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International Journal of Hydrogen Energy 2025年 145卷 345-357页

作者： Yanxin Li Xiaoqu Han Yiming Zhang Nikolaos Skordoulias Xuanhua Guo Junjie Yan Sotirios Karellas Emmanuel Kakaras State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong University Xi'an 710049 China Laboratory of Thermal Processes National Technical University of Athens Athens 15780 Greece Qingdao Huaru Energy Technology Company Limited Qingdao 266071 China Mitsubishi Hitachi Power Systems Europe GmbH Schifferstraße 80 Duisburg 47059 Germany

The high percentage of renewable energy penetration poses volatility and intermittency challenges, making it imperative to explore pathways for large-scale green hydrogen production and utilization. In the present work, a novel power-to-H 2 -to-power (PtH2tP) system is proposed for onshore wind accommodation, incorporating hydrogen mixed gas turbines (HMGTs). An innovative methodology integrating economic and carbon emissions assessment with optimal dispatch is developed, in which the HMGT off-design operational characteristics and policy compensation for green hydrogen are considered. A case study in China demonstrates the feasibility of the PtH2tP system in achieving flexible energy conversion and hydrogen self-sufficiency. Particularly, a levelized cost of electricity of 0.0537 €/kWh and carbon emissions of 0.29 kg CO 2 eq/kWh are observed. The fuel consumption of HMGTs and purchased grid electricity are significant contributors to carbon emissions. A comprehensive sensitivity analysis indicates an optimal hydrogen substitution ratio of 31% as the threshold for balancing economics and environmental benefits.

关键词： Windmill

Experiments and Predictions for Severe Slugging of Gas-Liquid Two-Phase flows in a Long-Distance Pipeline-Riser System

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SSRN 2023年

作者： Chang, Yingjie Xu, Qiang Zou, Suifeng Zhao, Xiangyuan Wu, Quanhong Wang, Yechun Thévenin, Dominique Guo, Liejin State Key Laboratory of Multiphase Flow in Power Engineering Xi’an Jiaotong University Xi’an710049 China Laboratory of Fluid Dynamics and Technical Flows Otto-von-Guericke-Universität Magdeburg Magdeburg39106 Germany

Experiments concerning the flow regimes observed in gas-liquid two-phase flows in a long pipeline-riser system have been carried out and are analyzed in this paper. The test loop with 0.075 m inner diameter consists of a 314 m horizontal pipeline, followed by a 25 m downward-inclined pipe, and finally a 21.5 m riser pipe. An industrial-scale global flow regime map is derived from differential pressure measurements in the riser. Electrical capacitance volume tomography installed in the horizontal section was used to reconstruct the phase interface in order to calculate the average gas void fraction (GVF). An appropriate model for this system is selected by comparing the experimental GVF with different, widely used models. The occurrence of a severe slugging flow (SS) can be well predicted using the model involving additional corrections (taking into account pipeline length, accurate GVF results, and gas density). This study supports the development of a suitable SS prediction model enabling safe design, operation, and control of practical systems. © 2023, The Authors. All rights reserved.

关键词： Pipelines

A study on free radical behaviors and reactions in supercritical water using quantum chemical simulation

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Journal of Molecular Liquids 2025年 419卷

作者： Ding, Weijing Takahashi, Osamu Wang, Junying Jin, Hui School of Transportation and Vehicle Engineering Shandong University of Technology Shandong Zi'bo255000 China State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong University Shaanxi Xi'an710049 China of Advanced Science and Engineering Hiroshima University Higashi-Hiroshima739-8526 Japan

Supercritical water (SCW) gasification is one of clean and efficient utilization way of biomass, other organic matters or coal for hydrogen production, in which radical reactions studies in SCW are limited but crucial. Density-functional tight-binding (DFTB) molecular simulation is one of efficient and convenient approaches to investigate these microscopic processes. Therefore, free radical reactions in severe SCW environment were investigated via DFTB calculations in this work. The results showed that the order of the free radicals containing bond cleavages reacted in SCW environment was ·OH, ·CH, ·CH2, ·HO2, ·CH3 and ·C6H5 under the same conditions. The reaction processes of different radicals in SCW were obtained. ·H was the most active free radical of reactions. This work is expected to understand the properties of free radicals in SCW better and explore intrinsic reaction mechanisms, which may provide a theoretical support for accomplishing efficient and low-carbon complete SCW gasification for hydrogen production. © 2024 Elsevier B.V.

关键词： Free radical Gasification Hydrogen production Reaction Supercritical Water (SCW)

Numerical Investigation on the Thermal-Hydraulic Performance of a Cryogenic Printed Circuit Heat Exchanger for Liquid Air Energy Storage

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SSRN 2022年

作者： Yu, Pengfei Liu, Hu Xue, Jingwen Zhang, Yankang Che, Defu State Key Laboratory of Multiphase Flow in Power Engineering School of Energy and Power Engineering Xi'an Jiaotong University Xi'An710049 China

The liquid air energy storage integrated with liquefied natural gas regasification is a promising large-scale storage method, but its development is limited by the lack of the thermal-hydraulic data of the cryogenic printed circuit heat exchanger. In this paper, a reduced numerical model for conjugate heat transfer was established, and the effect of the inclined angle (0°, 15°, 30°, 45°, and 60°) was investigated. The minimum internal temperature approach for optimal system operation is approximately 6 K, located in the middle of the heat exchanger. The nature of local flow and heat transfer was analyzed by quantifying the vortex strength and visualizing the vortex core. Results indicate that the evolution of Dean vortices plays a crucial role in heat transfer augmentation. The secondary flow caused by the elbow forces the velocity and temperature cores to strike the windward side periodically, which disturbs the boundary layer and enhances the fluid mixing. Entropy production analysis shows that the thermal entropy generation has a dominant share of the irreversibility. The zigzag channel with an inclined angle of 45° yields the best comprehensive performance since the irreversibility is reduced by augmenting the heat transfer. © 2022, The Authors. All rights reserved.

关键词： Air

Investigation of the Solar-Driven Chemical Looping Methane Dry Reforming on Rh-Doped LaCeO3.5 Oxygen Carrier

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SSRN 2024年

作者： Li, Peng Gai, Zhongrui Zhang, Jinrui Rao, Qiong Tang, Sanli Shen, Yuanhui Pan, Ying Jin, Hongguang Institute of Engineering Thermophysics Chinese Academy of Sciences Beijing100190 China State Key Laboratory of Multiphase Flow in Power Engineering Xi’an Jiaotong University Xi’an710049 China University of Chinese Academy of Sciences Beijing100049 China

The feasibility of a solar-driven chemical looping dry reforming of methane (DRM) process, which converts solar energy and methane into syngas via a looping material oxygen carrier is investigated experimentally. Thermogravimetric analysis (TGA) experiments were firstly carried out to verify the effect of the Rh-doped LaCeO3.5 which were synthesized via modified Pechini method and incipient wetness method and the result shows that Rh greatly improved the reaction kinetics. Photo-TGA experiments were conducted to evaluate the light effect in chemical looping DRM. Under the light condition, the Rh-doped LaCeO3.5 shows higher methane conversion, oxygen extraction rate and CO selectivity compared with the undoped one, decreasing the apparent activation energy of the reaction at the same time. Insights obtained from the UV-Vis spectroscopy verified that the surface Rh under the light could promote the activation of surface methane species and increase the light absorbance. Meanwhile, the FEM methods were used to obtain the distributions of the temperature fields of the photo-TGA reactor through the calculation of the coupling of the fluid, reaction and temperature fields. In this way, the conversion mechanism of the solar, heating and chemical energy was illustrated and furthermore, the calculated surface reaction rate and the variation tendency of the outlet-gas were consistent with the experimental results. Through the integration of solar energy, a high methane to solar fuel conversion efficiency could be achieved. The proposed process has the potential to produce solar fuels at high efficiency with reduced carbon footprint. © 2024, The Authors. All rights reserved.

关键词： Methane

The Performance Study on Hydrogen Production From Medium Temperature Methane Chemical Looping Steam Reforming Using Lithium-based Absorbent

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Kung Cheng Je Wu Li Hsueh Pao/Journal of Engineering Thermophysics 2025年第5期46卷 1401-1408页

作者： Wang, Xuyun Li, Yang Gai, Zhongrui Rao, Qiong Liu, Mingkai Pan, Ying School of Engineering Science University of Science and Technology of China Hefei230027 China Institute of Engineering Thermophysics Chinese Academy of Sciences Beijing100190 China University of Chinese Academy of Sciences Beijing100049 China International Research Center for Renewable Energy State Key Laboratory of Multiphase Flow in Power Engineering Xi’an Jiaotong University Xi’an710049 China

Lithium silicate serves as a novel CO2 absorbent with moderate absorptionregeneration temperature range (500∼700◦C) and excellent cycling stability. In this study, Li2CO3 was selected as the precursor for the preparation of lithium silicate. Additionally, a eutectic co-doping method with potassium elements was employed to enhance its reactivity. Using extrusion-spheronization, we successfully produced absorbent particles with high mechanical strength and cycling stability. The effects of absorption-regeneration temperature, CO2 concentration and particle diameter on the performance of absorbent particles have been studied in detail. Furthermore, mixed with NiO oxygen carriers, sorption-enhanced chemical looping reforming (SE-CLR) experiments were conducted at the range of 500∼650◦C for hydrogen production and in situ CO2 capture factors such as reaction temperatures and oxygen carrier to absorbent mass ratios were then investigated The results showcase that at the optimal reaction temperature of 600◦C, the SE-CLR process effectively lowered the reaction temperature by 25◦C, achieving a 13% increase in methane conversion rate and hydrogen purity and CO2 capture rate above 90% were attained. © 2025 Science Press. All rights reserved.

关键词： Silicates

Water Washing of Biomass and Biochar

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SSRN 2022年

作者： Huang, Xiaole Tie, Yuan Jiang, Jiahao Deng, Lei Che, Defu State Key Laboratory of Multiphase Flow in Power Engineering School of Energy and Power Engineering Xi’an Jiaotong University Xi’an710049 China

To investigate the differences of organics composition between leachates of biomass and biochar, four biomass materials and the corresponding biochar are water washed. The distributions of organic compounds in leachates are characterized by GC-MS. Raw and washed biomass, and biomass leachates dried at 333 K are sent for TG/DTG analysis. The results show that considering the content of aromatic hydrocarbons, corn and sorghum stalk are referred to be washed after high-temperature pyrolysis at 303 K, with the value of 11% and 29.95% respectively. Wheat straw and rice husk are proposed to wash directly. Considering the alkanes, cycloalkanes and heterocyclic hydrocarbons contents in leachates, it is proposed to washing low-temperature pyrolyzed biochar. It is recommended to wash biomass directly to inhibit acidic organics release. Washed and raw biomass have similar DTG curves. The combustion stage of dried leachate is more complicated, with one or two peaks during the third stage. The activation energy follows an order of washed biomass > raw biomass > biomass leachate. © 2022, The Authors. All rights reserved.

关键词： Biomass

Water Washing of Biomass and Biochar

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SSRN 2022年

To investigate the differences in organics composition between leachates of biomass and biochar, four biomass materials and the corresponding biochar are water washed. GC-MS is employed to characterize the distributions of organic components in leachates. Raw and washed biomass, and biomass leachates dried at 333 K are sent for TG/DTG analysis. The results show that corn and sorghum stalks should be washed after the high-temperature pyrolysis at 303 K, with aromatic hydrocarbon contents of 11.00% and 29.95%, respectively. It is proposed that wheat straw and rice husk should be washed directly. Considering the contents of alkanes, cycloalkanes, and heterocyclic hydrocarbon in leachates, biomass should be pyrolyzed at a relatively low temperature and then be washed. It is recommended to wash biomass directly to inhibit the acidic organic release. Washed and raw biomass samples have the similar DTG curves. The combustion of dried leachate is more complicated, with one or two peaks during the third stage. The activation energy follows an order of washed biomass > raw biomass > biomass leachate. © 2022, The Authors. All rights reserved.

关键词： Biomass

Recent advancement and future challenges of photothermal catalysis for VOCs elimination:From catalyst design to applications

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Green Energy & Environment 2023年第3期8卷 654-672页

作者： Yang Yang Shenghao Zhao Lifeng Cui Fukun Bi Yining Zhang Ning Liu Yuxin Wang Fudong Liu Chi He Xiaodong Zhang Environment and Low-Carbon Research Center School of Environment and ArchitectureUniversity of Shanghai for Science and TechnologyShanghai 200093China College of Smart Energy Shanghai Jiao Tong UniversityShanghai 200240China Institute of Applied Biotechnology Taizhou Vocation&Technical CollegeTaizhou Zhejiang 318000China Department of Civil Environmentaland Construction EngineeringCatalysis Cluster for Renewable Energy and Chemical Transformations(REACT)NanoScience Technology Center(NSTC)University of Central FloridaOrlandoFL 32816United States State Key Laboratory of Multiphase Flow in Power Engineering School of Energy and Power EngineeringXi'an Jiaotong UniversityXi'anShaanxi 710049China

Photothermal catalysis realizes the synergistic effect of solar energy and thermochemistry,which also has the potential to improve the reaction rate and optimize the *** this review,the research progress of photothermal catalytic removal of volatile organic compounds(VOCs)by nano-catalysts in recent years is systematically ***,the fundamentals of photothermal catalysis and the fabrication of catalysts are described,and the design strategy of optimizing photothermal catalysis performance is ***,the performance for VOC degradation with photothermal catalysis is evaluated and compared for the batch and continuous ***,the catalytic mechanism of VOC oxidation is systematically introduced based on experimental and theoretical ***,the future limitations and challenges have been discussed,and potential research directions and priorities are highlighted.A broad view of recent photothermal catalyst fabrication,applications,challenges,and prospects can be systemically provided by this review.

关键词： Photothermal catalysis VOCs Catalyst design Light-driven thermal catalysis Photothermal synergistic effect

Characteristics and Prediction Model of Co-Pyrolysis of Sewage Sludge and Camellia Seed Shell

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SSRN 2022年

作者： Wang, Bo Liu, Yinhe Guan, Yu Feng, Yiwei Pan, Hejitian State Key Laboratory of Multiphase Flow in Power Engineering School of Energy and Power Engineering Xi'an Jiaotong University Xi’an710049 China

Tar is an undesired product in the process of sewage sludge pyrolysis, which affects the normal operation of the equipment. In this paper, the characteristics of co-pyrolysis of sewage sludge and camellia seed shell for tar reduction and syngas production were explored. The content and composition of tar and pyrolysis gas co-pyrolyzed with different proportions of sewage sludge (JAS) and camellia seed shell samples (CSS) were studied. The weight loss characteristics of the samples were studied by thermogravimetric experiment, and the synergistic effects of different stages were analyzed. The performances of back propagation (BP) neural network and particle swarm optimization-back propagation neural network (PSO-BP) in reflecting the nonlinear relationship between temperature, mixing ratio, heating rate and remaining weight were compared. The results show that the tar yield was the lowest when 40JAS60CSS was pyrolyzed, which could alleviate the serious problems caused by the tar. Compared with the JAS single pyrolysis, the co-pyrolysis of JAS and CSS improved the content of PAHs and reduced the content of aliphatic hydrocarbons in the tar. The inhibition and promotion effects of co-pyrolysis would be transformed into each other with the progress of the pyrolysis, and the transformations were concentrated in the S 2 stage where the weight loss of the sample is the largest. The constructed PSO-BP-30 model contained two hidden layers, each with 12 neurons, which accurately reflected the nonlinear relationship between the temperature, mixing ratio, heating rate and residual weight. © 2022, The Authors. All rights reserved.

关键词： Pyrolysis