohua Shen International Research Center for Renewable Energy State Key Laboratory of Multiphase Flow in Power EngineeringXi’an Jiaotong UniversityXi’an 710049China

n-Si,believed as a promising photoanode candidate,has suffered from sluggish oxygen evolution reaction(OER)kinetics and poor chemical stability when exposed to aqueous ***,CoO_(x)/Ni:CoOOH bilayers were successfully deposited on n-Si substrate by atomic layer-deposition(ALD)and photoassisted electrochemical deposition(PED)for stabilizing and catalyzing photoelectrochemical(PEC)water *** comparison to the n-Si/CoO_(x)photoanode as reference,the prepared n-Si/CoO_(x)/Ni:CoOOH photoanode upon the optimized PED process presents a much improved PEC performance for water splitting,with the onset potential cathodically shifted to~1.03 V *** hydrogen electrode(RHE)and the photocurrent density much increased to 20 mA cm^(−2)at 1.23 V *** is revealed that the introduction of Ni dopants increases the work functions of the deposited Ni:CoOOH overlayers,which gives rise to the upward band bending weakened at the n-Si/CoO_(x)/Ni:CoOOH cascading interface while strengthened at the Ni:CoOOH/electrolyte interface(with the band bending shifted from downward to upward),contributing to the decreased and the increased driving forces for charge transfer at the interfaces,***,the balanced driving forces at the interfaces would endow the n-Si/CoO_(x)/Ni:CoOOH photoanode with the best PEC ***,PED has been evidenced superior to ED to dope Ni into CoOOH with the formed overlayer effectively catalyzing and stabilizing PEC water splitting.

关键词： n-Si photoanode work function photoelectrochemical water splitting

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Numerical Study on Influence of Platen Super-Heaters on Heat Deviation in a 600 MW Tangentially Fired Pulverized-Coal Boiler 9th

Numerical Study on Influence of Platen Super-Heaters on Heat...

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9th International Symposium on Coal Combustion, ISCC 2019

作者： Chen, Kai Zhang, Yan Deng, Lei Che, Defu School of Mechanic Engineering Xijing University Xi’an710123 China State Key Laboratory of Multiphase Flow in Power Engineering Xi’an Jiaotong University Xi’an710049 China

ISBN: (纸本)9789811616563

In order to investigate effects of platen super-heaters on the heat deviation in the cross-over pass, numerical simulation of a 600 MW tangentially fired pulverized-coal boiler has been studied. Two cases, building super-heaters or not, were established by FLUENT software in this study. Numerical results agree well with measured data of the utility boiler. Results show platen super-heaters break symmetry of velocity distribution at the furnace outlet. The position where peak temperature occurs is affected by platen super-heaters, while the position where peak velocity occurs is not. Platen super-heaters slightly reduce the temperature deviation at the furnace outlet, and enhances the velocity deviation at the furnace outlet. For this boiler, the velocity deviation is the main reason for the heat deviation in the cross-over pass. The simulation results in this study can provide reference for optimization of temperature deviation and velocity deviation in tangentially fired pulverized-coal boiler. © 2022, Tsinghua University Press.

关键词： Furnaces

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