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SSRN 2023年

作者： Zhang, Dan Tu, Maoping Yuan, Yang Han, Wei State Key Laboratory of Multiphase Flow in Power Engineering School of Energy & Power Engineering Xi'an Jiaotong University Shaanxi Xi’an710049 China Xi'an Thermal Power Research Institute Co. Ltd Shaanxi Xi’an710054 China

Directly heat water droplet by thermal radiation was the key process of coupling solar energy to achieve green production in many industrial applications, such as desalination, carbon capture, energy storage, and so on. The radiative transfer of single water droplet for given irradiation, including reflection, absorption, transmission and their dependences on external irradiation, droplet geometry and radiative properties were investigated through a calculation model set up according to zone method. In current study, the ranges of equivalent diameter and length-width ratio of droplet were 0.1-1.0 mm, 1-10 respectively, its absorption coefficient was 10-15000 m-1 and refractive index was 1.2-2.0. Results suggested that, (1) the absorption mode of droplet could be classified into surface absorption (SA) and volumetric absorption (VA) depending on whether its optical thickness was greater than 1. In VA, droplet could get uniform and fast temperature increasing, and its absorptivity and mean temperature increase rate could be simultaneously improved by increasing absorption coefficient. (2) Scattering included reflection and transmission. Compared with incident irradiation, reflection distributed mainly on the same side of droplet's long axis, while transmission mainly on the opposite side. The overall reflectivity increased with rising refractive index, but was independent on droplet size. While its transmissivity increased with enlarging length-width ratio or reducing equivalent diameter. (3) In VA, at least 40% of incident irradiation was scattered out. The total quantity of scattering could be adjusted by changing absorption coefficient in VA or refractive index in SA. The proportion of transmission in scattering could always be increased by reducing refractive index. © 2023, The Authors. All rights reserved.

关键词： Drops

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Effect of Tungsten Size on Thermal Analysis and Mechanism of Lithium Perchlorate-Based Electrically Controlled Solid Propellant

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SSRN 2023年

作者： Yang, Meng Yoh, Jack J. Tang, Chenglong Huang, Zuohua State Key Laboratory of Multiphase Flow in Power Engineering Xi’an Jiaotong University Xi’an710049 China Department of Aerospace Engineering Seoul National University Seoul08826 Korea Republic of

Electrically controlled solid propellant (ECSP) is a novel and potential of propellant with excellent properties, which can achieve multiple ignitions and extinguishments through supplying and cutting electric power. At present, thermochemistry coupled with electrochemical reaction processes are complex and not understood clearly, especially its based thermal decomposition mechanism without electric power. In this work, the baseline ECSP was prepared using lithium perchlorate (LiClO4, LP) as oxidant, and tungsten as metal additive to obtain high energy ECSP samples. The scanning electron microscope (SEM), differential scanning calorimeter (DSC) and thermogravimetry (TGA) were used to investigate thermal analysis characteristics of ECSP and the effect of metal tungsten sizes on reaction process and mechanism. The heat release and effective activation energy (Eα) of baseline ECSP were lower than those of metalized ECSP. In addition, with W size increasing, heat release and Eα of ECSP increase. Based on thermal analysis and kinetic results, the decomposition mechanisms of ECSP main components and samples were proposed. The absorbed and crystal water evaporated, then main components molten for all cases at low temperature ( © 2023, The Authors. All rights reserved.

关键词： Thermogravimetric analysis

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Hydrodynamic Pattern in Drying Saline Droplet with Suspended Nanoparticles

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Journal of Bionic engineering 2020年第4期17卷 802-808页

作者： Junheng Ren Xin Zhong Lu Shen Fei Duan School of Mechanical and Aerospace Engineering Nanyang Technological UniversitySingapore 639798Singapore State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong UniversityXi'an 710049China

Evaporation of multicomponent droplets has gained much attention nowadays because of their complex flow fields and various deposition *** we observe strong flows in evaporating sodium chloride saline droplets with suspended alumina oxide *** evolution of flow pattern was studied by tracking the trajectories of particles and the velocity field was investigated with Particle Image Velocimetry *** non-uniform evaporation rate along the droplet surface leads to a concentration gradient which induces the convection *** the evaporation process before crystallization happens,evolution of the flow can be divided into two *** Regime I,a centrosymmetric convection recirculation is formed *** RegimeⅡ,the convection recirculation migrates to the droplet edge and evolves into several small *** the late evaporation stage,crystallization could induce strong convection *** is shown that the flow tends to become more chaotic with a lower salt concentration.

关键词： convection flow concentration gradient saline droplet crystallization

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Mild Combustion of a Premixed Nh3/Air Jet Flame in Hot Coflow Versus its Ch4/Air Counterpart

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SSRN 2023年

作者： Li, Pengfei Wang, Guochang Liu, Xiangtao Shi, Guodong Cai, Xiao Liu, Zhaohui Mi, Jianchun State Key Laboratory of Coal Combustion School of Energy and Power Engineering Huazhong University of Science and Technology Wuhan430074 China College of Engineering Peking University Beijing100871 China State Key Laboratory of Multiphase Flow in Power Engineering Xi’an Jiaotong University Xi’an710049 China Dalian Maritime University China

MILD combustion is very suitable for solving the problems of unstable flame and high NOx emission (ENOx ) for ammonia fuel, but the related studies are rare. This work numerically investigates the MILD combustion characteristics of a premixed NH3/air jet flame in hot coflow (JHC) under different jet equivalence ratio (ΦJ), coflow temperature (TC) and oxygen level (XO2,C). For comparison, the similar CH4/air MILD-JHC flames are also calculated. Results show that the NH3 flame generally has lower temperature rise and heat release as well as larger reaction zone than CH4. This may suggest that the former flame can develop to the MILD regime more easily. ENOx is two orders higher from the NH3 than CH4 flame at all TC and XO2,C for ΦJ 1, ENOx of the NH3 flame quickly drops to near zero, but ENH3 and EH2 are very high (~1000 ppm) and the combustion efficiency is low. Moreover, ENOx increases quickly (slowly) with XO2,C (TC) while ENH3 and EH2 are quite low at TC ≥ 1300 K and XO2,C ≥ 1% for the NH3 flame. ENOx mainly comes from NO but N2O is also important at low ΦJ and TC. Therefore, considering all ENOx , ENH3, EH2 and the burning efficiency, the optimal conditions for NH3 MILD combustion are ΦJ =1, TC ≥ 1500 K and XO2,C =1%-3%. In addition, compared to the conventional flame, the NH3 MILD combustion can reduce ENOx by 1-2 orders. © 2023, The Authors. All rights reserved.

关键词： Ammonia

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Numerical Study of High-Energy Spark Ignition Characteristics in a Scramjet Combustor

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SSRN 2024年

作者： Gao, Ziyan Zhang, Meng Zhang, Zhibo Wu, Yun Zheng, Xing Miao, Huifeng National Key Lab of Aerospace Power System and Plasma Technology Xi’an Jiaotong University Xi’an710049 China State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong Universiy Xi’an710049 China National Key Lab of Aerospace Power System and Plasma Technology Air Force Engineering University Xi’an710038 China Shaanxi Key Laboratory of Environment and Control for Flight Vehicle School of Aerospace Engineering Xi’an Jiaotong University Shaanxi 710049 China

Reliable ignition is a fundamental prerequisite for the scramjet engines. In order to improve the reliability of ignition, further enhance the application of spark ignition in engineering, and improve the ignition ability in the field of supersonic combustion, an innovative long electrode distance high-energy spark igniter (LHSI) system was proposed by our research team. To reveal the instantaneous ignition characteristics of the LHSI, a simulation model of the LHSI is established and verified by experiments. Based on this, the formation and development of the initial fire core of vaporized kerosene and the ignition characteristics of LHSI in a scramjet combustor were simulated and compared with the conventional high-energy spark igniter (HSI). The analysis revealed that the success of the cavity ignition is greatly influenced by the local equivalent ratio of the initial flow field and the penetration depth of the initial flame core. Meanwhile, the fore recirculation zone of the cavity plays a key role in stabilization and development of the initial fire core. Compared with the HSI, the LHSI can produce initial flame core with higher penetration and greater size, which is the main reason for why LHSI has a broader ignition boundary. © 2024, The Authors. All rights reserved.

关键词： Ignition

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Theoretical Study on Predicting the Performance of Steam Ejector by Analogy Method

Theoretical Study on Predicting the Performance of Steam Eje...

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IEEE Asia power and Energy engineering Conference (APEEC)

作者： Yiguo Mei Keneng Qian Yuyan Hou Weixiong Chen Huaxin Consulting Design and Research Institute Co. Hangzhou China State Key Laboratory of Multiphase Flow in Power Engineering Xi’an Jiaotong University Xi’an China

At present, it is difficult to obtain steam with high pressure under conventional laboratory conditions, and there are certain operational risks in the production of high-pressure and high-temperature steam devices. In this paper, a method to predict the critical entrainment ratio of the steam ejector by using the critical entrainment ratio of the air ejector is proposed. According to the one-dimensional calculation model of the ejector, the parameters related to the critical entrainment ratio are derived. The mathematical relationship between the entrainment ratio and each parameter is found through the mathematical tool Matlab. The performance of the ejector with different working mediums is simulated and verified by Fluent. The research results in this paper show that the entrainment ratio of air and steam ejector is linear with the pressure ratio within a certain range of pressure ratio. Under this linear relationship, the experimental entrainment ratio of the air ejector can be used to predict the entrainment ratio of the steam ejector. In a certain linear range, the relative error between the entrainment ratio predicted by the method proposed in this paper and the simulation results is within 10%.

关键词： Electrical engineering Simulation Fitting Production Media Numerical simulation Market research

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金属原子诱导的微环境调控在聚合氮化碳光催化析氢中的研究

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Science China Materials 2024年第6期67卷 1765-1779页

作者：赵大明杨雨骁 Vasileios Binas 沈少华 School of Advanced Energy Shenzhen Campus of Sun Yat-sen UniversityShenzhen 518107China International Research Center for Renewable Energy State Key Laboratory of Multiphase Flow in Power EngineeringXi’an Jiaotong UniversityXi’an 710049China Institute of Electronic Structure and Laser(IESL) Vasilika VoutonHeraklion GR-71110Greece Physical Chemistry Laboratory Chemistry DepartmentAristotle University of ThessalonikiThessaloniki 54124Greece

开发高效稳定的半导体光催化剂对光催化技术迈向实际应用至关重要.聚合物氮化碳(CN)因其优异的物理化学性质而被视为最具发展前景的制氢光催化剂之一.在过去几十年中,从热力学或动力学角度开发的一系列改性策略已经显著提升了CN的光催... 详细信息

开发高效稳定的半导体光催化剂对光催化技术迈向实际应用至关重要.聚合物氮化碳(CN)因其优异的物理化学性质而被视为最具发展前景的制氢光催化剂之一.在过去几十年中,从热力学或动力学角度开发的一系列改性策略已经显著提升了CN的光催化制氢性能.近期,金属原子修饰策略为CN改性提供了一条新途径,这种策略可以精确调控CN的微环境.本文全面回顾了金属原子修饰的CN光催化剂在光催化分解水制氢领域的最新研究进展,包括金属单原子修饰的CN、金属双原子修饰的CN、金属单原子与团簇共修饰的CN,重点阐述了金属原子对提升光催化性能的关键作用.此外,本文还全面总结了发展先进的金属原子修饰的CN光催化剂所面临的挑战与机遇.

关键词： metal atom polymeric carbon nitride hydrogen evolution photocatalysis solar energy conversion

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Editor, Applied Energy Paper Entitled: "Industrialized Bimetallic Nano Oxygen Carrier for Dual-Stage Hydrogen Production from Mid-Temperature Chemical Looping Reforming"

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SSRN 2024年

作者： Tang, Sanli Gai, Zhongrui Li, Yang Liu, Yunlian Liu, Mingkai Pan, Ying Jin, Hongguang Institute of Engineering Thermophysics Chinese Academy of Sciences Beijing100190 China State Key Laboratory of Multiphase Flow in Power Engineering Xi’an Jiaotong University Xi’an710049 China University of Chinese Academy of Sciences Beijing100049 China

Chemical looping methane reforming has emerged as a promising avenue to produce blue hydrogen. Among the various oxygen carriers investigated for this process, Fe2O3 and NiO have garnered significant attention due to their affordability and favorable thermodynamic properties. Usually, such oxygen carriers had satisfactory H2 yields only in the oxidation stage with temperatures over 800 °C. This limitation poses challenges for industrial reactor design and product gas separation. In this study, we present a nanoscale Fe/Ni bimetallic oxygen carrier for dual-stage hydrogen generation from mid-temperature chemical looping methane reforming. The lab-scale oxygen carrier can produce H2 in both the reduction and the oxidation steps, reaching 75% overall H2 purity while reducing the temperature to 500-600 °C. Moreover, the 10-kg scale oxygen carrier achieved >90% CH4 conversion, >78% H2 purity and 2.8-3.5 H2 molecules produced per CH4 molecule. Made into beads, the 10-kg scale oxygen carrier still maintained an outlet H2 purity of >70% with redox stability over 150 cycles. These findings contribute to the advancement of chemical looping methane reforming for blue hydrogen production and supply. © 2024, The Authors. All rights reserved.

关键词： Hydrogen production

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From Lab to Industry: Scaling-Up Fe-Ni Bimetallic Nano Oxygen Carrier for Mid-Temperature Methane Chemical Looping Reforming

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SSRN 2024年

Chemical looping methane reforming has emerged as a promising avenue to produce blue hydrogen. Currently, the satisfactory CH4 conversion and H2 productivity are usually seen under temperatures above 800 °C. Such temperature requirement poses challenges for industrial reactor design and product gas separation. Investigated widely in chemical looping, bimetallic oxygen carrier has both catalytic and oxygen releasing functions, thus expected to realize both lower reaction temperature and high performance. In this study, we present a nanoscale Fe-Ni bimetallic oxygen carrier for mid-temperature chemical looping methane reforming which can be implemented at large scale. By virtue of a synergy from nanoscale Fe-Ni dispersion, all oxygen carriers from lab-scale to 10-kg scale can operate at 500-600 °C. The lab-scale oxygen carrier was found to convert >90% CH4, produce 3.5 H2 per CH4 molecule with 80-82% overall H2 purity at 575-600 °C. Following the proposed large-scale synthesis workflow, we acquired the 10-kg scale oxygen carrier powder with 70% with 2.8 H2 from per CH4 molecule. The 10-kg powders and beads both persisted phase, morphology and redox stability over 150 cycles. Further explorations revealed the similarity in structure and reaction performance between the lab-scale and 10-kg scale powders, and differences in reaction dynamics between the 10-kg powder and beads. These findings contribute to the mid-temperature chemical looping methane reforming by bridging laboratory practices and industrial application. © 2024, The Authors. All rights reserved.

关键词： Powders

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Navigating the Dual Pathways of Ion Removal in flow-Electrode Capacitive Deionization: Capacitive Trapping vs. Electrodialytic Migration

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SSRN 2025年

作者： Gu, Haibo Hou, Chengsi Mao, Yunfeng Wu, Deli School of Energy and Power Engineering University of Shanghai for Science and Technology Shanghai200093 China State Key Laboratory of Pollution Control and Resources Reuse College of Environmental Science & Engineering Tongji University Shanghai200092 China Shanghai Key Laboratory of Multiphase Flow and Heat Transfer in Power Engineering Shanghai200093 China Shanghai Institute of Pollution Control and Ecological Security Shanghai200092 China

By introducing flowing electrodes, FCDI enables desalination through dual mechanisms of electrodialytic and capacitive effects. Clarifying their distinct roles is essential to advance tailored system design and performance enhancement. This work elucidates the antagonistic interplay between capacitive trapping and electrodialytic migration in flow-electrode capacitive deionization (FCDI) through both electrochemical characterization and multiphysics modeling. Experimental analyses reveal that elevated flow rates enhance electrodialytic migration but impair capacitive adsorption. Multivariate parametric studies demonstrate that capacitive dominance prevails at high current densities and low electrolyte concentrations, whereas electrodialytic effects peak under high electrolyte concentration and moderate flow rates. The balance between the effects of electrodialysis (ED) and capacitive deionization (CDI) is greatly impacted by convective mass transfer, which is caused by the electrode flow rate. While higher solid weight percentages in the flow electrode improve the CDI effect by increasing the number of active sites for salt adsorption, increased electrode flow rates maximize the ED effect by encouraging ion transport in the electrolyte. In short words, strategies to promote free ions dispersing in the electrolyte would enhance the electrodialytic contribution, whereas the concentration polarization would benefit the capacitive contribution. This work opens the door for the exploration of upgrading FCDI architectures and optimizing operation parameters while providing insights into the intricate interactions within the system. © 2025, The Authors. All rights reserved.

关键词： Desalination

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