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Development in the application of laser-induced breakdown spectroscopy in recent years:A review

Frontiers of physics 2021年第2期16卷 45-69页

作者： Lian-Bo Guo Deng Zhang Lan-Xiang Sun Shun-Chun Yao Lei Zhang Zhen-Zhen Wang Qian-Qian Wang Hong-Bin Ding Yuan Lu Zong-Yu Hou Zhe Wang Wuhan National Laboratory for Optoelectronics(WNLO) Huazhong University of Science and TechnologyWuhan 430074China State Key Laboratory of Robotics Shenyang Institute of AutomationChinese Academy of SciencesSheyang 110016China School of Electric Power South China University of TechnologyGuangzhou 510640China State Key Laboratory of Quantum Optics and Quantum Optics Devices Institute of Laser SpectroscopyShanxi UniversityTaiyuan 030006China State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong UniversityXi'an 710049China Key Laboratory of Photonic Information Technology School of Optics and PhotonicsBeijing Institute of TechnologyBeijing 100081China School of Physics Dalian University of TechnologyNo.2 Linggong RoadGanjingzi DistrictDalian 116024China Optics and Optoelectronics Laboratory Ocean University of ChinaQingdao 266100China State Key Lab of Power Systems Department of Energy and Power EngineeringTsinghua UniversityBeijing 100084China

Laser-induced breakdown spectroscopy(LIBS)has been widely studied due to its unique advantages such as remote sensing,real-time multi-elemental detection and none-to-little *** the efforts of researchers around the world,LIBS has been developed by leaps and ***,in recent years,more and more Chinese LIBS researchers have put tremendous energy in promoting LIBS *** is worth mentioning that the application of LIBS in a specific field has its special application background and technical difficulties,therefore it may develop in different stages.A review summarizing the current development status of LIBS in various fields would be helpful for the development of LIBS technology as well as its applications especially for Chinese LIBS community since most of the researchers in this field work in *** the present work,we summarized the research status and latest progress of main research groups in coal,metallurgy,and water,*** on the current research status,the challenges and opportunities of LIBS were evaluated,and suggestions were made to further promote LIBS applications.

关键词： laser-induced breakdown spectroscopy application

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Preliminary Conceptual Design with Neutronics and Thermal-Hydraulics Assessments of Fustar

SSRN

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SSRN 2023年

作者： Zhou, Xingguang Zhang, Dalin Li, Xinyu Lv, Xindi Jiang, Dianqiang Tian, Wenxi Qiu, Suizheng State Key Laboratory of Multiphase Flow in Power Engineering Shaanxi Key Lab. of Advanced Nuclear Energy and Technology School of Nuclear Science and Technology Xi'an Jiaotong University Xi'An710049 China

The fluoride-salt-cooled high-temperature advanced reactor (FuSTAR) is an advanced small modular reactor, which aims to the electric supplement and clean heat production to western China. In this study, neutronics and thermal-hydraulics analysis are also carried out, and established the core layout and material ratio under the near-critical condition. The parameters of the designed core are evaluated quantitatively from various aspects. The results show that FuSTAR has sufficient shutdown depth, the equilibrium cycle is 3.24 years, and the discharge burnup depth is 106 GWd/MtU. The analysis of 1/6 core porous media shows that the peak fuel temperature under normal operating condition is 1009.3 K, which is far below the limit of 1573 K. Relevant design and analysis results can provide the reference for the subsequent small modular FHR design and construction. © 2023, The Authors. All rights reserved.

关键词： Computational fluid dynamics

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Evaluation of R513A as an environmentally friendly alternative to R134a in spray cooling for laser surgery: Heat transfer performance and optimization

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International Journal of Thermal Sciences 2025年 215卷

作者： He, Zhi-Zhong Lin, Xiang-Wei Li, Chen-Xi Kong, Chen Shen, Lin-Xin Zhou, Zhi-Fu State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong University Shaanxi Xi'an710049 China School of Future Technology Xi'an Jiaotong University Shaanxi Xi'an710049 China Xi'an Jiaotong University Health Science Center Shaanxi Xi'an710049 China

Spray cooling plays a pivotal role in mitigating thermal injuries to the epidermis during laser surgery. However, the widespread use of R134a, a refrigerant with a high global warming potential (GWP) of 1300, poses significant environmental concerns. In this study, R513A, a more environmental-friendly cryogen with a GWP of 573, is used to investigate the feasibility of replacing R134a and the effects of spray height, spurt duration, nozzle orifice diameter, and spray pressure on R513A spray cooling through a self-built open-loop spray system. Experimental results demonstrate that R513A exhibits superior cooling performance, achieving a minimum surface temperature (Tmin) 12 °C lower and a maximum heat flux (qmax) 27.5 % higher than R134a. Additionally, R513A offers a broader optimal spray height range (30–50 mm) in which Tmin is 4 °C and 13 °C lower than those at 20 mm and 10 mm, respectively. qmax in this range is 10 % and 16 % higher than those at 20 mm and 10 mm, respectively. While extending the spurt duration consumes more cryogen and prolongs the liquid film lifetime, the differences in Tmin and qmax are less than 4 °C and 10 kW/m2. With the nozzle orifice increasing from 0.6 mm to 1.0 mm, Tmin remains approximately −42 °C but qmax gradually increases by 6 kW/m2. Macroscopic analysis reveals that higher spray pressure induces a more dispersive spray, though this does not significantly improve cooling efficiency. To advance the understanding of R513A spray cooling dynamics, a dimensionless correlation was developed to predict the dynamic heat transfer coefficient across diverse conditions. This study not only highlights the potential of R513A as a sustainable alternative but also provides critical insights into optimizing spray cooling parameters for enhanced thermal management in laser surgery. © 2025 Elsevier Masson SAS

关键词： Chilling

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Best estimate plus uncertainty analysis of the China advanced large-scale PWR during LBLOCA scenarios

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International Journal of Advanced Nuclear Reactor Design and Technology 2020年 2卷 34-42页

作者： Chang, Yuhao Wang, Mingjun Zhang, Jing Tian, Wenxi Qiu, Suizheng Su, G.H. Department of Nuclear Science and Technology State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong University Xi'an710049 China

China advanced large-scale Pressurized Water Reactor (PWR) implements series of passive safety systems to provide core cooling and decay heat removal in case of some unexpected accidents. The development of reactor best estimate system analysis codes has realized the transition from conservative safety analysis to Best Estimate plus Uncertainty (BEPU) analysis for the purpose of achieving more realistic results and digging larger safety margins. The BEPU analysis during Large Break Loss of Coolant Accident (LBLOCA) has been widely used for the licensing application of Nuclear power Plants (NPPs). In this paper, the BEPU analysis of China advanced large-scale PWR was performed under the conditions of LBLOCA scenarios employing RELAP5 code. The models of reactor coolant system with all the passive safety systems were established and the influence of uncertainties of important parameters on the Peak Cladding Temperature (PCT) was evaluated. The results show the obtained PTC (1314 K) through the BEPU analysis is far below the 10CFR50.46 PCT acceptance criteria (1477 K) in case of LBLOCA and is also lower than the conservative calculation value (1348 K), indicating a larger safety margin. This work provides a meaningful evaluation method for China advanced large-scale PWR safety assessment. © 2020 Xi'an Jiaotong University

关键词： Pressurized water reactors

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Light doping of tungsten into copper-platinum nanoalloys for boosting their electrocatalytic performance in methanol oxidation

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Nano Research Energy 2022年第2期1卷 194-200页

作者： Danye Liu Qing Zeng Chaoquan Hu Dong Chen Hui Liu Yongsheng Han Lin Xu Qingbo Zhang Jun Yang State Key Laboratory of Multiphase Complex Systems Institute of Process EngineeringChinese Academy of SciencesBeijing 100190China Center of Materials Science and Optoelectronics Engineering University of Chinese Academy of SciencesBeijing 100049China Nanjing IPE Institute of Green Manufacturing Industry Nanjing 211100China School of Chemistry and Materials Science Jiangsu Key Laboratory of New Power BatteriesJiangsu Collaborative Innovation Centre of Biomedical Functional MaterialsNanjing Normal UniversityNanjing 210023China Department of Bioengineering Rice UniversityHoustonTexas 77005USA

Coupling the bi-functional mechanism with compressive lattice strain might be an effective way to boost the electrocatalysis of platinum(Pt)-based nanoparticles for methanol oxidation reaction(MOR).This strategy weakens the chemisorption of poisoning CO-like intermediates generated during MOR on the active Pt sites by lowering their d-band *** this context,we herein report the synthesis of ternary copper-tungsten-platinum(CuWPt)nanoalloys with light doping of W element by simply co-reducing their precursors at elevated *** this ternary alloy system,the presence of only small amount of W element not only weakens the chemisorption of CO-like intermediates by lowering the Pt d-band center through compressive lattice strain,but also cleans the active Pt sites by“hydrogen spillover effect”,endowing the as-prepared CuWPt nanoalloys at an appropriate Cu/W/Pt ratio with good activity for *** specific,the ternary CuWPt alloy nanoparticles at a Cu/W/Pt molar ratio of 21/4/75 show a specific activity of 2.5 mA·cm^(−2)and a mass activity of 2.11 A·mg^(−1)with a better durability,outperforming those ternary CuWPt alloy nanoparticles at other Cu/W/Pt ratios,binary CuPt alloys and commercial Pt/C catalyst as well as a large number of reported Pt-based *** addition,a single direct methanol fuel cell(DMFC)assembled using ternary CuWPt nanoalloys as anodic catalysts shows a power density of 24.3 mW·cm^(−2)and an open-circle voltage of 0.6 V,also much higher than those of the single DMFC assembled from commercial Pt/C catalysts.

关键词： lattice strain d-band center electrocatalysis hydrogen spillover methanol oxidation reaction

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Hydrodynamic Characteristics Prediction Models for Water-Cooled Wall Under Different Loads Based on Artificial Neural Network

SSRN

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SSRN 2024年

作者： Yang, Jiahui Zhang, Yong Li, Ruiyu Han, Lei Yue, Yang Wang, Jin Deng, Lei Che, Defu State Key Laboratory of Multiphase Flow in Power Engineering School of Energy and Power Engineering Xi’an Jiaotong University Xi’an710049 China Yantai Longyuan Power Technology Co. Ltd Yantai264000 China Shunde Institute of Inspection Guangdong Institute of Special Equipment Inspection and Research Foshan528300 China

Real-time monitoring of hydrodynamic characteristics in water-cooled wall is crucial for boiler safety. Comprehensive numerical simulations are employed in this study to determine the heat flux distribution on the water-cooled wall across 38 different operating conditions. The heat flux results are applied to calculate hydrodynamic characteristics. Subsequently, the hydrodynamic characteristics results, along with the corresponding operating parameters, form the dataset for the Artificial Neural Network (ANN) models. The proposed methodology generates high-quality datasets, with a maximum root mean square error (RMSE) of only 6.8 K when comparing the results of working fluid temperature to the measured values. Two dataset partitioning methods are compared. Compared with random partitioning (control group), Considering each working condition as a whole during dataset partitioning (experimental group) reduces the average RMSE of predicted results in the test set by 47.6%, along with a 31.8% decrease in average number of neurons. The developed models exhibit excellent agreement with four working conditions in the test set, both in trends and absolute values, with acceptable error ranges. On the validation and test sets, the maximum RMSEs between the predicted and calculated values for flow rate, pressure, temperature and enthalpy are 0.033 kg s-1, 0.49 MPa, 5.7 K and 89.5 kJ kg-1, respectively, underscoring the reliability and practicality of the predictive models. © 2024, The Authors. All rights reserved.

关键词： Hydrodynamics

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Numerical Study on Benchmark Analysis of NACIE-UP Facility with Uniform and Non-Uniform power Distribution

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SSRN 2024年

作者： Li, Haoyang Zhang, Dalin Zhou, Lei Deng, Jian Tian, Wenxi Su, Guanghui Qiu, Suizheng State Key Laboratory of Multiphase Flow in Power Engineering Shaanxi Key Laboratory of Advanced Nuclear Energy and Technology School of Nuclear Science and Technology Xi’an Jiaotong University Xi’an710049 China Nuclear Power Institute of China 328 Changshun Avenue Chengdu610213 China Science and Technology on Reactor System Design Technology Laboratory Nuclear Power Institute of China Chengdu610213 China

The NACIE-UP facility is located at the ENEA Brasimone Research Centre and is designed to investigate the thermo-hydraulic properties of LBE within a wire-spaced assembly under uniform and non-uniform power distribution conditions. In this study, the thermo-hydraulic characteristics of FPS are analyzed. ANSYS Fluent solver is applied with the COUPLE algorithm of RANS [[EQUATION]] model. Cheng&Tak correlation and computational conditions are implanted into Fluent in the form of UDFs. The results show that the RMSEs of ADP10SS1 and ADP10SS2 are 2.52 K and 3.69 K, 7.05 K and 8.48 K for ADP06SS1 and ADP06SS2, respectively, which indicate that the adopted models have good prediction ability for the temperature of the experimental conditions. Meanwhile, the heat transfer characteristics are investigated and compared with the correlations of Ushakov, Mikityuk, Kazimi and Carelli. Above all, this study provides quantitative and qualitative analysis for verification and validation of CFD/STH code and stand-alone CFD simulation. © 2024, The Authors. All rights reserved.

关键词： Heat transfer

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Pani Grafted Onto Waste Poros Polyurethane for Co-Adsorption of Multiple Pollutants in Industrial Wastewater

SSRN

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SSRN 2023年

作者： Wang, Ning Guo, Yirui Song, Yi Yan, Wei Gong, Xuesong Li, Yunfeng Mu, Ruihua Liu, Yonghong Zhang, Luohong School of Environmental and Chemical Engineering Xi'an Polytechnic University Xi'An710048 China Department of Environmental Science and Engineering State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong University Xi'An710049 China

Up-taking the pollutants simultaneously from industrial wastewater is an urgent in the advanced treatment. In this work, the polyaniline (PANI)-based efficient adsorbent supported by the waste polyurethane(PU) was designed for synchronous adsorption of pollutants (acid red G (ARG), methylene blue (MB), hexavalent chromium Cr(VI), phosphorus (TP), NH4+-N (ammonia nitrogen), NO3-N (nitrate nitrogen) and COD (chemical oxygen demand)). The results showed that the synchronous removal efficiency of ARG, MB, Cr(VI), TP, NH4+-N, NO3-N and COD in simulated wastewater reached 88%, 40%, 90%, 58%, 42%, 30% and 63%, respectively. The adsorption lasted for 1800 min (144 columns) before saturation, and no significant decrease was observed after 5 cycles of regeneration. Combined with the XPS (X-ray photoelectron spectroscopy) and EEM (excitation-emission matrix spectroscopy) analysis, ARG, Cr(VI), NO3-N and TP competed for the same adsorption sites, and the adsorption affinity order was ARG>Cr(Ⅵ)>TP>NO3-. During the adsorption process, Cr(VI) and =N- in PANI chain underwent redox reaction to form Cr(III) and -NH+-, which further promoted the adsorption of anionic pollutants, like H2PO4-. Redox reactions also occurred between Cr(VI) and MB before adsorption forming Cr(III) and small organic fragments. These conclusions prove the feasibility and effectiveness of PU-P/T as a potential engineering adsorbent for co-adsorption of a variety of pollutants. © 2023, The Authors. All rights reserved.

关键词： Adsorption

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Efficient Water Recovery and power Generation System Based on Air-Cooled Fuel Cell with Semi-Closed Cathode Circulation Mode

SSRN

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SSRN 2024年

作者： Yang, Yuchen Wu, Zhen Yao, Jing Wang, Bofei Yang, Fusheng Zhang, Zaoxiao Ren, Jianwei School of Chemical Engineering and Technology Xi’an Jiaotong University Xi’an710049 China State Key Laboratory of Multiphase Flow in Power Engineering Xi’an Jiaotong University Xi’an710049 China Department of Mechanical Engineering Science University of Johannesburg Johannesburg2092 South Africa

Air-cooled proton exchange membrane hydrogen fuel cell with on-line hydrogen production by hydrolysis has potential for portable applications due to its high volumetric power density and self-humidification. However, plenty of reserve water significantly reduces the power density of fuel cell system. Moreover, water recovery from fuel cell tail gas is difficult, because the tail gas humidity is very low due to excess cathode air as coolant. In this work, the dead-ended anode and semi-closed cathode proton exchange membrane fuel cell is proposed to achieve efficient water recovery and energy conversion via semi-closed cathode circulation mode. In this mode, cathode O2-poor tail gas is recycled as coolant instead of fresh air, which helps to enlarge the tail gas humidity by reducing the stoichiometric ratio of cathode to anode gas. The system lumped model with detailed component description is developed for optimization. More than 96% water production can be recycled under atmosphere temperature. The demand of fresh air is greatly reduced from 56 to 2 times of the consumption. Besides, the multi-objective optimization between water recovery and electrochemical performance shows high-efficiency water recovery of 94.70% and high energy conversion efficiency of 54.82%. © 2024, The Authors. All rights reserved.

关键词： Cathodes

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Influence of Bi3+ Doping on the Electrochemical Properties of Ti/Sb-Sno2/Pbo2 Electrode for Zinc Electrowinning

SSRN

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SSRN 2024年

作者： Wu, Jia Kang, Xuanqi Xu, Shuangwen Wei, Zhen Xu, Shangyuan Liu, Kang Feng, Qing Jia, Bo Wang, Yunhai Xían Taijin New Energy & Materials Sci-Tech CO. Ltd Xi’an710016 China Department of Environmental Science and Engineering State Key Laboratory of Multiphase Flow in Power Engineering Xi’an Jiao tong University Xi’an710049 China

Bi3+ doped Ti/Sb-SnO2/PbO2 electrode materials were fabricated by electrodeposition to improve its electrochemical performance in zinc electrowinning. The surface morphology, chemical composition and hydrophilicity of the as-prepared electrodes are characterized by scanning electron microscopy (SEM), energy dispersive X-ray spectroscopy (EDS), X-ray diffraction (XRD), X-ray photoelectron spectroscopy (XPS) and contact angle. The electrochemical measurement and the accelerate lifetime experiment are also conduct to investigate the electrocatalytic performance and stability of the electrodes. The results showed that Bi3+ modification electrode has an important effect on the coating morphology, crystal structure, surface hydrophilicity, electrocatalytic activity and stability. The electrode prepared from the solution containing 2 mmol·L-1 Bi(NO3)3 (marked as the Ti/Sb-SnO2/2Bi-PbO2 electrode) exhibits the best hydrophilicity performance (θ=21.6°) and the longest service life (1196 h). During the electrochemical characterization analysis, the Ti/Sb-SnO2/2Bi-PbO2 electrode showed the highest oxygen evolution activity, which can be attributed to the highest electroactive surface (qT*=21.20 C·cm-2) and the best charge transfer efficiency. DFT calculation demonstrate that the doping of Bi lead to the decrease in the OER reaction barrier and increase the DOS of the electrode, which further enhanced the catalytic activity and conductivity of the electrode. Moreover, the simulated zinc electrowinning experiment demonstrate that the Ti/Sb-SnO2/2Bi-PbO2 electrode consume less energy than other electrodes. Therefore, it is expected that the Bi modified electrodes may become a very promising electrode material for zinc electrowinning in the future. © 2024, The Authors. All rights reserved.

关键词： Hydrophilicity

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