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Wall-to-bed heat transfer in supercritical water fluidized bed using CFD-DEM

Particuology 2021年第3期19卷 113-123页

作者： Tianning Zhang Youjun Lu State Key Laboratory of Multiphase Flow in Power Engineering(SKLMFPE) Xi’an Jiaotong UniversityXi’anShaanxi 710049PR China

Supercritical water fluidized bed(SCWFB)reactors are designed to gasify biomass or coal with high *** this paper,the wall-to-bed heat transfer characteristics in SCWFB are studied using the computational fluid dynamics and discrete element method(CFD-DEM)coupled with a constant heat flux *** different methods are considered to deal with the multiphase heat flux boundary in CFD-DEM because there is currently no single widely accepted ***’s method predicts a more accurate wall-to-bed heat transfer coefficient in SCWFB than Lattanzi’s method according to comparisons of the simulation results with an empirical *** influences of temperature,pressure,velocity,and the solid phase properties,such as the particle diameter,particle heat capacity,particle thermal conductivity,and particle density,on the SCWFB wall-to-bed heat transfer characteristics are studied based on Zhang’s *** simulation results help reveal the SCWFB heat transfer characteristics.

关键词： Supercritical water Fluidized bed Heat transfer DEM-CFD Constant heat flux

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Technological innovations on direct carbon mitigation by ordered energy conversion and full resource utilization

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Carbon Neutrality 2022年第1期1卷 598-619页

作者： Liejin Guo Zhisong Ou Ya Liu Zhiwei Ge Hui Jin Guobiao Ou Mengmeng Song Zihao Jiao Wenhao Jing State Key Laboratory of Multiphase Flow in Power Engineering Xi’an Jiaotong UniversityNo.28Xianning West RoadXi’an 710049People’s Republic of China

Coal consumption leads to over 15 billion tons of global CO_(2) emissions annually,which will continue at a considerable intensity in the foreseeable *** remove the huge amount of CO_(2),a practically feasible way of direct carbon mitigation,instead of capturing that from dilute tail gases,should be developed;as intended,we developed two innovative supporting technologies,of which the status,strengths,applications,and perspective are discussed in this *** is supercritical water gasification-based coal/biomass utilization technology,which orderly converts chemical energy of coal and low-grade heat into hydrogen energy,and can achieve poly-generation of steam,heat,hydrogen,power,pure CO_(2),and *** other one is the renewables-powered CO_(2) reduction techniques,which uses CO_(2) as the resource for carbon-based fuel *** combining the above two technical loops,one can achieve a full resource utilization and zero CO_(2) emission,making it a practically feasible way for China and global countries to achieve carbon neutrality while creating substantial domestic benefits of economic growth,competitiveness,well-beings,and new industries.

关键词： Carbon neutrality Coal utilization Direct carbon mitigation Supercritical water gasification Renewable energy CO_(2)reduction

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氧化铁光阳极界面内建电场调控强化光生电荷空间分离

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Science China Materials 2023年第2期66卷 603-613页

作者：卯连连邓豪李明涛沈少华 International Research Center for Renewable Energy State Key Laboratory of Multiphase Flow in Power EngineeringXi’an Jiaotong UniversityXi’an 710049China

为了缓解氧化铁光阳极内部和表面的电荷复合,本文引入了一种界面电荷调控策略,利用界面内建电场(IEF)促进电荷的空间分离.水热生长的钛掺杂氧化铁(Hem)纳米棒通过简单的两步浸渍涂层过程,以石墨相氮化碳(g-C_(3)N_(4))和小的三氧化钼(Mo... 详细信息

为了缓解氧化铁光阳极内部和表面的电荷复合,本文引入了一种界面电荷调控策略,利用界面内建电场(IEF)促进电荷的空间分离.水热生长的钛掺杂氧化铁(Hem)纳米棒通过简单的两步浸渍涂层过程,以石墨相氮化碳(g-C_(3)N_(4))和小的三氧化钼(MoO_(3))团簇进行修饰.与原始的Hem相比,得到的Hem/C_(3)N_(4)/MoO_(3)表现出显著增强的光电化学分解水性能,相对于可逆氢电极,在1.23 V时,光阳极电流密度从0.3 mA cm^(-2)显著提高到1.6 mA cm^(-2),入射光子-电流转换效率在300 nm时达到18.4%.结果表明,在Hem/C_(3)N_(4)/MoO_(3)异质结中引入IEF是通过调控界面电荷特性实现的,此界面电荷特性是由Hem/C_(3)N_(4)界面的TypeⅡ能带排列和光阳极表面增强的能带弯曲所引起的,IEF能显著促进电荷的空间分离.研究这一界面电荷调控过程能为基于氧化铁的光阳极和其他半导体器件提供一种简单有效的策略,通过缓解载流子传输动力学的瓶颈,促进电荷的空间分离,实现高效的太阳能转换.

关键词：太阳能转换阳极电流密度半导体器件能带弯曲入射光子石墨相氮化碳载流子传输氢电极

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Data-Driven Surrogate Model for the Dynamic Characteristics of Supercritical Units

Data-Driven Surrogate Model for the Dynamic Characteristics ...

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2024 Boao New Power System International Forum - Power System and New Energy Technology Innovation Forum, NPSIF 2024

作者： Dong, Shuai Zheng, An Jiang, Junyao Gao, Wei Liu, Ming Huaneng Yimin Coal-Power Co. Ltd. Hulunbuir021130 China State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong University Xi'an710049 China

ISBN: (纸本)9798331504557

Coal-fired power generation units are characterized by large inertia, strong coupling, and high delay, making dynamic characteristic modeling inherently complex and computationally intensive. To address this, this paper utilizes GSE software to explore the dynamic characteristics of supercritical units. Data-driven approaches are then employed to develop surrogate model for these dynamics, comparing neural networks and support vector regression methods in the process. The study indicates that the surrogate model achieves a relative prediction error of less than 1% for live steam temperature, reheater steam outlet temperature, and power output. For live steam pressure and reheater steam outlet pressure, the model maintains a relative error within 10%. © 2024 IEEE.

关键词： Support vector regression

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利用三元合金保护和催化的硅光阳极与廉价硅太阳能电池相结合实现12.0%的太阳能制氢效率

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Engineering 2023年第6期25卷 128-137,M0006页

作者：何凌云洪欣王亦清邢众航耿嘉峰郭鹏慧苏进展沈少华 International Research Center for Renewable Energy State Key Laboratory of Multiphase Flow in Power EngineeringXi’an Jiaotong UniversityXi’an 710049China

n型硅(n-Si)表面在水溶液中容易被氧化和钝化,导致其在光电化学(PEC)分解水的析氧反应(OER)动力学缓慢。本工作通过欠电位沉积成功地在p^(+)n-Si基底上电沉积了三金属Ni_(0.9)Fe_(0.05)Co_(0.05)保护层。制备的Ni_(0.9)Fe_(0.05)Co_(0.0... 详细信息

n型硅(n-Si)表面在水溶液中容易被氧化和钝化,导致其在光电化学(PEC)分解水的析氧反应(OER)动力学缓慢。本工作通过欠电位沉积成功地在p^(+)n-Si基底上电沉积了三金属Ni_(0.9)Fe_(0.05)Co_(0.05)保护层。制备的Ni_(0.9)Fe_(0.05)Co_(0.05)/p^(+)n-Si光阳极具有优异的稳定性和PEC水氧化活性,具有相对低的OER起始电位(相对于可逆氢电极电势(RHE)仅为0.938 V),并且在1.23 V ***电位时具有较高的光电流密度(33.1 m A·cm^(-2)),显著优于Ni/p^(+)n-Si光阳极。工作证明了Fe在Ni层的掺杂会在Ni_(0.9)Fe_(0.05)Co_(0.05)/p^(+)n-Si界面处产生较大的能带弯曲,促进界面电荷分离。此外,Co的加入会产生丰富的Ni^(3+)和氧空位(Ov),作为活性位点可以加速OER动力学过程,协同促进PEC过程中的水氧化的活性。令人鼓舞的是,通过将Ni_(0.9)Fe_(0.05)Co_(0.05)/p^(+)n-Si光阳极连接到廉价的硅太阳能电池上,所制备的集成光伏/PEC(PV/PEC)器件实现了无偏压下高达12.0%的太阳制氢能量转换效率。这项工作提供了一种简单的方法来设计高效、稳定的n-Si基光阳极,并对其构效关系有了深刻的理解;这种方法制备的材料在集成低成本PV/PEC器件用于无辅助太阳能驱动水分解方面具有巨大的潜力。

关键词：欠电位沉积电极电势阳极连接硅太阳能电池能量转换效率太阳能制氢能带弯曲光阳极

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Influence of active and passive equipment for advanced pressurized water reactor on thermal hydraulic and source term behavior in severe accidents

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Energy Storage and Saving 2023年第1期2卷 392-402页

作者： Jishen Li Bin Zhang School of Nuclear Science and Technology Xi’an Jiaotong UniversityXi’an710049China State Key Laboratory of Multiphase Flow in Power Engineering Xi’an Jiaotong UniversityXi’an710049China

Extensive studies have been carried out on the behavior of core degradation and fission products of common pressurized water reactors(PWRs).However,few of them have investigated the relationship between thermal hydraulic and fission product behavior in advanced passive *** to the impact of thermal hydraulic be-haviors in different accident sequences on the release and transportation of fission products,an integrated severe accident analysis(ISAA)code with highly coupled thermal hydraulic and source term calculations is required to simultaneously analyze thermal hydraulic and source term *** advanced passive PWRs,important safety systems that may affect the behavior of the core and fission products should be *** is therefore necessary to simulate the thermal hydraulic and fission product behavior of advanced passive *** this study,the ISAA code is adopted to simulate the occurrence of a hypothetical double ended cold leg LBLOCA of HPR1000 in three scenarios of equipment *** results show that the high-temperature fuel rods and cladding ma-terials exhibit delayed failure at the lower position of the active core,whereas earlier failure at higher position during the *** and passive equipment affects fuel temperature,the oxidation conditions of the fuel,the interaction of fission products and structural materials,and the state of the fuel,thereby affecting the release of fission products in the ***1000 only relies on passive equipment to relieve the core degradation in severe accidents,realize the in-vessel retention of melt,and eliminate the ex-vessel release possibility of fission *** is hoped that the results can provide references for HPR1000 to formulate the severe accident management guidelines(SAMG).

关键词： Nuclear safety LBLOCA Severe accident Source term HPR1000 Active and passive equipment

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Assisting effect of Al_(2)O_(3) on MnO_(x) for NO catalytic oxidation

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Green Energy & Environment 2021年第6期6卷 903-909页

作者： Denghui Wang Hui Li Qi Yao Shien Hui Yanqing Niu State Key Laboratory of Multiphase Flow in Power Engineering School of Energy and Power EngineeringXi'an Jiaotong UniversityXi'an710049China

Various Mn-based catalysts for NO oxidation were prepared using MnO_(x)as active compound,while Ti O_(2)and Al_(2)O_(3)were adopted as catalyst *** performance of the catalysts was tested to study the effect of support on Mn-based catalyst *** of the catalysts followed as Mn_(0.4)/Al>Mn_(0.2)/Al>Mn_(0.4)/Ti>Mn_(0.2)/Ti>MnO_(x)>Al_(2)O_(3)on the whole,indicating the synergism of MnO_(x)and Al_(2)O_(3)for NO catalytic *** were analyzed according to characterization *** oxygen on catalyst rather than lattice oxygen was detected as the active oxidizer for NO *** catalyst support,Al_(2)O_(3)provided more sites to carry surface adsorbed oxygen than TiO_(2),resulting in the presence of more active oxygen on Mn O_(x)/Al_(2)O_(3)than on MnO_(x)/TiO_(2).Moreover,MnO_(x)/Al_(2)O_(3)possessed high surface area and pore volume,which greatly benefited the adsorption of NO on catalyst and further favored the oxidation of NO by active *** these advantages helped Mn_(0.4)/Al exhibited the best catalytic efficiency.

关键词： NO catalytic oxidation MnO_(x)/Al_(2)O_(3) NO_(2) Active oxygen

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Concurrently Boosting Activity and Stability of Oxygen Reduction Reaction Catalysts via Judiciously Crafting Fe-Mn Dual Atoms for Fuel Cells

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Nano-Micro Letters 2025年第4期17卷 275-289页

作者： Lei Zhang Yuchen Dong Lubing Li Yuchuan Shi Yan Zhang Liting Wei Chung-Li Dong Zhiqun Lin Jinzhan Su International Research Center for Renewable Energy State Key Laboratory of Multiphase Flow in Power EngineeringXi’an Jiaotong UniversityXi’an 710049People’s Republic of China Department of Physics Tamkang UniversityNew Taipei CityTaiwan 25137People’s Republic of China Department of Chemical and Biomolecular Engineering National University of SingaporeEngineering Drive 4Singapore 117585Singapore

The ability to unlock the interplay between the activity and stability of oxygen reduction reaction(ORR)represents an important endeavor toward creating robust ORR catalysts for efficient fuel ***,we report an effective strategy to concurrent enhance the activity and stability of ORR catalysts via constructing atomically dispersed Fe-Mn dualmetal sites on N-doped carbon(denoted(FeMn-DA)-N-C)for both anion-exchange membrane fuel cells(AEMFC)and proton exchange membrane fuel cells(PEMFC).The(FeMn-DA)-N-C catalysts possess ample dual-metal atoms consisting of adjacent Fe-N_(4)and Mn-N_(4)sites on the carbon surface,yielded via a facile doping-adsorption-pyrolysis *** introduction of Mn carries several advantageous attributes:increasing the number of active sites,effectively anchoring Fe due to effective electron transfer to Mn(revealed by X-ray absorption spectroscopy and density-functional theory(DFT),thus preventing the aggregation of Fe),and effectively circumventing the occurrence of Fenton reaction,thus reducing the consumption of ***(FeMn-DA)-N-C catalysts showcase half-wave potentials of 0.92 and 0.82 V in 0.1 M KOH and 0.1 M HClO_(4),respectively,as well as outstanding *** manifested by DFT calculations,the introduction of Mn affects the electronic structure of Fe,down-shifts the d-band Fe active center,accelerates the desorption of OH groups,and creates higher limiting *** AEMFC and PEMFC with(FeMn-DA)-N-C as the cathode catalyst display high power densities of 1060 and 746 mW cm^(-2),respectively,underscoring their promising potential for practical *** study highlights the robustness of designing Fe-containing dual-atom ORR catalysts to promote both activity and stability for energy conversion and storage materials and devices.

关键词： Doping-adsorption-pyrolysis Dual-atom catalysts Oxygen reduction reaction Fuel cells

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Unconventional energetics of small vacancy clusters in BCC high-entropy alloy Nb_(0.75)ZrTiV_(0.5)

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Journal of Materials Science & Technology 2023年第15期146卷 61-71页

作者： Tan Shi Xi Qiu Yundi Zhou Sixin Lyu Jing Li Dan Sun Qing Peng Yong Xin Chenyang Lu School of Nuclear Science and Technology Xi’an Jiaotong UniversityXi’an 710049China Nuclear Power Institute of China Chengdu 610213China State Key Laboratory of Nonlinear Mechanics Institute of MechanicsChinese Academy of SciencesBeijing 100190China School of Engineering Sciences University of Chinese Academy of SciencesBeijing 100049China State Key Laboratory of Multiphase Flow in Power Engineering Xi’an Jiaotong UniversityXi’an 710049China

The stability of small vacancy clusters including divacancy,trivacancy and tetravacancy has been studied in body-centered cubic high-entropy alloy Nb_(0.75)ZrTiV_(0.5) in structures of random solid solution and short-range order by first-principles calculations and molecular dynamics *** from conventional body-centered cubic metals,the tightly bound configurations have a lower structural stability and are not preferred energetically in the studied high-entropy *** of vacancy configurations leads to vacancy-atom exchanges that favor less compact *** formation energy of small vacancy clusters is much smaller than its constituent elements of Nb and V due to the large structural adjustment induced by severe local lattice *** difference in local lattice distortion and elemental arrangement in the vacancy neighborhood leads to significant site-to-site variation in vacancy cluster energy and *** formation energy has a strong correlation with the local energy state of the vacancy configuration and the extent of structural *** to random solid solution,the structure of short-range order has a higher stability for the most compact cluster configurations and tends to have higher vacancy cluster formation *** to classical molecular dynamics simulations of cluster diffusion at high temperature,the studied high-entropy alloy has a higher probability of cluster dissociation compared to Nb and *** unconventional energetics of small vacancy clusters is expected to have a profound impact on their generation,diffusion,dissociation,coalescence,as well as the defect microstructure evolution during irradiation.

关键词： Refractory high-entropy alloys Small vacancy clusters First-principles calculations Defect energetics Radiation defect evolution

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Investigation on the Parallel Computing Technique Using on the Numerical Simulation of Carbon Free Fuel 4

Investigation on the Parallel Computing Technique Using on t...

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4th International Conference on Information Science, Parallel and Distributed Systems, ISPDS 2023

作者： Wang, Weibin Wei, Xutao Xi'an Fanyi University Department of Computer Science Xi'an China Xi'an Jiaotong University State Key Laboratory of Multiphase Flow in Power Engineering Xi'an China

ISBN: (纸本)9798350337181

The numerical simulation of the turbulent combustion is identified as one of the most promising methods on the designs of the combustion devices, for example: the internal combustion engine and gas turbine. This mainly depends on the development of parallel computing technique. However, the computational efficiency for different cases on different compute nodes and number of cores still needs to be studied. On the other hand, due to the requirements from the aim of peaking carbon dioxide emissions before 2030 and achieving carbon neutrality before 2060, modern energy system is requesting low carbon or carbon free fuels, such as ammonia (NH3). Therefore, the simulations of ammonia/air flame were performed in present investigation. The comparison between simulation cases on different compute nodes and number of cores illustrates that different cases requires different number of cores to achieve the best computational efficiency. The computational efficiency of each compute nodes are dissimilar, which can decrease the efficiency. Meanwhile, the methods in present study can predict the ammonia/air flames. The initial condition of velocity fluctuation is necessary for simulating turbulent flame. The wrinkles of the flames can be well predicted by the velocity fluctuation initial boundary condition. © 2023 IEEE.

关键词： Computational efficiency

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