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Spontaneous photoelectric field-enhancement effect prompts the low cost hierarchical growth of highly ordered heteronanostructures for solar water splitting

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Nano Research 2016年第6期9卷 1561-1569页

作者： Yankuan Wei Jinzhan Su XiaokangWan Liejin Guo Lionel Vayssieres International Research Center for Renewable Energy State Key Laboratory for Multiphase Flow in Power Engineering School of Energy &Power Engineering Xi'an Jiaotong University Xi'an 710049 China

In this study, a potentially universal new strategy is reported for the large-scale, low-cost fabrication of visible-light-active highly ordered heteronanostructures based on the spontaneous photoelectric-field-enhancement effect inherent in pyramidal morphology. The hierarchical vertically oriented arrayed structures comprise an active molecular co-catalyst at the apex of a visible-light-active large band gap semiconductor for low-cost solar water splitting in a neutral aqueous medium without the use of a sacrificial agent.

关键词： bismuth vanadate co-catalysts photocatalysis solar water splitting oxygen evolution

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Integration of Organic Rankine Cycle with Lignite Flue Gas Pre-drying for Waste Heat and Water Recovery from Dryer Exhaust Gas: Thermodynamic and Economic Analysis

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Energy Procedia 2017年 105卷 1614-1621页

作者： Xiaoqu Han Sotirios Karellas Ming Liu Konstantinos Braimakis Weixiong Chen Junjie Yan Emmanuel Kakaras State Key Laboratory of Multiphase Flow in Power Engineering Xi’an Jiaotong University Xi’an 710049 China Laboratory of Steam Boilers and Thermal Plants National Technical University of Athens Athens 15780 Greece

The flue gas pre-drying of lignite produces a moisture rich dryer exhaust gas which can be further cooled to recover the waste heat and water vapor. An environmental friendly power system is investigated in the present work, which integrates the lignite flue gas pre-drying system with an organic Rankine cycle (ORC) to utilize the waste heat to generate power and capture the condensed water. Simulation models of the integrated system are developed, incorporating thermodynamic and economic evaluation indicators. The optimal energy and exergy efficiencies of the ORC system are calculated to be 3.10% and 24.57%, respectively, for an evaporation temperature of 51 °C when R245fa is used as the working fluid. Accordingly, the ORC power output is 3.61 MW and the absolute plant efficiency improvement is 0.27% points. Moreover, 55.17% of the water vapor can be recovered. The economic performance significantly relies on the specific investment cost of ORC and the electricity selling price. Typically, the break-even points of the specific investment cost are 2300 €/kW and 3700 €/kW when electricity selling prices are 0.05 €/kWh and 0.08 €/kWh, respectively.

关键词： Lignite Flue gas pre-drying Waste heat recovery Organic Rankine cycle

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Thermodynamic Optimization of a Double-pressure Organic Rankine Cycle Driven by Geothermal Heat Source

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Energy Procedia 2017年 129卷 591-598页

作者： Qingxuan Sun Yaxiong Wang Ziyang Cheng Jiangfeng Wang Pan Zhao Yiping Dai Institute of Turbomachinery State Key Laboratory of Multiphase Flow in Power Engineering School of Energy and Power Engineering Xi’an Jiaotong University Xi’an 710049 People’s Republic of China

Geothermal energy, as a typical low-temperature heat source, has been exploited for decades to generate electricity. Organic Rankine cycle (ORC) system has a high energy conversion efficiency due to the good performance of organic fluids under the geothermal water temperature. In this study, a double-pressure organic Rankine cycle system driven by geothermal heat source is used to generate electricity. The double-pressure ORC system achieves the cascaded utilization of energy, which can improve the efficiency of energy conversion. Mathematical model is established based on thermodynamic laws, and the overall system performance has been evaluated. A parametric analysis is conducted to examine the effects of some key thermodynamic parameters, namely turbine high-level inlet pressure, turbine low-level inlet pressure, turbine high-level inlet temperature, on the system performance. Parametric optimization is conducted by means of genetic algorithm (GA) to find the maximum system performance. At the same time, the performances of three organic working fluids are examined. Results indicate that R245fa has a better performance among the three organic fluids. The exergy efficiency of overall system exceeds 5.8% under the supply water of 120℃, and it produce more than 800kW electricity with the geothermal water at the mass flow rate of 250t/h. It is also found that the exergy efficiency has peak value under the effect of turbine high-level inlet pressure and turbine low-level inlet pressure. In addition, increasing turbine high-level inlet temperature brings a positive effect to the system performance. Exergy analysis is also conducted and the result shows that the main exergy loss occurs in high-pressure evaporator. By system optimization, the double-pressure organic Rankine cycle has a better performance in utilizing geothermal energy than single-pressure system.

关键词： Geothermal Organic Rankine cycle Double-pressure

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Towards efficient solar-to-hydrogen conversion: Fundamentals and recent progress in copper-based chalcogenide photocathodes

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Nanophotonics 2016年第4期5卷 468-491页

作者： Chen, Yubin Feng, Xiaoyang Liu, Maochang Su, Jinzhan Shen, Shaohua International Research Center for Renewable Energy State Key Laboratory of Multiphase Flow in Power Engineering Xi'An Jiaotong University Shaanxi710049 China

Photoelectrochemical (PEC) water splitting for hydrogen generation has been considered as a promising route to convert and store solar energy into chemical fuels. In terms of its large-scale application, seeking semiconductor photoelectrodes with high efficiency and good stability should be essential. Although an enormous number of materials have been explored for solar water splitting in the last several decades, challenges still remain for the practical application. P-type copper-based chalcogenides, such as Cu(In, Ga)Se2 and Cu2ZnSnS4, have shown impressive performance in photovoltaics due to narrow bandgaps, high absorption coefficients, and good carrier transport properties. The obtained high efficiencies in photovoltaics have promoted the utilization of these materials into the field of PEC water splitting. A comprehensive review on copper-based chalcogenides for solar-to-hydrogen conversion would help advance the research in this expanding area. This review will cover the physicochemical properties of copper-based chalco-genides, developments of various photocathodes, strategies to enhance the PEC activity and stability, introductions of tandem PEC cells, and finally, prospects on their potential for the practical solar-to-hydrogen conversion. We believe this review article can provide some insights of fundamentals and applications of copper-based chalco-genide thin films for PEC water splitting. © 2016 Y. Chen et al.

关键词： Photocathodes

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Correlations of Coal Chemical Properties in China: Quantitative Analysis from Thousands of Data

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Energy Procedia 2017年 105卷 1339-1343页

作者： Chang’an Wang Song Wu Wufeng Chen Qiang Lv Defu Che State Key Laboratory of Multiphase Flow in Power Engineering School of Energy and Power Engineering Xi’an Jiaotong University No 28 Xianning West Road Xi’an 710049 China

Coal chemical properties show conspicuous impacts on its reactivity and thermal conversion. Nevertheless, the quantitative analysis of coal property indice in China is insufficient. Here, we quantitatively analyzed the correlations of various chemical properties of coals from thousands of data. Noteworthy variations were captured with some quantified expressions between coal properties obtained.

关键词： coal property quantitative analysis fuel ratio coal rank energy conversion fossil fuel

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Product-based Carbon Constraint Energy Planning with pinch analysis for sustainable methanol industry in China

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Chemical Engineering Transactions 2017年 61卷 103-108页

作者： Qin, Zhen Tang, Kai Wu, Xiaomei Yu, Yunsong Zhang, Zaoxiao School of Chemical Engineering and Technology Xi'an Jiaotong University Xi'an710049 China State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong University Xi'an710049 China

For the purpose of greenhouse gas control in chemical industries, the industrial structure adjustment and lowcarbon technology retrofit are the alternatives for policymakers and plants to simultaneously meet the energy demand and carbon emission limit. Considering the various technological sources and predictable product demand in methanol production industries, this paper presents the method of Product-based Carbon Constraint Energy Planning (PCEP) combined with improved GM(1,1) model to analyse the practical interaction between energy demand and carbon emission for methanol industry in 2020 in China. The results show that without any emission reduction measures, the total carbon emissions of methanol industry in 2020 would be 4.84 times larger than that of 2011. By enhancing the methanol production of biomass routing and conducting the project of CO2 capture and storage (CCS) in all coal-to-methanol plants, the total carbon emissions would be 36.01 % less than the given carbon constraint. Besides, at least 65 % of coal-to-methanol plants should be retrofitted with CCS on the consideration of the current challenges of biofuel development in order to meet the carbon constraint. The energy structure of China and the inherent property with high carbon content in coal determine that the coal-to-methanol routing contributes the most of methanol supply but also the maximum carbon emissions in the methanol industry, even if policymakers and plants take measures to adjust the industrial structure and retrofit the existing plants with low-carbon technology. Copyright © 2017, AIDIC Servizi S.r.l.

关键词： Chemical industry

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[email protected] 2 O 4 fiber-in-tube mesoporous nanostructure: Formation mechanism and high electrochemical performance as an anode for lithium-ion batteries

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Journal of Alloys and Compounds 2017年 693卷 110-117页

作者： Jianan Wang Guorui Yang Ling Wang Wei Yan Wei Wei Department of Environmental Science and Engineering State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong University Xi'an 710049 China Department of Applied Chemistry School of Science Xi'an Jiaotong University 710049 China

In this paper, [email protected] 2 O 4 with a fiber-in-tube mesoporous nanostructure has been fabricated via a one-step single-spinneret electrospinning technique. This unique nanostructure is made of an outer spinel CoFe 2 O 4 tube and a loose inner fiber composed of the residual carbonaceous materials and metal precursors. The nanostructure's properties, such as morphology, components, structures and thermal stability, are characterized by scanning electron microscopy (SEM), transmission electron microscopy (TEM), X-Ray diffraction (XRD), thermogravimetric analysis (TGA), Brunauer, Emmett and Teller type specific area (S BET ) determination, X-ray photoelectron spectroscopy (XPS) and inductively coupled plasma-atomic emission spectrometry (ICP-AES). As an anode material for lithium-ion batteries, the [email protected] 2 O 4 composite (6.25 wt% carbon content) exhibits a high reversible capacity of 740 mA h g −1 after over 200 cycles at the current density of 200 mA g −1 with excellent cycling stability, which is attributed to its one dimensional continuous fiber-in-tube mesoporous morphology, as well as its stable structure benefiting from the existence of carbonaceous yolk. In addition, pure CoFe 2 O 4 nanotubes can also be obtained by sequentially agitating this product in water, which provides more potential applications of CoFe 2 O 4 .

关键词： Electrospinning [email protected] 2 O 4 Fiber-in-tube Mesoporous nanostructure Li-ion batteries

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Investigation on Correlations between Chemical Properties of High-alkali Solid Fuels

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Energy Procedia 2017年 142卷 1040-1044页

作者： Chang’an Wang Xin Zhu Jun Song Xuan Liu Qiang Lv Defu Che State Key Laboratory of Multiphase Flow in Power Engineering School of Energy and Power Engineering Xi’an Jiaotong University Xi’an 710049 China Ningxia Electric Power Research Institute Yinchuan 750002 China

The ash-related issues due to the high-alkali characteristic are still unresolved during utilization of biomass and Zhundong coal. Here, the correlations of several chemical properties of high-alkali solid fuels were investigated. The distributions of ash compositions in various biomass exhibit obvious diversity, while the distribution of K 2 O content within wheat and corn straws are the most scattered. The ash content in biomass shows a decrease tendency with the increase of carbon content. Zhundong coals generally have medium but close ash fusion points despite of quite different ash compositions sometimes.

关键词： high alkali chemical property Zhundong coal biomass ternary distribution

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Correction to: Glucose in Conjunction with Multiple Laser Pulses on Laser Treatment of Port-wine Stain: An in vivo Study

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Lasers in medical science 2018年第9期33卷 2015页

作者： Jun Ma Bin Chen Dong Li Yue Zhang Zhaoxia Ying State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong University Xi'an 710049 Shaanxi China. State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong University Xi'an 710049 Shaanxi China. chenbin@***. Department of Dermatology Second Affiliated Hospital Xi'an Jiaotong University Xi'an 710049 Shaanxi China. yzx1919@***.

In the originally published article, the title was incorrectly copied from another article. The correct title is "Glucose in Conjunction with Multiple Laser Pulses on Laser Treatment of Port-wine Stain: An in viv...

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Effects of Coal Blending and Operating Conditions on Combustion and NO x Emission Characteristics in a Tangentially-fired Utility Boiler

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Energy Procedia 2017年 105卷 4015-4020页

作者： Debo Li Qiang Lv Yongxin Feng Chang’an Wang Xuan Liu Kai Chen Kai Xu Jun Zhong Defu Che Electric Power Research Institute of Guangdong Power Grid Corporation Guangzhou 510080 China State Key Laboratory of Multiphase Flow in Power Engineering School of Energy and Power Engineering Xi’an Jiaotong University Xi’an 710049 China

The influences of operating conditions, such as excess air ratio and SOFA arrangement, on temperature distributions, species distributions, NO x emissions and burnout of a tangentially-fired utility boiler using bituminous and blended coal were investigated by numerical approach in the present study. The simulation results show that the fuel type exhibits certain effect on the temperature distributions and the NO x emissions. Moreover, higher excess air ratio could restrain the CO formation but promote NO x emission. The temperature and the species distributions are highly related to the SOFA arrangement. In addition, SOFA technology is still an effective approach to control the NO x emissions during blended coal combustion, while the disadvantageous effect on char burnout should be considered.

关键词： coal blending combustion NOx emission numerical simulation utility boiler

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