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Ni-based electrocatalysts for urea-assisted water splitting

Chinese Journal of Structural Chemistry 2024年第8期43卷 10-11页

作者： Shuyuan Pan Zehui Yang Fang Luo Faculty of Materials Science and Chemistry China University of Geosciences Wuhan388 Lumo RDWuhan430074China College of Materials Science and Engineering State Key Laboratory of New Textile Materials&Advanced Processing TechnologyWuhan Textile UniversityWuhan430200China

Hydrogen,as one of the environmentally-friendly energy sources,has garnered much *** splitting is one promising technology to electrochemically produce hydrogen driven by intermittent renewable energy sources without ... 详细信息

关键词： splitting hydrogen electrochemical

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Parametric study on the ballistic performance of seamed woven fabrics

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Defence technology（防务技术） 2023年第6期24卷 173-189页

作者： Hang Li Rui Zhang Shengnan Min Yi Zhou Jiuxiao Sun State Key Laboratory of New Textile Materials and Advanced Processing Technologies Wuhan Textile UniversityChina School of Materials Design&Engineering Beijing Institute of Fashion Technology100029BeijingChina

The ballistic perforation response of composite fabrics made by combining plain weaves with seaming technology is reported and compared with conventional unseamed plain *** effect of the seaming technique on the ballistic resistance of aramid plain fabrics is investigated by varying the seaming *** ballistic experiment uses 8 mm diameter spherical projectiles to impact different fabric sample targets with velocities of 230 m/s and 400 m/*** ballistic performance of seamed and unseamed fabrics is characterized by the specific energy absorption(SEA)values of the *** results show that the seamed fabric has a better energy absorption capacity than the unseamed fabric,e.g.,the SEA of sample 5(seaming lines on every four yarns in a single-ply fabric system)is 135%of sample 1(plain weave without thread seaming).In the single-layer system,the effect of the seaming technique on the energy absorption of the fabric in significant when considering seaming density,seaming orientation,seaming distance,and seaming material on the plain fabric;In addition,it is found that in multi-layer systems,seamed panels(e.g.,sample 7)exhibit better ballistic performance than multi-layer fabrics(e.g.,sample 2),and the specific energy absorption of sample 7 is approximately 156%and 200%of sample 6 and sample 2,***,the energy absorption of the fabric decreases with the increase of impact velocity,which is related to the energy absorption mechanism of the soft fabric system at high impact *** yarn pull-out tests shows that the constraint provided by the seaming thread increases the friction between the fabric-forming ***,when the constraint exceeds a certain level,it is detrimental to the energy absorption of the fabric,which may be due to the overconstraint of yarn mobility.

关键词： Fabric Ballistic performance Seaming technology Energy absorption

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Spatial confinement of free-standing graphene sponge enables excellent stability of conversion-type Fe_(2)O_(3)anode for sodium storage

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Chinese Chemical Letters 2025年第3期36卷 544-549页

作者： Jun Dong Senyuan Tan Sunbin Yang Yalong Jiang Ruxing Wang Jian Ao Zilun Chen Chaohai Zhang Qinyou An Xiaoxing Zhang Hubei Key Laboratory for High-efficiency Utilization of Solar Energy and Operation Control of Energy Storage System Hubei University of TechnologyWuhan 430068China State Key Laboratory of New Textile Materials and Advanced Processing Technologies Wuhan Textile UniversityWuhan 430200China State Key Laboratory of Advanced Technology for Materials Synthesis and Processing Wuhan University of TechnologyWuhan 430070China Nanjing University of Aeronautics and Astronautics Nanjing 210016China

Conversion-type anode materials are highly desirable for Na-ion batteries(NIBs)due to their high theoretical ***,the active materials undergo severe expansion and pulverization during the sodiation,resulting in inferior cycling ***,a self-supporting three-dimensional(3D)graphene sponge decorated with Fe_(2)O_(3)nanocubes(rGO@Fe_(2)O_(3))is ***,the 3D graphene sponge with resilience and high porosity benefits to accommodate the volume expansion of the Fe_(2)O_(3)nanocubes and facilitates the rapid electrons/ions transport,enabling spatial confinement to achieve outstanding ***,the free-standing rGO@Fe_(2)O_(3)can be directly used as an electrode without additional binders and conductive additives,which helps to obtain a higher energy *** on the total mass of the rGO@Fe_(2)O_(3)material,the rGO@Fe_(2)O_(3)anode presents a specific capacity of 859 mAh/g at 0.1 A/*** also delivers an impressive cycling performance(327 mAh/g after 2000 cycles at 1 A/g)and a superior rate capacity(162mAh/g at 20 A/g).The coin-type Na_(3)V_(2)(PO_(4))_(3)@C//rGO@Fe_(2)O_(3)NIB exhibits an energy density of 265.3Wh/*** unique 3D ionic/electronic conductive network may provide new strategies to design advanced conversion-type anode materials for high-performance NIBs.

关键词： Conversion-type anode Spatial confinement Fe_(2)O_(3) Graphene network Self-supporting Sodium-ion batteries

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Multi-scale structure engineering of covalent organic framework for electrochemical charge storage

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SusMat 2024年第1期4卷 4-33页

作者： Xiaofang Zhang Fangling Li Shuangqiao Yang Baiqi Song Richu Luo Rui Xiong Weilin Xu State Key Laboratory of New Textile Materials and Advanced Processing Technologies Wuhan Textile UniversityWuhanChina State Key Laboratory of Polymer Materials Engineering Polymer Research Institute at Sichuan UniversityChengduChina

Covalent organic frameworks(COFs),which are constructed by linking organic building blocks via dynamic covalent bonds,are newly emerged and burgeoning crystalline porous copolymers with features including programmable topological architecture,pre-designable periodic skeleton,well-defined micro-/meso-pore,large specific surface area,and customizable electroactive *** benefits make COFs as promising candidates for advanced electrochemical energy ***,for now,structure engineering of COFs from multiscale aspects has been conducted to enable optimal overall electrochemical performance in terms of structure durability,electrical conductivity,redox activity,and charge *** this review,we give a fundamental and insightful study on the correlations between multi-scale structure engineering and eventual electrochemical properties of COFs,started with introducing their basic chemistries and charge storage *** careful discussion on the significant achievements in structure engineering of COFs from linkages,redox sites,polygon skeleton,crystal nanostructures,and composite microstructures,and further their effects on the electrochemical behavior of COFs are ***,the timely cutting-edge perspectives and in-depth insights into COFbased electrodematerials to rationally screen their electrochemical behaviors for addressing future challenges and implementing electrochemical energy storage applications are proposed.

关键词： covalent organic frameworks electrochemical energy storage multi-scale structure engineering structure-performance correlation

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A self-powered system to electrochemically generate ammonia driven by palladium single atomelectrocatalyst

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SusMat 2024年第5期4卷 178-188页

作者： Hao Hu Shuyuan Pan Zhiyong Ma Kaiyi Liu Yi Li Haifeng Bao Chengwei Deng Fang Luo Zehui Yang State Key Laboratory of New Textile Materials&Advanced Processing Technology College of Materials Science and EngineeringWuhan Textile UniversityWuhanChina Faculty of Materials Science and Chemistry China University of GeosciencesWuhanChina Shaanxi Coal Chemical Industry Technology Research Institute Co. Ltd.Xi’anChina State Key Laboratory of Space Power-Sources Technology Shanghai Institute of Space Power SourcesShanghaiChina Hubei Key Laboratory for New Textile Materials and Applications Wuhan Textile UniversityWuhanChina

The utilization of single atoms(SAs)as trifunctional electrocatalyst for nitro-gen reduction,oxygen reduction,and oxygen evolution reactions(NRR,ORR,and OER)is still a formidable ***,we devise one-pot synthesized palladium SAs stabilized on nitrogen-doped carbon palladium SA electrocat-alyst(Pd-SA/NC)as efficient trifunctional electrocatalyst for NRR,ORR,and ***-SA/NC performs a robust catalytic activity toward NRR with faradaic efficiency of 22.5%at-0.25 V versus reversible hydrogen electrode(RHE),and the relative Pd utilization efficiency is enhanced by 17-fold than Pd-NP/*** addition,the half-wave potential reaches 0.876 V versus RHE,amounting to a 58-time higher mass activity than commercial Pt/***,the overpotential at 10 mA cm-2 is as low as 287 mV for Pd-SA/NC,outperforming the commer-cial IrO2 by 360 times in turnover frequency at 1.6 V versus ***,the assembled rechargeable zinc-air battery(ZAB)achieves a maximum power den-sity of 170 mW cm-2,boosted by 2.3 times than Pt/C–*** constructed ZABs efficiently power the NRR-OER system to electrochemically generate ammonia implying its superior trifunctionality.

关键词： nitrogen reduction reaction oxygen evolution reaction oxygen reduction reaction single atom

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Correlative Mn-Co catalyst excels Pt in oxygen reduction reaction of quasi-solid-state zinc-air batteries

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Nano Research 2024年第5期17卷 4118-4124页

作者： Tingting Wang Jincheng Huang Wei Sang Cai Zhou Bohan Zhang Wei Zhu Kang Du Zongkui Kou Shengxiang Wang School of Mathematical and Physical Sciences Wuhan Textile UniversityWuhan 430200China State Key Laboratory of Advanced Technology for Materials Synthesis and Processing Wuhan University of TechnologyWuhan 430070China

Zn-air batteries(ZABs)as a class of promising energy storage setups are generally powered by efficient and robust catalysts at the oxygen-involving *** the existing non-noble catalysts have outperformed noble Pt benchmark in the alkaline liquid-state ZABs,to the best of our knowledge few have excelled Pt in quasi-solid-state(QSS)***,we found that an integrated Mn-Co cathode derived from the bimetallic Mn/Co metal organic frameworks generates a 1.4-fold greater power density in the QSS ZABs than a Pt cathode while its power density in liquid-state ZABs is only 0.8-fold of the ***,such Mn-Co catalyst delivers high-rate oxygen reduction reaction(ORR)capability with half-wave potential of 0.84 *** in-depth characterizations and analyses have demonstrated that the Co and Mn species show the specific affinity towards H_(2)O and O_(2),respectively,synergizing the ORR process in the water-deficient environment of QSS *** work has enlightened the rational design of non-noble metal catalysts to improve the power density of QSS ZABs.

关键词： non-noble metal catalysts zinc-air battery quasi-solid-state synergistic effect

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Ultrafast Laser Irradiation Induced Oxidation of Dopant-Free Spiro-OMeTAD for Improving the Perovskite Solar Cells Performance

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Energy & Environmental materials 2025年第2期8卷 288-294页

作者： Jiaqi Meng Xiangyu Chen Weihan Li Nianyao Chai Zhongle Zeng Yunfan Yue Fengyi Zhao Xuewen Wang Center of Femtosecond Laser Manufacturing for Advanced Materials and Devices State Key Laboratory of Advanced Technology for Materials Synthesis and Processing Wuhan University of Technology School of Materials Science and Engineering Wuhan University of Technology International School of Materials Science and Engineering Wuhan University of Technology National Energy Key Laboratory for New Hydrogen-Ammonia Energy Technologies Foshan Xianhu Laboratory

The exceptional photoelectric performance and high compatibility of perovskite materials render perovskite solar cells highly promising for extensive development,thus garnering significant *** perovskite solar cells,the hole transport layer plays a crucial *** the commonly employed organic small molecule hole transport material Spiro-OMeTAD,a certain period of oxidation treatment is required to achieve complete transport ***,this posttreatment oxidation processes typically rely on ambient oxidation,which poses challenges in terms of precise control and leads to degradation of the perovskite light absorption *** approach fails to meet the demands for high efficiency and stability in practical ***,the mechanism of ultrafast laser on Spiro-OMeTAD and the reaction process for laser-induced oxidation of it are ***2at Perovskite/Spiro-OMeTAD interface breaks down to produce I2upon ultrafast laser irradiation and I2promote the oxidation *** the laser irradiation oxidation processing,a higher stability of perovskite solar cells is *** work establishes a new approach toward oxidation treatment of Spiro-OMeTAD.

关键词： hole transport layer perovskite solar cells ultrafast laser irradiation undoped Spiro-OMeTAD

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Biomimetic,fire-resistant,ultralight and porous carbon fiber sponges enabling safe and efficient remediation of crude oil spills in harsh environments

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Journal of materials Science & technology 2023年第27期158卷 77-85页

作者： Yushan Li Songjun Yao Song Yan Mei Xu Long Zheng Fei Pan Yeqiang Tan Xianze Yin College of Materials Science and Engineering State Key Laboratory of New Textile Materials&Advanced Processing TechnologyWuhan Textile UniversityWuhan 430200China National Local Joint Laboratory for Advanced Textile Processing and Clean Production Wuhan Textile UniversityWuhan 430200China Engineering Research Center of Ministry of Education for Clean Production of Textile Printing and Dyeing Wuhan Textile UniversityWuhan 430200China College of School of Environmental Engineering Wuhan Textile UniversityWuhan 430200China State Key Laboratory of Bio-Fibers and Eco-Textiles Collaborative Innovation Center of Marine Biobased Fiber and Ecological Textile Technology Institute of Marine Biobased MaterialsCollege of Materials Science and EngineeringQingdao UniversityQingdao 266071China

advanced absorbents must meet the requirements of superior hydrophobic/oleophilic behavior,favorable adsorption efficiency,and high photothermal and Joule heating performance to handle frequent crude oil ***,current carbon-based absorbents suffer from poor fire resistance,thus severely limiting their application in harsh ***,inspired by a bird’s nest,a polymer“welding”strategy is proposed to design a versatile absorbent in which the polymer serves as a“binder”to interconnect discontinuous fibers together to form a 3D welded *** continuous conductive networks endow the absorbent with high photothermal and Joule heating effect,thus achieving all-weather adsorption,and improving the adsorption efficiency of crude oil via the self-heating *** with other absorbents,the absorbent prepared via polymer welding technology exhibited preferable comprehensive performance,such as superhydrophobicity,high fire resistance,and high absorption ***,the noninflammable absorbent can restrain the combustion of crude oil,thereby reducing its combustion in case of *** versatile absorbent is expected to provide a promising solution for the safe and effi-cient cleanup of crude oil spills in harsh ***,the unique polymer welding strategy can be developed into a universal strategy for other material systems to expand their applications.

关键词： Polymer welding strategy Photothermal effect Joule heating effect Fire resistance Crude oil recovery

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Preparation of Silica Nanosphere with Vertical Pore and Its Application in Oil-water Separation

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Journal of Wuhan University of technology(materials Science) 2023年第2期38卷 299-303页

作者： FAN Hui CAI Yun BAI Ping YUAN Qinwen WANG Dong CHEN Yuanli State Key Laboratory of New Textile Materials and Advanced Processing Technologies of China Key Laboratory of Textile Fiber and ProductsMinistry of EducationHubei International Scientific and Technological Cooperation Base of Intelligent Textile Materials&ApplicationWuhan Textile UniversityWuhan430200China

Uniform monodispersed mesoporous silica nanospheres with vertical pores were successfully synthesized using chiral amphiphilic small molecule L-16Ala5PyClO4and solvents as dual templates via solgel *** morphologies and pore sizes of silicas are adjustable by changing the type and amount of solvents in the reaction *** the increase of the organic solvent content,the morphologies of the obtained silica changed from nanospheres with vertical pore structures to nanosheets *** 1 mL of benzene,cyclohexane or toluene were used as solvents,only silica nanospheres were obtained,the BET surface areas of silica nanospheres reached 600.7,669.5,and 560.8 m^(2)/g,*** pore sizes were 3.51,3.54,and 3.46 nm,***,these ordered silica nanospheres/poly(vinyl alcohol-co-ethylene)(PVAco-PE)nanofiber membranes have high separation efficiencies(>99%)for n-hexane/water mixtures.

关键词： sol-gel preparation mesoporous silica nanosphere oil-water separation

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Thickness-dependent magnetic property of FeNi thin film grown on flexible graphene substrate

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Chinese Physics B 2025年第2期34卷 448-452页

作者： Suixin Zhan Shaokang Yuan Yuming Bai Fu Liu Bohan Zhang Weijia Han Tao Wang Shengxiang Wang Cai Zhou State Key Laboratory of New Textile Materials and Advanced Processing Technologies Wuhan Textile UniversityWuhan 430200China School of Mathematical and Physical Sciences Wuhan Textile UniversityWuhan 430200China School of Integrated Circuits Huazhong University of Science and TechnologyWuhan 430074China Key Laboratory for Magnetism and Magnetic Materials Ministry of EducationLanzhou UniversityLanzhou 730000China

Electronics over flexible substrates offer advantages of flexibility, portability and low cost, and promising applications in the areas of energy, information, defense science and medical service. In recent years, tremendous progress has been witnessed in the development of flexible wearable devices that can be potentially massively deployed. Of particular interest are intelligent wearable devices, such as sensors and storage cells, which can be integrated by flexible magnetoelectronic devices based on magnetic thin films. To examine this further, the magnetic properties of FeNi thin films with different thicknesses grown on flexible graphene substrate are investigated at room temperature. The coercivity increases with increasing thicknesses of FeNi thin film, which can be attributed to the increase of grain size and decrease of surface roughness. Moreover, the thickness modulated magnetic property shows a magnetic anisotropy shift increase with varying thicknesses of FeNi thin film by using measurements based on ferromagnetic resonance, which further enhances the resonance frequency. In addition, the resonance peak is quite stable after bending it for ten cycles. The result is promising for the future design of flexible magnetoelectronic devices.

关键词： resonance frequency FeNi thin film flexible graphene substrate magnetic property

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