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White matter regeneration induced by aligned fibrin nanofiber hydrogel contributes to motor functional recovery in canine T12 spinal cord injury

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Regenerative Biomaterials 2022年第1期9卷 260-270页

作者： Zheng Cao Weitao Man Yuhui Xiong Yi Guo Shuhui Yang Dongkang Liu He Zhao Yongdong Yang Shenglian Yao Chuzhong Li Lingyun Zhao Xiaodan Sun Hua Guo Guihuai Wang Xiumei Wang State Key Laboratory of New Ceramics and Fine Processing Key Laboratory of Advanced MaterialsSchool of Materials Science and EngineeringTsinghua UniversityBeijing 100084China Department of Neurosurgery Beijing Tsinghua Changgung HospitalSchool of Clinical MedicineTsinghua UniversityBeijing 102218China Center for Biomedical Imaging Research Tsinghua UniversityBeijing 100084China Department of Orthopedics Dongzhimen HospitalBeijing 100007China School of Materials Science and Engineering University of Science and Technology BeijingBeijing 100083China Beijing Neurosurgical Institute Beijing Tiantan HospitalBeijing 100070China

A hierarchically aligned fibrin hydrogel(AFG)that possesses soft stiffness and aligned nanofiber structure has been successfully proven to facilitate neuroregeneration in vitro and in ***,its potential in promoting nerve regeneration in large animal models that is critical for clinical translation has not been sufficiently ***,the effects of AFG on directing neuroregeneration in canine hemisected T12 spinal cord injuries were *** obvious white matter regeneration consisting of a large area of consecutive,compact and aligned nerve fibers is induced by AFG,leading to a significant motor functional *** canines with AFG implantation start to stand well with their defective legs from 3 to 4 weeks postoperatively and even effortlessly climb the steps from 7 to 8 ***,high-resolution multi-shot diffusion tensor imaging illustrates the spatiotemporal dynamics of nerve regeneration rapidly crossing the lesion within 4 weeks in the AFG *** findings indicate that AFG could be a potential therapeutic vehicle for spinal cord injury by inducing rapid white matter regeneration and restoring locomotion,pointing out its promising prospect in clinic practice.

关键词： aligned fibrin hydrogel spinal cord injury white matter regeneration diffusion tensor imaging canine

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Recent Advances in Fibrous materials for Hydroelectricity Generation

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Nano-Micro Letters 2025年第2期17卷 109-133页

作者： Can Ge Duo Xu Xiao Feng Xing Yang Zheheng Song Yuhang Song Jingyu Chen Yingcun Liu Chong Gao Yong Du Zhe Sun Weilin Xu Jian Fang College of Textile and Clothing Engineering Soochow UniversitySuzhou 215123People’s Republic of China National Engineering Laboratory for Modern Silk Soochow UniversitySuzhou 215123People’s Republic of China State Key Laboratory of New Textile Materials and Advanced Processing Technologies Wuhan Textile UniversityWuhan 430200People’s Republic of China Institute of Functional Nano&Soft Materials(FUNSOM) Soochow UniversitySuzhou 215123People’s Republic of China Department of Electrical and Computer Engineering University of MassachusettsAmherstMA 01003USA Department of Materials Imperial College LondonSouth Kensington CampusLondon SW72AZUK College of Textile Science and Engineering Zhejiang Sci-Tech UniversityHangzhou 310018People’s Republic of China School of Materials Science and Engineering Shanghai Institute of Technology100 Haiquan RoadShanghai 201418People’s Republic of China

Depleting fossil energy sources and conventional polluting power generation pose a threat to sustainable *** generation from ubiquitous and spontaneous phase transitions between liquid and gaseous water has been considered a promising strategy for mitigating the energy *** materials with unique flexibility,processability,multifunctionality,and practicability have been widely applied for fibrous materials-based hydroelectricity generation(FHG).In this review,the power generation mechanisms,design principles,and electricity enhancement factors of FHG are first ***,the fabrication strategies and characteristics of varied constructions including 1D fiber,1D yarn,2D fabric,2D membrane,3D fibrous framework,and 3D fibrous gel are ***,the advanced functions of FHG during water harvesting,proton dissociation,ion separation,and charge accumulation processes are analyzed in ***,the potential applications including power supply,energy storage,electrical sensor,and information expression are also ***,some existing challenges are considered and prospects for future development are sincerely proposed.

关键词： Hydroelectricity Fibrous material Streaming potential Ion diffusion

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Recent progress on surface chemistryⅠ:Assembly and reaction

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Chinese Chemical Letters 2024年第12期35卷 43-94页

作者： Xin Li Zhen Xu Donglei Bu Jinming Cai Huamei Chen Qi Chen Ting Chen Fang Cheng Lifeng Chi Wenjie Dong Zhenchao Dong Shixuan Du Qitang Fan Xing Fan Qiang Fu Song Gao Jing Guo Weijun Guo Yang He Shimin Hou Ying Jiang Huihui Kong Baojun Li Dengyuan Li Jie Li Qing Li Ruoning Li Shuying Li Yuxuan Lin Mengxi Liu Peinian Liu Yanyan Liu Jingtao Lü Chuanxu Ma Haoyang Pan JinLiang Pan Minghu Pan Xiaohui Qiu Ziyong Shen Shijing Tan Bing Wang Dong Wang Li Wang Lili Wang Tao Wang Xiang Wang Xingyue Wang Xueyan Wang Yansong Wang Yu Wang Kai Wu Wei Xu Na Xue Linghao Yan Fan Yang Zhiyong Yang Chi Zhang Xue Zhang Yang Zhang Yao Zhang Xiong Zhou Junfa Zhu Yajie Zhang Feixue Gao Yongfeng Wang Center for Carbon-based Electronics and Key Laboratory for the Physics and Chemistry of Nanodevices School of ElectronicsPeking UniversityBeijing 100871China Spin-X Institute School of MicroelectronicsSouth China University of TechnologyGuangzhou 511442China School of Materials and Energy Guangzhou Key Laboratory of Low-Dimensional Materials and Energy Storage DevicesGuangdong University of TechnologyGuangzhou 510006China Faculty of Materials Science and Engineering Kunming University of Science and TechnologyKunming 650093 China i-Lab CAS Key Laboratory of Nanophotonic Materials and DevicesSuzhou Institute of Nano-Tech and Nano-BionicsChinese Academy of SciencesSuzhou 215123China CAS Key Laboratory of Molecular Nanostructure and Nanotechnology CAS Research/Education Center for Excellence in Molecular SciencesBeijing National Laboratory for Molecular Sciences(BNLMS)Institute of ChemistryChinese Academy of SciencesBeijing 100190China State Key Laboratory for Organic Electronics and Information Displays&Jiangsu Key Laboratory for Biosensors Institute of Advanced MaterialsJiangsu National Synergetic Innovation Center for Advanced MaterialsNanjing University of Posts and TelecommunicationsNanjing 210023China Institute of Functional Nano and Soft Materials(FUNSOM) Jiangsu Key Laboratory for Carbon-Based Functional Materials and DevicesSoochow UniversitySuzhou 215123China Hefei National Research Center for Physical Sciences at the Microscale and Synergetic Innovation Center of Quantum Information and Quantum Physics University of Science and Technology of ChinaHefei 230026China Institute of Physics&University of Chinese Academy of Sciences Beijing 100190China State Key Laboratory of Catalysis Dalian Institute of Chemical PhysicsChinese Academy of SciencesDalian 116023China College of Chemistry Beijing Normal UniversityBeijing 100875China Beijing National Laboratory for Molecular Sciences(BNLMS) College of Chemistry and Molecular EngineeringPeking UniversityBeijing 100871China School

Surface chemistry focuses on the investigation of the adsorption,migration,assembly,activation,reaction,and desorption of atoms and molecules at *** chemistry plays the pivotal roles in both fundamental science and applied *** review will summarize the recent progresses on surface assembly,synthesis and catalysis investigated mainly by scanning tunneling microscopy and atomic force *** assemblies of water and small biomolecules,construction of Sierpin′ski triangles and surface chirality are ***-surface synthesis of conjugated carbo-and heterocycles and other kinds of carbon nanostructures are *** model catalysis,including single-atom catalysis and electrochemical catalysis,are discussed at the single-atom level.

关键词： Surface chemistry Assembly Surface synthesis Catalysis on surface Surface electrochemical processes

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Boosting hydrogen evolution via work-function-accelerated electronic reconfiguration of Mo-based heterojunction

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Science China materials 2025年第1期68卷 189-198页

作者： Xiang Chen Shuai Feng Song Xie Yaping Miao Biao Gao Xuming Zhang Li Huang Yun Li Paul K.Chu Xiang Peng Hubei Key Laboratory of Plasma Chemistry and Advanced Materials Engineering Research Center of Phosphorus Resources Development and Utilization of Ministry of EducationSchool of Materials Science and EngineeringWuhan Institute of TechnologyWuhan 430205China Department of Physics Department of Materials Science and Engineeringand Department of Biomedical EngineeringCity University of Hong KongHong Kong 999077China School of Textile Science and Engineering Xi’an Polytechnic UniversityXi’an 710048China The State Key Laboratory of Refractories and Metallurgy Institute of Advanced Materials and NanotechnologyWuhan University of Science and TechnologyWuhan 430081China Guizhou Wujiang Hydropower Development Co. Ltd.Guiyang 550002China

Molybdenum-based catalysts have demonstrated significant potential in the electrocatalytic hydrogen evolution reaction(HER).However,the limited exposure of active sites and strong hydrogen adsorption result in suboptimal ***,a Mo_(2)N±MoSe_(2) heterojunction is prepared on carbon cloth(MNS/CC)to enhance the *** strong electronic interaction between Mo_(2)N and MoSe_(2),combined with the lower work function of Mo_(2)N,creates an intrinsic electric field at the heterojunction interface,which markedly improves charge transfer ***,the optimized electronic structure of Mo sites further enhances charge transfer and intrinsically catalytic activity in *** a result,MNS/CC requires overpotentials of mere 65 and 210 mV to achieve current densities of 20 mA cm^(−2) and 1 A cm^(−2),respectively,with a Tafel slope of only 96 mV dec−***,MNS/CC maintains stable operation at 1 A cm^(−2) for 240 h without significant *** results offer insights into the design of non-precious metal-based electrocatalysts for industrial hydrogen production.

关键词： water splitting hydrogen evolution reaction molybdenum-based catalyst heterojunction electronic interaction

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Tuning electrochemical water activation over NiIr single-atom alloy aerogels for stable electrochemiluminescence

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Science Bulletin 2024年第15期69卷 2387-2394页

作者： Ling Ling Mengzhen Xi Hengjia Wang Runshi Xiao Lirong Zheng Liuyong Hu Wenling Gu Chengzhou Zhu State Key Laboratory of Green Pesticide International Joint Research Center for Intelligent Biosensing Technology and HealthCollege of ChemistryCentral China Normal UniversityWuhan 430079China Hubei Key Laboratory of Plasma Chemistry and Advanced Materials Hubei Engineering Technology Research Center of Optoelectronic and New Energy MaterialsWuhan Institute of TechnologyWuhan 430205China Institute of High Energy Physics Chinese Academy of SciencesBeijing 100049China

The anodic oxygen evolution reaction is a well-acknowledged side reaction in traditional aqueous electrochemiluminescence(ECL) systems due to the generation and surface aggregation of oxygen at the electrode, which detrimentally impacts the stability and efficiency of ECL emission. However, the effect of reactive oxygen species generated during water oxidation on ECL luminophores has been largely overlooked. Taking the typical luminol emitter as an example, herein, we employed NiIr single-atom alloy aerogels possessing efficient water oxidation activity as a prototype co-reaction accelerator to elucidate the relationship between ECL behavior and water oxidation reaction kinetics for the first time. By regulating the concentration of hydroxide ions in the electrolyte, the electrochemical oxidation processes of both luminol and water are finely tuned. When the concentration of hydroxide ions in electrolyte is low,the kinetics of water oxidation is attenuated, which limits the generation of oxygen, effectively mitigates the influence of oxygen accumulation on the ECL strength, and offers a novel perspective for harnessing side reactions in ECL systems. Finally, a sensitive and stable sensor for antioxidant detection was constructed and applied to the practical sample detection.

关键词： Electrochemiluminescence Luminol Water activation Single-atom doping Sensing

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An orbital strategy for regulating the Jahn-Teller effect

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National Science Review 2024年第9期11卷 243-252页

作者： Tongtong Shang Ang Gao Dongdong Xiao Qinghua Zhang Xiaohui Rong Zhexin Tang Weiguang Lin Ting Lin Fanqi Meng Xinyan Li Yuren Wen Xuefeng Wang Dong Su Zhen Chen Yong-Sheng Hu Hong Li Qian Yu Ze Zhang Lijun Wu Lin Gu Jian-Min Zuo Yimei Zhu Liquan Chen Ce-Wen Nan State Key Laboratory of New Ceramics and Fine Processing National Center for Electron Microscopy in Beijing School of Materials Science and Engineering Tsinghua University Beijing National Laboratory for Condensed Matter Physics Institute of Physics Chinese Academy of Sciences Songshan Lake Materials Laboratory School of Materials Science and Engineering University of Science and Technology Beijing Department of Materials Science and Engineering Center of Electron Microscopy and State Key Laboratory of Silicon Materials Zhejiang University Condensed Matter Physics and Materials Science Division Brookhaven National Laboratory Department of Materials Science and Engineering University of Illinois at Urbana Champaign

The Jahn-Teller effect（JTE） arising from lattice-electron coupling is a fascinating phenomenon that profoundly affects important physical properties in a number of transition-metal *** JT distortions and their corresponding electronic structures is highly desirable to tailor the functionalities of ***,we propose a local coordinate strategy to regulate the JTE through quantifying occupancy in the dz2and dx2-y2orbitals of Mn and scrutinizing the symmetries of the ligand oxygen atoms in MnO6octahedra in LiMn2O4and *** effectiveness of such a strategy has been demonstrated by constructing P2-type NaLixMn1-xO2oxides with different Li/Mn ordering *** addition,this strategy is also tenable for most 3d transition-metal compounds in spinel and perovskite frameworks,indicating the univers ality of local coordinate strategy and the tunability of the lattice-orbital coupling in transition-metal *** work demonstrates a useful strategy to regulate JT distortion and provides useful guidelines for future design of functional materials with specific physical properties.

关键词： quantitative convergent-beam electron diffraction Jahn–Teller effect transition-metal oxide local coordinate strategy orbital degenerate

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One-step synthesis and electromagnetic absorption properties of high entropy rare earth hexaborides(HE REB6)and high entropy rare earth hexaborides/borates(HE REB6/HE REB03)composite powders

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Journal of advanced Ceramics 2021年第1期10卷 62-77页

作者： Weiming ZHANG Biao ZHAO Huimin XIANG Fu-Zhi DAI Shijiang WU Yanchun ZHOU Science and Technology on Advanced Functional Composite Laboratory Aerospace Research Institute of Materials&Processing TechnologyBeijing 100076China Henan Key Laboratory of Aeronautical Materials and Application Technology School of Material Science and EngineeringZhengzhou University of AeronauticsZhengzhou 450046China Zibo Firststar New Material Incorporated Co. Ltd.Zibo 255000China

Considering the emergence of severe electromagnetic interference problems,it is vital to develop electromagnetic(EM)wave absorbing materials with high dielectric,magnetic loss and optimized impedance ***,realizing the synergistic dielectric and magnetic losses in a single phase material is still a ***,high entropy(HE)rare earth hexaborides(REB6)powders with coupling of dielectric and magnetic losses were designed and successfully synthesized through a facial one-step boron carbide reduction method,and the effects of high entropy borates intermedia phases on the EM wave absorption properties were *** HE REB6 ceramics including(Ce0.2Y0.2Sm0.2Er0.2Yb0.2)B6,(Ce0.2Hu0.2Sm0.2Er0.2Yb0.2)B6,(Ce0.2Y0.2Eu0.2Er0.2Yb0.2)B6,(Ce0.2Ya2Sm0.2Eu0.2Yb0.2)B6,and(Nd0.2Y0.2Sm0.2Eu0.2Yb0.2)B6 possess CsCl-type cubic crystal structure,and their theoretical densities range from 4.84 to 5.25 g/cm^(3).(Ce02Y0.2Sm0.2Er0.2Yb02)B6 powders with the average particle size of 1.86 jim were found to possess the best EM wave absorption properties among these *** RLmin value of(Ce0.2Y0.2Sm0.2Er0.2Yb0.2)B6 reaches-33.4 dB at 11.5 GHz at thickness of 2 mm;meanwhile,the optimized effective absorption bandwidth(EAB)is 3.9 GHz from 13.6 to 17.5 GHz with a thickness of 1.5 *** introduction of HE REB03(RE=Ce,Y,Sm,Eu,Er,Yb)as intermediate phase will give rise to the mismatching impedance,which will further lead to the reduction of reflection ***,the HEREB6/HEREB03 still possess wide effective absorption bandwidth of 4.1 GHz with the relative low thickness of 1.7 *** the better stability,low density,and good EM wave absorption properties,HE REB6 ceramics are promising as a new type of EM wave absorbing materials.

关键词： high entropy rare earth hexaborides(HE REB6) one-step synthesis electromagnetic wave absorbing properties synergistic dielectric and magnetic losses wide effective absorption bandwidth

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Continuous Basalt Fibers into Fireproof and Thermal Insulation Architectures Using an Additive Manufacturing Manipulator

SSRN

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SSRN 2023年

作者： Yan, Chunze Shi, Yusheng Su, Bin Liu, Zhufeng Zhang, Lichao Li, Zhaoqing Wang, Changshun Wu, Zhenhua Wu, Siqi Wu, Hongzhi Geng, Peng Chen, Si Liu, Guizhou Yang, Lei Xia, Zhigang State Key Laboratory of Materials Processing and Die & Mould Technology Huazhong University of Science and Technology Wuhan430074 China Engineering Research Center of Ceramic Materials for Additive Manufacturing Ministry of Education Wuhan430074 China Wuhan Zeqing Technology Co. Ltd. Wuhan430074 China School of Transportation and Logistics Engineering Wuhan University of Technology Wuhan430063 China State Key Laboratory of New Textile Materials and Advanced Processing Technologies Wuhan Textile University Wuhan430200 China

The weaving technique used for basalt fibers is suitable for making architectures with a two-dimensional (2D) structure, but in practical applications, three-dimensional (3D) structure architectures are required in many fields. Additive manufacturing (AM) technology is suitable for fabricating 3D complex parts. However, the existing AM technology is only used to process continuous basalt fibers reinforced polymers for mechanical enhancement. Therefore, here, we report the fabrication of continuous basalt fibers with fireproof and thermal insulation performance through the combination of an AM manipulator, two-step precursor infiltration and pyrolysis (PIP) processes. Using SiOC ceramics to fill between continuous basalt fibers will help improve the architectures' fire and thermal insulation performance. In order to reduce the structural defects generated by the first PIP process, the final part with fireproof and thermal insulation performance was fabricated through the second PIP process. We further demonstrated the final part with excellent fireproof and thermal insulation performance. The final part had a shell temperature of 788.8℃ and an internal temperature of about 50℃ under the flame spray gun for the 20 s. By replacing polymers with inorganic materials, our basalt architectures exhibit their potential applications in military, aviation, and civil fireproof and thermal insulation equipment. © 2023, The Authors. All rights reserved.

关键词： 3D printing

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Intrinsic ion migration-induced susceptible two-dimensional phase-transition memristor with ultralow power consumption

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Science Bulletin 2025年

作者： Qin, Lanhao Yu, Yimeng Fang, Cheng Liu, Yujie Zhu, Kaichen Ouyang, Decai Liu, Shenghong Song, Bailing Zhou, Ruochen Lanza, Mario Hu, Wenhua Wu, Jinsong Li, Yuan Zhai, Tianyou State Key Laboratory of Materials Processing and Die & Mould Technology School of Materials Science and Engineering Huazhong University of Science and Technology Wuhan430074 China State Key Laboratory of Advanced Technology for Materials Synthesis and Processing Wuhan University of Technology Wuhan430070 China Center of Hydrogen Science State Key Laboratory of Metal Matrix Composites School of Materials Science and Engineering Innovation Center for Future Materials Shanghai Jiao Tong University Shanghai200240 China Physical Science and Engineering Division King Abdullah University of Science and Technology Thuwal23955-6900 Saudi Arabia School of Computer Science and Artificial Intelligence Wuhan University of Technology Wuhan430070 China

Two-dimensional (2D) phase-transition memristors have demonstrated transformative potential for neuromorphic computing, yet challenges like high power consumption, limited endurance, and crystal damage from external ion intercalation persist. Here, we introduce a novel 2D phase-transition memristor leveraging a paradigm-shifting mechanism by exploiting the ultrafast intrinsic Cu+ ion migration within Cu2S. This approach eliminates the need for external ion insertion, significantly reducing crystal damage and enabling exceptional cycling stability with over 400 DC cycles and 500 pulse cycles. The susceptible monoclinic-tetragonal phase-transition induced by intrinsic Cu+ migration achieves an unprecedented SET power consumption of 1 μW at 100 mV, significantly lower in currently reported phase-transition memristors. To further demonstrate the potential of intrinsic ion migration-induced (IIM) memristor, we simulated an IIM memristor crossbar array for image preprocessing in gesture recognition with a high SSIM value of 0.94, showcasing its potential for scalable neuromorphic hardware. This work establishes a new paradigm in low-power, high-performance phase-transition memristors, advancing their practical application in next-generation computing. © 2025 Science China Press

关键词： Memristor Neuromorphic device Two-dimensional materials

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N-Heterocycles Extended π-Conjugation Enables Ultrahigh Capacity,Long-Lived,and Fast-Charging Organic Cathodes for Aqueous Zinc Batteries

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CCS Chemistry 2023年第8期5卷 1789-1801页

作者： Huiling Peng Jin Xiao Zhonghan Wu Lei Zhang Yaheng Geng Wenli Xin Junwei Li Zichao Yan Kai Zhang Zhiqiang Zhu State Key Laboratory of Chemo/Biosensing and Chemometrics College of Chemistry and Chemical EngineeringHunan UniversityChangsha 410082 School of Science Hunan University of TechnologyZhuzhou 412007 Frontiers Science Center for New Organic Matter Renewable Energy Conversion and Storage Center(RECAST)Key Laboratory of Advanced Energy Materials ChemistryMinistry of EducationCollege of ChemistryNankai UniversityTianjin 300071

The aqueous zinc-organic battery is a promising candidate for large-scale energy ***,the rational design of advanced organic cathodes with high capacity,long lifespan,and high rate capability remains a big ***,we propose that extending theπ-conjugation by N-heterocycles can provide more active sites,lead to insolubility,and facilitate charge transfer,thus boosting the overall electrochemical performance of organic *** on this concept,a novel organic compound,dipyrido[3ʹ,2ʹ:5,6;2″,3″:7,8]quinoxalino[2,3-i]dipyrido[3,2-a:2ʹ,3ʹ-c]phenazine-10,21-dione(DQDPD),has been rationally designed and evaluated as the cathode for aqueous zinc ***,DQDPD shows a record high capacity(509 mAh g^(−1) at 0.1 A g^(−1),corresponding to a record-breaking energy density of 348 Wh kg^(−1)),excellent cycling stability(92%capacity retention after 7500 cycles at 10 A g^(−1)),and fast-charging capability(161 mAh g^(−1) at 20 A g^(−1)).Our work offers new ideas in the molecular engineering of organic electrodes for high-performance rechargeable batteries.

关键词： aqueous zinc batteries organic cathodes H^(+)/Zn^(2+)coinsertion N-heterocycles extendedπ-conjugation

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